Converse magnetoelectric (CME) effect is investigated in a FeCoBSi/0.7Pb(Mg1/3Nb2/3)O3-0.3PbTiO3 laminated composite by using induction method within different frequencies. A large CME coefficient of 3.05 G/V is observed at the resonance frequency of 76.5 kHz under a low bias magnetic field of 50 Oe. The CME coefficient of the heterostructure is almost constant and exhibits a relatively high value in a wide frequency span of 1–64 kHz. The origin of large CME effect and the advantages of Metglas acting as ferromagnetic layer are discussed in the present paper.