Multiphoton Applications Research Articles

Deterministic photon source interfaced with a programmable silicon-nitride integrated circuit

We develop a quantum photonic platform that interconnects a high-quality quantum dot single-photon source and a low-loss photonic integrated circuit made in silicon nitride. The platform is characterized and programmed to demonstrate various multiphoton applications, including bosonic suppression laws and photonic entanglement generation. The results show a promising technological route forward to scale-up photonic quantum hardware.

Multi-Channel SPAD Chip for Silicon Photonics With Multi-Photon CoIncidence Detection

We present the design and characterization of a microelectronic chip consisting of 32 independent single-photon counting and multi-photon time-coincidence channels, based on Single Photon Avalanche Diodes (SPADs). The chip aims at easing the assembly together with Silicon Photonics substrates and chips, for a broad spectrum of quantum applications. More specifically we targeted the Quantum Random Number Generation by exploiting the randomness in the optical path of single photons through multi-channel waveguides. To this purpose, the chip provides not only 32 independent pulse outputs for multi-channel single-photon counting, but it features other two operation modalities. For single-photon applications, the chip provides the single-hit digital address of the channel detecting the photon among the 32 ones. For multi-photon applications, the chip provides an event-driven pulse every time more than n photons (n selectable between 2 and 4) concurrently trigger different channels. Each detection channel consists of 4 independent SPADs with different diameter (5 m, 10 m, 20 m, and 50 m), in order to easily match the waveguides and collection efficiency.

Ultrashort-pulsed optical parametric oscillator employing Brewster angle prism retroreflectors.

We demonstrate a synchronously-pumped optical parametric oscillator (OPO) cavity in which traditional dielectric mirrors are replaced by all-planar Brewster angle prism retroreflectors, also known as Pellin-Broca prisms. Exploiting total internal reflection, these prisms form a cavity supporting >350-fs chirped signal pulses that were externally compressible to sub-150-fs durations. This simple architecture produces wavelengths tuneable across 1100 - 1350 nm, suitable for basic multi-photon applications.

Halide perovskite nanocrystals for multiphoton applications.

Halide perovskite nanocrystals (NCs) are a unique class of NCs with novel properties distinct from those of traditional semiconductor NCs. These exceptional properties of defect tolerance, large absorption coefficients, high brightness, and narrow emission linewidths stem from their atypical band structure. Their facile synthesis and broad colour tunability have attracted widespread interest for application in light emitting devices and lasers. One fledging niche area is the field of multiphoton excited emission where their giant nonlinear optical action cross-sections are highly favorable for imaging applications. This Frontier article examines the state-of-the-art in perovskite NCs for multiphoton applications from the materials science and physics perspectives that include their synthesis and nonlinear optical characterization. Opportunities and challenges of these exceptional NCs as potential fluorescent labels for multiphoton deep tissue microscopy are also highlighted.

Demonstration of flat-top beam illumination in widefield multiphoton microscopy.

.Multiphoton microscopy provides a suitable technique for imaging biological tissues with submicrometer resolution. Usually a Gaussian beam (GB) is used for illumination, leading to a reduced power efficiency in the multiphoton response and vignetting for a square-shaped imaging area. A flat-top beam (FTB) provides a uniform spatial intensity distribution that equalizes the probability of a multiphoton effect across the imaging area. We employ a customized widefield multiphoton microscope to compare the performance of a square-shaped FTB illumination with that based on using a GB, for both two-photon fluorescence (TPF) and second-harmonic generation (SHG) imaging. The variation in signal-to-noise ratio across TPF images of fluorescent dyes spans for the GB and for the FTB illumination, respectively. For the GB modality, TPF images of mouse colon and Convallaria root, and SHG images of chicken tendon and human breast biopsy tissue showcase area that are not imaged due to either insufficient or lack of illumination. For quantitative analysis that depends on the illuminated area, this effect can potentially lead to inaccuracies. This work emphasizes the applicability of FTB illumination to multiphoton applications.

Comparing the performance of a femto fiber-based laser and a Ti:sapphire used for multiphoton microscopy applications.

Ti:sapphire laser systems are the more extended excitation sources in multiphoton (MP) microscopy. Although tunable, the cost, size, and lack of portability often limit their use in some research fields. Femtosecond fiber-based lasers represent an attractive alternative since they are portable, compact, and affordable. Most MP applications using these devices employ wavelengths beyond 1000 nm. This work evaluates the performance of a mode-locked fiber-based laser emitting at 780 nm (within the spectral region often used with Ti:sapphire devices) for use in MP imaging microscopy. MP images acquired with this laser system have been compared with those obtained with a "regular" solid-state source. Results herein show that the images recorded with both laser sources were similar, independently of the depth location of the imaged plane. The structural information contained in the images hardly differed. Moreover, the images of deeper layers improved by means of adaptive optics were also similar. These ultrafast laser sources are expected to enhance the impact of MP microscopy in basic research, as well as in biomedical environments.

Spectral multiplexing for scalable quantum photonics using an atomic frequency comb quantum memory and feed-forward control.

Future multiphoton applications of quantum optics and quantum information science require quantum memories that simultaneously store many photon states, each encoded into a different optical mode, and enable one to select the mapping between any input and a specific retrieved mode during storage. Here we show, with the example of a quantum repeater, how to employ spectrally multiplexed states and memories with fixed storage times that allow such mapping between spectral modes. Furthermore, using a Ti:Tm:LiNbO_{3} waveguide cooled to 3K, a phase modulator, and a spectral filter, we demonstrate storage followed by the required feed-forward-controlled frequency manipulation with time-bin qubits encoded into up to 26 multiplexed spectral modes and 97% fidelity.

Enhanced two-photon excitation through optical fiber by single-mode propagation in a large core.

Multiphoton excitation through optical fibers is limited by pulse broadening caused by self-phase modulation. We show that for short fiber lengths (approximately 2 m) two-photon excitation efficiency at the fiber output can be substantially improved by single-mode propagation in a large-area multimode fiber (10-microm core diameter) instead of a standard 5.5-microm core fiber. Measurements and numerical simulations of postfiber spectra and pulse widths demonstrate that the increase in efficiency is due to a reduction of nonlinear pulse broadening. Single-mode propagation in a large-core fiber is thus suitable for multiphoton applications for which pulse recompression is not possible at the fiber end.

Single line high efficiency tunable fir generation by resonant four-wave mixing in CH3 pumped by a multiatmosphere tunable CO2 laser

By pumping CH3F with a high pressure tunable TE-CO2 laser, the resonant four-wave mixing process (RFWM) generates a very efficient tunable single line FIR emission at the Raman frequency. This result is strictly related to the spectroscopic structure of the CH3F molecule. By means of this process, a tunable FIR emission on a 0.1 cm−1 bandwidth 150 kW (8 mJ) single line, is obtained which can be used for many FIR multiphoton applications.