Magnonic Band Research Articles

Thermal Hall conductivity with sign change in the Heisenberg–Kitaev kagome magnet

The Heisenberg–Kitaev (HK) model on various lattices has attracted a lot of attention because it may lead to exotic states such as quantum spin liquid and topological orders. The rare-earth-based kagome lattice (KL) compounds and have q = 0, 120° order and canted ferromagnetic (CFM) order, respectively. Interestingly, the HK model on the KL has the same ground state long-range orders. In the theoretical phase diagram, the CFM phase resides in a continuous parameter region and there is no phase change across special parameter points, such as the Kitaev ferromagnetic (KFM) point, the ferromagnetic (FM) point and its dual FM point. However, a ground state property cannot distinguish a system with or without topological nontrivial excitations and related phase transitions. Here, we study the topological magnon excitations and related thermal Hall conductivity in the HK model on the KL with CFM order. The CFM phase can be divided into two regions related by the Klein duality, with the self dual KFM point as their boundary. We find that the scalar spin chirality, which is intrinsic in the CFM order, changes sign across the KFM point. This leads to the opposite Chern numbers of corresponding magnon bands in the two regions, and also the sign change of the magnon thermal Hall conductivity.

Long-distance coupling of spin qubits via topological magnons

We consider two distant spin qubits in quantum dots, both coupled to a two-dimensional topological ferromagnet hosting chiral magnon edge states at the boundary. The chiral magnon is used to mediate entanglement between the spin qubits, realizing a fundamental building block of scalable quantum computing architectures: a long-distance two-qubit gate. Previous proposals for long-distance coupling with magnons involved off-resonant coupling, where the detuning of the spin-qubit frequency from the magnonic band edge provides protection against spontaneous relaxation. The topological magnon mode, on the other hand, lies in between two magnonic bands far away from any bulk magnon resonances, facilitating strong and highly tuneable coupling between the two spin qubits. Even though the coupling between the qubit and the chiral magnon is resonant for a wide range of qubit splittings, we find that the magnon-induced qubit relaxation is vastly suppressed if the coupling between the qubit and the ferromagnet is antiferromagnetic. A fast and high-fidelity long-distance coupling protocol is presented capable of achieving spin-qubit entanglement over micrometer distances with $1\phantom{\rule{0.16em}{0ex}}\mathrm{MHz}$ gate speed and up to $99.9%$ fidelities. The resulting spin-qubit entanglement may be used as a probe for the long-sought detection of topological edge magnons.

Ab initio study of spin fluctuations in the itinerant kagome magnet FeSn

Kagome antiferromagnetic metal FeSn has become an attracting platform for the exploration of novel electronic states, such as topological Dirac states and the formation of flat bands by localized electrons. Apart from the electronic properties, Dirac magnons and flat magnon bands have also been proposed by applying simplified Heisenberg models to kagome magnetic systems.Inelastic neutron scattering studies on FeSn found well defined magnon dispersions at low energies,but magnons at high energies are strongly dampled, which can not be explained by localized spin models. In this paper, we utilize both linear spin wave theory and time-dependent density functional perturbation theory to investigate spin fluctuations of FeSn. Through the comparison of calculated spin wave spectra and Stoner continuum, we explicitly show that the damping of magnons at high energies are due to the Landau damping, and the appearance of high energy optical-magnon like branches at the M and K point are resulted by relatively low Stoner excitation intensity at those regions.

Spin Excitation Spectra of Anisotropic Spin-1/2 Triangular Lattice Heisenberg Antiferromagnets.

Investigation of dynamical excitations is difficult but crucial to the understanding of many exotic quantum phenomena discovered in quantum materials. This is particularly true for highly frustrated quantum antiferromagnets whose dynamical properties deviate strongly from theoretical predictions made based on the spin-wave or other approximations. Here, we present a large-scale numerical calculation on the dynamical correlation functions of spin-1/2 triangular Heisenberg model using a state-of-the-art tensor network renormalization group method. The calculated results allow us to gain for the first time a comprehensive picture on the nature of spin excitation spectra in this highly frustrated quantum system. It provides a quantitative account for all the key features of the dynamical spectra disclosed by inelastic neutron scattering measurements for Ba_{3}CoSb_{2}O_{9}, revealing the importance of the interplay between low- and high-energy excitations and its renormalization effect to the low-energy magnon bands and high-energy continuums. We identify the longitudinal Higgs modes in the intermediate-energy scale and predict the energy and momentum dependence of spectral functions along the three principal axes that can be verified by polarized neutron scattering experiments. Furthermore, we find that the spin excitation spectra weakly depend on the anisotropic ratio of the antiferromagnetic interaction.

Planar thermal Hall effect of topological bosons in the Kitaev magnet α-RuCl3.

The honeycomb magnet α-RuCl3 has attracted considerable interest because it is proximate to the Kitaev Hamiltonian whose excitations are Majoranas and vortices. The thermal Hall conductivity κxy of Majorana fermions is predicted to be half-quantized. Half-quantization of κxy/T (T, temperature) was recently reported, but this observation has proven difficult to reproduce. Here, we report detailed measurements of κxy on α-RuCl3 with the magnetic field B ∥ a (zigzag axis). In our experiment, κxy/T is observed to be strongly temperature dependent between 0.5 and 10 K. We show that its temperature profile matches the distinct form expected for topological bosonic modes in a Chern-insulator-like model. Our analysis yields magnon band energies in agreement with spectroscopic experiments. At high B, the spin excitations evolve into magnon-like modes with a Chern number of ~1. The bosonic character is incompatible with half-quantization of κxy/T.

Entanglement Negativity and Concurrence in Some Low-Dimensional Spin Systems.

The influence of magnon bands on entanglement in the antiferromagnetic XXZ model on a triangular lattice, which models the bilayer structure consisting of an antiferromagnetic insulator and normal metal, is investigated. This effect was studied in ferromagnetic as well as antiferromagnetic triangular lattices. Quantum entanglement measures given by the entanglement negativity have been studied, where a magnon current is induced in the antiferromagnet due to interfacial exchange coupling between localized spins in the antiferromagnet and itinerant electrons in a normal metal. Moreover, quantum correlations in other frustrated models, namely the metal-insulation antiferromagnetic bilayer model and the Heisenberg model with biquadratic and bicubic interactions, are analyzed.

Exact results for the orbital angular momentum of magnons on honeycomb lattices

We obtain exact results for the orbital angular momentum (OAM) of magnons at the high symmetry points of ferromagnetic (FM) and antiferromagnetic (AF) honeycomb lattices in the presence of Dzyallonshinskii–Moriya (DM) interactions. For the FM honeycomb lattice in the absence of DM interactions, the values of the OAM at the corners of the Brillouin zone (BZ) (, ) are alternately for both magnon bands. The presence of DM interactions dramatically changes those values by breaking the degeneracy of the two magnon bands. The OAM values are alternately and 0 for the lower magnon band and and 0 for the upper magnon band. For the AF honeycomb lattice, the values of the OAM at the corners of the BZ are on one of the degenerate magnon bands and on the other, where κ measures the anisotropy and the result is independent of the DM interaction.

Krein-unitary Schrieffer-Wolff transformation and band touchings in bosonic Bogoliubov–de Gennes and other Krein-Hermitian Hamiltonians

Krein-Hermitian Hamiltonians, i.e., Hamiltonians Hermitian with respect to an indefinite inner product, have emerged as an important class of non-Hermitian Hamiltonians in physics, encompassing both single-particle bosonic Bogoliubov-de Gennes (BdG) Hamiltonians and so-called "$PT$-symmetric" non-Hermitian Hamiltonians. In particular, they have attracted considerable scrutiny owing to the recent surge in interest for boson topology. Motivated by these developments, we formulate a perturbative Krein-unitary Schrieffer-Wolff transformation for finite-size dynamically stable Krein-Hermitian Hamiltonians, yielding an effective Hamiltonian for a subspace of interest. The effective Hamiltonian is Krein Hermitian and, for sufficiently small perturbations, also dynamically stable. As an application, we use this transformation to justify codimension-based analyses of band touchings in bosonic BdG Hamiltonians, which complement topological characterization. We use this simple approach based on symmetry and codimension to revisit known topological magnon band touchings in several materials of recent interest.

Omnidirectional flat bands in chiral magnonic crystals

The magnonic band structure of two-dimensional chiral magnonic crystals is theoretically investigated. The proposed metamaterial involves a three-dimensional architecture, where a thin ferromagnetic layer is in contact with a two-dimensional periodic array of heavy-metal square islands. When these two materials are in contact, an anti-symmetric exchange coupling known as the Dzyaloshinskii–Moriya interaction (DMI) arises, which generates nonreciprocal spin waves and chiral magnetic order. The Landau–Lifshitz equation and the plane-wave method are employed to study the dynamic magnetic behavior. A systematic variation of geometric parameters, the DMI constant, and the filling fraction allows the examination of spin-wave propagation features, such as the spatial profiles of the dynamic magnetization, the isofrequency contours, and group velocities. In this study, it is found that omnidirectional flat magnonic bands are induced by a sufficiently strong Dzyaloshinskii–Moriya interaction underneath the heavy-metal islands, where the spin excitations are active. The theoretical results were substantiated by micromagnetic simulations. These findings are relevant for envisioning applications associated with spin-wave-based logic devices, where the nonreciprocity and channeling of the spin waves are of fundamental and practical scientific interest.

Topological phase transition in magnon bands in a honeycomb ferromagnet driven by sublattice symmetry breaking

Ferromagnetic honeycomb systems are known to exhibit a magnonic topological phase under the existence of the next-nearest neighbor Dzyaloshinskii-Moriya interaction (DMI). Motivated by the recent progress in the sublattice-specific control of magnetic anisotropy, we study the topological phase of magnon bands of honeycomb ferromagnetic monolayer and bilayer with the sublattice symmetry breaking due to the different anisotropy energy in the presence of the DMI. We show that there is a topological phase transition between the topological magnon insulator and the topologically trivial magnon phase driven by the change of the relative size of the DMI and the anisotropy differences between the sublattices. The magnon thermal Hall conductivity is proposed as an experimental probe of the magnon topology.

Large Photogalvanic Spin Current by Magnetic Resonance in Bilayer Cr Trihalides.

Spin current is a key to realizing various phenomena and functionalities related to spintronics. Recently, the possibility of generating spin current through a photogalvanic effect of magnons was pointed out theoretically. However, neither a candidate material nor a general formula for calculating the photogalvanic spin current in materials is known so far. In this Letter, we develop a general formula for the photogalvanic spin current through a magnetic resonance process. This mechanism involves a one-magnon excitation process in contrast to the two-particle processes studied in earlier works. Using the formula, we show that GHz and THz waves create a large photogalvanic spin current in the antiferromagnetic phase of bilayer CrI_{3} and CrBr_{3}. The large spin current arises from an optical process involving two magnon bands, which is a contribution unknown to date. This spin current appears only in the antiferromagnetic ordered phase and is reversible by controlling the order parameter. These results open a route to material design for the photogalvanic effect of magnetic excitations.

Spin-wave nonreciprocity and formation of lateral standing spin waves in CoFeB/Ta/NiFe meander-shaped films

Studying the spin-wave (SW) propagation in 3D periodic structures opens new possibilities for joining functional units placed on the different layers of the magnonic circuitry. In the path toward 3D magnonics, the main challenge is the fabrication of large-scale 3D magnetic structures with nanometric precision control of geometry and material composition. In this work, we study the dependence on the Ta spacer thickness of the magnonic band structure, measured by Brillouin light scattering spectroscopy, of CoFeB/Ta/NiFe meander-shaped bilayers fabricated on pre-patterned Si substrate with thickness steps of 50 nm. Both propagating and stationary SW modes are observed. While the frequency of the dispersive mode slightly depends on the Ta spacer thickness, the frequency position of the three stationary modes in the lowest frequency range of the spectra significantly increases by increasing the Ta thickness. Micromagnetic calculations indicate that each of the three stationary modes is composed of a doublet of modes whose frequency separation, within each doublet, increases by increasing the mode frequency. The origin of this frequency separation is ascribed to the dynamic dipolar coupling between the magnetic layers that generate a significant frequency nonreciprocity of counterpropagating SWs. For these reasons, the investigated structures offer potential application as the nonreciprocal versatile interconnections performing the frequency selective regimes of signal propagation in magnonic circuits.

Theory of ultrasound propagation in LuCo3 near the low-spin–high-spin crossover

The possibility of experimental observation of the ultrasonic attenuation in the ferromagnet $\mathrm{LuCo}{}_{3}$ near the low-spin-high-spin crossover is discussed. We show that ultrasound propagation gives rise to transitions between states of the magnon band due to absorption of phonons, and this process is highly sensitive to the value of magnetization. The high magnetic field, which governs the crossover, alters the ultrasound propagation regime from off-resonant to resonant and we formulate a criterion of the change. Calculated temperature and field dependences of the ultrasonic wave number and attenuation clearly demonstrate anomalies in these characteristics in the vicinity of the crossover at intermediate temperatures far below the Curie temperature.

Quantum topological phase transitions in skyrmion crystals

Topological order is important in many aspects of condensed matter physics, and has been extended to bosonic systems. In this Letter we report on the nontrivial topology of the magnon bands in two distinct quantum skyrmion crystals appearing in zero external magnetic field. This is revealed by nonzero Chern numbers for some of the bands. As a bosonic analog of the quantum anomalous Hall effect, we show that topological magnons can appear in skyrmion crystals without explicitly breaking time-reversal symmetry with an external magnetic field. By tuning the value of the easy-axis anisotropy at zero temperature, we find eight quantum topological phase transitions signaled by discontinuous jumps in certain Chern numbers. We connect these quantum topological phase transitions to gaps closing and reopening between magnon bands.

Dipolar spin-waves and tunable band gap at the Dirac points in the 2D magnet ErBr3

Topological magnon insulators constitute a growing field of research for their potential use as information carriers without heat dissipation. We report an experimental and theoretical study of the magnetic ground-state and excitations in the van der Waals two-dimensional honeycomb magnet ErBr3. We show that the magnetic properties of this compound are entirely governed by the dipolar interactions which generate a continuously degenerate non-collinear ground-state on the honeycomb lattice with spins confined in the plane. We find that the magnon dispersion exhibits Dirac-like cones when the magnetic moments in the ground-state are related by time-reversal and inversion symmetries associated with a Berry phase π as in single-layer graphene. A magnon band gap opens when the dipoles are rotated away from this state, entailing a finite Berry curvature in the vicinity of the K and K’ Dirac points. Our results illustrate that the spin-wave dispersion of dipoles on the honeycomb lattice can be reversibly controlled from a magnetic phase with Dirac cones to a topological antiferromagnetic insulator with non-trivial valley Chern number.

Thermal Hall responses in frustrated honeycomb spin systems

We study geometrical responses of magnons driven by a temperature gradient in frustrated spin systems. While Dzyaloshinskii-Moriya (DM) interactions are usually incorporated to obtain geometrically nontrivial magnon bands, here we investigate thermal Hall responses of magnons that do not rely on the DM interactions. Specifically, we focus on frustrated spin systems with sublattice degrees of freedom and show that a nonzero Berry curvature requires breaking of an effective $PT$ symmetry. According to this symmetry consideration, we study the ${J}_{1}\text{\ensuremath{-}}{J}_{2}\text{\ensuremath{-}}{J}_{2}^{\ensuremath{'}}$ Heisenberg models on a honeycomb lattice as a representative example and demonstrate that magnons in the spiral phase support the thermal Hall effect once we introduce a magnetic field and asymmetry between the two sublattices. We also show that driving the magnons by a temperature gradient induces spin current generation (i.e., magnon spin Nernst effect) in the ${J}_{1}\text{\ensuremath{-}}{J}_{2}\text{\ensuremath{-}}{J}_{2}^{\ensuremath{'}}$ Heisenberg models.

Quantum entanglement and magnon Hall effect on the Lieb lattice model

Entanglement of magnons in the nearest-neighbor Heisenberg model on Lieb lattice (LL) with out-of-plane Dzyaloshinskii–Moriya (DM) antisymmetric spin coupling and external magnetic field is studied. We obtain the behavior of the von Neumann entropy (VN) and concurrence as a function of the DM strength, analyzing the effect of magnon bands on quantum entanglement . Furthermore, the quantum correlations in some fermions models such as the two-dimensional non-Hermitian model (NH) on LL lattice and the tight-binding model (TB) on the LL lattice have been also analyzed. The effect of opening of the gap in the spectrum in these models generates an effect on the entanglement quantifiers as von Neumann entropy, concurrence and negativity. • Quantum entanglement on two-dimensional Lieb lattice is studied. • von Neumann entropy, concurrence and entanglement negativity are studied. • Influence of magnon bands on entanglement is investigated.

Topological edge states in dipolar zig-zag stripes

We study the magnon spectrum of stacked zig-zag chains of point magnetic dipoles with an easy axis. The anisotropy due to the dipolar interactions and the two-point basis of the zig-zag chain unit cell combine to give rise to topologically non-trivial magnon bands in 2D zig-zag lattices. Adjusting the distance between the two sublattice sites in the unit cell causes a band touching, which triggers the exchange of the Chern numbers of volume bands switching the sign of the thermal conductivity and the sense of motion of edges modes in zig-zag stripes. We show that these topological features survive when the range of the dipolar interactions is truncated up to the second nearest neighbors.

Steady state entanglement of distant nitrogen-vacancy centers in a coherent thermal magnon bath

We investigate steady state entanglement (SSE) between two nitrogen-vacancy (NV) center defects in a diamond host on an ultrathin yttrium iron garnet (YIG) strip. We determine the dephasing and dissipative interactions of the qubits with the quanta of spin waves (magnon bath) in the YIG depending on the qubit positions on the strip. We show that the magnon's dephasing effect can be eliminated, and we can transform the bath into a multimode displaced thermal state using external magnetic fields. Entanglement dynamics of the qubits in such a displaced thermal bath have been analyzed by deriving and solving the master equation. An additional electric field is considered to engineer the magnon dispersion relation at the band edge to control the Markovian character of the open system dynamics. We determine the optimum geometrical parameters of the system of distant qubits and the YIG strip to get SSE. Furthermore, parameter regimes for which the shared displaced magnon bath can sustain significant SSE against the local dephasing and decoherence of NV centers to their nuclear spin environments have been determined. Along with SSE, we investigate the steady state coherence (SSC) and explain the physical mechanism of how delayed SSE appears following a rapid generation and sudden death of entanglement using the interplay of decoherence-free subspace states, system geometry, displacement of the thermal bath, and enhancement of the qubit dissipation near the magnon band edge. A nonmonotonic relation between bath coherence and SSE is found, and critical coherence for maximum SSE is determined. Our results illuminate the efficient use of system geometry, band edge in bath spectrum, and reservoir coherence to engineer system-reservoir interactions for robust SSE and SSC.

Tunable Magnonic Chern Bands and Chiral Spin Currents in Magnetic Multilayers.

Realization of novel topological phases in magnonic band structures represents a new opportunity for the development of spintronics and magnonics with low power consumption. In this work, we show that in antiparallelly aligned magnetic multilayers, the long-range, chiral dipolar interaction between propagating magnons generates bulk bands with nonzero Chern integers and magnonic surface states carrying chiral spin currents. The surface states are highly localized and can be easily toggled between nontrivial and trivial phases through an external magnetic field. The realization of chiral surface spin currents in this dipolarly coupled heterostructure represents a magnonic implementation of the coupled wire model that has been extensively explored in electronic systems. Our work presents an easy-to-implement system for realizing topological magnonic surface states and low-dissipation spin current transport in a tunable manner.