The study deals with the manufacture of so-called fly-eye mirror in EUV lithography by means of an ultraprecision 5-axis control milling. It is extremely difficult to manufacture a highly accurate fly-eye mirror by conventional methods such as photolithography, mechanical cutting by a lathe and so on since it consists of 500 circular arc mirror elements of 15 mm in length and 1 mm in width having a spherical surface of 660 mm in radius and there are minute steps among them. ln order to manufacture fly-eye mirror with high accuracy and efficiency, the study proposes two new machining methods to manufacture spherical surface by employing a rotational single-crystal diamond tool. 0ne is to use a sphere type tool with circular arc cutting edge of 660 mm in radius. The rotation of the cutting tool forms a convex spherical surface of 600 mm in radius within a circle of 1 mm in diameter. The movement of the cutting tool along the circular arc of a mirror elements makes it possible to machine fly-eye mirror elements. Though the method is theoretically efficient, it is found that it is not practical due to the difficulty of manufacturing the tool accurately. The other is to use a flat type tool with the cutting edge angle of 90 degree. The tool enables to manufacture spherical surfaces with any radius by feeding it along the mirror surface and bears practical use because the cutting method is independent of tool form accuracy. Machining experiment was conducted by use of the latter tool. The machined circular are mirror elements of oxgen-free copper show smooth spherical surface and required steps among them without any burrs. lt is found that the proposed method has the potential of producing the fly-eye mirror correctly.