We examine a strategy for using neutral current measurements in long-baseline neutrino oscillation experiments to put limits on the existence of more than three light, active neutrinos. We determine the relative contributions of statistics, cross-section uncertainties, event misidentification and other systematic errors to the overall uncertainty of these measurements. As specific case studies, we make simulations of beams and detectors that are like the K2K, T2K and MINOS experiments. We find that the neutral current cross-section uncertainty and contamination of the neutral current signal by charge current events allow a sensitivity for determining the presence of sterile neutinos at the 0.10–0.15 level in probablility.