Magnetic Domain Research Articles

Switchable-magnetization planar probe MFM sensor for imaging magnetic textures of complex metal oxide perovskite

We introduce an alternative method for switching-magnetization magnetic force microscopy that utilizes planar tip-on-chip probes. Unlike conventional needle-like tips, the planar probe technique incorporates a microdevice near the tip apex on a 1×1mm2 chip, which allows for thin-film engineering and micro/nano-customization aimed at application-specific tip functionalization. In this study, we establish a microscale current pathway near the tip end to manage the tip magnetization state. This planar probe was used to investigate the intricate disordered magnetic domain structure of an epitaxial thin film of the transition metal oxide perovskite LaMnO3, a material previously demonstrated to exhibit complex domains related to superparamagnetism, antiferromagnetism, and ferromagnetism. We successfully visualized an inhomogeneous distribution of magnetic islands near the Curie temperature, with a resolution exceeding 10nm.

Numerical study of turbulent eddy self-interaction in tokamaks with low magnetic shear. Part I: Linear simulations

Abstract This study examines the impact of low and zero magnetic shear, along with rational values of safety factor, on linear mode behavior in tokamak plasmas. We focus on how magnetic field line topology and parallel domain length influence linear mode structures and growth rates as magnetic shear decreases. Our results
show that as magnetic shear is reduced to low values, linear modes can transition between different branches, significantly affecting their characteristics. At zero magnetic shear, accurate modeling requires precisely capturing magnetic topology, as small deviations near rational surfaces can greatly impact growth rates. These findings are extended to nonlinear simulations in a companion paper (Volčokas, 2024), revealing that long turbulent eddies and magnetic field line topology play a crucial role in turbulence self-interaction and plasma transport.

Anomalous Nernst Effect-Based Near-Field Imaging of Magnetic Nanostructures.

The anomalous Nernst effect (ANE) gives rise to an electrical response transverse to magnetization and an applied temperature gradient in a magnetic metal. A nanoscale temperature gradient can be generated by the use of a laser beam applied to the apex of an atomic force microscope tip, thereby allowing for spatially resolved ANE measurements beyond the optical diffraction limit. Such a method has been previously used to map in-plane magnetized magnetic textures. However, the spatial distribution of the out-of-plane temperature gradient, which is needed to fully interpret such ANE-based imaging, was not studied. We therefore use a well-known magnetic texture, a magnetic vortex core, to demonstrate the reliability of the ANE method for imaging of magnetic domains with nanoscale resolution. Moreover, since the ANE signal is directly proportional to the temperature gradient, we can also consider the inverse problem and deduce information about the nanoscale temperature distribution. Our results together with finite element modeling indicate that besides the out-of-plane temperature gradients there are even larger in-plane temperature gradients. Thus, we extend the ANE imaging to study the out-of-plane magnetization in a racetrack nanowire by detecting the ANE signal generated by in-plane temperature gradients. In all cases, a spatial resolution of ≈70 nm is obtained. These results are significant for the rapidly growing field of thermoelectric imaging of antiferromagnetic spintronic device structures.

Electron states emerging at magnetic domain walls of magnetic semiconductors with strong Rashba effect

Electron states emerging at magnetic domain walls of magnetic semiconductors with strong Rashba effect

Giant antisymmetric magnetoresistance arising across optically controlled domain walls in the magnetic Weyl semimetal Co3Sn2S2

Domain walls (DWs) in magnetic materials host various interesting magneto-transport phenomena. Recent theoretical proposals focusing on DWs of magnetic Weyl semimetals (mWSMs) suggest the emergence of even more exotic transport owing to topologically protected Weyl domains with opposite chirality. However, techniques for controlling and characterizing DWs in mWSMs have not yet matured sufficiently to identify the distinct features of electrical conduction on DWs. Here, by adopting an optical technique to manipulate magnetic domains in mWSM Co3Sn2S2 Hall-bar devices, we discover giant antisymmetric magnetoresistance arising across a DW formed by serially connected upward- and downward-magnetized Weyl domains. This phenomenon originates from the large tangent of the Hall angle associated with the intrinsic anomalous Hall effect in the oppositely magnetized Weyl domains. Furthermore, we quantitatively evaluate DW resistance by systematically controlling the number of DWs. These results underscore the promising avenue of Weyl DW engineering for advanced research on topological magnets.

The influence of laser process parameters on the Iron loss of grain-oriented silicon steel

Laser scribing effectively reduces the energy loss of grain-oriented silicon steel in alternating and pulsating magnetic fields. This study focuses on the 27Q120 material, analyzes the macroscopic surface morphology and iron loss variations of grain-oriented silicon steel under the influence of two types of laser spots (circular spots without the application of a diffractive optical element (DOE) and rectangular spots formed by a DOE), laser power (600W to 2400W), and scribing spacing (3.5mm to 7.5mm) as process parameters. The relationship between magnetic domain width, stress, and iron loss was analyzed. The result shows that the iron loss improvement rates (β) achieved with circular and rectangular spot scribing were 16.054% and 17.116%, respectively. Corresponding magnetic domain widths were 0.17754 mm and 0.1636 mm, with hysteresis losses of 0.5114 W/kg and 0.5033 W/kg, respectively. Under the same laser power and scribing spacing, a lower energy density significantly reduced the damage to the surface macroscopic morphology by the laser, leading to improved iron loss. Furthermore, the iron loss of grain-oriented steel is positively correlated with the width of magnetic domains and negatively correlated with compressive stress.

Magnetic Field Evolution of the Solar Active Region 13664

On 2024 May 10–11, the strongest geomagnetic storm since 2003 November occurred, with a peak Dst index of −412 nT. The storm was caused by NOAA active region (AR) 13664, which was the source of a large number of coronal mass ejections and flares, including 12 X-class flares. Starting from about May 7, AR 13664 showed a steep increase in its size and (free) magnetic energy, along with increased flare activity. In this study, we perform 3D magnetic field extrapolations with the NF2 nonlinear force-free code based on physics-informed neural networks (R. Jarolim et al.). In addition, we introduce the computation of the vector potential to achieve divergence-free solutions. We extrapolate vector magnetograms from the Solar Dynamics Observatory’s Helioseismic and Magnetic Imager at the full 12 minute cadence from 2024 May 5 00:00 to 11 04:36 UT, in order to understand the AR’s magnetic evolution and the large eruptions it produced. A decrease in the calculated relative free magnetic energy can be related to solar flares in ∼90% of the cases, and all considered X-class flares are reflected by a decrease in the relative free magnetic energy. Regions of enhanced free magnetic energy and depleted magnetic energy between the start and end times of major X-class flares show spatial alignment with brightness increases in extreme-ultraviolet observations. We provide a detailed analysis of the X3.9-class flare on May 10, where we show that the interaction between separated magnetic domains is directly linked to major flaring events. With this study, we provide a comprehensive data set of the magnetic evolution of AR 13664 and make it publicly available for further analysis.

Effect of epoxidation level on rheological properties of epoxidized natural rubber-based magnetorheological elastomer

Epoxidized natural rubbers (ENR)are potential to be an alternative of natural rubber as matrix of magnetorheological elastomers (MREs). These ENR-based MREs offer various advantages such as excellent mechanical properties and damping characteristics that are well-suited for applications in vibration control and noise reduction devices. However, there is a paucity information in regard to the effect of different epoxidation levels on rheological properties of MRE. Therefore, the main aim of this study is to explore the influence of epoxidation level on rheological properties of MRE using commercialized ENR corresponding to ENR 25 and ENR 50. ENR-based MREs were created by blending with carbonyl iron particles (CIPs) and other additives, followed by curing at 150 °C for 30 min. The study involved producing ten MRE samples with various weight percentages of CIP (0,10,30,50 and 70 wt%). The storage modulus of ENR 50 exhibited a significant increment from 0.73 MPa to 1.04 MPa as compared to ENR 25 which caused the storage modulus to increase from 0.77 to 0.88 MPa. This showed that ENR 50-based MRE are stiffer in comparison to ENR 25-based MRE. Initial loss modulus value for ENR 50 (0.098 MPa) was lower than that of ENR 25 (0.112 MPa), consequently less energy is dissipated to surrounding for ENR 50-based MRE compare ENR 25-based MRE. The loss factor that represents damping properties showed that ENR 50 reached higher values (0.120 MPa) compared to ENR 25 (0.106 MPa). The increasing of CIPs content from 0 to 70 wt% contributed to increasing of magnetorheological effect for both ENR-based MRE where ENR 25 produced slightly higher with increment of 1.88 % to 22.6 % than ENR 50-based MRE with increment of 2.47 % to 18.18 % due to rise of magnetic forces generated from interaction of magnetic moments in magnetic domains of each CIPs. The results and analysis indicate that different levels of epoxidation in ENR have a marginal impact on the rheological properties of ENR-based MREs.

MHz High Performance of Soft Magnetic Composite with Ordered Domain Structure for Efficient Conversion of Electrical Energy

AbstractSoft magnetic materials are a core element of power electronics and electrical machines. However, none of the soft magnetic materials is able to exploit the full potential of wide bandgap semiconductors, which operate above MHz frequency for efficient energy conversion in power electronic systems. Here, a high‐performance Fe–Si soft magnetic composites with a 2D ordered domain structure are reported, enabling efficient energy conversion at MHz frequencies. By transforming spherical particles into flakes and arranging them in layers, 2D magnetic domains are created within the composite. This leads to a 90% increase in permeability and a tenfold decrease in loss at 3 MHz compared to composite made with spherical particles. The significantly increased cut‐off frequency indicates that the ordered flaky particles are suitable for MHz applications, unlike the disordered spherical particles. These findings provide an effective approach for fabricating high performance soft magnetic composites from traditional spherical particles and miniaturizing magnetic devices for efficient power electronics operation.

Diode and Selective Routing Functionalities Controlled by Geometry in Current-Induced Spin-Orbit Torque Driven Magnetic Domain Wall Devices.

Research on current-induced domain wall (DW) motion in heavy metal/ferromagnet structures is crucial for advancing memory, logic, and computing devices. Here, we demonstrate that adjusting the angle between the DW conduit and the current direction provides an additional degree of control over the current-induced DW motion. A DW conduit with a 45° section relative to the current direction enables asymmetrical DW behavior: for one DW polarity, motion proceeds freely, while for the opposite polarity, motion is impeded or even blocked in the 45° zone, depending on the interfacial Dzyaloshinskii-Moriya interaction strength. This enables the device to function as a DW diode. Leveraging this velocity asymmetry, we designed a Y-shaped DW conduit with one input and two output branches at +45° and -45°, functioning as a DW selector. A DW injected into the junction exits through one branch, while a reverse polarity DW exits through the other, demonstrating selective DW routing.

Decoding the magnetic bit positioning error in a ferrimagnetic racetrack.

Current-driven motion of magnetic domain walls is one of the key technologies for developing storage class memory devices. Extensive studies have revealed a variety of material systems that exhibit high-speed and/or lower power propagation of the domain walls driven by electric current. However, few studies have assessed the reliability of the operations of the memory technology. Here, we decode the errors associated with writing and shifting domain walls using nanosecond current pulses in a ~5-micrometer-wide wire composed of a Pt/GdFeCo bilayer. We find that writing a domain wall at the edge of the wire causes a bit positioning error of ~0.3 micrometers, whereas the shifting process induces an error of ~0.1 micrometers per a 2-nanosecond-long current pulse. The error correlation among successive shifting is negligible when the current drive is sufficiently large. These features allow reliable operation of highly packed domain walls in a ferrimagnetic racetrack.

Magnetometric and seismic investigation of the Nova Colinas impact structure, Parnaíba Basin, Brazil

Nova Colinas (NC) is a complex-type impact structure located in the northeast region of Brazil. It was formed in the volcano-sedimentary strata of the Parnaíba Basin, in the northern part of Western Gondwana. With an apparent diameter of approximately 6.5–7 km, its rim exhibits a distinctive magnetic signal, likely associated to basic volcanic rocks from the Mosquito Formation. These rocks present shock deformation, bracketing the maximum age of the impact event to 197 Ma. We use the magnetometric and seismic methods to establish the geophysical signature of NC and it is the structural framework in subsurface, as well as for characterizing the occurrence and extent of the volcanics. The magnetometric maps present two distinct magnetic domains in the region of NC: (i) the northern area is characterized by short-wavelength magnetic anomalies related to the basaltic flows of the Mosquito Formation; and (ii) the southern region, where sedimentary rocks from the Sambaiba Formation occur, which lacks significant magnetic anomalies, a typical pattern of siliciclastic sedimentary strata. The magnetic sources at the structure's rim reach an estimated depth of ∼250 m, and the position of the rim itself has been effectively established by the total horizontal derivative of the tilt derivative (THDR_TDR) technique. The regional magnetic anomaly suggests a deeper source at the center of the structure, possibly caused by strata with high magnetic susceptibility uplifted in the modification stage of crater formation. Magnetometric modeling using the magnetization vector inversion (MVI) method allowed detailed mapping of the volcanic rocks that form NC's rim. Additionally, analysis of the seismic data allowed the identification of two well-marked horizons, interpreted as diabase sills, located at depths of 600 m and 1200 m, respectively. Impact-related deformation represented by structures such as fractures, a central uplift, and reflector discontinuities associated with faulting, fracturing, and brecciation, were also unveiled by the seismic data, as well as the establishment of the depth of the crystalline basement at ca. 2200 m.

Multiferroic Microstructure Created from Invariant Line Constraint

AbstractFerroic materials enable a multitude of emerging applications, and optimum functional properties are achieved when ferromagnetic and ferroelectric properties are coupled to a first‐order ferroelastic transition. In bulk materials, this first‐order transition involves an invariant habit plane, connecting coexisting phases: austenite and martensite. Theory predicts that this plane should converge to a line in thin films, but experimental evidence is missing. Here, the martensitic and magnetic microstructure of a freestanding epitaxial magnetic shape memory film is analyzed. It is shown that the martensite microstructure is determined by an invariant line constraint using lattice parameters of both phases as the only input. This line constraint explains most of the observable features, which differ fundamentally from bulk and constrained films. Furthermore, this finite‐size effect creates a remarkable checkerboard magnetic domain pattern through multiferroic coupling. The findings highlight the decisive role of finite‐size effects in multiferroics.

Feature extraction and classification of microstructure and magnetic tomography images of an advanced Nd-Fe-B sintered magnet

Abstract Although the microstructure and magnetic tomography images of an advanced Nd-Fe-B sintered magnet were previously reported [Takeuchi, SO., NPG Asia Mater. 14, 70 (2022)], the relationship between these three-dimensional images has not been well analyzed. In this work, a feature extraction method of histogram of oriented gradients and a classification method of uniform manifold approximation and projection are employed for this issue. The microstructural features with superimposing the information of magnetic domain structure are classified into two groups depending on the external magnetic field, resulting in the different microstructural features for the different magnetization states are successfully classified. These differences of the microstructural features are difficult to be found by human recognition. Further detailed analysis of these microstructural features may clarify the key microstructures for the nucleation of reversed domains and their propagations.

Fabrication of Nd-Ho Cosubstituted Co0.5Ni0.5Fe2O4 Nanospinel Ferrites and Exploration of Their Microstructure, Magnetic, and Electromagnetic Characteristics.

The composition and hyperfine structures of Nd3+-Ho3+ ions cosubstituted CoNi nanospinel ferrites (Co0.5Ni0.5NdxHoxFe2-2xO4 (x ≤ 0.05) NSFs) as well as their magnetic and electrodynamic behavior have been presented. The compound Nd-Ho → CoNiFe2O4 (x ≤ 0.05) NSFs were produced using the sol-gel method. XRD powder patterns indicated phase- and substituent-induced modifications of crystallites. The SEM analysis indicated the homogeneous distribution of grains with Nd-Ho cosubstitution. It was found that the values of x had an impact on the hyperfine magnetic field of the A and B sites. The cation distribution was determined by using Mössbauer spectroscopy. The M-H loops' investigations showed that the current NSFs behave ferrimagnetically at both room and low temperatures. An almost continuous rise in the strength of the coercive field was noticed with a rise in Ho-Nd content. The value of calculated squareness ratio values was above 0.5 at both temperatures, entailing that the studied NSFs' structure is made of single magnetic domains. The electromagnetic characteristics of the samples can be explained by the main contribution to electromagnetic absorption being the electric energy losses. Electromagnetic absorbed materials can be applied to provide electromagnetic compatibility and develop functional electromagnetic shields.

Dynamics of converting skyrmion bags with different topological degrees into skyrmions in synthetic antiferromagnetic nanotracks

Skyrmion bags are spin textures with any integer topological degree, which can be driven by spin-polarized currents and generate multiple skyrmions when passing through racetracks with special geometries. We have proposed three nanotrack configurations with different narrow channels on synthetic antiferromagnetic racetracks and investigated the dynamic process of current-induced conversion of skyrmion bags into skyrmions. We have found that when skyrmion bags enter narrow channels, they can be converted into magnetic domains, while when the driving force from spin-transfer torque is strong enough, the magnetic domains can break free from the pinning at the ends of channels and form skyrmions. Both the number of channels and driving current density affect the number of generated skyrmions. As the number of channels rises, magnetic domains split at the junctions of channels, forming more magnetic domains and producing more skyrmions. Furthermore, the number of generated skyrmions is also related to the quantity, arrangement, and interaction forces of inner antiskyrmions. When the number of channels remains constant, the number of antiskyrmions only affects the transition of skyrmion bags to magnetic domains and does not affect the movement of magnetic domains or the transition of magnetic domains to skyrmions. The maximum of generated skyrmions in nanotracks with triple channels reaches 9. Dzyaloshinskii–Moriya interaction and anisotropy may play an important role in the structural stability of skyrmion bags, which can affect the splitting behavior of skyrmion bags. This work is beneficial for the design of artificial synapses and the application of neuromorphic computing based on skyrmion bags.

Microstructure, phase compositions, and coercivity evolution in micron-thick SmCo-based permanent magnetic films

Permanent magnetic thick films are increasingly used in Micro-Electro-Mechanical Systems (MEMS) devices, but the interplay between magnetic properties, microstructure, and film thickness remains underexplored. We deposited SmCo-based films with thicknesses ranging from 350 nm to 1300 nm using magnetron sputtering at room temperature, followed by in-situ annealing. Our study examined the evolution of microstructure, phase composition, magnetic properties, and domain structures as thickness increases. The films displayed dense, fibrous structures typical of the zone T-type region, with 3D morphologies forming a network structure and an arc-shaped surface that expands with thickness. At thinner levels (around 350 nm), an amorphous SmCo phase predominates, prone to oxidation, while at greater thicknesses, the SmCo5 phase dominates but maintains a grain size of 12–15 nm. Coercivity decreases significantly from 33 kOe to 8 kOe as thickness increases from 630 to 1300 nm due to the diminishing pinning effect and dominance of the reversal domain nucleation mechanism. Analysis using magnetic force microscopy and micromagnetic simulations indicates that this reduction in coercivity is mainly due to the decomposition of the SmCo5 phase and a reduction in magnetic domain size.

Strain-controlled switching of magnetic skyrmioniums in ultrathin nanodisks

Magnetic skyrmions and skyrmioniums have garnered significant attention due to their distinctive topologically nontrivial spin structures. Gaining a deep understanding of the magnetization dynamics of these structures and their interconversion processes is essential for fully leveraging their potential in magnetic storage technology. Here, the dynamics of strain-controlled generation and annihilation of skyrmions and skyrmioniums are investigated using phase field simulation methods. It is discovered that tensile strain can induce the transformation of a single domain into skyrmions and skyrmioniums, which can still exist stably after the strain is released. Notably, skyrmioniums demonstrate robust stability within a specific strain window of −0.2% to 0.5%. Beyond this, escalating the compressive strain magnitude induces a phase transition from skyrmioniums to skyrmions, culminating in a direct collapse to a single-domain state at a critical compressive strain of −0.8%. This study reveals that strain can effectively control a variety of topological magnetic domain structures and achieve their interconversion, providing guidance for the design of low-power, nonvolatile, multi-state spin storage devices.

Imaging magnetic transition of magnetite to megabar pressures using quantum sensors in diamond anvil cell

High-pressure diamond anvil cells have been widely used to create novel states of matter. Nevertheless, the lack of universal in-situ magnetic measurement techniques at megabar pressures makes it difficult to understand the underlying physics of materials’ behavior at extreme conditions, such as high-temperature superconductivity of hydrides and the formation or destruction of the local magnetic moments in magnetic systems. Here, we break through the limitations of pressure on quantum sensors by modulating the uniaxial stress along the nitrogen-vacancy axis and develop the in-situ magnetic detection technique at megabar pressures with high sensitivity (~1μT/Hz\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\\sim 1{{{\\rm{\\mu }}}}{{{\\rm{T}}}}/\\sqrt{{{{\\rm{Hz}}}}}$$\\end{document}) and sub-microscale spatial resolution. By directly imaging the magnetic field and the evolution of magnetic domains, we observe the macroscopic magnetic transition of Fe3O4 in the megabar pressure range from ferrimagnetic (α-Fe3O4) to weak ferromagnetic (β-Fe3O4) and finally to paramagnetic (γ-Fe3O4). The scenarios for magnetic changes in Fe3O4 characterized here shed light on the direct magnetic microstructure observation in bulk materials at high pressure and contribute to understanding magnetism evolution in the presence of numerous complex factors such as spin crossover, altered magnetic interactions and structural phase transitions.

Direct magnetoelectric coupling in Pr doping Bi6Ti3Fe2O18 relaxor ferroics

Single-phase multiferroics are fractional and rarely meet at room temperature. Direct magnetoelectric coupling in relaxor ferroic phase was observed in Bi6−xPrxTi3Fe2O18 (x = 0.0, 0.3, 0.6, 0.9, and 1.2) films, where the chemical disorder doping-induced effective internal pressure played a key role. It is analytically formulated from the phase-structure shift, ferroelectric domain, and origin of the magnetic order. The strip magnetic domains are broken into a dotted domain structure following a quantitatively increase in lattice stress. A Monte Carlo simulation including stress energy items is used to unveil the hitherto unexplored coupling mechanism by tuning the symmetric exchange restriction of Fe3+–O–Fe3+. Moreover, the observation of coefficient 78.8 mV/cm·Oe at room temperature is intriguing for potential application.