Microphysical Measurements Research Articles

Evaporative and Radiative Cooling in POST Stratocumulus

Abstract Buoyancy reversal by evaporative cooling in entrainment holes has a minimal influence on stratocumulus (Sc) observed during the Physics of Stratocumulus Top (POST) aircraft field study held off the California coast in 2008. High-resolution temperature and microphysics measurements show only small differences for Sc with and without buoyancy reversal predicted by mixing fraction analysis that relates mixtures of cloudy air and free-atmospheric air to buoyancies of the mixtures. The reduction of LWC due to evaporation in the holes is a small percentage (average ~12%) of liquid water diluted in the Sc by entrainment from the entrainment interface layer (EIL) located above unbroken cloud top where most mixing, evaporation, and reduction of the large buoyancy jump between the cloud and free atmosphere occur. Entrainment is dominated by radiative cooling at cloud top.

Impact of different IFS microphysics on a warm conveyor belt and the downstream flow evolution

The influence of microphysical processes on the upper‐level flow features associated with an extratropical cyclone is investigated with the ECMWF global atmospheric model. A control simulation with the model version operational at ECMWF during 2014/early 2015 and a simulation with new parametrizations of rain autoconversion/accretion, rain evaporation and snow riming operational since May 2015 are compared in detail. In order to investigate the impact of each microphysical process separately, the diabatic heating rate for each microphysical process and the associated change in potential vorticity (PV) is calculated and compared for the two simulations. The influence on the upper‐level ridge building and the downstream flow evolution is investigated. The changes in the microphysical parametrization led to differences in the position of the warm conveyor belt (WCB) outflow. The WCB reaches the upper troposphere with low PV values and shifts the location of the tropopause in a slightly different way in the two simulations. Although these differences are relatively small at the beginning, they are advected downstream and amplify, leading to distinct differences in the upper‐level PV pattern. These results highlight the importance of correct representation of microphysical processes for large‐scale flow features. Additionally they emphasise the need for detailed microphysical measurements in extratropical cyclones in order to better understand and constrain the microphysical processes in NWP models.

Spectral optical layer properties of cirrus from collocated airborne measurements and simulations

Abstract. Spectral upward and downward solar irradiances from vertically collocated measurements above and below a cirrus layer are used to derive cirrus optical layer properties such as spectral transmissivity, absorptivity, reflectivity, and cloud top albedo. The radiation measurements are complemented by in situ cirrus crystal size distribution measurements and radiative transfer simulations based on the microphysical data. The close collocation of the radiative and microphysical measurements, above, beneath, and inside the cirrus, is accomplished by using a research aircraft (Learjet 35A) in tandem with the towed sensor platform AIRTOSS (AIRcraft TOwed Sensor Shuttle). AIRTOSS can be released from and retracted back to the research aircraft by means of a cable up to a distance of 4 km. Data were collected from two field campaigns over the North Sea and the Baltic Sea in spring and late summer 2013. One measurement flight over the North Sea proved to be exemplary, and as such the results are used to illustrate the benefits of collocated sampling. The radiative transfer simulations were applied to quantify the impact of cloud particle properties such as crystal shape, effective radius reff, and optical thickness τ on cirrus spectral optical layer properties. Furthermore, the radiative effects of low-level, liquid water (warm) clouds as frequently observed beneath the cirrus are evaluated. They may cause changes in the radiative forcing of the cirrus by a factor of 2. When low-level clouds below the cirrus are not taken into account, the radiative cooling effect (caused by reflection of solar radiation) due to the cirrus in the solar (shortwave) spectral range is significantly overestimated.

LABEX L-IPSL Arctic Metadata Portal

The Institut Pierre Simon Laplace (IPSL) encompasses a wide diversity of projects that focus on the Arctic. From these observations the IPSL has generated a large number of datasets gathering Arctic observations. These observations include measurements on atmospheric chemical composition, snow micro-physical properties or ocean measurements. However, some of these datasets remain locally stored and there is a lack of public awareness regarding these resources, which has hindered their visualisation and sharing. This motivated the creation of the LABEX L-IPSL Arctic metadata Portal ( http://climserv.ipsl.polytechnique.fr/arcticportal/ ), presented here, which improves the visibility of the variety of observations collected within the institute as well as the evaluation of numerical models. The LABEX L-IPSL Arctic metadata Portal will also promote new avenues in Arctic research within the IPSL and with other collaborating institutions.

COMMIT in 7-SEAS/BASELInE: Operation of and Observations from a Novel, Mobile Laboratory for Measuring In-Situ Properties of Aerosols and Gases

Trace gases and aerosols (particularly biomass-burning aerosols) have important implications for air quality and climate studies in Southeast Asia (SEA). This paper describes the purpose, operation, and datasets collected from NASA Goddard Space Flight Center’s (NASA/GSFC) Chemical, Optical, and Microphysical Measurements of In-situ Troposphere (COMMIT) laboratory, a mobile platform designed to measure trace gases and optical/microphysical properties of naturally occurring and anthropogenic aerosols. More importantly, the laboratory houses a specialized humidification system to characterize hygroscopic growth/enhancement, a behavior that affects aerosol properties and cloud-aerosol interactions and is generally underrepresented in the current literature. A summary of the trace gas and optical/microphysical measurements is provided, along with additional detail and analysis of data collected from the hygroscopic system during the 2015 Seven South-East Asian Studies (7-SEAS) field campaign. The results suggest that data from the platform are reliable and will complement future studies of aerosols and air quality in SEA and other regions of interest.

A Comparison of Airborne In Situ Cloud Microphysical Measurement with Ground-Based C-Band Radar Observations in Deep Stratiform Regions of African Squall Lines

AbstractThis study addresses clouds with significant ice water content (IWC) in the stratiform regions downwind of the convective cores of African squall lines in the framework of the French–Indian satellite Megha-Tropiques project, observed in August 2010 next to Niamey (13.5°N, 2°E) in the southwestern part of Niger. The objectives included comparing the IWC–Z reflectivity relationship for precipitation radars in deep stratiform anvils, collocating reflectivity observed from ground radar with the calculated reflectivity from in situ microphysics for all aircraft locations inside the radar range, and interpreting the role of large ice crystals in the reflectivity of centimeter radars through analysis of their microphysical characteristics as ice crystals larger than 5 mm frequently occurred. It was found that, in the range of 20–30 dBZ, IWC and C-band reflectivity are not really correlated. Cloud regions with high IWC caused by important crystal number concentrations can lead to the same reflectivity factor as cloud regions with low IWC formed by a few millimeter-sized ice crystals.

Quantitative evaluation of seven optical sensors for cloud microphysical measurements at the Puy-de-Dôme Observatory, France

Abstract. Clouds have an important role in Earth's radiative budget. Since the late 1970s, considerable instrumental developments have been made in order to quantify cloud microphysical and optical properties, for both airborne and ground-based applications. Intercomparison studies have been carried out in the past to assess the reliability of cloud microphysical properties inferred from various measurement techniques. However, observational uncertainties still exist, especially for droplet size distribution measurements and need to be reduced. In this work, we discuss results from an intercomparison campaign, performed at the Puy de Dôme in May 2013. During this campaign, a unique set of cloud instruments was operating simultaneously in ambient air conditions and in a wind tunnel. A Particle Volume Monitor (PVM-100), a Forward Scattering Spectrometer Probe (FSSP), a Fog Monitor (FM-100), and a Present Weather Detector (PWD) were sampling on the roof of the station. Within a wind tunnel located underneath the roof, two Cloud Droplet Probes (CDPs) and a modified FSSP (SPP-100) were operating. The main objectives of this paper are (1) to study the effects of wind direction and speed on ground-based cloud observations, (2) to quantify the cloud parameters discrepancies observed by the different instruments, and (3) to develop methods to improve the quantification of the measurements. The results revealed that all instruments showed a good agreement in their sizing abilities, both in terms of amplitude and variability. However, some of them, especially the FM-100, the FSSP and the SPP, displayed large discrepancies in their capability to assess the magnitude of the total number concentration of the cloud droplets. As a result, the total liquid water content can differ by up to a factor of 5 between the probes. The use of a standardization procedure, based on data of integrating probes (PVM-100 or visibilimeter) and extinction coefficient comparison substantially enhanced the instrumental agreement. During this experiment, the total concentration agreed in variations with the visibilimeter, except for the FSSP, so a corrective factor can be applied and it ranges from 0.44 to 2.2. This intercomparison study highlights the necessity to have an instrument which provides a bulk measurement of cloud microphysical or optical properties during cloud ground-based campaigns. Moreover, the FM and FSSP orientation was modified with an angle ranging from 30 to 90° angle with wind speeds from 3 to 7 m s−1. The results show that the induced number concentration loss is between 29 and 98 % for the FSSP and between 15 and 68 % for the FM-100. In particular, FSSP experiments showed strong discrepancies when the wind speed was lower than 3 m s−1 and/or when the angle between the wind direction and the orientation of the instruments is greater than 30°. An inadequate orientation of the FSSP towards the wind direction leads to an underestimation of the measured effective diameter.

A Balloonborne Particle Size, Imaging, and Velocity Probe for in Situ Microphysical Measurements

AbstractA balloonborne instrument known as the Particle Size, Image, and Velocity (PASIV) probe has been developed at the National Severe Storms Laboratory to provide in situ microphysical measurements in storms. These observations represent a critical need of microphysics observations for use in lightning studies, cloud microphysics simulations, and dual-polarization radar validation. The instrument weighs approximately 2.72 kg and consists of a high-definition (HD) video camera, a camera viewing chamber, and a modified Particle Size and Velocity (Parsivel) laser disdrometer mounted above the camera viewing chamber. Precipitation particles fall through the Parsivel sampling area and then into the camera viewing chamber, effectively allowing both devices to sample the same particles. The data are collected on board for analysis after retrieval. Taken together, these two instruments are capable of providing a vertical profile of the size, shape, velocity, orientation, and composition of particles along the balloon path within severe weather.The PASIV probe has been deployed across several types of weather environments, including thunderstorms, supercells, and winter storms. Initial results from two cases in the Deep Convective Clouds and Chemistry Experiment are shown that demonstrate the ability of the instrument to obtain high-spatiotemporal- resolution observations of the particle size distributions within convection.

High-resolution measurement of cloud microphysics and turbulence at a mountaintop station

Abstract. Mountain research stations are advantageous not only for long-term sampling of cloud properties but also for measurements that are prohibitively difficult to perform on airborne platforms due to the large true air speed or adverse factors such as weight and complexity of the equipment necessary. Some cloud–turbulence measurements, especially Lagrangian in nature, fall into this category. We report results from simultaneous, high-resolution and collocated measurements of cloud microphysical and turbulence properties during several warm cloud events at the Umweltforschungsstation Schneefernerhaus (UFS) on Zugspitze in the German Alps. The data gathered were found to be representative of observations made with similar instrumentation in free clouds. The observed turbulence shared all features known for high-Reynolds-number flows: it exhibited approximately Gaussian fluctuations for all three velocity components, a clearly defined inertial subrange following Kolmogorov scaling (power spectrum, and second- and third-order Eulerian structure functions), and highly intermittent velocity gradients, as well as approximately lognormal kinetic energy dissipation rates. The clouds were observed to have liquid water contents on the order of 1 g m−3 and size distributions typical of continental clouds, sometimes exhibiting long positive tails indicative of large drop production through turbulent mixing or coalescence growth. Dimensionless parameters relevant to cloud–turbulence interactions, the Stokes number and settling parameter are in the range typically observed in atmospheric clouds. Observed fluctuations in droplet number concentration and diameter suggest a preference for inhomogeneous mixing. Finally, enhanced variance in liquid water content fluctuations is observed at high frequencies, and the scale break occurs at a value consistent with the independently estimated phase relaxation time from microphysical measurements.

The Ice Selective Inlet: a novel technique for exclusive extraction of pristine ice crystals in mixed-phase clouds

Abstract. Climate predictions are affected by high uncertainties partially due to an insufficient knowledge of aerosol–cloud interactions. One of the poorly understood processes is formation of mixed-phase clouds (MPCs) via heterogeneous ice nucleation. Field measurements of the atmospheric ice phase in MPCs are challenging due to the presence of much more numerous liquid droplets. The Ice Selective Inlet (ISI), presented in this paper, is a novel inlet designed to selectively sample pristine ice crystals in mixed-phase clouds and extract the ice residual particles contained within the crystals for physical and chemical characterization. Using a modular setup composed of a cyclone impactor, droplet evaporation unit and pumped counterflow virtual impactor (PCVI), the ISI segregates particles based on their inertia and phase, exclusively extracting small ice particles between 5 and 20 μm in diameter. The setup also includes optical particle spectrometers for analysis of the number size distribution and shape of the sampled hydrometeors. The novelty of the ISI is a droplet evaporation unit, which separates liquid droplets and ice crystals in the airborne state, thus avoiding physical impaction of the hydrometeors and limiting potential artefacts. The design and validation of the droplet evaporation unit is based on modelling studies of droplet evaporation rates and computational fluid dynamics simulations of gas and particle flows through the unit. Prior to deployment in the field, an inter-comparison of the optical particle size spectrometers and a characterization of the transmission efficiency of the PCVI was conducted in the laboratory. The ISI was subsequently deployed during the Cloud and Aerosol Characterization Experiment (CLACE) 2013 and 2014 – two extensive international field campaigns encompassing comprehensive measurements of cloud microphysics, as well as bulk aerosol, ice residual and ice nuclei properties. The campaigns provided an important opportunity for a proof of concept of the inlet design. In this work we present the setup of the ISI, including the modelling and laboratory characterization of its components, as well as field measurements demonstrating the ISI performance and validating the working principle of the inlet. Finally, measurements of biological aerosol during a Saharan dust event (SDE) are presented, showing a first indication of enrichment of bio-material in sub-2 μm ice residuals.

Improving representation of convective transport for scale‐aware parameterization: 1. Convection and cloud properties simulated with spectral bin and bulk microphysics

AbstractThe ultimate goal of this study is to improve the representation of convective transport by cumulus parameterization for mesoscale and climate models. As Part 1 of the study, we perform extensive evaluations of cloud‐resolving simulations of a squall line and mesoscale convective complexes in midlatitude continent and tropical regions using the Weather Research and Forecasting model with spectral bin microphysics (SBM) and with two double‐moment bulk microphysics schemes: a modified Morrison (MOR) and Milbrandt and Yau (MY2). Compared to observations, in general, SBM gives better simulations of precipitation and vertical velocity of convective cores than MOR and MY2 and therefore will be used for analysis of scale dependence of eddy transport in Part 2. The common features of the simulations for all convective systems are (1) the model tends to overestimate convection intensity in the middle and upper troposphere, but SBM can alleviate much of the overestimation and reproduce the observed convection intensity well; (2) the model greatly overestimates Ze in convective cores, especially for the weak updraft velocity; and (3) the model performs better for midlatitude convective systems than the tropical system. The modeled mass fluxes of the midlatitude systems are not sensitive to microphysics schemes but are very sensitive for the tropical case indicating strong microphysics modification to convection. Cloud microphysical measurements of rain, snow, and graupel in convective cores will be critically important to further elucidate issues within cloud microphysics schemes.

In-situ measurements of cloud-precipitation microphysics in the East Asian monsoon region since 1960

A large number of in-situ measurements of cloud-precipitation microphysical properties have been made since 1960, including measurements of particle size distribution, particle concentration, and liquid water content of clouds and rain. These measurements have contributed to considerable progress in understanding microphysical processes in clouds and precipitation and significant improvements in parameterizations of cloud microphysics in numerical models. This work reviews key findings regarding cloud-precipitation microphysics over China. The total number concentrations of various particles vary significantly, with certain characteristic spatial scales. The size distributions of cloud droplets in stratiform clouds can generally be fit with gamma distributions, but the fit parameters cover a wide range. Raindrop size distributions (RSDs) associated with stratiform clouds can be fit with either exponential or gamma distributions, while RSDs associated with convective or mixed stratiform-cumuliform clouds are best fit with gamma distributions. Concentrations of ice nuclei (IN) over China are higher than those observed over other regions, and increase exponentially as temperature decreases. The particle size distributions of ice crystals, snow crystals, and hailstones sampled at a variety of locations can be reliably approximated by using exponential distributions, while aerosol particle size distributions are best described as the sum of a modified gamma distribution and a Junge power-law distribution. These results are helpful for evaluating and improving the fidelity of physical processes and hydrometeor fields simulated by microphysical parameterizations. The comprehensive summary and analysis of previous work presented here also provide useful guidelines for the design of future observational programs.

Observations of the Origin and Distribution of Ice in Cold, Warm, and Occluded Frontal Systems during the DIAMET Campaign

Abstract Three case studies in frontal clouds from the Diabatic Influences on Mesoscale Structures in Extratropical Storms (DIAMET) project are described to understand the microphysical development of the mixed phase regions of these clouds. The cases are a kata-type cold front, a wintertime warm front, and a summertime occluded frontal system. The clouds were observed by radar, satellite, and in situ microphysics measurements from the U.K. Facility for Airborne Atmospheric Measurements (FAAM) research aircraft. The kata cold front cloud was shallow with a cloud-top temperature of approximately −13°C. Cloud-top heterogeneous ice nucleation was found to be consistent with predictions by a primary ice nucleation scheme. The other case studies had high cloud tops (< −40°C) and despite no direct cloud-top measurements in these regions, homogeneous ice nucleation would be expected. The maximum ice crystal concentrations and ice water contents in all clouds were observed at temperatures around −5°C. Graupel was not observed, hence, secondary ice was produced by riming on snow falling through regions of supercooled liquid water. Within these regions substantial concentrations (10–150 L−1) of supercooled drizzle were observed. The freezing of these drops increases the riming rate due to the increase in rimer surface area. Increasing rime accretion has been shown to lead to higher ice splinter production rates. Despite differences in the cloud structure, the maximum ice crystal number concentration in all three clouds was ~100 L−1. Ice water contents were similar in the warm and occluded frontal cases, where median values in both cases reached ~0.2–0.3 g m−3, but lower in the cold front case.

Diabatic Heating and Cooling Rates Derived from In Situ Microphysics Measurements: A Case Study of a Wintertime U.K. Cold Front

AbstractIn situ measurements associated with the passage of a kata cold front over the United Kingdom on 29 November 2011 are used to initialize a Lagrangian parcel model for the purpose of calculating rates of diabatic heating and cooling associated with the phase changes of water within the cloud system. The parcel model calculations are performed with both bin-resolved and bulk treatments of microphysical processes. The in situ data from this case study reveal droplet number concentrations up to 100 cm−3, with planar ice crystals detected at cloud top, as well as columnar crystals produced by rime splinter ejection within the prefrontal warm sector. The results show that in terms of magnitude, the most significant rates of diabatic heating and cooling are produced by condensation growth of liquid water within the convective updrafts at the leading edge of the front. The peak temperature tendencies associated with condensation are typically found to be at least an order of magnitude larger than those associated with the ice phase, although the cooling effect from sublimation and melting occurs over a wide region. The parcel model framework is used in conjunction with the observations to assess the suitability of existing bulk microphysical treatments, of the kind used in operational weather forecast models. It is found that the assumption of spherical ice crystals (with diameters equal to the maximum dimension of those sampled), along with the use of negative exponential functions to describe ice particle size distributions, can lead to an overestimation of local diabatic heating and cooling rates by a factor of 2 or more.

The next generation airborne polarimetric Doppler weather radar

Abstract. Results from airborne field deployments emphasized the need to obtain concurrently high temporal and spatial resolution measurements of 3-D winds and microphysics. A phased array radar on an airborne platform using dual-polarization antenna has the potential for retrieving high-resolution, collocated 3-D winds and microphysical measurements. Recently, ground-based phased array radar (PAR) has demonstrated the high time-resolution estimation of accurate Doppler velocity and reflectivity of precipitation and clouds when compared to mechanically scanning radar. PAR uses the electronic scanning (e-scan) to rapidly collect radar measurements. Since an airborne radar has a limited amount of time to collect measurements over a specified sample volume, the e-scan will significantly enhance temporal and spatial resolution of airborne radar observations. At present, airborne weather radars use mechanical scans, and they are not designed for collecting dual-polarization measurements to remotely estimate microphysics. This paper presents a possible configuration of a novel airborne phased array radar (APAR) to be installed on an aircraft for retrieving improved dynamical and microphysical scientific products. The proposed APAR would replace the aging, X-band Electra Doppler radar (ELDORA). The ELDORA X-band radar's penetration into precipitation is limited by attenuation. Since attenuation at C-band is lower than at X-band, the design specification of a C-band airborne phased array radar (APAR) and its measurement accuracies are presented. Preliminary design specifications suggest the proposed APAR will meet or exceed ELDORA's current sensitivity, spatial resolution and Doppler measurement accuracies of ELDORA and it will also acquire dual-polarization measurements.

Chemical properties of insoluble precipitation residue particles

Precipitation chemistry can provide unique insights into the composition of aerosol particles involved in precipitation processes. Until recently, precipitation chemistry studies focused predominantly on soluble components. Analyzing the single particle insoluble components in addition to soluble ions in precipitation can provide detailed information on the individual particles originally in the cloud or removed by precipitation as well as the source of the aerosols. Herein, we present an in-depth analysis of resuspended residues from precipitation samples collected at a remote site in the Sierra Nevada Mountains in California during the 2009–2011 winter seasons. In addition, we present results from laboratory control experiments of dust, leaf litter, smoke, and sea salt samples that were conducted to better understand how insoluble and soluble residues are distributed during the atomization process and aid in the classification of the residue compositions in the precipitation samples. Further, immersion freezing ice nuclei (IN) measurements of insoluble residues from precipitation water enabled the determination of residue types that likely seeded clouds. Long-range transported dust mixed with biological material tended to be more IN active, while purely biological residues contained a variety of high and low temperature IN. Overall, results from this study can be used as a benchmark for classification of insoluble precipitation residues in future studies. Knowledge of the precipitation chemistry of insoluble residues coupled with meteorological and cloud microphysical measurements will ultimately improve our understanding of the link between aerosols, clouds, and precipitation.

Influence of aerosols on the life cycle of a radiation fog event. A numerical and observational study

Despite the knowledge gained on the physical processes dominating the formation, development and dissipation of radiation fog events, uncertainties still exist about the role of the microphysical processes related to aerosol characteristics. The objective of this work is to analyze the sensitivity of fog to aerosols through their impacts on the fog droplets. A radiation fog event that formed on 15/11/2011 at the SIRTA Observatory near Paris in the context of the 2011–2012 ParisFog field campaign is the basis of this study. The selected case is one that initially forms a few hundred meters above the surface and within half an hour lowers down to the surface. A combination of SIRTA's sophisticated observations and 1D numerical simulations is employed with the aim of better understanding the influence of thermodynamics and microphysics on the life-cycle of the fog event and the degree to which aerosol characteristics such as concentration of potentially activated aerosols, size and solubility affect its characteristics. It results that the model simulates fairly well the fog life cycle, with only one half hour advance in the onset and one hour in the dissipation at the surface. The quality of the reference simulation is evaluated against several in-situ and remote sensing measurements. A numerical sensitivity analysis shows that the fog characteristics are strongly influenced by the aerosols. Doubling (halving) the cloud condensation nuclei (CCN) number translates into a 160% increase (65% decrease) in the production of fog droplets, and a 60% increase (40% decrease) of the liquid water path (LWP). The aerosols influence up to 10% the fog geometrical thickness. The necessity for more detailed local forcings that will produce better thermohygrometric conditions in the upper levels above the formed fog layer is underlined, as well as the addition of microphysical measurements in the vertical that will allow to improve two-moment microphysics schemes.

Stability and Charging Characteristics of the Comma Head Region of Continental Winter Cyclones

Abstract This paper presents analyses of the finescale structure of convection in the comma head of two continental winter cyclones and a 16-storm climatology analyzing the distribution of lightning within the comma head. A case study of a deep cyclone is presented illustrating how upper-tropospheric dry air associated with the dry slot can intrude over moist Gulf air, creating two zones of precipitation within the comma head: a northern zone characterized by deep stratiform clouds topped by generating cells and a southern zone marked by elevated convection. Lightning, when it occurred, originated from the elevated convection. A second case study of a cutoff low is presented to examine the relationship between lightning flashes and wintertime convection. Updrafts within convective cells in both storms approached 6–8 m s−1, and convective available potential energy in the cell environment reached approximately 50–250 J kg−1. Radar measurements obtained in convective updraft regions showed enhanced spectral width within the temperature range from −10° to −20°C, while microphysical measurements showed the simultaneous presence of graupel, ice particles, and supercooled water at the same temperatures, together supporting noninductive charging as an important charging mechanism in these storms. A climatology of lightning flashes across the comma head of 16 winter cyclones shows that lightning flashes commonly occur on the southern side of the comma head where dry-slot air is more likely to overrun lower-level moist air. Over 90% of the cloud-to-ground flashes had negative polarity, suggesting the cells were not strongly sheared aloft. About 55% of the flashes were associated with cloud-to-ground flashes while 45% were in-cloud flashes.

Ice cloud single-scattering property models with the full phase matrix at wavelengths from 0.2 to 100 µm

Ice cloud bulk scattering models are derived for 445 discrete wavelengths between 0.2µm and 100µm. The methodology for deriving these optical models is based on microphysical data from 11 field campaigns using a variety of in situ probes, and incorporates a correction to mitigate the impact of ice particles that shatter at the probe inlets. The models are also based on a new library of ice habit single scattering properties developed for plates, droxtals, hollow and solid columns, hollow and solid bullet rosettes, an aggregate of solid columns, and a small/large aggregate of plates. Three sets of models are developed that assume the use of solid columns only, the aggregate of solid columns only, and a general habit mixture that incorporates all the habits. The consistency of the resulting models is explored. While the general habit mixture provides consistency with in situ microphysical measurements and the closest agreement with polarized reflectivities observed by the POLDER instrument on the PARASOL satellite, the aggregate of severely roughened solid columns provides the closest agreement between solar and infrared optical thicknesses. Finally, spectral results are presented for the shortwave and longwave models.

On the microphysical behaviour of wind-forced water surfaces and consequent re-aeration

AbstractA detailed laboratory investigation of the mechanical and low-solubility gas coupling between wind and water has been undertaken using a suite of microphysical measurement techniques. Under a variety of wind conditions and in the presence and absence of mechanically generated short waves, approximately fetch-independent surface conditions have been achieved over short laboratory fetches of several metres. The mechanical coupling of the surface is found to be consistent with Banner (J. Fluid Mech. vol. 211, 1990, pp. 463–495) and Banner & Peirson (J. Fluid Mech. vol. 364, 1998, pp. 115–145). Bulk observations of re-aeration are consistent with previous laboratory studies. The surface kinematical behaviour is in accordance with the observations of Peirson & Banner (J. Fluid Mech. vol. 479, 2003, pp. 1–38). Also, their predictions of a strong enhancement of low-solubility gas flux at the onset of microscale breaking is confirmed and direct observations show a concomitant onset of very thin aqueous diffusion sublayers. It is found that the development of strong parasitic capillary waves towards the incipient breaking limit does not noticeably enhance constituent transfer. Across the broad range of conditions investigated during this study, the local instantaneous constituent transfer rate remains approximately log-normally distributed with an approximately constant standard deviation of $0.62\pm 0.15({\mathrm{log}}_e(\mathrm{m}~ {\mathrm{s}}^{-1}))$. Although wind-forced water surfaces are shown to be punctuated by intense tangential stresses and local surface convergence, localized surface convergence does not appear to be the single critical factor determining exchange rate. Larger-scale orbital wave straining is found to be a significant constituent transfer process in contrast to Witting (J. Fluid Mech. vol. 50, 1971, pp. 321–334) findings for heat fluxes, but the measured effects are consistent with his model. By comparing transfer rates in the presence and absence of microscale breaking, low-solubility gas transfer was decomposed into its turbulent/capillary ripple, gravity-wave-related and microscale breaking contributions. It was found that an efficiency factor of approximately $17\, \%$ needs to be applied to Peirson & Banner’s model, which is extended to field conditions. Although bulk thermal effects were observed and thermal diffusion layers are presumed thicker than their mass diffusion counterparts, significant thermal influences were not observed in the results.