Magnon States Research Articles

Quantum Control of a Single Magnon in a Macroscopic Spin System.

Nonclassical quantum states are the pivotal features of a quantum system that differs from its classical counterpart. However, the generation and coherent control of quantum states in a macroscopic spin system remain an outstanding challenge. Here we experimentally demonstrate the quantum control of a single magnon in a macroscopic spin system (i.e., 1mm-diameter yttrium-iron-garnet sphere) coupled to a superconducting qubit via a microwave cavity. By tuning the qubit frequency insitu via the Autler-Townes effect, we manipulate this single magnon to generate its nonclassical quantum states, including the single-magnon state and the superposition of single-magnon state and vacuum (zero magnon) state. Moreover, we confirm the deterministic generation of these nonclassical states by Wigner tomography. Our experiment offers the first reported deterministic generation of the nonclassical quantum states in a macroscopic spin system and paves a way to explore its promising applications in quantum engineering.

Optical registration of a coherent magnon state outside of the excitation region.

Magnons have demonstrated enormous potential for the next generation of information technology and quantum computing. In particular, the coherent state of magnons resulting from their Bose-Einstein condensation (mBEC) is of great interest. Typically, mBEC is formed in the magnon excitation region. Here we demonstrate for the first time by optical methods the permanent existence of mBEC at large distances from the magnon excitation region. The homogeneity of the mBEC phase is also demonstrated. The experiments were carried out on films of yttrium iron garnet magnetized perpendicular to the surface and at room temperature. We use the method described in this article to develop coherent magnonics and quantum logic devices.

Localized Surface Magnon Modes in Cubic Ferromagnetic Lattices

A theoretical formalism for calculating the bulk and surface spin modes in Heisenberg semi-infinite lattices is presented on a ferromagnetic cubic network of spins, coupled via nearest and next-nearest neighbors exchange interactions. The magnetic surface can be considered as semi-infinite slabs at the end of the bulk structures. The breakdown of translation symmetry, in the normal direction of the surface, gives rise to localized spin wave modes in its neighborhood. The localized magnon spectrum is derived as elements of a Landauer-type scattering matrix, in the three cubic lattices sc, bcc and fcc. The magnon properties are simulated and determined numerically for each cubic lattice by using the matching technique. The observed fluctuations in the numerical results demonstrate the interference magnon effects between scattered spinwaves and the localized magnon states, generated by the surface region with characteristic Fano resonances. In cubic leads, the localized surface spin states are sensitive to the local magnetic coupling and the incident direction in the surface boundary. In this contribution, the normalized energy of spinwaves arising from the absence of translation symmetry is analyzed for each cubic system as a function of the exchange integral parameters. This addresses the dependence of the surface magnon on the different possibilities of the of the exchange parameters variation from softening to hardening in the neighborhood of the surface region.

Direct Optical Probe of Magnon Topology in Two-Dimensional Quantum Magnets.

Controlling edge states of topological magnon insulators is a promising route to stable spintronics devices. However, to experimentally ascertain the topology of magnon bands is a challenging task. Here we derive a fundamental relation between the light-matter coupling and the quantum geometry of magnon states. This allows us to establish the two-magnon Raman circular dichroism as an optical probe of magnon topology in honeycomb magnets, in particular of the Chern number and the topological gap. Our results pave the way for interfacing light and topological magnons in functional quantum devices.

Radiation-free and non-Hermitian topology inertial defect states of on-chip magnons

Radiative damping is a strong dissipation source for the quantum emitters hybridized with propagating photons, electrons, or phonons, which is not easily avoidable for on-chip magnonic emitters as well that can radiate via the surface acoustic waves of the substrate. Here we demonstrate in an array of on-chip nanomagnets coupled in a long range via exchanging the surface acoustic waves that a point defect in the array, which can be introduced by the local magnon frequency shift by a local biased magnetic field or the absence of a magnetic wire, strongly localizes the magnons, in contrast to the well spreading Bloch-like collective magnon modes in such an array setting. The radiation of the magnon defect states is exponentially suppressed by the distance of the defect to the array edges. Moreover, this defect state is strikingly inertial to the non-Hermitian topology that localizes all the extended states at one boundary. Such configuration robust magnon defect states towards radiation-free limit may be suitable for high-fidelity magnon quantum information storage in the future on-chip magnonic devices.

Particle zoo in a doped spin chain: Correlated states of mesons and magnons

It is a widely accepted view that the interplay of spin- and charge-degrees of freedom in doped antiferromagnets (AFMs) gives rise to the rich physics of high-temperature superconductors. Nevertheless, it remains unclear how effective low-energy degrees of freedom and the corresponding field theories emerge from microscopic models, including the $t-J$ and Hubbard Hamiltonians. A promising view comprises that the charge carriers have a rich internal parton structure on intermediate scales, but the interplay of the emergent partons with collective magnon excitations of the surrounding AFM remains unexplored. Here we study a doped one-dimensional spin chain in a staggered magnetic field and demonstrate that it supports a zoo of various long-lived excitations. These include magnons; mesonic pairs of spinons and chargons, along with their ro-vibrational excitations; and tetra-parton bound states of mesons and magnons. We identify these types of quasiparticles in various spectra using DMRG simulations. Moreover, we introduce a strong-coupling theory describing the polaronic dressing and molecular binding of mesons to collective magnon excitations. The effective theory can be solved by standard tools developed for polaronic problems, and can be extended to study similar physics in two-dimensional doped AFMs in the future. Experimentally, the doped spin-chain in a staggered field can be directly realized in quantum gas microscopes.

Entangling mechanical vibrations of two massive ferrimagnets by fully exploiting the nonlinearity of magnetostriction

Quantum entanglement in the motion of macroscopic objects is of significance to both fundamental studies and quantum technologies. Here we show how to entangle the mechanical vibration modes of two massive ferrimagnets that are placed in the same microwave cavity. Each ferrimagnet supports a magnon mode and a low-frequency vibration mode coupled by the magnetostrictive force. The two magnon modes are, respectively, coupled to the microwave cavity by the magnetic dipole interaction. We first generate a stationary nonlocal entangled state between the vibration mode of the ferrimagnet-1 and the magnon mode of the ferrimagnet-2. This is realized by continuously driving the ferrimagnet-1 with a strong red-detuned microwave field and the entanglement is achieved by exploiting the magnomechanical parametric down-conversion and the cavity–magnon state-swap interaction. We then switch off the pump on the ferrimagnet-1 and, simultaneously, turn on a red-detuned pulsed drive on the ferrimagnet-2. The latter drive is used to activate the magnomechanical beamsplitter interaction, which swaps the magnonic and mechanical states of the ferrimagnet-2. Consequently, the previously generated phonon–magnon entanglement is transferred to the mechanical modes of two ferrimagnets. The work provides a scheme to prepare entangled states of mechanical motion of two massive objects, which may find applications in various studies exploiting macroscopic entangled states.

Master equation approach to magnon relaxation and dephasing

There has been a recent upsurge of interest in the quantum properties of magnons for quantum information processing. An important issue is to examine the stability of quantum states of magnons against various relaxation and dephasing channels. Since the interaction of magnons in magnetic systems may fall in the ultrastrong and even deep-strong coupling regimes, the relaxation process of magnon states is quite different from the more common quantum optical systems. Here we study the relaxation and dephasing of magnons based on the Lindblad formalism and derive a generalized master equation that describes the quantum dynamics of magnons. Employing this master equation, we identify two distinct dissipation channels for squeezed magnons, i.e., the local dissipation and collective dissipation, which play a role for both ferromagnets and antiferromagnets. The local dissipation is caused by the independent exchange of angular momentum between the magnonic system and the environment, while the collective dissipation is dressed by the parametric interactions of magnons and it enhances the quantumness and thermal stability of squeezed magnons. Further, we show how this formalism can be applied to study the pure dephasing of magnons caused by four-magnon scattering and magnon-phonon interactions. Our results provide the theoretical tools to study the decoherence of magnons within a full quantum-mechanical framework and further benefit the use of quantum states of magnons for information processing.

Symmetry resolved entanglement of excited states in quantum field theory. Part II. Numerics, interacting theories and higher dimensions

In a recent paper we studied the entanglement content of zero-density excited states in complex free quantum field theories, focusing on the symmetry resolved entanglement entropy (SREE). By zero-density states we mean states consisting of a fixed, finite number of excitations above the ground state in an infinite-volume system. The SREE is defined for theories that possess an internal symmetry and provides a measure of the contribution to the total entanglement of each symmetry sector. In our work, we showed that the ratio of Fourier-transforms of the SREEs (i.e. the ratio of charged moments) takes a very simple and universal form for these states, which depends only on the number, statistics and symmetry charge of the excitations as well as the relative size of the entanglement region with respect to the whole system’s size. In this paper we provide numerical evidence for our formulae by computing functions of the charged moments in two free lattice theories: a 1D Fermi gas and a complex harmonic chain. We also extend our results in two directions: by showing that they apply also to excited states of interacting theories (i.e. magnon states) and by developing a higher dimensional generalisation of the branch point twist field picture, leading to results in (interacting) higher-dimensional models.

Exchange-mediated magnon-phonon scattering in monolayer CrI3

The interplay between magnons and phonons and its influences on magnon dissipation have attracted widespread attentions. Whereas the previous theoretical works were usually restricted to the interactions between low-frequency magnons and acoustic phonons in the long-wavelength region, in the present work we go beyond this limit and investigate the magnon relaxation in a two-dimensional ferromagnet, a monolayer ${\mathrm{CrI}}_{3}$, through magnon-phonon scattering channels mediated by the variation of the exchange strength resulting from all-wavelength acoustic phonons as well as the optical ones. With a precise description of the magnon and phonon Bloch states from first principles, we evaluate the magnon relaxation rate due to these exchange-mediated magnon-phonon scatterings and reveal rich features in its momentum dependence, which reflects nicely the role of the associated phonons with in-plane atomic vibrations. The magnon-number-conserving scattering is found to be orders of magnitude stronger than the magnon-number-nonconserving scattering due to the weak anisotropic exchange coupling or dipole-dipole interaction. Our first-principles-based approach provides a better solution for the quantitative evaluation of the magnon dissipation by phonons.

Time-dependent strain-tuned topological magnon phase transition

Collinear magnets in honeycomb lattices under the action of time-dependent strains are investigated. Given the limits of high-frequency periodically varying deformations, we derive an effective Floquet theory for spin systems that results in the emergence of a spin chirality. We find that the coupling between magnons and spin chirality depends on the details of the strain such as the spatial dependence and applied direction. Magnonic fluctuations about the ferromagnetic state are determined, and it is found that spatially homogeneous strains drive the magnon system into topologically protected phases. In particular, we show that certain uniform strain fields play the role of an out-of-plane nearest-neighbor Dzyaloshinskii-Moriya interaction. Furthermore, we explore the application of nonuniform strains, which lead to a confinement of magnon states that for uniaxial strains propagates along the direction that preserves translational symmetry. Our work demonstrates a direct way in which to manipulate the magnon spectrum based on time-dependent strain engineering that is relevant for exploring topological transitions in quantum magnonics.

Interaction between magnon and skyrmion: Toward quantum magnonics

In recent years, magnon and spin texture are attracting great interest in condensed matter physics and magnetism. Magnonics is aiming to use magnon as information carriers to realize functions for storage, transmission, and processing. Magnetic skyrmion is representative spin texture due to its topologically nontrivial properties. Since skyrmions are topologically protected, their transformation to other spin configurations requires overcoming additional topological energy barriers. Therefore, skyrmions are more stable than other trivial spin textures. In addition, the characters of nanoscale size, quasiparticle properties, and various excitation modes make them a potential candidate for spintronic application. Magnon and skyrmion, as two fundamental excitations, can coexist in magnetic systems and interplay with each other through direct exchange interactions. In this review, we provide an overview of recent theoretical and experimental studies on magnon–skyrmion interactions. We mainly focus on three kinds of magnon–skyrmion interactions: (i) magnon scattering by skyrmion, (ii) skyrmion motion driven by magnon, and (iii) coupling between magnon and skyrmion modes. The first two kinds of interactions could be clearly explained by the wave-particle interaction model on the classical level. Alternatively, the last kind of interaction could be understood by the coupled harmonic oscillator model on the quantum level, which indicates fast energy exchange and hybrid magnon states. The exploration focused on quantum phenomena of magnon has led to the emerging field of quantum magnonics and promoted applications of magnon in quantum information storage and processing. In the end, we give a perspective on the exploration of magnon–skyrmion interaction in quantum magnonics.

Elemental excitations in MoI3 one-dimensional van der Waals nanowires

We report the polarization-dependent Raman spectra of exfoliated MoI3, a van der Waals material with a “true one-dimensional” crystal structure that can be exfoliated to individual atomic chains. The temperature evolution of several Raman features reveals an anomalous behavior suggesting a phase transition of magnetic origin. Theoretical considerations indicate that MoI3 is an easy-plane antiferromagnet with alternating spins along the dimerized chains and with inter-chain helical spin ordering. The calculated frequencies of phonons and magnons are consistent with the interpretation of the experimental Raman data. The obtained results shed light on the specifics of the phononic and magnonic states in MoI3 and provide a strong motivation for further study of this unique material with potential for future spintronic applications.

Molecular beam epitaxy, photoluminescence from Mn2+ multiplets and self-trapped exciton states of γ-MnTe single-crystalline thin films

Single-crystalline γ-MnTe thin films with zinc-blende structure were grown epitaxially on InP(111) by molecular beam epitaxy. Two-dimensional growth regime and atomic surface flatness are achieved, and appearance of Laue’s oscillation peaks illustrates the superior crystalline quality and interface of γ-MnTe films. A pseudocrystalbuffer layer is formed at interface releasing the strain led by the large lattice mismatch between γ-MnTe and InP, and then growth of γ-MnTe films with a perfect lattice evidences the high-quality crystallinity in a fully relaxed state. Photoluminescence (PL) emissions from 4T1g(4G) and 4T1(4G) related to Mn2+ ions d-d multiplets are observed with their respective activation energies of ∼142.5 meV and ∼323.5 meV. Such high potentials reflecting the nonradiative recombination indicate the thermal stability of these PL. Moreover, two extra PL transitions assigned to be the emissions from self-trapped exciton (STE) states are found below TN. Time-resolved PL (TRPL) spectra at various temperatures indicate that the relaxation dynamics of photoexcited d-electrons is strongly correlated to the antiferromagnetic ordering transition due to the synergy of magnon, phonon and STE states. These findings suggest that introduction of STE states in a material by controlling its magnetic ordering qualifies the competition in optoelectronics devices.

Pure dephasing of magnonic quantum states

For a wide range of nonclassical magnonic states that have been proposed and demonstrated recently, a new time scale besides the magnon lifetime---the magnon dephasing time---becomes important, but this time scale is rarely studied. Considering exchange interaction and spin-phonon coupling, we evaluate the pure magnon dephasing time and find it to be smaller than the magnon lifetime at temperatures of a few kelvins. By examining a magnonic cat state as an example, we show how pure dephasing of magnons destroys and limits the survival of quantum superpositions. Thus it will be critical to perform quantum operations within the pure dephasing time. We further derive the master equation for the density matrix describing such magnonic quantum states taking into account the role of pure dephasing. This methodology can be generalized to include additional dephasing channels that experiments are likely to encounter in the future. Our findings enable one to design and manipulate robust quantum states of magnons for information processing.

Non‐Classical Correlations between Single Photons and Magnons

AbstractA scheme is proposed to realize the non‐classical correlation between magnons and photons in a cavity optomagnonic system, which supports both photon modes and a magnon mode. Starting with the system being initially prepared in its ground state, two laser pulses successively drive corresponding optical mode. A two‐mode squeezing interaction between optical mode 1 and the magnon mode is created by the first pulse, which leads to a non‐classical correlation between photons and magnons. To verify this non‐classical correlation, the second pulse is utilized to transfer the magnon state to another optical mode, thus the correlated photon–photon pairs are generated out of the cavity. By discussing the violation of Cauchy–Schwarz inequality, based on numerical simulation, it is confirmed that non‐classical correlated photon–magnon pairs can be created in the weak coupling regime, which relaxes the requirements of experimental conditions. The result indicates that cavity optomagnonics can be a promising platform for studying magnon‐based quantum information processing.

High-fidelity quantum sensing of magnon excitations with a single electron spin in quantum dots

Single-electron spins in quantum dots are the leading platform for qubits, while magnons in solids are one of the emerging candidates for quantum technologies. How to manipulate a composite system composed of both systems is an outstanding challenge. Here, we use spin–charge hybridization to effectively couple the single-electron spin state in quantum dots to the cavity and further to the magnons. Through this coupling, quantum dots can entangle and detect magnon states. The detection efficiency can reach 0.94 in a realistic experimental situation. We also demonstrate the electrical tunability of the scheme for various parameters. These results pave a practical pathway for applications of composite systems based on quantum dots and magnons.

Tunable Magnonic Chern Bands and Chiral Spin Currents in Magnetic Multilayers.

Realization of novel topological phases in magnonic band structures represents a new opportunity for the development of spintronics and magnonics with low power consumption. In this work, we show that in antiparallelly aligned magnetic multilayers, the long-range, chiral dipolar interaction between propagating magnons generates bulk bands with nonzero Chern integers and magnonic surface states carrying chiral spin currents. The surface states are highly localized and can be easily toggled between nontrivial and trivial phases through an external magnetic field. The realization of chiral surface spin currents in this dipolarly coupled heterostructure represents a magnonic implementation of the coupled wire model that has been extensively explored in electronic systems. Our work presents an easy-to-implement system for realizing topological magnonic surface states and low-dissipation spin current transport in a tunable manner.

On certain classes of exact solutions of two magnon states in the Heisenberg spin chain

On certain classes of exact solutions of two magnon states in the Heisenberg spin chain

Topological thermal Hall effect and magnonic edge states in kagome ferromagnets with bond anisotropy

The magnon band topology due to the Dzyaloshinskii–Moriya interaction (DMI) and its relevant topological thermal Hall effect has been extensively studied in kagome lattice magnets. In this theoretical investigation, we report a new mechanism for phase transitions between topological phases of magnons in kagome ferromagnets by tuning the anisotropic nearest-neighbor ferromagnetic interaction and DMI. Using the linear spin-wave theory, we calculate the Chern number and thermal Hall conductivity of magnons in low temperature regime. We show the magnon band structures and magnonic edge states in each topological phase. From the topological phase diagram, we find a sign reversal of the thermal Hall conductivity upon tuning the modulation factors. We explicitly demonstrate the correspondence of thermal Hall conductivity with the propagation direction of the magnonic edge states. Finally, we discuss candidate materials as experimental realizations of our theoretical model.