Sustainable livelihood of farmers is the key to rural revitalization. The purpose of this study was to establish livelihood capital cultivation models suitable for farmers in different agricultural regions and to enhance the sustainability of farmers’ livelihoods by selecting four agricultural regions (suburban agriculture, intensive agriculture, plain field agriculture, and mountain agriculture) and 1025 rural households and employing Participatory Rural Appraisal (PRA) to systematically analyze the characteristics of livelihood capital and livelihood stability of farmers in different agricultural regions and the coupling coordination relationship between them based on a Sustainable Livelihood Framework (SLF). The results show that: (1) The average household livelihood capital is highest in intensive agricultural regions and lowest in mountain agricultural regions. (2) Farmers in suburban agricultural regions have a variety of sources of income; thus, the livelihood stability is the highest. while it is lowest in intensive agricultural regions. (3) The coupling coordination degree of livelihood capital and livelihood stability in suburban agricultural regions and plain field agricultural regions is primary coordination, while in intensive agricultural regions and mountain agricultural regions, livelihood capital and stability are slightly out of balance.