In this study, the Mg 58Cu 29.5Y 6Nd 5Ag 1.5 bulk metallic glasses (BMGs) with superior glass forming ability are made by Cu-mold casting and injection casting processes. Critical rod size of the Mg 58Cu 29.5Y 6Nd 5Ag 1.5 BMGs (base alloys) reached ∼4 mm in diameter. The results of Vickers indentation and compression tests of Mg 58Cu 29.5Y 6Nd 5Ag 1.5 alloy reveal that the mechanical performance of the BMG base alloy is brittle. The highest fracture toughness and plastic strain of the base alloy are only ∼9 MPa m 1/2 and ∼0%, respectively. SEM observation is followed after the mechanical properties tests. It showed that the dominant patterns of the fracture surface are the featureless mirror-like and river-like regions. For enhancing the mechanical properties of the base alloys, porous Mo particles are added to form Mg 58Cu 29.5Y 6Nd 5Ag 1.5–Mo BMG composites (BMGCs). It is found that the fracture toughness and the fracture strength of the 30 vol.% Mo particles reinforced Mg 58Cu 29.5Y 6Nd 5Ag 1.5 BMGCs is promoted to ∼50 MPa m 1/2 and ∼1100 MPa. The observation of the fracture surface of Mg 58Cu 29.5Y 6Nd 5Ag 1.5–30 vol.% Mo BMG composite via the compression test reveals that the shear bands and cracks propagation is resisted by the dispersion of Mo particles and secondary shear bands are formed during the plastic deformation. It is also observed that the fracture surface is occupied by vein-like pattern, instead of mirror-like region. Moreover, the plastic strain of the Mg 58Cu 29.5Y 6Nd 5Ag 1.5–30 vol.% Mo BMG composite increased to ∼29%.