Macroscopic Distances Research Articles

Repairable Macroscopic Monodomain Arrays from Block Copolymers Enabled by Photoplastic and Photodielectric Effects

Upon exposure to UV light (120 mW/cm2, λ = 365 nm), a trans-cis isomerization occurs in a cylinder-forming, azobenzene-containing block copolymer of polydimethylsiloxane-b-poly((4(phenyldiazenyl)phenoxy)hexyl acrylate) (PDMS-b-PPHA) that enables the generation of monodomains of healable, long-range ordered arrays of nanoscopic domains over macroscopic distances. The trans-cis isomerization gives rise to a significant increase in the dielectric constant (from 6.52 to 19.8 at 100 Hz, photodielectric behavior) and a dramatic decrease in the Tg (from 54 to 1 °C, photoplastic behavior) of the PPHA block. By combining these characteristics with an in-plane electric field, macroscopic monodomains of near-perfectly aligned cylindrical microdomains are achieved at low temperatures, and a damage repair is clearly uncovered, where the 300 nm wide scratches can be completely healed at 40 °C, leaving a smooth, uniformly thick film where the continuity and orientation of the aligned microdomains are restored. Subsequent exposure to visible light causes a cis-trans isomerization, increasing the matrix Tg to 54 °C, producing highly oriented and aligned PDMS cylindrical microdomains in a PPHA matrix.

Quick Macroscopic Diffusion-Based Molecular Communication With Wavelike Propagation by Use of a Suspension of Relay Cells

In order to enable molecular communication on macroscopic distances without a moving medium, the model of diffusion-based information transmission with a large number of relays suspended in the medium, hence at random positions, is proposed. With an increasing number of relays, the stochastic variations approach zero and the system exhibits a quasi-deterministic behavior. Furthermore, the transmission time becomes inversely proportional to the number of relays and the impulse response independent of the channel length. Thus, the model describes a wave-like propagation, which is fundamentally different from the established flow- and diffusion-based approaches in molecular communication.

Reversal of nanomagnets by propagating magnons in ferrimagnetic yttrium iron garnet enabling nonvolatile magnon memory

Despite the unprecedented downscaling of CMOS integrated circuits, memory-intensive machine learning and artificial intelligence applications are limited by data conversion between memory and processor. There is a challenging quest for novel approaches to overcome this so-called von Neumann bottleneck. Magnons are the quanta of spin waves. Their angular momentum enables power-efficient computation without charge flow. The conversion problem would be solved if spin wave amplitudes could be stored directly in a magnetic memory. Here, we report the reversal of ferromagnetic nanostripes by spin waves which propagate in an underlying spin-wave bus. Thereby, the charge-free angular momentum flow is stored after transmission over a macroscopic distance. We show that the spin waves can reverse large arrays of ferromagnetic stripes at a strikingly small power level. Combined with the already existing wave logic, our discovery is path-breaking for the new era of magnonics-based in-memory computation and beyond von Neumann computer architectures.

Flavor-changing light bosons with accidental longevity

We consider a model with a complex scalar field that couples to (e, μ) or (μ, τ) within the “longevity” window: left[|{m}_{l_1}-{m}_{l_2}|,{m}_{l_1}+{m}_{l_2}right] in which l1 and l2 are the two different charged leptons. Within such a mass window, even a relatively large coupling (e.g. of the size commensurate with the current accuracy/discrepancy in the muon g − 2 experiment) leads to long lifetimes and macroscopic propagation distance between production and decay points. We propose to exploit several existing neutrino experiments and one future experiment to probe the parameter space of this model. For the μ − e sector, we exploit the muonium decay branching ratio and the production and decay sequence at the LSND experiment, excluding the parametric region suggested by gμ − 2 anomaly. For the τ − μ sector, we analyze three main production mechanisms of scalars at beam dump experiments: the Drell-Yan process, the heavy meson decay, and the muon scattering. We explore the constraints from the past CHARM and NuTeV experiments, and evaluate sensitivity for the proposed beam dump experiment, SHiP. The latter can thoroughly probe the parameter space relevant for the gμ− 2 anomaly.

Spatial Spreading of the Condensate of Magnetoexcitons in a Quantum Hall Insulator

The spatial spreading of a dense ensemble of spin cyclotron magnetoexcitons in a quantum Hall insulator at the filling factor ν = 2 is visualized using an optical system with a high aperture ratio. It is found that nondiffusive propagation over macroscopic distances is characteristic not only of excitons with a momentum on the order of the reciprocal magnetic length, which form a coherent condensate of magnetoexcitons, but also of excitons with very low momenta. The nondiffusive propagation of magnetoexciton condensates in real space is accompanied by a huge threshold increase in the amplitude of light reflection from excitations. The possible explanations of the observed behavior are discussed.

Optically trapped room temperature polariton condensate in an organic semiconductor

The strong nonlinearities of exciton-polariton condensates in lattices make them suitable candidates for neuromorphic computing and physical simulations of complex problems. So far, all room temperature polariton condensate lattices have been achieved by nanoimprinting microcavities, which by nature lacks the crucial tunability required for realistic reconfigurable simulators. Here, we report the observation of a quantised oscillating nonlinear quantum fluid in 1D and 2D potentials in an organic microcavity at room temperature, achieved by an on-the-fly fully tuneable optical approach. Remarkably, the condensate is delocalised from the excitation region by macroscopic distances, leading both to longer coherence and a threshold one order of magnitude lower than that with a conventional Gaussian excitation profile. We observe different mode selection behaviour compared to inorganic materials, which highlights the anomalous scaling of blueshift with pump intensity and the presence of sizeable energy-relaxation mechanisms. Our work is a major step towards a fully tuneable polariton simulator at room temperature.

The effective theory of gravity and dynamical vacuum energy

Gravity and general relativity are considered as an Effective Field Theory (EFT) at low energies and macroscopic distances. The effective action of the conformal anomaly of light or massless quantum fields has significant effects on macroscopic scales, due to associated light cone singularities that are not captured by an expansion in local curvature invariants. A compact local form for the Wess-Zumino effective action of the conformal anomaly and stress tensor is given, requiring the introduction of a new light scalar field, which it is argued should be included in the low energy effective action for gravity. This scalar conformalon couples to the conformal part of the spacetime metric and allows the effective value of the vacuum energy, described as a condensate of an exact 4-form abelian gauge field strength F = dA, to change in space and time. This is achieved by the identification of the torsion dependent part of the Chern-Simons 3-form of the Euler class with the gauge potential A, which enters the effective action of the conformal anomaly as a J · A interaction analogous to electromagnetism. The conserved 3-current J describes the worldtube of 2-surfaces that separate regions of differing vacuum energy. The resulting EFT thus replaces the fixed constant Λ of classical gravity, and its apparently unnaturally large sensitivity to UV physics, with a dynamical condensate whose ground state value in empty flat space is Λeff = 0 identically. By allowing Λeff to vary rapidly near the 2-surface of a black hole horizon, the proposed EFT of dynamical vacuum energy provides an effective Lagrangian framework for gravitational condensate stars, as the final state of complete gravitational collapse consistent with quantum theory. The possible consequences of dynamical vacuum dark energy for cosmology, the cosmic coincidence problem, and the role of conformal invariance for other fine tuning issues in the Standard Model are discussed.

Metastability for expanding bubbles on a sticky substrate

We study the dynamical behavior of a one dimensional interface interacting with a sticky impenetrable substrate or wall. The interface is subject to two effects going in opposite directions. Contacts between the interface and the substrate are given an energetic bonus while an external force with constant intensity pulls the interface away from the wall. Our interface is modeled by the graph of a one-dimensional nearest-neighbor path on Z+, starting at 0 and ending at 0 after 2N steps, with the wall being the horizontal axis. At equilibrium each path ξ=(ξx)x=02N is given a probability proportional to λH(ξ)exp(σNA(ξ)), where H(ξ):=#{x:ξx=0} and A(ξ) is the area enclosed between the path ξ and the x-axis. We then consider the classical heat-bath dynamics which equilibrates the value of each ξx at a constant rate via corner-flip. Investigating the statics of the model, we derive the full phase diagram in λ and σ of this model, and identify the critical line which separates a localized phase where the pinning force sticks the interface to the wall and a delocalized one, for which the external force stabilizes ξ around a deterministic shape at a macroscopic distance of the wall. On the dynamical side, we identify a second critical line, which separates a rapidly mixing phase (for which the system mixes in polynomial time) to a slow phase where the mixing time grows exponentially. In this slowly mixing regime, we obtain a sharp estimate of the mixing time on the log scale, and provide evidences of a metastable behavior.

Ensemble origins and distance-dependence of long-range mutational effects in proteins

SummaryMutational effects in globular proteins exhibit an exponential-like decreasing dependence on distance from the mutated site, suggestive of long-range modulation of structural-thermodynamic features. Here, we extract the physical origins of this pattern by employing a statistical-mechanical model to construct conformational ensembles of three archetypal proteins. Through large-scale in silico alanine-scanning mutagenesis, we show that inter-residue differential coupling free energies, which are characteristic ensemble thermodynamic properties, follow a similar exponential distance dependence with the effects felt until ∼15–20 Å from the mutated site. From the perspective of an ensemble-averaged structure, this feature arises via long-range reorganization of the interaction network on mutations which is more significant for charged residues compared to hydrophobic residues. Our work highlights how subtle alterations in the microscopic distribution of states manifest as a macroscopic distance dependence, the physical origins of mutation-induced dynamic allostery, and the necessity to consider the global intra-protein interaction network to understand mutational outcomes.

Topological Order, Quantum Codes, and Quantum Computation on Fractal Geometries

We investigate topological order on fractal geometries embedded in $n$ dimensions. In particular, we diagnose the existence of the topological order through the lens of quantum information and geometry, i.e., via its equivalence to a quantum error-correcting code with a macroscopic code distance or the presence of macroscopic systoles in systolic geometry. We first prove a no-go theorem that $\mathbb{Z}_N$ topological order cannot survive on any fractal embedded in 2D. For fractal lattice models embedded in 3D or higher spatial dimensions, $\mathbb{Z}_N$ topological order survives if the boundaries of the interior holes condense only loop or membrane excitations. Moreover, for a class of models containing only loop or membrane excitations, and are hence self-correcting on an $n$-dimensional manifold, we prove that topological order survives on a large class of fractal geometries independent of the type of hole boundaries. We further construct fault-tolerant logical gates using their connection to global and higher-form topological symmetries. In particular, we have discovered a logical CCZ gate corresponding to a global symmetry in a class of fractal codes embedded in 3D with Hausdorff dimension asymptotically approaching $D_H=2+\epsilon$ for arbitrarily small $\epsilon$, which hence only requires a space-overhead $\Omega(d^{2+\epsilon})$ with $d$ being the code distance. This in turn leads to the surprising discovery of certain exotic gapped boundaries that only condense the combination of loop excitations and gapped domain walls. We further obtain logical $\text{C}^{p}\text{Z}$ gates with $p\le n-1$ on fractal codes embedded in $n$D. In particular, for the logical $\text{C}^{n-1}\text{Z}$ in the $n^\text{th}$ level of Clifford hierarchy, we can reduce the space overhead to $\Omega(d^{n-1+\epsilon})$. Mathematically, our findings correspond to macroscopic relative systoles in fractals.

Observation of heat transport mediated by the propagation distance of surface phonon-polaritons over hundreds of micrometers

Efficient heat dissipation in micro/nano electronics requires long-distance propagation of heat carriers operated above room temperature. However, thermal phonons—the primary heat carriers in dielectric nanomaterials—dissipate the thermal energy after just a few hundred nanometers. Theory predicts that the mean free path of surface phonon-polaritons (SPhPs) can be hundreds of micrometers, which may improve the overall dissipation of heat in nanomaterials. In this work, we experimentally demonstrate such long-distance heat transport by SPhPs. Using the 3ω technique, we measure the in-plane thermal conductivity of SiN nanomembranes for different heater-sensor distances, membrane thicknesses, and temperatures. We find that thin nanomembranes support heat transport by SPhPs, as evidenced by an increase in the thermal conductivity with temperature. Remarkably, the thermal conductivity measured 200 μm away from the heater is consistently higher than that measured 100 μm closer. This result suggests that heat conduction by SPhPs is quasi-ballistically over at least hundreds of micrometers. Our findings pave the way for coherent heat manipulations above room temperature over macroscopic distances, which impacts the applications in thermal management and polaritonics.

Geuine tripartite entanglement in three-flavor neutrino oscillations

The violation of Leggett–Garg inequalities tested the quantumness of neutrino oscillations (NOs) across macroscopic distances. The quantumness can be quantified by using the tools of the quantum resource theories. Recently, a new genuine tripartite entanglement measure (Xie et al. in Phys Rev Lett 127:040403, 2021), concurrence fill, is defined as the square root of the area of the concurrence triangle satisfying all genuine multipartite entanglement conditions. It has several advantages compared to other existing tripartite measures. Here, we focus on using concurrence fill to quantify the tripartite entanglement in three-flavor NOs. Concurrence fill can reach its maximum 0.89 for the experimentally-observed electron antineutrino oscillations, but it cannot for the muon antineutrino oscillations. In both cases, we compare its performance with other three tripartite entanglement measures, including the generalized geometric measure (GGM), the three-pi entanglement, and the genuinely multipartite concurrence (GMC), in the neutrino propagation, and accordingly show that concurrence fill contains the most quantum resource. Furthermore, concurrence fill and the three-pi entanglement are always smooth, while GGM and GMC measures have several sharp peaks. The genuine tripartite quantification of the quantumness of three-flavor NOs represents the first step towards the further potential application of neutrinos on quantum information processing.

An elementary quantum network of entangled optical atomic clocks.

Optical atomic clocks are our most precise tools to measure time and frequency1-3. Precision frequency comparisons between clocks in separate locations enable one to probe the space-time variation of fundamental constants4,5 and the properties of dark matter6,7, to perform geodesy8-10 and to evaluate systematic clock shifts. Measurements on independent systems are limited by the standard quantum limit; measurements on entangled systems can surpass the standard quantum limit to reach the ultimate precision allowed by quantum theory-the Heisenberg limit. Although local entangling operations have demonstrated this enhancement at microscopic distances11-16, comparisons between remote atomic clocks require the rapid generation of high-fidelity entanglement between systems that have no intrinsic interactions. Here we report the use of a photonic link17,18 to entangle two 88Sr+ ions separated by a macroscopic distance19 (approximately 2 m) to demonstrate an elementary quantum network of entangled optical clocks. For frequency comparisons between the ions, we find that entanglement reduces the measurement uncertainty by nearly [Formula: see text], the value predicted for the Heisenberg limit. Today's optical clocks are typically limited by dephasing of the probe laser20; in this regime, we find that entanglement yields a factor of 2 reduction in the measurement uncertainty compared with conventional correlation spectroscopy techniques20-22. We demonstrate this enhancement for the measurement of a frequency shift applied to one of the clocks. This two-node network could be extended to additional nodes23, to other species of trapped particles or-through local operations-to larger entangled systems.

Light-Triggered Manipulations of Droplets All in One: Reversible Wetting, Transport, Splitting, and Merging.

Here, we establish different ways of light-triggered droplet manipulation such as reversible wetting, splitting, merging, and transport. The unique features of our approach are that the changes in the wetting properties of microscopic droplets of isotropic (oil) or anisotropic (liquid crystalline) liquids adsorbed on photoswitchable films can be triggered just by application of soft optical stimuli, which lead to dynamical, reversible changes in the local morphology of the structured surfaces. The adaptive films consist of an azobenzene-containing surfactant ionically attached to oppositely charged polymer chains. Under exposure to irradiation with light, the azobenzene photoisomerizes between two states, nonpolar trans-isomer and polar cis-isomer, resulting in the corresponding changes in the surface energy and orientation of the surfactant tails at the interface. Additionally, the local increase in the surface temperature due to absorption of light by the azobenzene groups enables diverse processes of manipulation of the adsorbed small droplets, such as the reversible increase of the droplet basal area up to 5 times, anisotropic wetting during irradiation with modulated light, and precise partition of the droplet into many small pieces, which can then be merged on demand to the desired number of larger droplets. Moreover, using a moving focused light spot, we experimentally demonstrate and theoretically explain the locomotion of the droplet over macroscopic distances with a velocity of up to 150 μm·s-1. Our findings could lead to the ultimate application of a programmable workbench for manipulating and operating an ensemble of droplets, just using simple and gentle optical stimuli.

Virtual neutrino propagation at short baselines

Within a covariant perturbative field-theoretical approach, the wave-packet modified neutrino propagator is expressed as an asymptotic expansion in powers of dimensionless Lorentz- and rotation-invariant variables. The expansion is valid at high energies and short but macroscopic space-time distances between the vertices of the proper Feynman macrodiagram. In terms of duality between the propagator and the effective neutrino wave packet, at short times and distances, neutrinos are deeply virtual and move quasi-classically. In the lowest-order approximation, this leads to the classical inverse-square dependence of the modulus squared flavor transition amplitude and related neutrino-induced event rate from distance L between the source and detector, and the above-mentioned asymptotics results in the corrections to the classical behavior represented by powers of L^2. This is very different from the long-baseline regime, where similar corrections are given by an asymptotic expansion in inverse powers of L^2. However, in both short- and long-baseline regimes, the main corrections lead to a decrease in number of neutrino events.

Shedding light on the electroweak phase transition from exotic Higgs boson decays at the lifetime frontiers

We study the scenarios where a strongly first-order electroweak phase transition (EWPT) is triggered by a light singlet scalar, which has feeble interactions to the Higgs. Since the singlet scalar is light and has weak couplings, it can decay at a macroscopic distance away from the collision point. Therefore, it can be regarded as a long-lived particles (LLP) in such scenarios. We perform the searches of the LLPs from the exotic Higgs decays, at the FASER, MAPP and CMS-Timing detectors of the 14 TeV HL-LHC, to probe the strongly first-order EWPT. In certain scenarios, we show that the LLP searches can help to reach the parameter space of the strongly first-order EWPT remarkably, where the searches for promptly exotic Higgs decays are not valid.

Drawing at the Nanoscale through Macroscopic Movement.

Nanopatterns are important for applications in various nanodevice fields. Existing nanopatterning techniques mainly directly manufacture the nanopatterns through various lithographic methods, which usually are laborious, time-consuming, and need expensive equipment. Here, an extremely simple drawing at the nanoscale (DAN) concept to indirectly fabricate rational nanopatterns through controlling the macroscopic movement of the substrate , is demonstrated. The structure of the nanopatterns is completely determined by and can be shrunk by millions of times from the moving track of the substrate. Multiple surface nanopatterns of different materials with accurately tailorable relative positions can be simply stacked together by moving the substrate by macroscopic distances during different DAN processes. In combination with sophisticated lithographic methods, the DAN method is anticipated to enable substantial advances in nanofabrication.

Topological graph states and quantum error-correction codes

Deciding if a given family of quantum states is topologically ordered is an important but nontrivial problem in condensed matter physics and quantum information theory. We derive necessary and sufficient conditions for a family of graph states to be in TQO-1, which is a class of quantum error correction code states whose code distance scales macroscopically with the number of physical qubits. Using these criteria, we consider a number of specific graph families, including the star and complete graphs, and the line graphs of complete and completely bipartite graphs, and discuss which are topologically ordered and how to construct the codewords. The formalism is then employed to construct several codes with macroscopic distance, including a three-dimensional topological code generated by local stabilizers that also has a macroscopic number of encoded logical qubits. The results indicate that graph states provide a fruitful approach to the construction and characterization of topological stabilizer quantum error correction codes.

Detection of magnetic force fields at macroscopic distances with a micromechanical cantilever oscillator

We report a procedure for measuring variations of the magnetic field gradients generated by a macroscopic coil. A micromechanical cantilever oscillator covered with a magnetic material is used to detect variations of the magnetic force field at distances exceeding several times the coil diameter (4 mm). The detection is based on the phase of the first eigenmode of the cantilever while modulating the magnetic field at low frequencies. The nanoscale oscillation of the cantilever along with the high-quality resonance factor are responsible for a coherent oscillation allowing high sensitivity. A detection sensitivity, under ambient conditions, of the order of 10−13 T/nm2 is estimated with the help of numerical calculations. The approach is useful for evaluating the spatial variation of the magnetic field gradients generated by any source of magnetic field when the magnetic field can be modified at rates below the resonant frequency of the cantilever. These results can be useful for gradient fields monitoring in macro- and micro-scale magnetic resonance imaging, non-contact electric currents identification from stray magnetic fields, electrical power monitoring, 3D-magnetic fields mapping, or miniature orientation devices.

Trajectories and the perception of classical motion in the free propagation of wave packets

AbstractThe free propagation in time of a normalisable wave packet is the oldest problem of continuum quantum mechanics. Its motion from microscopic to macroscopic distance is the way in which most quantum systems are detected experimentally. Although much studied and analysed since 1927 and presented in many textbooks, here the problem is re‐appraised from the standpoint of semi‐classical mechanics. Particular aspects are the emergence of deterministic trajectories of particles emanating from a region of atomic dimension and the interpretation of the wave function as describing a single particle or an ensemble of identical particles. Of possible wave packets, that of Gaussian form is most studied due to the simple exact form of the time‐dependent solution in real and in momentum space. Furthermore, this form is important in laser optics. Here the equivalence of the time‐dependent Schrödinger equation to the paraxial equation for the propagation of light is demonstrated explicitly. This parallel helps to understand the relevance of trajectory concepts and the conditions necessary for the perception of quantum motion as classical.Key Points The paper addresses a problem of fundamental quantum mechanics, important in both physics and chemistry. Within physics, the subject is relevant to the disciplines of both quantum mechanics and classical optics. The matter presented is topical also for researchers in the history and philosophy of physics.