Surface Plasmon Polariton Modes Research Articles

A Tunable artificial plasmonic nanolaser with wide spectrum emission operating at room temperature

Abstract With information and communication technology developing fast, a key objective in the field of optoelectronic integrated devices is the reduction of nano-laser size and energy consumption. Photonics nanolasers are unable to exceed the diffraction limit and typically exhibit low modulation rates of several GHz. In contrast, plasmonic nanolaser utilize highly confined surface plasmon polariton (SPP) modes that can surpass diffraction limit and their strong Purcell effect can accelerate the modulation rates to several THz. Here, we propose a parametrically tunable artificial plasmonic nanolasers based on Metal-Insulator-Semiconductor-Insulator-Metal (MISIM) structure, which demonstrates the capability to compress the mode field volume to λ/14. As the pump power increases, the proposed artificial plasmonic nanolasers exhibits wide output spectrum of 20nm. Additionally, we investigate the impact of various cavity parameters on the nanolaser’s output threshold, offering potentials for realizing low-threshold artificial plasmonic nanolasers. Moreover, we observe a blue shift in the center wavelength of the nanolaser output with thinner gain layer thickness, predominantly attributed to the increased exciton–photon coupling strength. Our work brings inspiration to several areas, including Spaser-based interconnects, Nano-LEDs, spontaneous emission control, miniaturization of photon condensates, eigenmode engineering of plasmonic nanolasers, and optimal design driven by Artificial Intelligence (AI).

Ultra-high sensitivity surface plasmon U-channel photonic crystal fiber for hemoglobin sensing

In order to increase the wavelength response range of the U-channel sensor, a numerical study has been conducted and then the sensing structure has been optimized. A sensor in photonic crystal fiber (PCF) is proposed in which a layer of titanium dioxide is coated on the surface of the U-channel and then coated with a gold film. These two different metal films are mainly used to control the Surface plasmon resonance (SPR) peak and the corresponding resonance wavelength, thus changing the sensor performance. Just below the metal layer are two special air holes on either side. They form a leakage window in the center. In the following sections, the effects of these variables on the sensor will be studied in detail by COMSOL. The modal transmission characteristics of this fiber optic sensor are analyzed in this paper. By analyzing the obtained loss spectrum, the energy variation in the surface plasmon polariton (SPP) mode and the influence of the core mode on the sensing performance of the fiber optic sensor presented, the general rule of the optimized PCF-SPR sensor is deduced. In addition, we can make subtle adjustments to the sensor to improve its sensitivity. We found with the refractive index (RI) ranging from 1.26 to 1.42, the maximum wavelength sensitivity is 7500 nm/RIU, which corresponds to a full width at half maximum (FWHM) of 11.83 nm，a figure of merit (FOM) of 634.1 RIU−1. In addition, we also have discussed the sensor and different concentrations of hemoglobin aqueous solution to detect its RI. It is evident from the results that the sensor demonstrates excellent sensitivity and a wide detection range, which is highly desirable for practical diagnostic purposes. The potential of this sensor for clinical trials and its application to medical diagnostics is promising. Compared with complex traditional methods, the PCF has obvious advantages such as clear structure, simple manufacture, high sensitivity and strong environmental adaptability. Moreover, it has the advantage of wide wavelength response range and has a clear development prospect in the field of biochemical sensing. It has foreseeable potential practical value.

Enhanced Fiber Long‐Range Surface Plasmon Sensing Enabled by Resonance Coupling to Surface Plasmon Polaritons

A tunable fiber optic (FO) long‐range surface plasmon (LRSP) sensor with strong coupling is developed and demonstrated theoretically in this article. The sensor consists of a square lattice array of Ag nanodisks resting on the FO end face. Utilizing nanodisks with small diameters leads to the pronounced excitation of two distinct and independent resonant modes: surface plasmon polaritons (SPP) and LRSP. A systematic investigation is performed to evaluate the sensing performance and capabilities of the sensor, focusing on its bulk and surface sensitivity. Significantly, the LRSP mode demonstrates high sensitivity and favorable linearity in response to refractive index (RI) changes, with an exceptionally high figure of merit (FOM). On the contrary, the SPP mode is regarded as an ideal self‐referencing mode due to its immunity to RI fluctuations. The enlargement of nanodisks diameters results in a swift redshift in the LRSP wavelength, leading to a strong coupling with the SPP mode. This coupling facilitates the transfer of electric fields within the SPP mode, promotes sensing capabilities, and enables the realization of dual‐channel sensing functionality. The occurrence of strong coupling phenomena along with the use of FO substrates provides an innovative option for achieving multifunctionality and miniaturization in sensor platforms.

Transmission enhancement effect of distributed Bragg reflector structure covered with metal grating

In order to observe the extraordinary optical transmission (EOT) through a metal gratings, induced by Tamm plasmon polaritons (TPPs), a layered structure consisting of a distributed Bragg reflector covered with a one-dimensional metal grating is proposed in this work. When an incident light wave passes through DBR regime and impinges on the DBR-metal interface normally, the generation of TPPs and the resulting highly localized energy on the metal-DBR interface are simulated in detail by the finite element method. As a result, the surface plasmon polariton (SPPs) modes accommodated inside the slits of metal gratings can be excited more effectively by the enhanced electromagnetic field associated with TPPs located on the interface. Furthermore, the enhanced transmission of incident light waves in the structure can be achieved when the SPP mode inside the grating slits satisfies the Fabry-Perot (FP)-like resonance condition, which reveals that the EOT in this structure comes from a TPPs-FP hybrid resonance. This inference can be confirmed by the relationships between the central wavelength and the grating height for the two transmission peaks, and the magnetic field modal profiles associated with the two peaks. Quantitative effects of the slit width and duty cycle on the transmission peak of the metal grating are analyzed numerically, and the results demonstrate that when the period is determined, as the slits width increases, the two peak transmittances first increase and then decrease. On the other hand, when the slit widths are chosen to be 40 nm, 50 nm, and 60 nm respectively, the peak transmittance first increases and then decreases with the duty cycle increasing. Meanwhile, it is found that the center wavelengths of the transmission peaks are related to the duty cycle in a nearly linear manner for three slit widths, which can be used to flexibly adjust the center wavelength of extraordinary optical transmission.

Strongly polarized color conversion of isotropic colloidal quantum dots coupled to fano resonances.

Colloidal quantum dots (QDs) offer high color purity essential to high-quality liquid crystal displays (LCDs), which enables unprecedented levels of color enrichment in LCD-TVs today. However, for LCDs requiring polarized backplane illumination in operation, highly polarized light generation using inherently isotropic QDs remains a fundamental challenge. Here, we show strongly polarized color conversion of isotropic QDs coupled to Fano resonances of v-grooved surfaces compatible with surface-normal LED illumination for next-generation QD-TVs. This architecture overcomes the critically oblique excitation of surface plasmon coupled emission by using v-shapes imprinted on the backlight unit (BLU). With isotropic QDs coated on the proposed v-BLU surface, we experimentally measured a far-field polarization contrast ratio of ∼10. Full electromagnetic solution shows Fano line-shape transmission in transverse magnetic polarization allowing for high transmission as an indication for forward-scattering configuration. Of these QDs coupled to the surface plasmon-polariton modes, we observed strong modifications in their emission kinetics revealed by time-resolved photoluminescence spectroscopy and via dipole orientations identified by back focal plane imaging. This collection of findings indicates conclusively that these isotropic QDs are forced to radiate in a linearly polarized state from the patterned planar surface under surface-normal excitation. For next-generation QD-TVs, the proposed polarized color-converting isotropic QDs on such v-BLUs can be deployed in bendable electronic displays.

Quasi-bound states in the continuum in a metal nanograting metasurface for a high figure-of-merit refractive index sensor.

In this work, we investigate the bound states in the continuum (BICs) in a gold nanograting metal-insulator-metal metasurface structure at oblique angles of incidence. The nanograting metasurface consists of a gold nanograting patterned on a silicon dioxide dielectric film deposited on a thick gold film supported by a substrate. With rigorous full-wave finite difference time domain simulations, two bound states in the continuum are revealed upon transverse magnetic wave angular incidence. One BIC is formed by the interference between the surface plasmon polariton mode of the gold nanograting and the FP cavity mode. Another BIC mode is formed by the interference between the metal-dielectric hybrid structure guided mode resonance mode and the FP cavity mode. While true BIC modes cannot be observed, quasi-BIC modes are investigated at angles of incidence slightly off from the corresponding true BIC angles. It is shown that quasi-BIC modes can suppress radiation loss, resulting in narrow resonance spectral linewidths and high quality-factors. The quasi-BIC mode associated with the surface plasmon polariton mode is investigated for refractive index sensing. As a result, a high sensitivity refractive index sensor with a large figure-of-merit of 364 has been obtained.

Nanoscale Manipulation of Exciton-Trion Interconversion in a MoSe2 Monolayer via Tip-Enhanced Cavity-Spectroscopy.

Emerging light-matter interactions in metal-semiconductor hybrid platforms have attracted considerable attention due to their potential applications in optoelectronic devices. Here, we demonstrate plasmon-induced near-field manipulation of trionic responses in a MoSe2 monolayer using tip-enhanced cavity-spectroscopy (TECS). The surface plasmon-polariton mode on the Au nanowire can locally manipulate the exciton (X0) and trion (X-) populations of MoSe2. Furthermore, we reveal that surface charges significantly influence the emission and interconversion processes of X0 and X-. In the TECS configuration, the localized plasmon significantly affects the distributions of X0 and X- due to the modified radiative decay rate. Additionally, within the TECS cavity, the electric doping effect and hot electron generation enable dynamic interconversion between X0 and X- at the nanoscale. This work advances our understanding of plasmon-exciton-hot electron interactions in metal-semiconductor-metal hybrid structures, providing a foundation for an optimal trion-based nano-optoelectronic platform.

Bayesian optimization of periodic multilayered slabs for passive absorptivity control

A vanadium dioxide (VO2) film grown on a titanium oxide crystal shows a metal–insulator transition at room temperature with drastically changed optical properties. A multilayered slab with a sub-micron scale VO2 film was proposed to utilize its unique properties for passive intensity control of sunlight absorption and radiative cooling. Its optimal geometries were numerically explored using the Bayesian optimization (BO) method. BO was applied for three types of multilayered slabs, those having one, two, or three isolated slabs of different widths. For each type of multilayered slab, BO could optimize geometric variables with practical calculation times considering the total number of possible combinations of variables, which is subsequently referred to as the total number of candidates. Optimization results revealed that two isolated slabs had the most suitable spectral absorptivity in both hot and cold environments. The infrared absorptivity of the double slab was kept low in cold conditions to suppress radiative cooling. However, the double slab exhibited good radiative cooling performance under hot conditions. Electromagnetic energy density surrounding the slab illustrated that metallic VO2 and gold placed in a parallel manner excited the coupled mode of surface plasmon polaritons to enhance absorptivity. Radiative cooling faded for the triple slab because each slab could couple with radiation propagating only across a portion of the cross-sectional area. Through three BO trials, improvement of the VO2 visible reflectivity was recognized as a future issue for further development of passive sunlight absorption control.

Fabrication Process of Metal-Assisted Chemical Etched Curved Mirror Structure for Extracting Surface Plasmon Polariton Mode of Top-Emitting Organic LED

Fabrication Process of Metal-Assisted Chemical Etched Curved Mirror Structure for Extracting Surface Plasmon Polariton Mode of Top-Emitting Organic LED

High refractive index sensing highly sensitive and low loss SPR sensor based on hollow-core D-shaped optical fiber

A hollow-core D-shaped optical fiber-based surface plasmon resonance (SPR) sensor for low-loss and highly sensitive liquid analytes detection is theoretically investigated. The gold (Au) metal nanolayer is coated on the cladding etched D-shaped flat surface to develop the plasmonic effect. The nanolayer coating on the outer flat surface is very easy compared to the inside hollow-core, so our hollow-core sensor manufacturing is too easy compared to other hollow-core refractive indices (RIs) detection sensors. The resonance effect between analytes filled fundamental guided core mode and surface plasmon polariton mode of the D-shaped hollow-core optical fiber sensor is used to obtain the detections of analytes RIs variations. We have found good linear results ([Formula: see text]) in analytes RIs versus resonance wavelength for gold layers thicknesses for the analytes RIs range of 1.45–1.52. This hollow-core D-shaped optical fiber sensor achieves the maximum wavelength sensitivity of 23500[Formula: see text]nm RIU[Formula: see text] and a corresponding resolution of [Formula: see text] RIU. We have obtained the maximum figure of merit (FOM) of 228 1/RIU. The proposed sensor may be highly active in detecting the biological and chemical liquid analytes.

Dual‐polarised end‐fire antenna based on the high‐order mode of spoof surface plasmon polaritons

AbstractA planar antenna with dual‐linearly polarised end‐fire radiation is proposed. A tapered double‐sided symmetrical spoof surface plasmon polariton (SSPP) transmission line (TL) with tilted unit cells is proposed. The SSPP TL can operate in two types of first high‐order modes: the first high‐order even mode and the first high‐order odd mode. A two‐port feeding structure is designed to feed the SSPP TL. When the signal is fed from port 1, the energy travels through the substrate integrated waveguide and eventually excites the even mode on the SSPP TL, leading to vertically polarised radiation. Conversely, when the signal is input from port 2, the energy travels through the stripline‐to‐slotline transition and eventually excites the odd mode on the SSPP TL, generating horizontally polarised radiation. According to the measured results, a 54.6% overlapping bandwidth is obtained. The horizontal and the vertical polarisations achieve a maximum gain of 14.7 and 12.2 dBi, respectively.

Terahertz Generation through Coherent Excitation of Slow Surface Waves in an Array of Carbon Nanotubes

In this paper, we present a scheme for generating terahertz (THz) radiation using an array of parallel double-walled carbon nanotubes (DWCNTs) subjected to a direct current (DC). The longitudinal surface plasmon polaritons (SPPs) in the DWCNTs are coherently excited by two near-infrared laser beams with slightly different frequencies. Through numerical methods, we investigate the spectral characteristics of the SPPs in the presence of a DC current in the nanotubes. We identify high-quality plasmonic modes with a slowdown factor exceeding 300 in the terahertz frequency region. The amplification of these slow SPP modes is facilitated by the DC current in the DWCNTs, fulfilling a synchronism condition. This condition ensures that the phase velocity of the SPPs is closely matched to the drift velocity of the charge carriers, allowing for an efficient energy exchange between the current and the surface electromagnetic wave. The high-frequency currents on the nanotube walls in the DWCNT array enable the emission of THz radiation into the far field, owing to an antenna effect.

Dynamic construction of refractive index-dependent vibrations using surface plasmon-phonon polaritons

One of the fundamental hurdles in infrared spectroscopy is the failure of molecular identification when their infrared vibrational fingerprints overlap. Refractive index (RI) is another intrinsic property of molecules associated with electronic polarizability, but with limited contribution to molecular identification in mixed environments currently. Here, we investigate the coupling mode of localized surface plasmon and surface phonon polaritons for vibrational de-overlapping. The coupling mode is sensitive to the molecular refractive index, attributed to the RI-induced vibrational variations of surface phonon polaritons (SPhP) within the Reststrahlen band, referred to as RI-dependent SPhP vibrations. The RI-dependent SPhP vibrations are linked to molecular RI features. According to the deep-learning-augmented demonstration of bond-breaking-bond-making dynamic profiling in biological reaction, we substantiate that the RI-dependent SPhP vibrations effectively disentangle overlapping vibrational modes, achieving a 92% identification accuracy even for the strongly overlapping vibrational modes in the reaction. Our findings offer insights into the realm of light-matter interaction and provide a valuable toolkit for biomedicine applications.

Optimization of a Weyl-semimetal-based near-field heat transfer system

Near-field radiative heat transfer (NFRHT) is inherently limited by Lorentz reciprocity, which can be partially mitigated through the application of an external magnetic field. However, recent studies have discovered that Weyl semimetals (WSMs) possess the ability to achieve nonreciprocal surface plasmon polariton modes without relying on an external magnetic field. Building upon the nonreciprocal nature of WSMs, this study investigates NFRHT between two WSM slabs and compares different WSM materials. The primary focus of the comparison lies in analyzing the heat flux under varying emitter and receiver temperatures. Three of the selected WSM materials exhibit similar performance in NFRHT, showing sensitivity to a decrease in the receiver temperature due to their low dielectric tensor components. In contrast, Eu2IrO7 displays distinctive characteristics, being sensitive to changes in the emitter temperature as a result of its higher dielectric tensor components. Additionally, a reassessment of the nonreciprocity in Co2MnGa, Eu2IrO7 and Co3Sn2S2 is conducted. Furthermore, Bayesian optimization algorithms are employed to optimize parameters and address the challenge of low thermal radiation observed in existing WSM NFRHT systems. The results highlight the achievement of an optimal WSM material that achieves an impressive heat flux of 5.29 × 108 (W/m2) at an emitter temperature of 310 K and a receiver temperature of 290 K. Notably, this heat flux surpasses that of Co2MnGa by 2.5 times in the context of NFRHT. The discoveries presented in this study promises to offer practical implications for the development of nonreciprocal thermal energy management systems.

Crossed grating sensing refractive index change in the non-laboratory environment.

Surface plasmon polaritons (SPPs) have been widely applied to refractive index (RI) sensing for their extremely high sensitivity to the surrounding RI change. Many efforts have been devoted to narrowing the linewidth of the SPP mode and enhancing the sensitivity of SPP sensors. However, most reported SPP-based RI sensing platforms could only operate in a laboratory environment for their bulky volume or sophisticated measuring systems. In this context, we have developed a miniaturized and portable RI sensing platform based on a 2D crossed grating coupled SPP sensor that can work under a non-laboratory environment. The crossed grating is fabricated by the laser interference lithography (LIL) method, which is cost-effective and reproductive. A series of glucose solutions with different concentrations have been used as analytes to verify the sensing performance of the fabricated crossed grating.

Exploring plasmonic effect on exciton transport: A theoretical insight from macroscopic quantum electrodynamics.

Exciton transport in extended molecular systems and how to manipulate such transport in a complex environment are essential to many energy and optical-related applications. We investigate the mechanism of plasmon-coupled exciton transport by using the Pauli master equation approach, combined with kinetic rates derived from macroscopic quantum electrodynamics. Through our theoretical framework, we demonstrate that the presence of a silver nanorod induces significant frequency dependence in the ability of transporting exciton through a molecule chain, indicated by the exciton diffusion coefficient, due to the dispersive nature of the silver dielectric response. Compared with the same system in vacuum, great enhancement (up to a factor of 103) in the diffusion coefficient can be achieved by coupling the resonance energy transfer process to localized surface plasmon polariton modes of the nanorod. Furthermore, our analysis reveals that the diffusion coefficients with the nearest-neighbor coupling approximation are ∼10 times smaller than the results obtained beyond this approximation, emphasizing the significance of long-range coupling in exciton transport influenced by plasmonic nanostructures. This study not only paves the way for exploring practical approaches to study plasmon-coupled exciton transport but also provides crucial insights for the design of innovative plasmon-assisted photovoltaic applications.

Broadband unidirectional surface plasmon polaritons with low loss.

Unidirectional surface plasmon polaritons (SPPs) have been proven to truly exist at an interface between a magnetized semiconductor and an opaque isotropic material, however, they suffer rather serious leakage loss (with propagation length shorter than two wavelengths) caused by nonlocality. In this work, we investigate an alternative category of unidirectional SPPs existing on a nonreciprocal plasmonic platform with a cladding composed of a dielectric heterostructure transversely terminated by metal. This unidirectional SPP mode exists for small wavenumbers within the entire upper bulk-mode bandgap of the magnetized semiconductor, hence it is robust against nonlocal effects over a broad band. In contrast to previous unidirectional SPPs, the leakage loss of the present unidirectional SPPs is significantly reduced by more than five times, since the portion of modal energy distributed in the cladding is substantially increased. A similar reduction in absorption losses associated with semiconductor dissipation is observed. Though the nonlocality induces a backward-propagating SPP with extremely large wavenumbers, it can be suppressed even at very small level of dissipation. Therefore, our proposed plasmonic waveguide actually exhibits exceptional unidirectional characteristics.

Photon recycling in organic semiconductor films using plasmonic metasurfaces

Photon recycling (PR) is a type of iterative self-absorption and re-emission by semiconductors. It plays an important but often-overlooked role in the performance of semiconductor optoelectronic devices. Additionally, it has not previously been investigated in the case of organic semiconductors, despite their propensity to exhibit for self-absorption. In this work, we study PR in thin films of three different organic semiconducting polymers on a variety of different surfaces to investigate the role of PR on the emission from the films. We show that PR is strongly affected by the substrate surface type and the morphology of the semiconductor. Silver grating-based metasurfaces and symmetric dielectric waveguides increase PR by up to a factor of 1.72 in all organic thin films compared to those on planar silver surfaces. However, polymer films with significant surface roughness do not show strong PR effects due to reduced guiding of emission in the plane of the film. Additionally, the luminescence quantum yield of all polymers is enhanced by both silver nanoparticle- and grating-based metasurfaces (by up to factors of 1.7 and 1.5, respectively) compared to the planar silver surfaces. This is attributed to the Purcell effect and improved extraction of emission coupled to surface plasmon polariton (SPP) modes. This study demonstrates that PR can be achieved in organic semiconductors, and it is strongest for surfaces and structures that promote both high quantum yield and in-plane waveguiding at the semiconductor emission wavelength.

Dual-core-enhanced surface plasmon resonance for sensing high refractive index liquid based on photonic crystal fiber

A dual-core photonic crystal fiber sensor based on surface plasmon resonance is theoretically proposed for the high-sensitive detection of high refractive index liquid analytes. Dual-core construction can effectively enhance the coupling effect between the fiber-core mode and the surface plasmon polariton modes, leading to sharp loss peaks at the resonance wavelengths. As the refractive index of the targeted analyte varies, the resonance condition will change as well and cause a certain shift of loss peak. Numeric results show that this dual-core fiber sensor exhibits an average linear sensitivity 9538 nm/RIU and a maximum sensitivity is 11400 nm/RIU with a resolution 8.77 × 10−6 RIU. The detected range is broad and covers the high refractive index range from 1.45 to 1.58 with an average figure of merit 284.5 RIU−1. The dependence of structure parameters and the thickness of coated-metal thin-film on sensing performance is performed systemically and suggests different responses. The proposed sensor is highly promising in detecting high refractive index liquid analytes in the fields of biological detection, environmental monitoring and chemical analysis.

Compact effective surface plasmon polariton transmission line with undiminished bandwidth and enhanced field confinement.

In this work, we propose a compact effective surface plasmon polariton (CESPP) transmission line (TL) based on a structural dispersion-induced surface plasmon polaritons (SPPs) mode, which can enhance confinement while ensuring that the working bandwidth is not reduced. The dispersion relation of the CESPPs proposed in this article indicates that the shallower the groove, the stronger the confinement. Furthermore, the CESPPs may facilitate longitudinal miniaturization, since the configuration of the unit cell is simple. The coupling effect between two CESPP TLs has been well studied, revealing that excellent cross talk suppression can be achieved. The measurement results exhibit strong agreement with full-wave simulations, suggesting that the proposed CESPP TL holds significant potential for valuable applications in modern high-speed circuits.