Mode-locked Thin-disk Oscillator Research Articles

Intra-oscillator high harmonic source reaching 100-eV photon energy

Resonant enhancement inside an optical cavity has been a wide-spread approach to increase efficiency of nonlinear optical conversion processes while reducing the demands on the driving laser power. This concept has been particularly important for high harmonic generation XUV sources, where passive femtosecond enhancement cavities allowed significant increase in repetition rates required for applications in photoelectron spectroscopy, XUV frequency comb spectroscopy, including the recent endeavor of thorium nuclear clock development. In addition to passive cavities, it has been shown that comparable driving conditions can be achieved inside mode-locked thin-disk laser oscillators, offering a simplified single-stage alternative. This approach is less sensitive to losses thanks to the presence of gain inside the cavity and should thus allow higher conversion efficiencies through tolerating higher intensity in the gas target. Here, we show that the intra-oscillator approach can indeed surpass the much more mature technology of passive enhancement cavities in terms of XUV flux, even reaching comparable values to single-pass sources based on chirped-pulse fiber amplifier lasers. Our system operates at 17 MHz repetition rate generating photon energies between 60 eV and 100 eV. Importantly, this covers the highly attractive wavelength for the silicon industry of 13.5 nm at which our source delivers 60 nW of outcoupled average power per harmonic order.

Self-started Kerr-lens mode-locked thin-disk oscillator.

Kerr-lens mode-locking (KLM) has been widely used in thin-disk oscillators to generate high-power femtosecond pulses. Here we demonstrate a Kerr-lens mode-locked Yb:YAG thin-disk oscillator that can be self-started under two configurations. The first can deliver 13-W, 235-fs pulses at a repetition rate of 103 MHz; the second delivers 49 W at a repetition rate of 46.5 MHz, whose corresponding pulse energy of 1.05 µJ is, to the best of our knowledge, the highest energy ever obtained in self-started Kerr-lens mode-locked oscillators. A new method to initiate KLM in the form of optical perturbation in a thin-disk oscillator has also been demonstrated.

110 MW thin-disk oscillator.

A compact Kerr-lens mode-locked thin-disk oscillator reproducibly delivering 110 MW output peak power, the highest among all oscillators, is reported. This simple and stable femtosecond oscillator delivering a unique combination of high average power (202 W) and peak power, is an ideal driver and an important milestone for the development of extreme ultraviolet transportable frequency comb sources.

Sub-100-fs Kerr-lens mode-locked Yb:YAG ring-cavity thin-disk oscillator.

Ultrafast ring-cavity thin-disk oscillators combine high output power with the flexibility of generating output either unidirectionally or bidirectionally. Here, we report a Kerr-lens mode-locked ring-cavity Yb:YAG thin-disk oscillator delivering unidirectional 89-fs pulses by inducing additional spectral broadening with nonlinear plates. This is the shortest pulse duration for a ring-cavity mode-locked thin-disk oscillator. Bidirectional mode-locking was also realized. These results lay the foundation for the more efficient generation of high-order harmonics at MHz repetition rates and high-power dual frequency combs.

High-efficiency 100-W Kerr-lens mode-locked Yb:YAG thin-disk oscillator

We demonstrate a Kerr-lens mode-locked femtosecond Yb:YAG thin-disk oscillator and investigate the approach to increase the optical-to-optical efficiency based on the scheme of direct multiple passes of the laser beam through the thin-disk medium. With twelve passes through the thin disk, 266-fs pulses were delivered from the oscillator with an average power of 105.6 W at a repetition rate of 20 MHz. The corresponding optical-to-optical efficiency is 31.1%, which is, to the best of our knowledge, the highest efficiency of any mode-locked thin-disk oscillator with pulse duration below 300 fs. This demonstration paves the way to even more efficient mode-locked femtosecond thin-disk oscillators, and provides an excellent laser source for the applications such as non-linear frequency conversion and high-precision industrial processing.

Influence of disk aberrations on high-power thin-disk laser cavities.

We present a systematic study on the influence of thin-disk aberrations on the performance of thin-disk laser oscillators. To evaluate these effects, we have developed a spatially resolved numerical model supporting arbitrary phase profiles on the intracavity components that estimates the intracavity beam shape and the output power of thin-disk laser oscillators. By combining this model with the experimentally determined phase profile of the thin-disk (measured with interferometry), we can predict the operation mode of high-power thin-disk lasers, including mode degradation, higher-order mode coupling, and stability zone shrinking, all of which are in good agreement with experiment. Our results show that one of the main mechanisms limiting the performance is the small deviation of the disk's phase profile from perfect radial symmetry. This result is an important step to scaling modelocked thin-disk oscillators to the kW-level and will be important in the design of future active multi-pass cavity arrangements.

High-power modelocked thin-disk oscillators as potential technology for high-rate material processing.

High average power femtosecond lasers have made spectacular progress in the last decades – moving from laboratory-based systems with maximum average powers of tens of watts to kilowatt-class mature industrial systems in a short time. The availability of such systems opens new possibilities in many fields; one of the most prominent ones that have driven many of these technological advances is precise high-speed material processing, where ultrashort pulses have long been recognized to provide highest precision processing of virtually any material, and high average power extends these capabilities to highest processing rates. Here, we focus our attention on one high-average power technology with large unexplored potential for this specific application: directly modelocked multi-MHz repetition frequency high-power thin-disk oscillators. We review their latest state-of-the-art and discuss future directions and challenges, specifically with this application field in mind.

SESAM mode-locked Yb:YAB thin-disk oscillator delivering an average power of 19 W

We report on a semiconductor saturable absorber mirror mode-locked thin-disk oscillator based on Yb:YAB delivering pulses with a duration of 462 fs at an average output power of 19.2 W and a pulse energy of 0.38 µJ.

Increasing the efficiency of the intra-cavity generation of ultra-short radially polarized pulses in thin-disk resonators with grating waveguide structures

In this paper, we report on the investigation of two different approaches based on grating waveguide structures (GWS) to generate radially polarized ultra-short pulses in thin-disk laser resonators. In previously reported mode-locked thin-disk oscillators emitting radially polarized pulses, a partly reflective GWS was employed as an outcoupling element for polarization shaping. This partly reflective GWS introduced significant losses for the outcoupled radiation, resulting in a reduced optical efficiency. The aim of the investigations presented here is to explore the possibility of improving the optical efficiency by using a highly reflective GWS in different resonator configurations, which circumvents the loss port present for the partly reflective GWS. The investigations show that using a highly reflective GWS as a folding mirror of the resonator enables a significant improvement of the optical efficiency compared to the previously reported configurations.

Single-cycle, MHz repetition rate THz source with 66 mW of average power.

We demonstrate terahertz (THz) generation using the tilted pulse front method in lithium niobate, driven at an unprecedented high average power of more than 100 W and at a 13.3 MHz repetition rate, provided by a compact amplifier-free mode-locked thin-disk oscillator. The conversion efficiency was optimized with respect to the pump spot size and pump pulse duration, enabling us to generate a maximum THz average power of 66 mW, which is, to the best of our knowledge, the highest reported to date from a laser-driven, few-cycle THz source. Furthermore, we identify beam walk-off as the main obstacle that currently limits the conversion efficiency in this excitation regime (with moderate pulse energies and small spot sizes). Further upscaling to the watt level and beyond is within reach, paving the way for linear and nonlinear high average power THz spectroscopy experiments with an exceptional signal-to-noise ratio at megahertz repetition rates.

Milliwatt-class broadband THz source driven by a 112 W, sub-100 fs thin-disk laser.

We demonstrate a high repetition-rate, single-cycle THz source with a maximum average power of 1.35 mW, operating at a center frequency of 2 THz. This result was obtained by optical rectification (OR) in GaP using an amplifier-free, nonlinearly compressed modelocked thin-disk oscillator based on Yb:YAG, delivering 8.4 µJ pulses with 88 fs duration at a repetition rate of 13.4 MHz, resulting in driving pulses for OR with 112 W average power and 80 MW peak power. To the best of our knowledge, our result represents the highest average power so far achieved with OR in GaP. The demonstrated performance is very attractive for improving current linear THz time-domain spectroscopy experiments, which are currently restricted by low signal-to-noise ratio and long measurement times.

Kerr-lens mode-locked thin-disk oscillator with 50% output coupling rate.

Several approaches to power scaling of mode-locked thin-disk oscillators exist. One of these approaches is based on the increased gain provided by multiple passes through the thin-disk laser medium. For the first time, to the best of our knowledge, we applied this approach to a Kerr-lens mode-locked thin-disk oscillator. The so obtained additional gain allowed mode-locked operation with up to 50% output coupling rate. This first demonstration is of particular importance for gain media with inherently low-emission cross sections and paves the way to even more powerful Kerr-lens mode-locked thin-disk oscillators. Moreover, the experimental results indicate an increased self-amplitude modulation related to an overall increase in the soft-aperture Kerr-lens effect.

Efficient nonlinear compression of a mode-locked thin-disk oscillator to 27 fs at 98 W average power.

We demonstrate efficient pulse compression of a 13.4MHz, 534fs, 123W, Yb:YAG thin-disk oscillator down to 27fs at 98W average power, resulting in a record-high 166MW peak power from an amplifier-free oscillator-driven setup. Our compressor is based on two stages: one multipass cell allowing us to reduce the pulse duration to sub-90fs and, subsequently, a multiple-plate compressor, allowing us to reach 27fs. The overall average power compression efficiency is 80%, and the beam has excellent beam quality and homogeneity. In addition, we demonstrate further spectral broadening that supports a transform limit of 5fs in a second multiple-plate stage, demonstrating the potential for reaching a 100W class, amplifier-free, few-cycle source in the near future. The performance of this unique source is very promising for applications previously restricted to amplified sources, such as efficient generation of extreme ultraviolet light at high repetition rate, and the generation of high-power broadband THz radiation.

Optical rectification of a 100 W average power mode-locked thin-disk oscillator.

We demonstrate terahertz (THz) generation at megahertz repetition rate by optical rectification in GaP crystals, using excitation average power levels exceeding 100 W. The laser source is a state-of-the-art diode-pumped Yb:YAG SESAM-mode-locked thin-disk laser, capable of generating 580 fs pulses at an average power up to 120 W and a repetition rate of 13.4 MHz directly from a one-box oscillator, without the need for any extra amplification stages. In this first demonstration, we measure a maximum THz average power of 78 μW at a central frequency of 0.8 THz. Our results show that optical rectification of state-of-the-art high average power ultrafast sources in nonlinear crystals is within reach and paves the way toward high average power, ultrafast laser pumped THz sources.

Radially polarized passively mode-locked thin-disk laser oscillator emitting sub-picosecond pulses with an average output power exceeding the 100 W level.

We report on a high-power passively mode-locked radially polarized Yb:YAG thin-disk oscillator providing 125 W of average output power. To the best of our knowledge, this is the highest average power ever reported from a mode-locked radially polarized oscillator without subsequent amplification stages. Mode-locking was achieved by implementing a SESAM as the cavity end mirror and the radial polarization of the LG*01 mode was obtained by means of a circular Grating Waveguide Output Coupler. The repetition rate was 78 MHz. A pulse duration of 0.97 ps and a spectral bandwidth of 1.4 nm (FWHM) were measured at the maximum output power. This corresponds to a pulse energy of 1.6 µJ and a pulse peak power of 1.45 MW. A high degree of radial polarization of 97.3 ± 1% and an M2-value of 2.16 which is close to the theoretical value for the LG*01 doughnut mode were measured.

Multi-mW, few-cycle mid-infrared continuum spanning from 500 to 2250\u2009cm\u22121

The demand for and usage of broadband coherent mid-infrared sources, such as those provided by synchrotron facilities, are growing. Since most organic molecules exhibit characteristic vibrational modes in the wavelength range between 500 and 4000 cm−1, such broadband coherent sources enable micro- or even nano-spectroscopic applications at or below the diffraction limit with a high signal-to-noise ratio1, 2, 3. These techniques have been applied in diverse fields ranging from life sciences, material analysis, and time-resolved spectroscopy. Here we demonstrate a broadband, coherent and intrinsically carrier-envelope-phase-stable source with a spectrum spanning from 500 to 2250 cm−1 (−30 dB) at an average power of 24 mW and a repetition rate of 77 MHz. This performance is enabled by the first mode-locked thin-disk oscillator operating at 2 μm wavelength, providing a tenfold increase in average power over femtosecond oscillators previously demonstrated in this wavelength range4. Multi-octave spectral coverage from this compact and power-scalable system opens up a range of time- and frequency-domain spectroscopic applications.

Extreme ultraviolet light source at a megahertz repetition rate based on high-harmonic generation inside a mode-locked thin-disk laser oscillator.

We demonstrate a compact extreme ultraviolet (XUV) source based on high-harmonic generation (HHG) driven directly inside the cavity of a mode-locked thin-disk laser oscillator. The laser is directly diode-pumped at a power of only 51 W and operates at a wavelength of 1034 nm and a 17.35 MHz repetition rate. We drive HHG in a high-pressure xenon gas jet with an intracavity peak intensity of 2.8×1013 W/cm2 and 320 W of intracavity average power. Despite the high-pressure gas jet, the laser operates at high stability. We detect harmonics up to the 17th order (60.8 nm, 20.4 eV) and estimate a flux of 2.6×108 photons/s for the 11th harmonic (94 nm, 13.2 eV). Due to the power scalability of the thin-disk concept, this class of compact XUV sources has the potential to become a versatile tool for areas such as attosecond science, XUV spectroscopy, and high-resolution imaging.

Powerful 100-fs-scale Kerr-lens mode-locked thin-disk oscillator.

We have recently demonstrated a simple power scaling procedure for Kerr-lens mode-locked thin-disk oscillators. Here we report on the extension of this scheme to a broadband high-peak-power thin-disk oscillator, delivering 140-fs pulses with a peak and average power of 62MW and 155W, respectively. This result shows that reaching the emission bandwidth of the gain material in Kerr-lens mode-locked thin-disk oscillators is feasible without sacrificing output power, efficiency, or stability by relying on high intracavity nonlinearities.

All solid-state spectral broadening: an average and peak power scalable method for compression of ultrashort pulses.

Spectral broadening in bulk material is a simple, robust and low-cost method to extend the bandwidth of a laser source. Consequently, it enables ultrashort pulse compression. Experiments with a 38 MHz repetition rate, 50 W average power Kerr-lens mode-locked thin-disk oscillator were performed. The initially 1.2 μJ, 250 fs pulses are compressed to 43 fs by means of self-phase modulation in a single 15 mm thick quartz crystal and subsequent chirped-mirror compression. The losses due to spatial nonlinear effects are only about 40 %. A second broadening stage reduced the Fourier transform limit to 15 fs. It is shown that the intensity noise of the oscillator is preserved independent of the broadening factor. Simulations manifest the peak power scalability of the concept and show that it is applicable to a wide range of input pulse durations and energies.

Carrier-envelope-phase stabilization via dual wavelength pumping.

A power-scalable concept for carrier-envelope-phase stabilization is presented. It takes advantage of simultaneous pumping of the zero- and first-phonon absorption line of Yb:YAG at 969 and 940 nm. The concept was implemented to lock the carrier-envelope-offset frequency of a 45 W average power Kerr-lens mode-locked thin-disk oscillator. The lock performance is compared to previous experiments where carrier-envelope-stabilization was realized by means of cavity loss modulation.