A temperature-dependent anisotropic material model for use in a coupled thermo-mechanical finite element analysis of the forming of aluminum sheets was developed. The anisotropic properties of the aluminum alloy sheet AA3003-H111 were characterized for a range of temperatures 25–260 °C (77–500 °F) and for different strain rates. Material hardening parameters (flow rule) and plastic anisotropy parameters ( R 0, R 45 and R 90) were calculated using standard ASTM uniaxial tensile tests. From this experimental data, the anisotropy coefficients for the Barlat YLD96 yield function [Barlat, F., Maeda, Y., Chung, K., Yanagawa, M., Brem, J.C., Hayashida, Y., Lege, D.J., Matsui, K., Murtha, S.J., Hattori, S., Becker, R.C., Makosey, S., 1997a. Yield function development for aluminum alloy sheets. J. Mech. Phys. Solids 45 (11/12), 1727–1763] in the plane stress condition were calculated for several elevated temperatures. Curve fitting was used to calculate the anisotropy coefficients of Barlat’s YLD96 model and the hardening parameters as a function of temperature. An analytical study of the accuracy and usability of this curve fitting technique is presented through the calculation of plastic anisotropy R-parameters and yield function plots at different temperatures.