Magnetic Vortex Research Articles

Dephasing of ion beams as magnetic vortex acceleration regime transitions into a bubble-like field structure

The interaction of an ultra-intense laser pulse with a near critical density target results in the formation of a plasma channel, a strong azimuthal magnetic field and moving vortices. An application of this is the generation of energetic and collimated ion beams via magnetic vortex acceleration. The optimized regime of magnetic vortex acceleration is becoming experimentally accessible with new high intensity laser beamlines coming online and advances made in near critical density target fabrication. The robustness of the acceleration mechanism with realistic experimental conditions is examined with three-dimensional simulations. Of particular interest is the acceleration performance with different laser temporal contrast conditions, in some cases leading to pre-expanded target profiles prior to the arrival of the main pulse. Preplasma effects on the structure of the accelerating fields are explored, including a detailed analysis of the ion beam properties and the efficiency of the process. Improved scaling laws for the magnetic vortex acceleration mechanism, including the laser focal spot size effects, are presented.

Anatomy of the Dynamics of the Nucleation of Skyrmions in Nanodots via the Voltage‐Controlled Magnetic Anisotropy

AbstractElectric fields can be employed to efficiently manipulate spin textures in low‐dimensional magnetic systems. In this work, the field‐free formation of magnetic skyrmions in ferromagnetic‐based patterned nanodots with perpendicular magnetic anisotropy and Dzyaloshinskii–Moriya interaction via the voltage‐controlled magnetic anisotropy is studied. By micromagnetic simulations it is demonstrated that by reducing the magnetic anisotropy via an electric voltage pulse with adequate intensity and raise and decay times, it is possible to achieve 100% skyrmion nucleation probability through an intermediate magnetic vortex. The nucleation path is investigated in a Graphene/Co/Pt nanodot varying Co thickness, temperature, and applied field. A complete nucleation/annihilation process via bipolar voltage pulses is also possible enabling the realization of a writing/deleting logic device. The results reveal the relevance of following a quasi‐equilibrium magnetization dynamical path and elucidates the relevance of the absolute stability of the magnetic skyrmion state against other possible magnetic configurations.

Observation of higher-order gyrotropic modes and energy transfer in cylindrical ferromagnetic nanodots-based square lattices

We investigated and reported on a wide variety of gyrotropic modes in both isolated thick cylindrical magnetic vortices and lattices of such magnetic vortices arranged in square-lattice structures. In significantly thicker magnetic vortices, we see a higher-order flexure modes in addition to the uniform gyrotropic modes. We thoroughly examined the variation of the frequency and intensity of these modes with the thickness of the magnetic nanodots forming a vortex. We specifically looked at how the thickness, diameter, and aspect ratio of a single magnetic vortex and magnetic vortex lattice in various configurations affect the mode frequencies. When the magnetic vortex at the center is excited by an a.c. spin-polarized current with an excitation frequency equal to the collective gyrotropic frequencies of the lattice, we discuss the dynamics of the transfer of magnetic energy at three high symmetry points of the three-dimensional lattice of Permalloy nanodots with a vortex structure. The energy transmission in these lattice systems is estimated using the power and phase distributions for such configurations. Lattice configurations with substantially thicker nanodots consisting of uniform modes and higher-order flexure modes in the Eigen spectrum have transmission with uniform modes in specific directions and suppression in others, acting as a magnonic filter, and no transmission at all with higher-order modes. Such magnonic vortex lattice structures seek to improve the future prospects of technology and provide emerging applications in information processing devices, magnonic filters, three-dimensional waveguides, and magnonic crystals.

Planar scanning probe microscopy enables vector magnetic field imaging at the nanoscale

Abstract Planar scanning probe microscopy is a recently emerging alternative approach to tip-based scanning probe imaging. It can scan an extended planar sensor, such as a polished bulk diamond doped with magnetic-field-sensitive nitrogen-vacancy (NV) centers, in nanometer-scale proximity of a planar sample. So far, this technique has been limited to optical near-field microscopy, and has required nanofabrication of the sample of interest. Here we extend this technique to magnetometry using NV centers, and present a modification that removes the need for sample-side nanofabrication. We harness this new ability to perform a hitherto infeasible measurement - direct imaging of the three-dimensional vector magnetic field of magnetic vortices in a thin film magnetic heterostructure, based on repeated scanning with NV centers with different orientations within the same scanning probe. Our result opens the door to quantum sensing using multiple qubits within the same scanning probe, a prerequisite for the use of entanglement-enhanced and massively parallel schemes.

Impact of submicron Nb3Sn stoichiometric surface defects on high-field superconducting radiofrequency cavity performance

Nb3Sn film coatings have the potential to drastically improve the accelerating performance of Nb superconducting radiofrequency (SRF) cavities in next-generation linear particle accelerators. Unfortunately, persistent Nb3Sn stoichiometric material defects formed during fabrication limit the cryogenic operating temperature and accelerating gradient by nucleating magnetic vortices that lead to premature cavity quenching. The SRF community currently lacks a predictive model that can explain the impact of chemical and morphological properties of Nb3Sn defects on vortex nucleation and maximum accelerating gradients. Both experimental and theoretical studies of the material and superconducting properties of the first 100 nm of Nb3Sn surfaces are complicated by significant variations in the volume distribution and topography of stoichiometric defects. This work contains a coordinated experimental study with supporting simulations to identify how the observed chemical composition and morphology of certain Sn-rich and Sn-deficient surface defects can impact the SRF performance. Nb3Sn films were prepared with varying degrees of stoichiometric defects, and the film surface morphologies were characterized. Both Sn-rich and Sn-deficient regions were identified in these samples. For Sn-rich defects, we focus on elemental Sn islands that are partially embedded into the Nb3Sn film. Using finite element simulations of the time-dependent Ginzburg-Landau equations, we estimate vortex nucleation field thresholds at Sn islands of varying size, geometry, and embedment. We find that these islands can lead to significant SRF performance degradation that could not have been predicted from the ensemble stoichiometry alone. For Sn-deficient Nb3Sn surfaces, we experimentally identify a periodic nanoscale surface corrugation that likely forms because of extensive Sn loss from the surface. Simulation results show that the surface corrugations contribute to the already substantial drop in the vortex nucleation field of Sn-deficient Nb3Sn surfaces. This work provides a systematic approach for future studies to further detail the relationship between experimental Nb3Sn growth conditions, stoichiometric defects, geometry, and vortex nucleation. These findings have technical implications that will help guide improvements to Nb3Sn fabrication procedures. Our outlined experiment-informed theoretical methods can assist future studies in making additional key insights about Nb3Sn stoichiometric defects that will help build the next generation of SRF cavities and support related superconducting materials development efforts. Published by the American Physical Society 2024

Microscopic examination of rf-cavity-quality niobium films through local nonlinear microwave response

The performance of superconducting radio-frequency (SRF) cavities is sometimes limited by local defects. To investigate the rf properties of these local defects, especially those that nucleate rf magnetic vortices, a near-field magnetic microwave microscope is employed. Local third-harmonic response (P3f) and its temperature dependence and rf power dependence are measured for one Nb/Cu film grown by direct current magnetron sputtering (DCMS) and six Nb/Cu films grown by high-power impulse magnetron sputtering (HiPIMS) with systematic variation of deposition conditions. Five out of the six HiPIMS Nb/Cu films show a strong third-harmonic response that is likely coming from rf vortex nucleation due to a low-Tc surface defect with a transition temperature between 6.3 and 6.8 K, suggesting that this defect is a generic feature of air-exposed HiPIMS Nb/Cu films. A phenomenological model of surface-defect grain boundaries hosting a low-Tc impurity phase is introduced and studied with time-dependent Ginzburg-Landau (TDGL) simulations of probe-sample interaction to better understand the measured third-harmonic response. The simulation results show that the third-harmonic response of rf vortex nucleation caused by surface defects exhibits the same general features as the data, including peaks in third-harmonic response with temperature, and their shift and broadening with higher microwave amplitude. We find that the parameters of the phenomenological model (the density of surface defects that nucleate rf vortices and the depth an rf vortex travels through these surface defects) vary systematically with film deposition conditions. From the point of view of these two properties, the Nb/Cu film that is most effective at reducing the nucleation of rf vortices associated with surface defects can be identified. Published by the American Physical Society 2024

Anomalous Nernst Effect-Based Near-Field Imaging of Magnetic Nanostructures.

The anomalous Nernst effect (ANE) gives rise to an electrical response transverse to magnetization and an applied temperature gradient in a magnetic metal. A nanoscale temperature gradient can be generated by the use of a laser beam applied to the apex of an atomic force microscope tip, thereby allowing for spatially resolved ANE measurements beyond the optical diffraction limit. Such a method has been previously used to map in-plane magnetized magnetic textures. However, the spatial distribution of the out-of-plane temperature gradient, which is needed to fully interpret such ANE-based imaging, was not studied. We therefore use a well-known magnetic texture, a magnetic vortex core, to demonstrate the reliability of the ANE method for imaging of magnetic domains with nanoscale resolution. Moreover, since the ANE signal is directly proportional to the temperature gradient, we can also consider the inverse problem and deduce information about the nanoscale temperature distribution. Our results together with finite element modeling indicate that besides the out-of-plane temperature gradients there are even larger in-plane temperature gradients. Thus, we extend the ANE imaging to study the out-of-plane magnetization in a racetrack nanowire by detecting the ANE signal generated by in-plane temperature gradients. In all cases, a spatial resolution of ≈70 nm is obtained. These results are significant for the rapidly growing field of thermoelectric imaging of antiferromagnetic spintronic device structures.

Suppression of magnetic vortex losses in submicron NbN coplanar waveguide resonators

We present a method for improving the performance of microwave coplanar resonators in magnetic fields, by using narrow superconducting strips of width close to the London penetration depth. In a range of low fields, the narrow strips inhibit the presence of magnetic vortices, thus preventing the generation of losses caused by their motion, leading to enhanced resistance to magnetic fields. Our method provides a more straightforward solution compared to previously proposed techniques designed to restrict vortex motion, holding potential for the development of improved devices based on microwave resonators.

Generation of quasi-monoenergetic proton beams from near-critical density plasmas irradiated by picosecond laser pulses

Laser-driven high-quality ion beams hold immense potential for applications in diverse fields such as tumor therapy, fast ignition, and so on. However, current experimental ion beams are often constrained by either a large energy spread or relatively low energy. In this paper, we proposed a novel scheme for generating quasi-monoenergetic proton beams by irradiating near-critical-density plasmas, which have a density gradient with a picosecond laser pulse. This approach leverages two key aspects: first, the sustained interaction between the laser pulse and the plasma enhances the duration of magnetic vortex acceleration, thereby promoting extended ion acceleration. Second, the utilization of a multi-species target facilitates the formation of a dual-peaked electric field, which leads to the accumulation of protons in the negative gradient of the accelerating phase, resulting in a quasi-monoenergetic proton beam. The two-dimensional particle-in-cell simulation reveals that by employing a laser intensity of 1.37 × 1020 W/cm2 with a pulse duration of 0.5 ps, we can achieve a carbon ion beam with an energy of 50 MeV/u, and a quasi-monoenergetic proton beam exhibiting a cutoff energy of 160 MeV/u, a peak energy of 75 MeV/u, an energy spread of 3.1 %, and an angle divergence of ∼ 3.2°. Furthermore, the quasi-monoenergetic property is corroborated in three-dimensional simulation results, underscoring the robustness and effectiveness of our proposed scheme.

Superconducting multi-vortices and a novel BPS bound in chiral perturbation theory

We derive a novel BPS bound from chiral perturbation theory minimally coupled to electrodynamics at finite isospin chemical potential. At a critical value of the isospin chemical potential, a system of three first-order differential field equations (which implies the second-order field equations) for the gauge field and the hadronic profile can be derived from the requirement to saturate the bound. These BPS configurations represent magnetic multi-vortices with quantized flux supported by a superconducting current. The corresponding topological charge density is related to the magnetic flux density, but is screened by the hadronic profile. Such a screening effect allows to derive the maximal value of the magnetic field generated by these BPS magnetic vortices, being Bmax = 2, 04 × 1014 G. The solution for a single BPS vortex is discussed in detail, and some physical consequences, together with the comparison with the magnetic vortices in the Ginzburg-Landau theory at critical coupling, are described.

Dual Frequency-Regulated Magnetic Vortex Nanorobots Empower Nattokinase for Focalized Microvascular Thrombolysis.

Magnetic nanorobots are emerging players in thrombolytic therapy due to their noninvasive remote actuation and drug loading capabilities. Although the nanorobots with a size under 100 nm are ideal to apply in microvascular systems, the propulsion performance of nanorobots is inevitably compromised due to the limited response to magnetic fields. Here, we demonstrate a nattokinase-loaded magnetic vortex nanorobot (NK-MNR) with an average size around 70 nm and high saturation magnetization for mechanical propelling and thermal responsive thrombolysis under a magnetic field with dual frequencies. The nanorobots are stable in suspension and undergo the magneto-steered assembly into chain-like NK-MNRs, which are regulated to generate magnetic forces to mechanically damage and penetrate the thrombus by the low-frequency rotating magnetic field. Synergistically, enhanced magnetic hyperthermia is triggered by an alternating magnetic field of high frequency, enabling heat-induced NK release and fibrinolysis. In this dual frequency-regulated magnetothrombolysis (fRMT) strategy, nanorobots collaborate under the dual magnetic energy conversion model to achieve the vasculature recanalization rate of 81.0% in thrombotic mice. Overall, the nanorobot with the special magnetic vortex property and multimodel controls is a promising nanoplatform for in vivo focalized microvascular thrombolysis.

Thermal gradient-induced critical current degradation in mesoscopic superconducting thin film

Abstract Superconducting materials inevitably suffer from the sudden change of temperature in localized areas in practical applications, and the concomitant thermal gradient may be detrimental to their performance. Critical current density is a key factor affecting the performance of superconductors. However, the effect of thermal gradient on the critical current density has not been identified. Here, by combining the time-dependent Ginzburg–Landau equations and the heat transfer equation, the thermal gradient and magnetic field dependence of the critical current density are systematically investigated and rationalized by exploring the behavior of vortex and magnetization. For lower magnetic fields, it is found that the thermal gradients strongly reduce the local surface barriers, which inhibits vortex entry and movement, leading to a rapid deterioration of the current-carrying capability. Under moderate magnetic fields, the critical current density corresponding to higher thermal gradients decreases more slowly with increasing magnetic field, which results from the thermal gradient-induced entry and moving of vortices along the current direction. As the magnetic field continues to increase, the variation of the critical current density transitions into a platform period and even slightly rises. The enhanced critical current is primarily attributed to the excess entry of vortices, which increases the surface barrier of the sample. With the further increase in the magnetic field, the critical current density continues to decrease due to increased magnetic field penetration. These results unveil the fundamental interplay between thermal gradients, external magnetic field, vortex, magnetization and critical current density, and provide a theoretical basis for understanding the heat-induced quenching of mesoscopic superconducting thin films in practical applications.

Magnetic vortex γ-Fe2O3 nanospheres decorated with gold nanoparticles for dual hyperthermia treatment

In this work, multifunctional systems with potential applications for dual control of thermal heat delivery are developed. For this purpose, the nanosystems produced consist of vortex iron oxide nanospheres (VIONS) decorated with different amounts of gold nanoparticles (AuNPs). The VIONS were synthesized using the solvothermal reduction method, resulting in a 204 ± 24 nm diameter and meeting the requirements for biomedical applications. Magnetic measurements revealed that these systems are composed mainly of maghemite (γ-Fe2O3), exhibiting relatively low coercivity and moderate saturation magnetization, both of which serve as indicative attributes of an exceptional magnetic vortex state as validated by electron holography microscopy. The decoration with gold NPs was achieved through deposition-precipitation, involving the deposition of gold hydroxide on the surface of the previously amine-modified iron oxide NPs, followed by the concurrent reduction of Au3+. Furthermore, the gold NP size modulation was investigated by consecutively adding Au3+ to obtain gold NPs that interact with light differently depending on their size. The study provides crucial information that can aid the decoration of magnetic iron oxide nanospheres with AuNPs with tailored magnetic and optical properties; consequently, they may be promising candidates for magnetic and photothermal hyperthermia based on three-dimensional magnetic vortex structures.

Chirality Control of Magnetic Vortices in Ferromagnetic Disk–Nanowire System

The results of experimental studies and micromagnetic modeling of magnetic states in a one-dimensional array are presented. The array has the form of a chain of ferromagnetic disks coupled with a ferromagnetic nanowire made of the same material. The disks are located on opposite sides of the nanowire, which makes it possible to obtain distributions when the chiralities of the magnetic vortex shells in neighboring disks alternate, which can find application in vortex spin nanooscillators. Using the application in situ of a magnetic field to an excited objective lens using Lorentz transmission electron microscopy, it is shown that in this system it is possible to control the chiralities of the shells of magnetic vortices, which is realized by magnetization in the sample plane along various azimuthal directions. When wire magnetized along a nanowire, vortex states with opposite chiralities are realized in disks located on opposite sides of it. An antivortex is formed in the nanowire itself at the boundary with the disk, since the local direction of magnetization in the wire and in the disk are anticollinear. When magnetized perpendicular to the nanowire, states with the same chirality are realized in all disks. In this case, two perpendicular domain walls are formed between the disks in the nanowire, and the vortex in the disk is shifted to one of the edges along the nanowire.

Excitation of the Gyrotropic Mode in a Magnetic Vortex by Time-Varying Strain.

We demonstrate the excitation of the gyrotropic mode in a magnetostrictive vortex by time-varying strain. The vortex dynamics is driven by a time-varying voltage applied to the piezoelectric substrate and detected electrically by spin rectification at subthreshold values of rf current. When the frequency of the time-varying strain matches the gyrotropic frequency at a given in-plane magnetic field, the strain-induced in-plane magnetic anisotropy leads to a resonant excitation of the gyration dynamics in the magnetic vortex. We show that nonlinear gyrotropic dynamics can be excited already for moderate amplitudes of the time-varying strain.

Steerable current-driven emission of spin waves in magnetic vortex pairs.

The efficient excitation of spin waves is a key challenge in the realization of magnonic devices. We demonstrate current-driven generation of spin waves in antiferromagnetically coupled magnetic vortices. We use time-resolved x-ray microscopy to directly image the emission of spin waves upon the application of alternating currents flowing directly through the magnetic stack. Micromagnetic simulations allow us to identify the current-driven Oersted field as the main origin of excitation, in contrast to spin-transfer torques. In our case, these internal Oersted fields have an orders of magnitude higher spin-wave excitation efficiency than commonly used stripline antennas. For magnetostrictive materials, we furthermore demonstrate that the direction of magnon propagation can be steered by increasing the excitation amplitude, which modifies the underlying magnetization profile through an additional anisotropy. The demonstrated methods allow for the efficient and tunable excitation of spin waves, marking a substantial advance concerning the design of magnonic devices.

From Magnetostatics to Topology: Antiferromagnetic Vortex States in NiO‐Fe Nanostructures

AbstractMagnetic vortices are topological spin structures frequently found in ferromagnets, yet novel to antiferromagnets. By combining experiment and theory, it is demonstrated that in a nanostructured antiferromagnetic‐ferromagnetic NiO(111)‐Fe(110) bilayer, a magnetic vortex is naturally stabilized by magnetostatic interactions in the ferromagnet and is imprinted onto the adjacent antiferromagnet via interface exchange coupling. Micromagnetic simulations are used to construct a corresponding phase diagram of the stability of the imprinted antiferromagnetic vortex state. The in‐depth analysis reveals that the interplay between interface exchange coupling and the antiferromagnet magnetic anisotropy plays a crucial role in locally reorienting the Néel vector out‐of‐plane in the prototypical in‐plane antiferromagnet NiO and thereby stabilizing the vortices in the antiferromagnet.

Micromagnetic analysis of magnetic vortex dynamics for reservoir computing

Reservoir computing (RC) has generated significant interest for its ability to reduce computational costs compared to traditional neural networks. The performance of the RC element is quantified by its memory capacity (MC) and prediction capability. In this study, we utilize micromagnetic simulations to investigate a magnetic vortex based on a permalloy ferromagnetic layer and its dynamics in RC. The nonlinear dynamics of the vortex core (VC), driven by continuous oscillating magnetic fields and binary digit data as spin-polarized current pulses, are analyzed. The highest MC observed is 4.1, corresponding to the nonlinear VC dynamics. Additionally, the prediction capability is evaluated using the Nonlinear Auto-Regressive Moving Average 2 task, demonstrating a normalized mean squared error of 0.0241 highlighting the time-series data prediction performance of the vortex as a reservoir.

Vortex superlattice induced second-order topological mid-gap states in first-order topological insulators and superconductors

Topological defects such as vortex and dislocations, support zero-energy localized states as a reflection of the bulk topology, in first-order topological insulators and superconductors. Furthermore, emergent first-order topological mid-gap states have been discovered driven by the magnetic vortex superlattice. However, whether the higher-order topological mid-gap states would emerge from the first-order topological insulators and superconductors with the vortex superlattice remains elusive. In this work, we propose vortex superlattice could induce second-order topological mid-gap states with staggered lattice spacings for vortices in first-order topological insulators and superconductors. These higher-order topological mid-gap states originate from the staggered tunneling between vortex-induced bound states and the emergent π flux on vortex superlattices, as an intrinsic exhibition of the interplay between vortices and bulk topology for the first-order topological states. Our work uncovers higher-topological characteristics of topological-defect superlattice in first-order topological states, and develops a controllable environment for the creation and exploration of higher-order topological states.

Higher Order Topological Defects in a Moiré Lattice

AbstractTopological defects are ubiquitous, they manifest in a wide variety of systems such as liquid crystals, magnets or superconductors. The recent quest for non‐abelian anyons in condensed matter physics stimulates the interest for topological defects since they can be hosted in vortices in quantum magnets or topological superconductors. In addition to these vortex defects, this study proposes to investigate edge dislocations in 2D magnets as new building blocks for topological physics since they can be described as vortices in the structural phase field. It demonstrates the existence of higher order topological dislocations within the higher order moiré pattern of the van der Waals 2D magnet CrCl3 deposited on Au(111). Surprisingly, these higher order dislocations arise from ordinary simple edge dislocations in the atomic lattice of CrCl3. This study provide a theoretical framework explaining the higher order dislocations as vortices with a winding Chern number of 2. It is expected that these original defects can stabilize some anyons either in a 2D quantum magnet or within a 2D superconductor coupled to it.