Multiphoton States Research Articles

Heisenberg-Limited Quantum Lidar for Joint Range and Velocity Estimation.

We propose a quantum lidar protocol to jointly estimate the range and velocity of a target by illuminating it with a single beam of pulsed displaced squeezed light. In the lossless scenario, we show that the mean-squared errors of both range and velocity estimations are inversely proportional to the squared number of signal photons, simultaneously attaining the Heisenberg limit. This is achieved by engineering the multiphoton squeezed state of the temporal modes and adopting standard homodyne detection. To assess the robustness of the quantum protocol, we incorporate photon losses and detuning of the homodyne receiver. Our findings reveal a quantum advantage over the best-known classical strategy across a wide range of round-trip transmissivities. Particularly, the quantum advantage is substantial for sufficiently small losses, even when compared to the optimal-potentially unattainable-classical performance limit. The quantum advantage also extends to the practical case where quantum engineering is done on top of a strong classical coherent state with watts of power. This, together with the robustness against losses and the feasibility of the measurement with state-of-the-art technology, make the protocol highly promising for near-term implementation.

Revealing nonclassicality of multiphoton optical beams via artificial neural networks

The identification of nonclassical features of multiphoton quantum states represents a crucial task in the development of many quantum photonic technologies. Under realistic experimental conditions, a photonic quantum state gets affected by its interaction with several nonideal optoelectronic devices, including those used to guide, detect, or characterize it. The result of such noisy interaction is that the nonclassical features of the original quantum state get considerably reduced or are completely absent in the detected, final state. In this work, the self-learning features of artificial neural networks are exploited to experimentally show that the nonclassicality of multiphoton quantum states can be assessed and fully characterized, even in the cases in which the nonclassical features are concealed by the measuring devices. Our work paves the way toward artificial-intelligence-assisted experimental-setup characterization, as well as quantum state nonclassicality identification. Published by the American Physical Society 2024

Optimized higher-order photon state classification by machine learning

The classification of higher-order photon emission becomes important with more methods being developed for deterministic multiphoton generation. The widely used second-order correlation g(2) is not sufficient to determine the quantum purity of higher photon Fock states. Traditional characterization methods require a large amount of photon detection events, which leads to increased measurement and computation time. Here, we demonstrate a machine learning model based on a 2D Convolutional Neural Network (CNN) for rapid classification of multiphoton Fock states up to |3⟩ with an overall accuracy of 94%. By fitting the g(3) correlation with simulated photon detection events, the model exhibits an efficient performance particularly with sparse correlation data, with 800 co-detection events to achieve an accuracy of 90%. Using the proposed experimental setup, this CNN classifier opens up the possibility for quasi-real-time classification of higher photon states, which holds broad applications in quantum technologies.

Birefringent Spin‐Photon Interface Generates Polarization Entanglement

AbstractA spin‐photon interface based on the luminescence of a singly charged quantum dot in a micropillar cavity allows for the creation of photonic entangled states. Current devices suffer from cavity birefringence, which limits the generation of spin‐photon entanglement. In this study, we conduct a theoretical analysis of the light absorption and emission by the interface with an anisotropic cavity and derive the maximal excitation and spin‐photon entanglement conditions. It is shown that the concurrence of the spin‐photon state equal to one and complete quantum dot population inversion can be reached for a micropillar cavity with any degree of birefringence by tuning the quantum dot resonance strictly between the cavity modes. This sweet spot is also valid for generating a multiphoton cluster state, as demonstrated by calculating the three‐tangle and fidelity with the maximally entangled state.

Generation of multi-photon Fock states at telecommunication wavelength using picosecond pulsed light

Multi-photon Fock states have diverse applications such as optical quantum information processing. For the implementation of quantum information processing, Fock states should be generated within the telecommunication wavelength band, particularly in the C-band (1530-1565 nm). This is because mature optical communication technologies can be leveraged for transmission, manipulation, and detection. Additionally, to achieve high-speed quantum information processing, Fock states should be generated in optical pulses with as short a duration as possible, as this allows embedding lots of information in the time domain. In this paper, we successfully generate picosecond pulsed multi-photon Fock states (single-photon and two-photon states) in the C-band with Wigner negativities for the first time, which are verified by pulsed homodyne tomography. In our experimental setup, we utilize a single-pixel superconducting nanostrip photon-number-resolving detector (SNSPD), which is expected to facilitate the high-rate generation of various quantum states. This capability stems from the high temporal resolution of SNSPDs (several tens of picoseconds in our case and also in general) allowing us to increase the repetition frequency of pulsed light from the conventional MHz range to the GHz range, although in this experiment the repetition frequency is limited to 10 MHz due to the bandwidth of the homodyne detector. Consequently, our experimental setup is anticipated to serve as a prototype of a high-speed optical quantum state generator for ultrafast quantum information processing at telecommunication wavelength.

Engineering quantum states from a spatially structured quantum eraser.

Quantum interference is a central resource in many quantum-enhanced tasks, from computation to communication. While usually occurring between identical photons, it can also be enabled by performing projective measurements that render the photons indistinguishable, a process known as quantum erasing. Structured light forms another hallmark of photonics, achieved by manipulating the degrees of freedom of light, and enables a multitude of applications in both classical and quantum regimes. By combining these ideas, we design and experimentally demonstrate a simple and robust scheme that tailors quantum interference to engineer photonic states with spatially structured coalescence along the transverse profile, a type of quantum mode with no classical counterpart. To achieve this, we locally tune the distinguishability of a photon pair by spatially structuring the polarization and creating a structured quantum eraser. We believe that these spatially engineered multiphoton quantum states may be of significance in fields such as quantum metrology, microscopy, and communication.

Deterministic single photon subtraction with a cascade of waveguide-coupled atoms

We present a specialized photon subtraction scheme that allows for the deterministic extraction of single photons from multiphoton states while preserving the input single-photon states unaltered. The proposed device integrates two Λ-type emitters with transitions selectively coupled to a single chiral waveguide through single photon Raman interaction (SPRINT). We develop a comprehensive theoretical model for the system using the input-output formalism within the SLH framework and conduct numerical simulations to analyze its interaction with traveling few-photon pulses of coherent light. We use these simulations to predict the scheme’s operation and highlight how this two-emitter extension improves the original SPRINT-based deterministic single-photon subtraction when it comes to implementing undetectable photon number splitting attack on a quantum key distribution channel.

Tailoring the nonclassicality of light states via mode detuning in waveguide beam splitters

The recent advent of integrated waveguide systems with reconfigurable propagation constants and coupling coefficients has opened the door to using waveguide detuning as a resource for readily tailoring the quantum properties of light states. Here we theoretically demonstrate that waveguide mode detuning can be used for molding the nonclassical properties of two interacting quantum optical fields in integrated waveguide couplers. In particular, we explore the states that are generated by conditional measurements when one of the input ports of the waveguide coupler is excited by coherent states, squeezed vacuum states, and thermal states, while the other port is excited by a single-photon Fock state. We explore the detuning range required to attain nonclassical states. Our findings could pave the way for a robust integrated-optics protocol, providing enhanced control and engineering capabilities over multiphoton quantum states.

Deterministic Generation of Qudit Photonic Graph States from Quantum Emitters

We propose and analyze deterministic protocols to generate qudit photonic graph states from quantum emitters. We show that our approach can be applied to generate any qudit graph state and we exemplify it by constructing protocols to generate one- and two-dimensional qudit cluster states, absolutely maximally entangled states, and logical states of quantum error-correcting codes. Some of these protocols make use of time-delayed feedback, while others do not. The only additional resource requirement compared to the qubit case is the ability to control multilevel emitters. These results significantly broaden the range of multiphoton entangled states that can be produced deterministically from quantum emitters. Published by the American Physical Society 2024

Single-shot characterization of photon indistinguishability with dielectric metasurfaces

Characterizing the indistinguishability of photons is a key task in quantum photonics, underpinning the tuning and stabilization of the photon sources and thereby increasing the accuracy of quantum operations. The protocols for measuring the degree of indistinguishability conventionally require photon-coincidence measurements at several different time or phase delays, which is a fundamental bottleneck towards fast measurements and real-time monitoring of indistinguishability. Here, we develop a static dielectric metasurface grating without any reconfigurable elements that realizes a tailored multiport transformation in the free-space configuration without the need for phase locking and enables single-shot characterization of the indistinguishability between two photons in multiple degrees of freedom including time, spectrum, spatial modes, and polarization. Topology optimization is employed to design a silicon metasurface with polarization independence, high transmission, and high tolerance to measurement noise. We fabricate the metasurface and experimentally quantify the indistinguishability of photons in the time domain with fidelity over 98.4%. We anticipate that the developed framework based on ultrathin metasurfaces can be further extended for multi-photon states and additional degrees of freedom associated with spatial modalities.

Error suppression in multicomponent cat codes with photon subtraction and teleamplification

It is known that multiphoton states can be protected from decoherence due to a passive loss channel by applying noiseless attenuation before and noiseless amplification after the channel. In this work, we propose the combined use of multiphoton subtraction on four-component cat codes and teleamplification to effectively suppress errors under detection and environmental losses. The back-action from multiphoton subtraction modifies the encoded qubit encoded on cat states by suppressing the higher photon numbers, while simultaneously ensuring that the original qubit can be recovered effectively through teleamplification followed by error correction, thus preserving its quantum information. With realistic photon subtraction and teleamplification-based scheme followed by optimal error-correcting maps, one can achieve a worst-case fidelity (over all encoded pure states) of over 93.5% (82% with only noisy teleamplification) at a minimum success probability of about 3.42%, under a 10% environmental-loss rate, 95% detector efficiency and sufficiently large cat states with the coherent-state amplitudes of 2. This sets a promising standard for combating large passive losses in quantum-information tasks in the noisy intermediate-scale quantum (NISQ) era, such as direct quantum communication or the storage of encoded qubits on the photonic platform.

High-fidelity four-photon GHZ states on chip

Mutually entangled multi-photon states are at the heart of all-optical quantum technologies. While impressive progresses have been reported in the generation of such quantum light states using free space apparatus, high-fidelity high-rate on-chip entanglement generation is crucial for future scalability. In this work, we use a bright quantum-dot based single-photon source to demonstrate the high fidelity generation of 4-photon Greenberg-Horne-Zeilinger (GHZ) states with a low-loss reconfigurable glass photonic circuit. We reconstruct the density matrix of the generated states using full quantum-state tomography reaching an experimental fidelity to the target state of FGHZ4=(86.0±0.4)%\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$${{{{\\mathcal{F}}}}}_{{{{{\\rm{GHZ}}}}}_{4}}=(86.0\\pm 0.4)\\, \\%$$\\end{document}, and a purity of PGHZ4=(76.3±0.6)%\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$${{{{\\mathcal{P}}}}}_{{{{{\\rm{GHZ}}}}}_{4}}=(76.3\\pm 0.6)\\, \\%$$\\end{document}. The entanglement of the generated states is certified with a semi device-independent approach through the violation of a Bell-like inequality by more than 39 standard deviations. Finally, we carry out a four-partite quantum secret sharing protocol on-chip where a regulator shares with three interlocutors a sifted key with up to 1978 bits, achieving a qubit-error rate of 10.87%. These results establish that the quantum-dot technology combined with glass photonic circuitry offers a viable path for entanglement generation and distribution.

Autonomous Stabilization of Fock States in an Oscillator against Multiphoton Losses.

Fock states with a well-defined number of photons in an oscillator have shown a wide range of applications in quantum information science. Nonetheless, their usefulness has been marred by single and multiphoton losses due to unavoidable environment-induced dissipation. Though several dissipation engineering methods have been developed to counteract the leading single-photon-loss error, averting multiple-photon losses remains elusive. Here, we experimentally demonstrate a dissipation engineering method that autonomously stabilizes multiphoton Fock states against losses of multiple photons using a cascaded selective photon-addition operation in a superconducting quantum circuit. Through measuring the photon-number populations and Wigner tomography of the oscillator states, we observe a prolonged preservation of nonclassical Wigner negativities for the stabilized Fock states |N⟩ with N=1, 2, 3 for a duration of about 10ms. Furthermore, the dissipation engineering method demonstrated here also facilitates the implementation of a nonunitary operation for resetting a binomially encoded logical qubit. These results highlight potential applications in error-correctable quantum information processing against multiple-photon-loss errors.

Efficient characterizations of multiphoton states with an ultra-thin optical device

Metasurface enables the generation and manipulation of multiphoton entanglement with flat optics, providing a more efficient platform for large-scale photonic quantum information processing. Here, we show that a single metasurface optical device would allow more efficient characterizations of multiphoton entangled states, such as shadow tomography, which generally requires fast and complicated control of optical setups to perform information-complete measurements, a demanding task using conventional optics. The compact and stable device here allows implementations of general positive operator valued measures with a reduced sample complexity and significantly alleviates the experimental complexity to implement shadow tomography. Integrating self-learning and calibration algorithms, we observe notable advantages in the reconstruction of multiphoton entanglement, including using fewer measurements, having higher accuracy, and being robust against experimental imperfections. Our work unveils the feasibility of metasurface as a favorable integrated optical device for efficient characterization of multiphoton entanglement, and sheds light on scalable photonic quantum technologies with ultra-thin optical devices.

Photonic Source of Heralded Greenberger-Horne-Zeilinger States.

Generating large multiphoton entangled states is of main interest due to enabling universal photonic quantum computing and all-optical quantum repeater nodes. These applications exploit measurement-based quantum computation using cluster states. Remarkably, it was shown that photonic cluster states of arbitrary size can be generated by using feasible heralded linear optics fusion gates that act on heralded three-photon Greenberger-Horne-Zeilinger (GHZ) states as the initial resource state. Thus, the capability of generating heralded GHZ states is of great importance for scaling up photonic quantum computing. Here, we experimentally demonstrate this required building block by reporting a polarisation-encoded heralded GHZ state of three photons, for which we build a high-rate six-photon source (547±2 Hz) from a solid-state quantum emitter and a stable polarization-based interferometer. The detection of three ancillary photons heralds the generation of three-photon GHZ states among the remaining particles with fidelities up to F=0.7278±0.0106. Our results initiate a path for scalable entangling operations using heralded linear-optics implementations.

Non-Gaussian quantum states generated via quantum catalysis and their statistical properties

Abstract A new kind of non-Gaussian quantum catalyzed state is proposed via multiphoton measurements and two-mode squeezing as an input of thermal state. The characteristics of generating multiphoton catalysis output state depends on the thermal parameter, catalyzed photon number and squeezing parameter. We then analyze the nonclassical properties by examining the photon number distribution, photocount distribution and partial negativity of the Wigner function. Our findings indicate that nonclassicality can be achieved through the implementation of multiphoton catalysis operations, and modulated by the thermal parameter, catalyzed photon number and squeezing parameter.

Robust Classical and Quantum Polarimetry with a Single Nanostructured Metagrating.

We formulate a new conceptual approach for one-shot complete polarization state measurement with nanostructured metasurfaces applicable to classical light and multiphoton quantum states by drawing on the principles of generalized quantum measurements based on positive operator-valued measures. Accurate polarization reconstruction from a combination of photon counts or correlations from several diffraction orders is robust with respect to even strong fabrication inaccuracies, requiring only a single classical calibration of the metasurface transmission. Furthermore, this approach operates with a single metagrating without interleaving, allowing for a reduction in metasurface size while preserving high transmission efficiency and output beam quality. We theoretically obtained original metasurface designs, fabricated the metasurface from amorphous silicon nanostructures deposited on glass, and experimentally confirmed accurate polarization reconstruction of laser beams. We also anticipate robust operation under changes in environmental conditions, opening new possibilities for space-based imaging and satellite optics.

Enhancing quantum features and teleportation fidelity of two-mode non-Gaussian states using conditional measurements

The family of two-mode non-Gaussian entangled states, including the pair coherent states (PCSs) and their genealogies, has been extensively investigated regarding their quantum properties and their practical applications in quantum information. Specifically, certain states, such as the multiphoton catalytic pair coherent states (MCPCSs), have been newly introduced under specific experimental conditions. For a more feasible approach, in this paper, we introduce novel nonclassical states obtained by subtracting photons through conditional measurements using beam splitters applied to the two modes of the PCSs. These states are called pair coherent states with conditional measurements (PCSCMs). Our purpose is to demonstrate that the quantum features, such as entanglement, Einstein–Podolsky–Rosen (EPR) correlation, EPR steering, and the average fidelity in teleportation can be enhanced in comparison with both the original PCSs and the MCPCSs. In specific cases, several characteristics are observed in PCSCMs but not inspected in both PCSs and MCPCSs. In our findings, we prove that the quantum characteristics within the PCSCMs are influenced not just by the number of detected photons, denoted by variables k and l, but also by the discrepancy in photon numbers, especially by the difference of k − l.

Controlled Emission of Entangled Multiphoton States from Cascaded Quantum Wells

Controlled Emission of Entangled Multiphoton States from Cascaded Quantum Wells

Single-active-element demultiplexed multi-photon source

Temporal-to-spatial mode demultiplexing routes non-simultaneous events of the same spatial mode to distinct output trajectories. This technique has now been widely adopted, because it gives access to higher-number multi-photon states when exploiting solid-state quantum emitters. However, implementations so far have required an always-increasing number of active elements and are therefore rapidly facing resource constraints. Here, we propose and demonstrate a demultiplexing approach that uses only a single active element for routing to, in principle, an arbitrary number of outputs. We employ our device in combination with a high-efficiency single-photon source based on a quantum dot, and measure up to eight demultiplexed highly indistinguishable single photons. We discuss the practical limitations of our approach, and describe in which conditions it can be used to demultiplex, e.g., tens of outputs. Our scheme thus provides a path for the preparation of resource-efficient larger-scale multi-photon sources.