mA Beam Research Articles

Physical start-up of the Nuclear Subcritical Facility “Neutron Source” of NSC KIPT

National Science Center “Kharkov Institute of Physics and Technology” jointly with the Argonne National Laboratory developed, designed and constructed the Subcritical Nuclear Facility “Neutron source based on the subcritical assembly driven by electron linear accelerator”. The article presents the main results obtained during the physical start-up of the plant, the program of which involved the staged loading of fuel assemblies into the core with subsequent measurements of its neutron-physical characteristics. In total, 37 fuel assemblies of WWR-M2 type were loaded into the facility core. The values o f the effective neutron multiplication factor keff and reactivity ρ of the subcritical assembly were measured after each loading step using the multiplication and area ratio methods. In addition, the neutron flux to electron current ratio method was tested for on-line reactivity monitoring. The investigations were performed when the accelerator was operated with 100 MeV electron beam energy, 2.7 μs electron pulse duration, 20 Hz pulse repetition rate and ≤ 40 mA beam pulse current. The obtained results were analyzed in terms of ensuring the facility nuclear safety at the next stage of its commissioning which is the pilot operation.

Status and Commissioning Plan of Korea-4GSR

Multipurpose Synchrotron Radiation Construction Project is in progress to construct 4th generation storage ring with a 800-m-long circumference in Ochang. Its beam parameter is 4 GeV electron beam energy, lower than 100 pm emittance, 100 mA beam current. Currently, Korea Basic Science Institute is in charge of construction and Pohang Accelerator Laboratory (PAL) is in charge of the accelerator complex and ten beamlines. Recently, PAL is finalizing technical design and producing prototypes. In this report we introduce status and commissioning plan of 4GSR project focusing on beam physics part.

Innovative Cesiation Deriving Incredible 145 mA Beam from J-PARC Cesiated RF-Driven H− Ion Source

In NIBS2022, the stable 8 hours operation of the J-PARC cesiated RF-driven H− ion source (IS) in a test-stand with a 69.9 keV 120 mA beam and a beam duty factor of 4 % (1 ms x 40 Hz) was reported. However, the Cesiation condition was produced after many times and rather large amount of Cs and H2Os injections. The fluctuation of the H− ion beam intensity (IH −) in a pulse and the transverse emittances were rather larger than those for the previous 65 keV 110 mA operation. The plasma electrode temperature (TPE) of 254 °C much higher than that not only for the usual J-PARC IS (about 70 °C) but also for the standard cesiated H− ion sources (180 ∼ 200 °C) suggested the existence of novel H2O mediated cesiation surviving against the high TPE. In this paper, the J-PARC IS improvements based upon a hypothesis of the best cesiation constituted of sub monolayer H2O (chemically bound with Mo) mediated cesiation and Cs half monolayer on remaining surface are presented. The innovative cesiation derived a 76.5 keV 145 mA beam stably with the small beam fluctuation and transverse emittances suitable for Radio Frequency Quadrupole LINACs of high energy LINACs. The measured results of the 145 mA / 83 mA beam, extraction electrode current and RF waveforms, parameter trends of an 8 hours 145 mA operation and the transverse emittances are presented. The optimum TPE was increased from 70 °C to 230 °C. Furthermore, the beam intensity for the J-PARC IS operation energy of 52.5 keV was increased from 72 mA to 83 mA, which was consistent with the 1.5 power perveance law on the beam energy compared with 145 mA for 76.5 keV.

Recent advancements with the H− injector performance for the Spallation Neutron Source operation and upgrade

The Spallation Neutron Source (SNS) located at the Oak Ridge National Laboratory is an accelerator-based, pulsed neutron facility utilized for a broad range of scientific research and industrial applications. In the past 5 years, the facility has reliably been operated at its baseline design beam power of 1.4 MW, and it is currently undertaking an upgrade to double its power to 2.8 MW. A 65-keV H− injector, which comprises an rf-driven H− ion source and an electrostatic low energy beam transport, delivers the required high-current, time-structured H− beam to the accelerator. The H− injector can reliably provide 50-60 mA beam current at 6% duty-factor (1 ms, 60 Hz) for a 3-4 month service cycle. To ensure sufficient operational margins for the SNS routine operations and ongoing upgrade requirements, the injector system has been continuously improved on a R&D test stand. This paper presents the operational status and recent advancements with the injector system performance including the enhanced ion source beam output capability up to ∼110 mA, the improved ion source plasma ignition reliability using a 27.12-MHz RF system, and the upgraded LEBT beam chopper system etc.

Development and commissioning of a hydrogen ion source for the CERN ALPHA experiment

The CERN ALPHA experiment makes precision measurements of antihydrogen atoms held in a superconducting magnetic minimum trap. Recent studies of the antihydrogen spectrum have provided unique tests of fundamental physics, and to improve on these studies ALPHA is now proposing upgrades to directly compare hydrogen and antihydrogen within their existing atom trap. One route towards producing cold, neutral hydrogen atoms is the integration of a hydrogen ion source into the experiment. Ideally, this should provide both positive (H+, H2 +, H3 +) and negative (H-) ions to facilitate different schemes for producing and trapping hydrogen atoms. For compatibility with ALPHA's existing beamlines, the source must produce modest (∼ 10 μA) beam currents at very low final energies (<100 eV). PELLIS, previously developed at JYFL, is a filament-driven ion source that generates 5–10 keV H- beams with small emittances and tens of microamps of beam current. Here, we present a modified PELLIS design to provide both positive and negative hydrogen ions for ALPHA. The use of an electromagnet filter field in PELLIS allows for the optimisation of H- volume production, and also tuning of the positive ion species fraction. We present simulations of H- (and similarly H+) transport through the initial extraction optics, which have been configured for a lower beam energy of 5 keV and designed to match a proposed beamline to interface with ALPHA. We present the results of detailed vacuum simulations that were used to guide the optics design, allowing the source (at 10-2 mbar) to interface with a transport beamline ∼ 0.5 m downstream that has strict vacuum requirements of < 10-9 mbar. We present experimental results from commissioning of the source, and show that it broadly performs as designed for both positive and negative hydrogen ions.

Magnetic Design of the Commutational Magnet and Quadrupoles for PERLE Accelerator

PERLE (Powerful Energy Recovery LINAC for Experiment) is a three turns high-power Energy Recovery LINAC (ERL) facility with 20 mA beam current and beam energy from 250 MeV to 500 MeV. It is a testbed to validate multi-turn high current ERL operation for the future LHeC and will be the first ERL for nuclear applications. In this work, the design and optimization of the commutational magnet (B-com) used to spread/combine the three beams and one series of quadrupole magnets is discussed. The B-com magnet is optimized for a 30° bending angle with harmonic content of 0.036%. The quadrupole magnets generate a field gradient of 34.15 T/m. Further studies to suppress saturation at a maximum gradient of 44.1 T/m are undergoing.

Production of pharmaceutical grade [201Tl]Thallous chloride using 30 MeV cyclotron

Multiple patient doses of [201Tl]TlCl has been produced using electrodeposited enriched 203Tl in 30 MeV cyclotron (Cyclone-30) with 28 MeV proton energy at 50 μA beam current for 8 h. Ion Exchange Column Chromatography (IECC) and liquid-liquid extraction has been employed for semi-automated radiochemical separation and purification of produced [201Tl]TlCl. The produced [201Tl]TlCl was used in coronary artery disease (CAD) patients.

Co-production of 155Tb and 152Tb irradiating 155Gd / 151Eu tandem target with a medium energy α-particle beam

IntroductionFour terbium isotopes 149,152,155,161Tb emitting various types of radiation can be used for both diagnostics and therapy. 152Tb emits positrons and is ideal for PET. 155Tb is considered a promising Auger emitter and a diagnostic pair for other terbium therapeutic isotopes. Several methods for the production of 155Tb using charged particle accelerators have been proposed, but they all have significant limitations. The restricted availability of this isotope hinders its medical applications. We have proposed a new method for production of 155Tb, irradiating enriched 155Gd by alpha particles. The possibility of simultaneous production of two isotopes of terbium, 152,155Tb, was also studied for more efficient cyclotron beam use. MethodsIrradiation of 155Gd enriched targets and 155Gd / 151Eu tandem target with alpha-particles with an energy of 54 MeV was carried out at the U-150 cyclotron at the NRC "Kurchatov Institute". The cross sections of nuclear reactions on enr-155Gd were measured by the stack foil technique, detecting the gamma-radiation of the activation products. The separation of rare earth elements was performed by extraction chromatography with the LN Resin. 155Tb was produced via 155Dy decay. ResultsThe cross sections for the 155,156Tb and 155,157Dy production were measured by the irradiation of a gadolinium target enriched with the 155Gd isotope with alpha-particles in an energy range of 54 → 33 MeV. The yield of 155Dy on a thick target at 54 MeV was 130 MBq/μAh, which makes it possible to obtain 1 GBq of 155Tb in 11 hour-irradiation with 20 μA beam current. The possibility of simultaneous production of 152,155Tb by irradiation of 155Gd and 151Eu tandem target with medium-energy alpha-particles is implemented. Optimal irradiation energy ranges of alpha -particles as 54 → 42 MeV for 155Tb and 42 → 34 MeV for 152Tb were suggested. Product activity and radionuclidic purity were calculated.

120 mA operation of J-PARC cesiated RF-driven H- ion source

The Japan Proton Accelerator Research Complex (J-PARC) cesiated RF-driven H- ion source (IS) has been stably operated for about eight years by using an internal-RF-antenna developed at the Spallation Neutron Source (SNS). From Sep. 2018, the J-PARC 400 MeV LINAC has been steadily operated with the design H- ion beam intensity (IH- ) of 50 mA, when an about 60 mA beam is injected from the IS. At each end of about 3 months J-PARC operation, the IS supplies a 52.5 keV 72 mA beam for the LINAC 60 mA acceleration. The IS superior emittances predicted in a test-stand were proven by the high RFQ acceleration efficiency of 94.3% (IH-RFQ = 67.9 mA). The high intensity beam with transverse emittances suitable for the RFQ is produced with several unique measures, such as, slight water molecules addition into hydrogen plasma, the low temperature (about 70°C) operation of 45°-tapered 16-mm thick plasma electrode with the precise cesium (Cs) density control, the impurity elimination in the hydrogen plasma along with the filter-field optimization, the continuous-wave igniter plasma driven with a 42-W 30-MHz RF, and so on. The 120 mA operation results of the IS in the test-stand are presented in this paper. A 69.9 keV 120 mA H- ion beam, about 107.8 mA of which was inside the transverse emittances used for a common RFQ design, was stably operated with a duty factor of 4% (1 ms × 40 Hz). The IS is the benchmark one for the next generation high energy H- LINACs aiming for 100 mA class intensity.

Development of Allison scanner to measure transverse emittance at low energy beam transport of rare-isotope accelerator complex for ON-line experiments

The Rare-isotope Accelerator complex for ON-line experiments is a heavy-ion accelerator facility that accelerates a stable or rare isotope beam up to 400 kW with an energy of 200 MeV/u. Various heavy-ion beams are generated from the Electron Cyclotron Resonance Ion Source, with an energy of 10 keV/u and separated according to A/Q at the first dipole magnet (DM). To measure beam transverse emittance at the Low Energy Beam Transport section, two Allison scanners are installed behind the DM for the X and Y directions. It consist of a servo motor for driving, a Faraday cup for current measurement, deflection plates, and electronic device. The measurable range of beam angle in of the Allison scanner is determined by the structure of the deflection plate and designed based on mathematical calculations. Experimental Physics and Industrial Control System (EPICS) is adopted to integrate and control a variety of devices. To control the complex measurement sequence of the Allison scanner, an EPICS sequencer module was used. Normalized emittance is calculated by python code with Pyepics module using phase space distribution data. In this paper, we present the detailed design of the Allison scanner, the configuration of the control system, and the experimental results using an Ar9+ 30 μA beam.

H- beam formation simulation in negative ion source for CERN's Linac4 accelerator

The caesiated surface negative ion (H-) source is the first element of CERN's LINAC4 a linear injector designed to accelerate negative hydrogen ions to 160 MeV. The IS03 ion source is operated at 35 mA beam intensity and reliably feeds CERN's accelerator chain, H- ions are generated via plasma volume and caesiated molybdenum (Cs-Mo) plasma electrode surface mechanisms. Studying the beam extraction region of this H- ion source is essential for optimizing the H- production. The 3D Particle-in-cell (PIC) Monte Carlo (MC) code ONIX (Orsay Negative Ion eXtraction [1]), written to study H- beam formation processes in neutral-beam injectors for fusion, has been adapted to single aperture accelerator H- sources. The code was modified to match the conditions of the beam formation and extraction regions of the Linac4 H- source [2]. A set of parameters was chosen to characterize the plasma and to match the specific volume and surface production modes. Simulated results of the extraction regions are presented and benchmarked with experimental results obtained at the Linac4 test stand [3].

Scanning electron microscope imaging by selective e-beaming using photoelectron beams from semiconductor photocathodes

Pulsed electron beams from a photocathode using an InGaN semiconductor have brought selectively scanning technology to scanning electron microscopes, where the electron beam irradiation intensity and area can be arbitrarily selected within the field of view in SEM images. The p-type InGaN semiconductor crystals grown in the metalorganic chemical vapor deposition equipment were used as the photocathode material for the electron beam source after the surface was activated to a negative electron affinity state in the electron gun under ultrahigh vacuum. The InGaN semiconductor photocathode produced a pulsed electron beam with a rise and fall time of 3 ns, consistent with the time structure of the irradiated pulsed laser used for the optical excitation of electrons. The InGaN photocathode-based electron gun achieved a total beam operation time of 1300 h at 15 μA beam current with a downtime rate of 4% and a current stability of 0.033% after 23 cycles of surface activation and continuous beam operation. The InGaN photocathode-based electron gun has been installed in the conventional scanning electron microscope by replacing the original field emission gun. SEM imaging was performed by selective electron beaming, in which the scanning signal of the SEM system was synchronized with the laser for photocathode excitation to irradiate arbitrary regions in the SEM image at arbitrary intensity. The accuracy of the selection of regions in the SEM image by the selective electron beam was pixel by pixel at the TV scan speed (80 ns/pix, 25 frame/s) of the SEM.

Efficient Production of the PET Radionuclide 133La for Theranostic Purposes in Targeted Alpha Therapy Using the 134Ba(p,2n)133La Reaction.

Targeted Alpha Therapy is a research field of highest interest in specialized radionuclide therapy. Over the last decades, several alpha-emitting radionuclides have entered and left research topics towards their clinical translation. Especially, 225Ac provides all necessary physical and chemical properties for a successful clinical application, which has already been shown by [225Ac]Ac-PSMA-617. While PSMA-617 carries the DOTA moiety as the complexing agent, the chelator macropa as a macrocyclic alternative provides even more beneficial properties regarding labeling and complex stability in vivo. Lanthanum-133 is an excellent positron-emitting diagnostic lanthanide to radiolabel macropa-functionalized therapeutics since 133La forms a perfectly matched theranostic pair of radionuclides with the therapeutic radionuclide 225Ac, which itself can optimally be complexed by macropa as well. 133La was thus produced by cyclotron-based proton irradiation of an enriched 134Ba target. The target (30 mg of [134Ba]BaCO3) was irradiated for 60 min at 22 MeV and 10–15 µA beam current. Irradiation side products in the raw target solution were identified and quantified: 135La (0.4%), 135mBa (0.03%), 133mBa (0.01%), and 133Ba (0.0004%). The subsequent workup and anion-exchange-based product purification process took approx. 30 min and led to a total amount of (1.2–1.8) GBq (decay-corrected to end of bombardment) of 133La, formulated as [133La]LaCl3. After the complete decay of 133La, a remainder of ca. 4 kBq of long-lived 133Ba per 100 MBq of 133La was detected and rated as uncritical regarding personal dose and waste management. Subsequent radiolabeling was successfully performed with previously published macropa-derived PSMA inhibitors at a micromolar range (quantitative labeling at 1 µM) and evaluated by radio-TLC and radio-HPLC analyses. The scale-up to radioactivity amounts that are needed for clinical application purposes would be easy to achieve by increasing target mass, beam current, and irradiation time to produce 133La of high radionuclide purity (>99.5%) regarding labeling properties and side products.

Radioactive and Stable Ion Beam production at GANIL

GANIL Facilities deliver ion beams from Proton to Uranium up to 95MeV/A. The Cyclotron facility combined with the SPIRAL1 facility provides Stable Ion Beams (SIB) since 1983 and Radioactive Ion Beams (RIB) since 2001 for Physics experiments. R&D of new stable and radioactive beams are continuously under progress matching physicist requirements. During the last ten years, the SPIRAL1 facility was upgraded to extend its capabilities to deliver RIBs of condensable elements. After a new one delivered in 2019, off-line R&D’s have been done on the Target Ions Source System and also on the Charge Breeder to improve efficiencies and achieve an operational and reliable facility.In parallel, the commissioning of the LINAC-SPIRAL2 facility started in 2019 with a proton beam production. In 2020, a 16 kW proton beam was delivered for the first time on the Neutron For Science physics area, and a 4 mA beam of 4He2+ was produced with the PhoenixV3 ECR ion source to mimic a deuteron beam. In this article, an overview of GANIL ion sources, beam properties and future developments are described.

Measurement and analysis techniques for a study of 12C(p,γ) and 13C(p,γ) deep underground

The 12C(p,γ) and 13C(p,γ) reaction cross sections are currently under investigation in the low-background environment of the Laboratory for Underground Nuclear Astrophysics. Both reactions are being studied using different types of solid targets, and employing complementary detection techniques (HPGe spectroscopy, total absorption spectroscopy and activation counting). To reduce systematic uncertainties, targets must be accurately characterized and their degradation monitored under the intense (~ 400 µA) beam of the LUNA400 accelerator. We present the experimental techniques employed, and the analyses developed for the study of these reactions.

Electron Beam Emission System for Space Welding Based on Indirectly-Heated Bombardment Cathode

An electron beam emission system developed for space welding and consisting of an indirectly-bombardment cathode fabricated using LaB6 was studied to improve the working life of the space welding electron gun. The energy transfer model of the indirectly-heated bombardment cathode was established based on the cooling effect of thermionic emission and the bombardment heating structure. The efficiency of the energy transfer model was verified by conducting emission tests and the differences between the test and theoretical values were analyzed. The designed electron beam emission system could emit 500 mA beam current in a stable manner at an acceleration voltage of 20 kV, and the diameter of the beam spot was less than 400 μm. The structure, indirectly heated by electron bombardment, exhibited a stable performance, could stabilize the working temperature of the cathode by exploiting the bombardment beam, and the total heating efficiency of the system could reach 76.04%.

High-current H2 + beams from a filament-driven multicusp ion source.

We report the results from a new multicusp ion source (MIST-1) that produces record steady-state currents of H2 + (1 mA) from this type of ion source with high purity (80% H2 +). We built MIST-1 to fulfill the stringent beam purity and beam quality requirements for IsoDAR, a proposed discovery-level neutrino experiment, requiring a 10 mA, 60 MeV/amu continuous wave (cw) proton beam on the target. IsoDAR will use a cyclotron accelerating H2 + ions and using a novel radio frequency quadrupole (RFQ) direct injection method. Systematic measurements, varying discharge voltage, discharge current, and gas pressure, indicate that the ideal operating regime is at low pressure, high discharge current, and high discharge voltage. We have measured the combined species emittance after the source extraction to be <0.05 π-mm-mrad (rms, normalized) for a 0.95 mA beam. Beyond showing high currents and high H2 + fraction, our measurements agree well with high fidelity simulations. These results show the feasibility of using a multicusp ion source for IsoDAR and the RFQ direct injection prototype and paves the way to record breaking cw beam currents of 5 mA H2 + (equivalent to 10 mA protons) from compact cyclotrons, ideal for underground installation.

Study of a hexagonal lattice defect photonic crystal waveguide slow wave structure for G-band traveling wave tube

A defect photonic crystal waveguide (DPCW) slow wave structure (SWS) for G-band traveling wave tube (TWT) is proposed. This DPCW SWS is arrayed in hexagonal lattice with the center defect cells. The TWT based on DPCW SWS operates at 16 kV beam voltage and 120 mA beam current with a 0.6 T focusing magnetic field. A saturated output power of 22.3W, corresponding to a gain of 36.5 dB, is achieved with an input power of 5 mW. The output power is over 10W in a 30 GHz bandwidth. Stable output signal can be achieved without attenuator or sever which shows that the proposed DPCW SWS can depress the oscillation and harmonic in nature. A DPCW SWS sample was fabricated by computer control (CNC) milling, and the measured results show great agreement with the simulation results.

A High-Current-Density Electron Beam for Millimeter-Wave Amplifiers

We present experimental characterization of a 20-kV, 130-mA thermionic electron gun, which is a component of a ${W}$ -band traveling-wave tube (TWT) power amplifier. The electron beam is strongly focused by a 6.6-kG permanent magnet solenoid, producing a peak current density up to 800 A/cm2. The cathode temperature, focus electrode voltage, and modulating anode voltage are varied to characterize the emitted cathode current and beam transport through the beam tunnel of the TWT RF circuit. We observe the variation of the cathode current from 107 to 155 mA and peak beam transmission of 95% measured at the collector. Experimental results are compared to 2-D simulations with the electron gun and collector design code MICHELLE.

The flux weighted cross sections of 179Hf(γ,γ’)179mHf and natHf(γ,x)179mHf reactions at 8 MeV and 15 MeV bremsstrahlung end point energies

For the hafnium element, the cross sections of 179Hf(γ,γ′)179mHf and natHf(γ,x)179mHf reactions were measured at 8 MeV and 15 MeV bremsstrahlung end point energies respectively using activation method and off-line gamma-ray spectroscopy. The bremsstrahlung radiation spectra were generated by bombarding a 0.1 mm tungsten target with 8 MeV and 15 MeV electrons at 5 μA beam current and also theoretically simulated by GEANT4 computer code. The flux weighted average cross sections of 179Hf (γ,γ′)179mHf and natHf(γ,x)179mHf reactions were measured by using 115In(γ,γ’)115mIn and 197Au(γ,n)196Au as flux monitor reactions at 8 MeV and 15 MeV bremsstrahlung radiation respectively. The measured cross sections are found close to the corresponding theoretical cross sections estimated by TALYS 1.95 and TENDL 2019 computer codes. These hafnium cross sections at 8 MeV and 15 MeV bremsstrahlung radiation will be new additions to the EXFOR library, as so far not reported in literature.