The total reflectance spectra of lunar simulant dusts (<20 m particles) were measured to determine their integrated solar absorptance and their thermal emittance for the purpose of analyzing the effect of dust on the performance of thermal control surfaces. All of the simulants exceptMinnesota Lunar Simulant 1 had awavelengthdependant reflectivity near 0.10 over the wavelength range of 8–25 m, and so are highly emitting at room temperature and lower. The anomalous behavior ofMinnesota Lunar Simulant 1 was attributed to its very low glass content. The 300 K emittance of all the lunar simulants, except Minnesota Lunar Simulant 1, ranged from 0.78 to 0.92. In all cases, the was lower for the <20 m particles than for larger particles reported earlier. There was considerably more variation in the lunar simulant reflectance in the solar spectral range (250–2500 nm) than in the thermal infrared. As expected, the lunar highlands simulants were more reflective in this wavelength range than the lunar mare simulants. The maxima at the Christiansen frequency were consistent with simulants being largely plagioclase and confirmed that, with the exception ofMinnesota Lunar Simulant 1P, addition of agglutinates did not change the mineralogical character of the simulants. The of the simulants ranged from 0.39 to 0.75. This is lower than values reported earlier for larger particles of the same simulants (0.41–0.82) and for representative mare and highlands lunar soils (0.74–0.91). Because the of somemare simulantsmore closelymatched that of highlands lunar soils, it is recommended that and values be the criteria for choosing a simulant for assessing the effects of dust on thermal control surfaces, rather than whether a simulant has been formulated as a highlands or a mare simulant.