High-resolution (0.1-Å) spectra of the 6815-Å band of methane are presented for Jupiter, Saturn, Uranus, and Neptune. Spectra for Uranus, Neptune, and the equatorial region of Saturn were acquired with the SPIFI ( W. H. Smith, T. R. Hicks, and J. P. Born (1978). Proceedings of the 4th International Colloquium on Astrophysics, Triest, July 3–7, 1978. pp. 593–599) at the 2.2-m telescope of the Mauna Kea Observatory during May and June 1980. Additional spectra were obtained for Jupiter and the northern temperate and polar regions of Saturn in December 1980 and January 1981 from Kitt Peak National Observatory's McMath Solar Telescope. The spectra show a dichotomy in strength of methane absorption between Jupiter-Saturn and Uranus-Neptune. A simple model analysis, based on homogeneous scattering models, is unable to resolve whether this dichotomy is due to an actual increase in the methane mixing ratio with solar distance or to the temperature dependence of line strengths and absorption pathlengths in these atmospheres. If the rotational quantum number for the prominent 6818.9-Å feature is J < 4, then significant aerosol extinction must exist within the visibly accessible portion of Uranus' atmosphere for the methane mixing ratio to be greater than the solar value.