This study investigates the use of 3-Aminopropyl triethoxy silane as a surface modifier for Cu-coated Carbon Fibers. The modified fibers were subsequently incorporated into Acrylonitrile Butadiene Styrene matrix composites through melt blending and high-temperature compression molding. The research evaluates the effect of 3-Aminopropyl triethoxy silane on the interfacial structure and mechanical performance of these composites. Results demonstrate a substantial enhancement in the wettability and surface energy of Cu-coated Carbon Fibers, with the static contact angle reduced from 111.2° to 84.5° and surface energy increased from 44.67 mN·m−1 to 56.66 mN·m−1. These surface modifications contributed to an 82.7 % increase in tensile strength and a 76.4 % improvement in tensile modulus of the resultant composites.