Carbon fiber-reinforced polymer (CFRP)/titanium alloy (Ti6Al4V) stacks are widely used in the aerospace industry due to their excellent physical properties. The substantial demand for drilling components in the aerospace industry necessitates the implementation of enhanced processing efficiency and drilling quality standards. Six-degrees-of-freedom robots are commonly used in the aerospace industry due to their high production efficiency, high flexibility, and low labor costs. However, due to the weak stiffness, chatter is prone to occur during processing, which has a detrimental impact on the quality of the finished product. As an advanced processing technology, ultrasonic-assisted machining technology can effectively reduce the cutting force and suppress the chatter in the drilling process, so it is widely used in production. In this paper, first, the robot kinematic (dexterity) and stiffness performance is analyzed. Then, the appropriate range of the machining plane and the posture of the robot in the workspace are selected. Finally, the vibration and CFRP entrance damage during the machining process are compared and studied in conventional robotic drilling (CRD) and ultrasonic-assisted robotic drilling (UARD). The experimental results demonstrate that the UARD is an effective method for reducing vibration during the machining process. Compared with the CRD, the CFRP entrance delamination damage in UARD is reduced. Under the appropriate processing parameters, the entrance delamination factor could be reduced by 15%, and the burr height could be reduced by 45%. Obviously, the UARD is a promising process to improve the CFRP entrance delamination damage.
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