The Palaeoproterozoic, ∼ 1.88–2.0 Ga, Mugford Group of northern Labrador is a relatively undeformed cover sequence developed on Archaean crust of the Nain craton. The Cod Island Formation occurs at the base of the group and consists of mixed shale, chert, dolostone and siltstone. Thin layers of highly matured organic material similar to anthracite have been found within a shale and chert sequence. Based on the nonmigrated and sedimentological context of the layers, the material may represent some of the earliest intact, in situ, organic deposits known. δ 13C isotope ratios of the organic matter in this deposit range from −31.79 to −32.22‰ and the H/C atomic ratios from 0.05 to 0.08. The material represents the first truly biological remains known from the Nain Province of Labrador and the earliest organic material in northeastern North America.