Magnetic Bias Research Articles

Voltage Control of Exchange Bias via Magneto-Ionic Approaches

The exchange bias (EB) effect denotes a magnetic bias phenomenon originating from the interfacial exchange coupling at the ferromagnetic/antiferromagnetic materials, which plays an indispensable role in the functionality of various devices, such as magnetic random-access memory (MRAM) and sensors. Voltage control of exchange bias offers a promising pathway to significantly reduce device power consumption, effectively fostering the evolution of low-energy spintronic devices. The “magneto-ionic” mechanism, characterized by its operational efficiency, low energy consumption, reversibility, and non-volatility, provides innovative approaches for voltage control of exchange bias and has led to a series of significant advancements. This review systematically synthesizes the research progress on voltage control of exchange bias based on the magneto-ionic mechanism from the perspectives of ionic species, material systems, underlying mechanisms, and performance parameters. Furthermore, it undertakes a comparative evaluation of the voltage-controlled exchange bias by different ions, ultimately providing a forward-looking perspective on the future trajectory of this research domain.

Weak-field FMR and magnetization near the collinear to conical ferrimagnetic phase transition in the U-type hexaferrite Sr4CoZnFe36O60 ceramics

ABSTRACT Temperature evolution of the ferromagnetic resonance (FMR) and its interference with other microwave (MW) magnons near the collinear to conical ferrimagnetic phase transition at T c2 = 305 K is found to correlate with the evolution of the weak-field magnetization: from two components in the conical phase to one component in the collinear phase. The FMR splitting above T c2 correlates with the splitting of the coercive fields of the two magnetization components. A high sensitivity of the FMR to the weak magnetic bias near T c2 is shown to be caused by the gradual transformation of the conical spin magnetic moments to the longitudinal ones. Application of the weak magnetic bias allows to adjust the MW absorption, and its level of above 30 dB is achieved near the FMR frequency (5.7–7.2 GHz), that allows to consider the Sr4CoZnFe36O60 hexaferrite ceramics as a possible MW absorbing material.

Frequency Tunable Film Bulk Acoustic Resonator Integrating PMN‐PT/FSMA Multiferroic Heterostructure for Flexible MEMS

AbstractFrequency tunable flexible piezo resonators exhibit significant potential for technological advances in wearable magnetic field sensing, futuristic wireless telecommunication devices, and flexible micro‐electromechanical systems. This study presents a multifunctional and flexible 0.67Pb(Mg1/3Nb2/3)O3−0.33PbTiO3(PMN‐PT)/Ni50Mn35In15 (Ni‐Mn‐In) multiferroic heterostructure‐based bulk acoustic wave (BAW) resonator fabricated over Kapton substrate. The fundamental resonance frequency (fR = 5.31 GHz) of the resonator is tunable with magnetic and electric fields. A significant change in resonance frequency (ΔfR) of 405 MHz has been achieved with 3.37 Hz nT−1 sensitivity using a direct current (DC) magnetic field of 1200 Oe, attributed to the delta‐E effect. The resonator displays a significant magnetic field tunability of 8.83%. Additionally, a substantial ΔfR of 360 MHz, 36 Hz µV−1 sensitivity and 6.78% tunability is attained with 10 V of DC bias voltage. The impact of magnetic field and DC bias voltage on the acoustic characteristics have been studied by fitting the resonance frequency curves with an equivalent modified Butterworth‐Van Dyke model. The fabricated BAW resonator exhibits outstanding flexibility with no discernible change in fR up to 2000 bending cycles. Such PMN‐PT/Ni‐Mn‐In‐based multiferroic BAW resonators displaying magnetic and electric field tunability are propitious for next‐generation flexible electronics and magnetic field sensors.

A coaxial solid state nonlinear pulse forming line with an exponentially tapered ferrite composite core.

The need to optimize size, weight, and power of high-power microwave (HPM) systems has motivated the development of solid-state HPM sources, such as nonlinear transmission lines (NLTLs), which utilize gyromagnetic precession or dispersion to generate RF. One recent development implemented the NLTL as a pulse forming line (PFL) to form a nonlinear pulse forming line (NPFL) system that substantially reduced the system's size by eliminating the need for a separate PFL; however, matching standard loads can be challenging. This paper describes the development of a tapered NPFL using an exponentially tapered composite based ferrite core containing 60% nickel zinc ferrite (by volume) encased in polydimethylsiloxane (PDMS) and encapsulated in a 5% barium strontium titanate shell. The tapers exponentially change the line's impedance from a 50Ω standard HN connection to 25Ω before tapering back to 50Ω. We characterized the core behavior by obtaining magnetization curves and ferromagnetic resonance measurements. The rise time (10%-90%) of the pulse decreased from ∼6ns for 5kV charging voltage to 1.8ns for 15kV charging voltage. Under unbiased conditions, the system generated HPM with a center frequency of ∼850MHz with a 3 dB bandwidth of 125MHz. Magnetic biases of 15 and 25 kA/m increased the modulation depth and decreased the center frequency to ∼500MHz for 15kV charging voltage.

Magnetically tunable bound states in the continuum with arbitrary polarization and intrinsic chirality

Bound states in the continuum (BICs), which are exotic localized eigenstates embedded in the continuum spectrum and exhibit topological polarization singularities in momentum space, have recently attracted great attention in both fundamental and applied physics. Here, based on a magneto-optical (MO) photonic crystal (PhC) slab placed in external magnetic fields with time-reversal symmetry (TRS) breaking, we theoretically propose magnetically tunable BICs with arbitrary polarization covering the entire Poincaré sphere and efficient off-Γ chiral emission of circularly polarized states (C point). More interestingly, by further breaking the in-plane inversion symmetry of the MO PhC slab to generate a pair of C points spawning from the eliminated BICs and tuning the external magnetic field strength to move one C point to the Γ point, an at-Γ intrinsic chiral BIC exhibits chiral characteristics on both sides of the PhC slab with near-unity circular dichroism exceeding 0.99 and a high-quality factor of 46,000 owing to the preserved out-of-plane mirror symmetry. Moreover, the chirality of the chiral BICs can be inverted by flipping the magnetic bias. Our work opens an unprecedented avenue to explore the unique topological photonics of BICs with broken TRS and promises multiple applications in chiral-optical effects, structured light, and tunable optical devices.

A microsystem for in vivo wireless monitoring of plastic biliary stents using magnetoelastic sensors.

With an interest in monitoring the patency of stents that are used to treat strictures in the bile duct, this paper reports the investigation of a wireless sensing system to interrogate a microsensor integrated into the stent. The microsensor is comprised of a 28-μm-thick magnetoelastic foil with 8.25-mm length and 1-mm width. Magnetic biasing is provided by permanent magnets attached to the foil. These elements are incorporated into a customized 3D polymeric package. The system electromagnetically excites the magnetoelastic resonant sensor and measures the resulting signal. Through shifts in resonant frequency and quality factor, the sensor is intended to provide an early indication of sludge accumulation in the stent. This work focuses on challenges associated with sensor miniaturization and placement, wireless range, drive signal feedthrough, and clinical use. A swine specimen in vivo experiment is described. Following endoscopic implantation of the sensor enabled plastic stent into the bile duct, at a range of approximately 17 cm, the signal-to-noise ratio of ~106 was observed with an interrogation time of 336 s. These are the first reported signals from a passive wireless magnetoelastic sensor implanted in a live animal.

Evidence of Spin Reorientation from Γ4 to Γ2 and Sign Reversal Exchange Bias in CeCrO3 Nanoparticles

Herein, the temperature‐dependent magnetic structure and sign reversal exchange bias in CeCrO3 using magnetization data and time‐of‐flight neutron diffraction data which is given less attention among RCrO3 are investigated. While nuclear structural analysis using Rietveld refinement exhibits distorted orthorhombic structure within Pnma space group, temperature dependence of the magnetic structure using neutron diffraction reveals possible spin configurations, namely, Γ4, Γ2, and Γ1, within the temperature range of 6–300 K. Temperature‐dependent magnetization shows compensation temperature, Tcomp, at 58 K, spin reorientation temperature, TSR, at 15 K along with a Neel temperature, TN, at 260 K which is the outcome of the competition between canted antiferromagnetic ordering of Cr3+ ions and Ce3+ ions in CeCrO3. Furthermore, the magnetization versus magnetic field (M vs H) measurements indicate transition of the Γ4 spin structure to Γ2 spin structure around TSR which is further supported by reversible‐to‐irreversible changes observed in temperature‐dependent MFCC and MFCW. Moreover, a temperature‐driven sign reversal of exchange bias in CeCrO3 is observed, resulting from the competition between antiferromagnetic coupling between chromium moment (MCr) and cerium moment (MCe) in these nanoparticles. This intriguing behavior holds significant potential for the development of thermally assisted magnetic random access memory.

Combining Magnetostriction with Variable Reluctance for Energy Harvesting at Low Frequency Vibrations

In this paper, we explore the benefits of using a magnetostrictive component in a variable reluctance energy harvester. The intrinsic magnetic field bias and the possibility to utilize magnetic force to achieve pre-stress leads to a synergetic combination between this type of energy harvester and magnetostriction. The proposed energy harvester system, to evaluate the concept, consists of a magnetostrictive cantilever beam with a cubic magnet as proof mass. Galfenol, Fe81.6Ga18.4, is used to implement magnetostriction. Variable reluctance is achieved by fixing the beam parallel to an iron core, with some margin to create an air gap between the tip magnet and core. The mechanical forces of the beam and the magnetic forces lead to a displaced equilibrium position of the beam and thus a pre-stress. Two configurations of the energy harvester were evaluated and compared. The initial configuration uses a simple beam of aluminum substrate and a layer of galfenol with an additional magnet fixing the beam to the core. The modified design reduces the magnetic field bias in the galfenol by replacing approximately half of the length of galfenol with aluminum and adds a layer of soft magnetic material above the galfenol to further reduce the magnetic field bias. The initial system was found to magnetically saturate the galfenol at equilibrium. This provided the opportunity to compare two equivalent systems, with and without a significant magnetostrictive effect on the output voltage. The resonance frequency tuning capability, from modifying the initial distance of the air gap, is shown to be maintained for the modified configuration (140 Hz/mm), while achieving RMS open-circuit coil voltages larger by a factor of two (2.4 V compared to 1.1 V). For a theoretically optimal load, the RMS power was simulated to be 5.1 mW. Given the size of the energy harvester (18.5 cm3) and the excitation acceleration (0.5 g), this results in a performance metric of 1.1 mW/cm3g2.

Whole-Head Noninvasive Brain Signal Measurement System with High Temporal and Spatial Resolution Using Static Magnetic Field Bias to the Brain.

Noninvasive brain signal measurement techniques are crucial for understanding human brain function and brain-machine interface applications. Conventionally, noninvasive brain signal measurement techniques, such as electroencephalography, magnetoencephalography, functional magnetic resonance imaging, and near-infrared spectroscopy, have been developed. However, currently, there is no practical noninvasive technique to measure brain function with high temporal and spatial resolution using one instrument. We developed a novel noninvasive brain signal measurement technique with high temporal and spatial resolution by biasing a static magnetic field emitted from a coil on the head to the brain. In this study, we applied this technique to develop a groundbreaking system for noninvasive whole-head brain function measurement with high spatiotemporal resolution across the entire head. We validated this system by measuring movement-related brain signals evoked by a right index finger extension movement and demonstrated that the proposed system can measure the dynamic activity of brain regions involved in finger movement with high spatiotemporal accuracy over the whole brain.

Microwave magnetic excitations in U-type hexaferrite Sr4CoZnFe36O60 ceramics

Microwave (MW) transmission, absorption, and reflection loss spectra of the ferrimagnetic U-type hexaferrite Sr4CoZnFe36O60 ceramics were studied from 100 MHz to 35 GHz at temperatures between 10 and 390 K. Nine MW magnetic excitations with anomalous behavior near ferrimagnetic phase transitions were revealed. They also change under the application of the weak bias magnetic field (0–700 Oe) at room temperature. Six pure magnetic modes are assigned to dynamics of the magnetic domain walls and inhomogeneous magnetic structure of the ceramics, to the natural ferromagnetic resonance (FMR), and to the higher-frequency magnons. Three modes are considered the magnetodielectric ones with the dominating influence of the magnetic properties on their temperature and field dependences. The presence of the natural FMR in all ferrimagnetic phases proves the existence of the non-zero internal magnetization and magnetocrystalline anisotropy. Splitting of the FMR into two components without magnetic bias was observed in the collinear phase and is attributed to a change in the magnetocrystalline anisotropy during phase transition. The high-frequency FMR component critically slows down to phase transition. At room temperature, FMR splitting and essential suppression of the higher-frequency modes were revealed under the weak bias field (300–700 Oe). The highly nonlinear MW response and FMR splitting are caused by the gradual evolution of the polydomain magnetic structure to a monodomain one. The high number of magnetic excitations observed in the MW region confirms the suitability of using hexaferrite Sr4CoZnFe36O60 ceramics as MW absorbers, shielding materials and highly tunable filters.

Development of Reconfigurable High-Frequency Devices Using Liquid Crystal in Substrate-Integrated Gap Waveguide Technology

This article presents the theoretical study, numerical simulation and fabrication of a phase shifter and a stub resonator for use in microstrip ridge gap waveguide (MRGW) technology, using a liquid crystal (LC) in the substrate as a reconfigurable material. The phase shifter and the stub resonator are filled with LC, and thanks to the LC’s dielectric anisotropy properties, the phase shift and the resonance response can be easily controlled using an external electric or magnetic bias field. The phase shifter was designed to operate in the range of 10 to 20 GHz, and the resonator was designed to operate in the range of 7.8 to 8.8 GHz. The phase shifter’s responses (including both phase shift and insertion losses), associated with both the parallel and perpendicular permittivity values of the LC, were computed and measured, and then the corresponding figure of merit (FoM) was extracted. The resonator’s frequency responses, associated with both the LC’s parallel and perpendicular permittivity, were computed. The resonator’s frequency responses, which provided different polarization voltages, were measured and compared to the simulation results. All technological issues related to both prototypes are also discussed here. The good agreement between the simulation and measurement results confirm this technology as a viable approach to the practical implementation of these microwave reconfigurable devices.

Wideband isolator based on one-way surface magnetoplasmons with ultra-high isolation

In this paper, we present a new type of isolator based on one-way surface magnetoplasmons (SMPs) at microwave frequencies, and it is the first time that an experimental prototype of isolator with wideband and ultra-high isolation is realized using SMP waveguide. The proposed model with gyromagnetic and dielectric layers is systematically analyzed to obtain the dispersion properties of all the possible modes, and a one-way SMP mode is found to have the unidirectional transmission property. In simulation and experiment with metallic waveguide loaded with yttrium–iron–garnet (YIG) ferrite, the scattering parameters and the field distributions agree well with the analysis and verify the one-way transmission property. The isolation is found to be as high as 80 dB and the typical value of insertion loss is 1 dB. Besides, the one-way transmission band can be controlled by changing the magnetic bias. From theoretical analysis and simulation, it is found that with a tiny value of 10 Oe of the magnetic bias, the relative bandwidth can be tuned to be greater than 50%. Compared with conventional isolators, this one-way SMP isolator has the advantages of ultra-high isolation, wide relative frequency band, and requires much smaller bias field, which has promising potential in non-reciprocal applications.

Contributions of the extended ELISE and BATMAN Upgrade test facilities to the roadmap towards ITER NBI

ITER’s NBI systems are a first of its kind system with very challenging targets for the RF-driven ion source and the acceleration stage. In a step ladder approach, the ion source test facilities BATMAN Upgrade (BUG) and ELISE support the activities carried out at the Neutral Beam Test Facility, Padua, which is equipped with the ion source facility SPIDER and with MITICA being equivalent to the ITER Heating Neutral Beam injector (HNB), capable of operating at the full power and pulse length of the ITER HNBs. The contributions of the prototype ion source at BUG (1/8 scale) and the size scaling experiment ELISE (1/2 size ITER source) to the roadmap are manifold: for hydrogen operation the ion source performance is demonstrated in several sequential 1000 s pulses, whereas long pulse deuterium operation is limited by the heat load of the co-extracted electrons on the extraction grid. Measures like special magnetic filter field configurations or biasing of surfaces and improved Cs management are identified. Both facilities have recently been extended to full steady state compatibility and very first insights of the ion source performance with steady state extraction compared to the previously used beam blips (10 s extraction every 150 s) are already gained. A pulse length of 400 s, as required for the first deuterium campaigns at ITER, seems to be feasible soon, whereas the one hour pulse imposes the highest challenge to overcome. Investigations on beam divergence revealed a divergence at the upper limit of the acceptable value for the HNB. Measurements on the beam uniformity on the scale of beamlet groups and grid segments at ELISE demonstrated a uniformity of better than the required 90%. BUG and ELISE gave input to recent implementations at SPIDER; MITICA and ITER’s NBI. Still open points and challenges are addressed, for which a continuation of the step ladder approach is essential.

Asymmetric Manipulation of Perpendicular Exchange Bias and Programmable Spin Logical Cells by Spin-Orbit Torque in a Ferromagnet/Antiferromagnet System.

Antiferromagnets are competitive candidates for the next generation of spintronic devices owing to their superiority in small-scale and low-power-consumption devices. The electrical manipulation of the magnetization and exchange bias (EB) driven by spin-orbit torque (SOT) in ferromagnetic (FM)/antiferromagnetic (AFM) systems has become focused in spintronics. Here, the realization of a large perpendicular EB field in Co/IrMn and the effective manipulation of the magnetic moments of the magnetic Co layer and EB field by SOT in Pt/Co/IrMn system is reported. During the SOT-driven switching process, an asymmetrically manipulated state is observed. Current pulses with the same amplitude but opposite directions induce different magnetization states. Magneto-optical Kerr measurements reveal that this is due to the coexistence of stable and metastable antiferromagnetic domains in the AFM. Exploiting the asymmetric properties of these FM/AFM structures, five spin logic gates, namely AND, OR, NOR, NAND, and NOT, are realized in a single cell via SOT. This study provides an insight into the special ability of SOT on AFMs and also paves an avenue to construct the logic-in-memory and neuromorphic computing cells based on the AFM spintronic system.

Wavelet scattering and multiclass support vector machine (WS_MSVM) for effective fault classification in transformers: a real-time experimental approach

The dependable operation of the protective system is affected by residual magnetism and magnetic bias during the activation of the transformer. Challenges arise in distinguishing between inrush current and fault current when the transformer circuit breaker switching angle and remnant flux attain specific values. This situation can lead to a lack of sensitivity or failure in the operation of the transformer protection system. Thus, this paper proposes an effective approach for classifying different faults in transformers (internal and non-internal faults) using wavelet scattering and multiclass support vector machine (MSVM) technique (WS_MSVM). The wavelet scattering method begins by transmitting the data through a sequence of wavelet transforms, nonlinear operations, and averaging processes. This series of operations aims to generate low-variance representations of time series data. Wavelet time scattering produces signal representations that remain unaffected by shifts in the input signal, while still preserving the ability to distinguish between internal and non-internal faults. Internal faults are those occurring within the zones of the current transformer (CT) connected on both sides of the transformer. On the other hand, non-internal faults consist of magnetizing inrush current, sympathetic inrush current, and external faults (faults occurring outside the CT zones). The efficacy of the proposed WS_SVM is evaluated on the real-time experimental results obtained from the differential path of a laboratory transformer. The experimental data generated over one power frequency cycle under diverse operating conditions is employed in MATLAB to assess the effectiveness of the proposed WS_SVM algorithm.

Insights into a Defective Potassium Sulfido Cobaltate: Giant Magnetic Exchange Bias, Ionic Conductivity, and Electrical Permittivity

AbstractThe novel potassium sulfido cobaltate, K2[Co3S4] is introduced, with 25% vacancies of the cobalt positions within a layered anionic sublattice. The impedance and dielectric investigations indicate a remarkable ionic conductivity of 21.4 mS cm−1 at room temperature, which is in the range of highest ever reported values for potassium‐ions, as well as a high electrical permittivity of 2650 at 1 kHz, respectively. Magnetometry results indicate an antiferromagnetic structure with giant intrinsic exchange bias fields of 0.432 and 0.161 T at 3 and 20 K respectively, potentially induced by a combination of the interfacial effect of combined magnetic anionic and nonmagnetic cationic sublattices, as well as partial spin canting. The stability of the exchange bias behavior is confirmed by a training effect of less than 18% upon 10 hysteresis cycles. The semiconductivity of the material is determined, both experimentally and theoretically, with a bandgap energy of 1.68 eV. The findings render this material as a promising candidate for both, active electrode material in potassium‐ion batteries, and for spintronic applications.

Polarization-multiplexed dual-band terahertz beam switching based on magneto-dielectric metasurfaces

Electrically tunable metasurfaces with pixel-level phase control are good candidates for dynamic manipulation of the beam direction in the terahertz band, which is a critical and highly desired technique for next generation communications. Yet the complex biasing, limited aperture and cross talk hinders its progress. In this study, we propose a magnetic-field-globally controlled metasurface for beam switching. The metasurface is composed of a bi-layer silicon metagrating on a magneto-optical substrate InSb. The beam direction is governed by two physical processes: the magnetically-controlled polarization and the polarization-controlled diffraction. By utilizing the circular dichroism and Faraday rotation effects in InSb, the metasurface can operate at two frequency bands. The beam is switched among four directions by properly choosing the magnetic field biasing and the frequency. This study offers a promising solution for beam management using magnetic field biasing and in a global manner.

Terahertz photon to dc current conversion via magnetic excitations of multiferroics

Direct conversion from terahertz photon to charge current is a key phenomenon for terahertz photonics. Quantum geometrical description of optical processes in crystalline solids predicts existence of field-unbiased dc photocurrent arising from terahertz-light generation of magnetic excitations in multiferroics, potentially leading to fast and energy-efficient terahertz devices. Here, we demonstrate the dc charge current generation from terahertz magnetic excitations in multiferroic perovskite manganites with spin-driven ferroelectricity, while keeping an insulating state with no free carrier. It is also revealed that electromagnon, which ranges sub-terahertz to 2 THz, as well as antiferromagnetic resonance shows the giant conversion efficiency. Polar asymmetry induced by the cycloidal spin order gives rise to this terahertz-photon-induced dc photocurrent, and no external magnetic and electric bias field are required for this conversion process. The observed phenomena are beyond the conventional photovoltaics in semi-classical regime and demonstrate the essential role of quantum geometrical aspect in low-energy optical processes. Our finding establishes a paradigm of terahertz photovoltaic phenomena, paving a way for terahertz photonic devices and energy harvesting.

Stabilizing perpendicular magnetic anisotropy with strong exchange bias in PtMn/Co by magneto-ionics

Electric field control of magnetic properties offers a broad and promising toolbox for enabling ultra-low power electronics. A key challenge with high technological relevance is to master the interplay between the magnetic anisotropy of a ferromagnet and the exchange coupling to an adjacent antiferromagnet. Here, we demonstrate that magneto-ionic gating can be used to achieve a very stable out-of-plane (OOP) oriented magnetization with strong exchange bias in samples with as-deposited preferred in-plane (IP) magnetization. We show that the perpendicular interfacial anisotropy can be increased by more than a factor 2 in the stack Ta/Pt/PtMn/Co/HfO2 by applying −2.5 V gate voltage over 3 nm HfO2, causing a reorientation of the magnetization from IP to OOP with a strong OOP exchange bias of more than 50 mT. Comparing two thicknesses of PtMn, we identify a notable trade-off: while thicker PtMn yields a significantly larger exchange bias, it also results in a slower response to ionic liquid gating within the accessible gate voltage window. These results pave the way for post-deposition electrical tailoring of magnetic anisotropy and exchange bias in samples requiring significant exchange bias.

Distributed-Parameter Modeling of High-Power Giant Magnetostrictive Transducers Considering Permanent Magnetic Bias

Distributed-Parameter Modeling of High-Power Giant Magnetostrictive Transducers Considering Permanent Magnetic Bias