Live 60Fe Research Articles

Origin of 60Fe nuclei in cosmic rays: the contribution of local OB associations

ABSTRACT The presence of live 60Fe nuclei (lifetime of 3.8 Myr) in cosmic rays detected by the Advanced Composition Explorer/Cosmic Ray Isotope Spectrometer instrument suggests a nearby nucleosynthesis source. 60Fe is primarily produced in core-collapse supernovae, and we aim to clarify whether the detected 60Fe nuclei can be associated with a particular local supernova. We consider 25 OB associations and subgroups located within 1 kpc of the Solar system based on recent Gaia census. A model is developed that combines stellar population synthesis within these OB associations, cosmic ray acceleration within associated superbubbles, and cosmic ray transport to the Solar system. The most critical model parameter impacting 60Fe cosmic ray production is the explodability criterion, which determines if a massive star ends its life as a supernova. Our study points to the Scorpius–Centaurus (Sco–Cen) OB association as the most probable origin of the observed 60Fe nuclei, particularly suggesting they were accelerated in the Sco–Cen superbubble by a young supernova aged ≤500 kyr with a progenitor mass of approximately 13–20 M⊙. A less likely source is the supernova at the origin of the Geminga pulsar 342 kyr ago, if the progenitor originated in the Orion OB1 association. The contribution of local OB associations to the cosmic ray density of stable 56Fe is estimated to be around 20 per cent, with some sensitivity to cosmic ray acceleration efficiency and diffusion coefficient. These findings shed light on the origins of cosmic ray nuclei, connecting them to nucleosynthesis events within our local cosmic neighbourhood.

High precision nickel isotope measurements of early Solar System materials and the origin of nucleosynthetic disk variability

Various chemical elements including nickel (Ni) exhibit mass-independent isotope heterogeneity on a bulk meteorite level, which is generally accepted to reflect the heterogeneous distribution of presolar carrier(s) from different nucleosynthetic sources. Thus, understanding the nature of the carriers can help decipher the origin of the observed nucleosynthetic variability, which remains elusive. In this study, we present the first high precision measurements of mass-independent and mass-dependent Ni isotope compositions for step-leaches of the CI chondrite Ivuna and Efremovka CAIs supplemented by bulk chondrite measurements. Step-leaches record highly anomalous Ni isotope signatures that can be attributed to at least four diverse nucleosynthetic sources. The most anomalous leachates show either large deficits (up to 0.1 %) in the neutron-poor 58Ni and 60Ni nuclides (L11, thought to contain mainly s-process derived Ni) or minor enrichments and deficits (∼100 ppm) in 60Ni or 64Ni (L6, L8, L9 and L10, all thought to derive mainly from supernovae). Pristine CAIs record Ni isotope compositions typified by enrichments in 58Ni of up to 400 ppm. Our new data for bulk chondrites agree with earlier work and emphasize the appropriateness of using the 62Ni/61Ni ratio for internal normalization. Based on the compositional relations between the step-leaches data, CAIs, and bulk meteorites, we show that 60Ni variability is consistent with being of nucleosynthetic origin as opposed to reflecting variable Fe/Ni ratios in the presence of live 60Fe. Finally, we infer that the observed Ni nucleosynthetic disk variability is predominantly driven by a combination of processes separating different nucleosynthetic carriers in the disk from each other, including thermal processing and size-based sorting.

Possible Implications of Relatively High Levels of Initial 60Fe in Iron Meteorites for the Noncarbonaceous–Carbonaceous Meteorite Dichotomy and Solar Nebula Formation

Cook et al. found that iron meteorites have an initial abundance ratio of the short-lived isotope 60Fe to the stable isotope 56Fe of 60Fe/56Fe ∼ (6.4 ± 2.0) × 10−7. This appears to require the injection of live 60Fe from a Type II supernova (SN II) into the presolar molecular cloud core, as the observed ratio is over a factor of 10 times higher than would be expected to be found in the ambient interstellar medium (ISM) as a result of galactic chemical evolution. The supernova triggering and injection scenario offers a ready explanation for an elevated initial 60Fe level, and in addition provides a physical mechanism for explaining the noncarbonaceous–carbonaceous (NC–CC) dichotomy of meteorites. The NC–CC scenario hypothesizes the solar nebula first accreted material that was enriched in supernova-derived nuclides, and then later accreted material depleted in supernova-derived nuclides. While the NC–CC dichotomy refers to stable nuclides, not short-lived isotopes like 60Fe, the SN II triggering hypothesis provides an explanation for the otherwise unexplained change in nuclides being accreted by the solar nebula. Three-dimensional hydrodynamical models of SN II shock-triggered collapse show that after triggering collapse of the presolar cloud core, the shock front sweeps away the local ISM while accelerating the resulting protostar/disk to a speed of several kilometers per second, sufficient for the protostar/disk system to encounter within ∼1 Myr the more distant regions of a giant molecular cloud complex that might be expected to have a depleted inventory of supernova-derived nuclides.

The Dyadic Radionuclide System 60Fe / 53Mn to Distinguish Interstellar from Interplanetary 60Fe

The discovery of live 60Fe in a deep-sea crust with proposed interstellar origin followed by evidence for elevated interplanetary 3He in the same crust raised the question on how to unambiguously identify the true production site of the identified 60Fe. Here, we show the implementation of the dyadic radionuclide system 60Fe / 53Mn to serve as a tool for the identification of surplus interstellar 60Fe over interplanetary production. The recent updates in experimental 60Fe and 53Mn data from iron meteorites as well as in production rate models confirm the validity and robustness of this dyadic system for future applications.

Iron and Nickel Isotopes in IID and IVB Iron Meteorites: Evidence for Admixture of an SN II Component and Implications for the Initial Abundance of 60Fe

Abstract We measured Fe and Ni isotopes in 13 iron meteorites from magmatic groups IID and IVB. Resolvable deficits (≈−0.14) are observed in ε 60Ni in both groups. Small deficits (≈−0.08) are also evident in ε 56Fe but not in the most neutron-rich isotope of Fe (58Fe). Relative to terrestrial material, the observed ε iFe values are consistent with the presence of a small excesses of material in the parent bodies of IID and IVB irons that was produced in a type II supernova. The ε 60Ni and ε 56Fe values are uncorrelated in both groups. This is consistent with a nucleosynthetic origin of the ε 56Fe deficits, whereas the ε 60Ni deficits are best explained as radiogenic in nature due to the former presence of live 60Fe (t 1/2 = 2.62 Ma) in the early solar system. The 60Ni deficits correspond to 60Fe/56Fe ratios of ≈3 × 10−7 at the time of core formation on the IID and IVB parent bodies. These data, in conjunction with previously published 182Hf–182W core formation ages, are used to estimate a solar system initial 60Fe/56Fe = (6.4 ± 2.0) × 10−7 for the formation region of carbonaceous chondrites.

Formation and evolution of the local interstellar environment: combined constraints from nucleosynthetic and X-ray data

ABSTRACT Several observations suggest that the Solar system has been located in a region affected by massive stellar feedback for at least a few Myr; these include detection of live 60Fe in deep-sea archives and Antarctic snow, the broad angular distribution of 26Al around the Galactic plane seen in all-sky γ-ray maps, and the all-sky soft X-ray background. However, our position inside the Galactic disc makes it difficult to fully characterize this environment, and our limited time baseline provides no information about its formation history or relation to large-scale galactic dynamics. We explore these questions by using an N-body + hydrodynamics simulation of a Milky-Way-like galaxy to identify stars on Sun-like orbits whose environments would produce conditions consistent with those we observe. We find that such stars are uncommon but not exceptionally rare. These stars are found predominantly near the edges of spiral arms, and lie inside kpc-scale bubbles that are created by multiple generations of star formation in the arm. We investigate the stars’ trajectories and find that the duration of the stay in the bubble ranges from 20 to 90 Myr. The duration is governed by the crossing time of stars across the spiral arm. This is generally shorter than the bubble lifetime, which is ∼100 Myr as a result of the continuous gas supply provided by the arm environment.

Nucleosynthesis in the Innermost Ejecta of Neutrino-driven Supernova Explosions in Two Dimensions

Abstract We examine nucleosynthesis in the innermost neutrino-processed ejecta (a few ) of self-consistent two-dimensional explosion models of core-collapse supernovae (CCSNe) for six progenitor stars with different initial masses. Three models have initial masses near the low-mass end of the SN range of (e8.8; electron-capture SN), (z9.6), and (u8.1), with initial metallicities of 1, 0, and 10−4 times the solar metallicity, respectively. The other three are solar-metallicity models with initial masses of (s11), (s15), and (s27). The low-mass models e8.8, z9.6, and u8.1 exhibit high production factors (nucleosynthetic abundances relative to the solar abundances) of 100–200 for light trans-Fe elements from Zn to Zr. This is associated with an appreciable ejection of neutron-rich matter in these models. Remarkably, the nucleosynthetic outcomes for the progenitors e8.8 and z9.6 are almost identical, including interesting productions of 48Ca and 60Fe, irrespective of their quite different (O–Ne–Mg and Fe) cores prior to collapse. In the more massive models s11, s15, and s27, several proton-rich isotopes of light trans-Fe elements including the p-isotope 92Mo (for s27) are made, up to production factors of ∼30. Both electron-capture SNe and CCSNe near the low-mass end can therefore be dominant contributors to the Galactic inventory of light trans-Fe elements from Zn to Zr and probably 48Ca and live 60Fe. The innermost ejecta of more massive SNe may have only subdominant contributions to the chemical enrichment of the Galaxy except for 92Mo.

ELECTRON-CAPTURE SUPERNOVAE AS SOURCES OF 60 Fe

We investigate the nucleosynthesis of the radionuclide 60Fe in electron-capture supernovae (ECSNe). The nucleosynthetic results are based on a self-consistent, two-dimensional simulation of an ECSN as well as models in which the densities are systematically increased by some factors (low-entropy models). 60Fe is found to be appreciably made in neutron-rich ejecta during the nuclear quasi-equilibrium phase with greater amounts being produced in the lower-entropy models. Our results, combining them with the yields of core-collapse supernovae (CCSNe) in the literature, suggest that ECSNe account for at least 4-30% of live 60Fe in the Milky Way. ECSNe co-produce neutron-rich isotopes, 48Ca, 50Ti, 54Cr, some light trans-iron elements, and possibly weak r-process elements including some radionuclides such as 93Zr, 99Tc, and 107Pd, whose association with 60Fe might have been imprinted in primitive meteorites or in the deep ocean crust on the Earth.

60Fe– 60Ni systematics in the eucrite parent body: A case study of Bouvante and Juvinas

Eucrites are basaltic meteorites that cooled rapidly but are in many instances thermally metamorphosed and impact brecciated. The exact timing of these events remains unclear. In this study, Ni isotopic compositions and Fe/Ni elemental ratios are presented for two non-cumulate eucrites, Bouvante and Juvinas, including mineral separates from the latter. The samples are characterized by variable, well-resolved 60Ni-excesses consistent with the former presence of live 60Fe ( t 1/2 = 2.62 Ma) at the time of eucrite crystallization. A significant fraction of Ni with a terrestrial-like composition appears to be surface correlated. This Ni may be the product of terrestrial contamination or was introduced by a chondritic impactor during brecciation. Altogether, the data provide evidence for a complex and probably multi-stage history of Fe and/or Ni redistribution, which impedes the interpretation of the chronological data.

Size of the group IVA iron meteorite core: Constraints from the age and composition of Muonionalusta

The group IVA fractionally crystallized iron meteorites display a diverse range of metallographic cooling rates. These have been attributed to their formation in a metallic core, approximately 150 km in radius, that cooled to crystallization in the absence of any appreciable insulating mantle. Here we build upon this formation model by incorporating several new constraints. These include (i) a recent U–Pb radiometric closure age of < 2.5 Myr after solar system formation for the group IVA iron Muonionalusta, (ii) new measurements and modeling of highly siderophile element compositions for a suite of IVAs, and (iii) consideration of the thermal effects of heating by the decay of the short-lived radionuclide 60Fe. Our model for the thermal evolution of the IVA core suggests that it was approximately 50–110 km in radius after being collisionally exposed. This range is due to uncertainties in the initial abundance of live 60Fe incorporated into the IVA core. Our models define a relationship between cooling rate and closure age, which is used to make several predictions that can be tested with future measurements. In general, our results show that diverse cooling rates and early U–Pb closure ages can only coexist on mantle-free bodies and that energy released by the decay of 60Fe reduces the core size necessary to produce diverse metallographic cooling rates. The influence of 60Fe on cooling rates has largely been neglected in previous core formation models; accounting for this heat source can affect size estimates for other iron meteorite cores that cooled to crystallization in the presence of live 60Fe. Candidates for such a scenario of early, mantle-free formation include the iron IIAB, IIIAB and IVB groups.

Penetration of nearby supernova dust in the inner solar system

We investigate the method by which nearby supernovae – within a few tens of pc of the solar system – can penetrate the solar system and deposit live radioactivities on earth. The radioactive isotopic signatures that could potentially leave an observable geological imprint are in the form of refractory metals; consequently, it is likely they would arrive in the form of supernova-produced dust grains. Such grains can penetrate into the solar system more easily than the bulk supernova plasma, which gets stalled and deflected near the solar system due to the solar wind plasma pressure. We therefore examine the motion of charged grains as they decouple from the supernova plasma and are influenced by the solar magnetic, radiation, and gravitational fields. We characterize the dust trajectories with analytical approximations which display the roles of grain size, initial velocity, and surface voltage. These results are verified with full numerical simulations for wide ranges of dust properties. We find that supernova dust grains traverse the inner solar system nearly undeflected, if the incoming grain velocity – which we take to be that of the incident supernova remnant – is comparable to the solar wind speeds and much larger than the escape velocity at 1 AU. Consequently, the dust penetration to 1 AU has essentially 100% transmission probability and the dust capture onto the earth should have a geometric cross section. Our results cast in a new light the terrestrial deposition of radioisotopes from nearby supernovae in the geological past. For explosions beyond ∼10 pc from earth, dust grains can still deliver supernova ejecta to earth, and thus the amount of supernova material deposited is set by the efficiency of dust condensation and survival in supernovae. Turning the problem around, we use observations of live 60Fe in both deep-ocean and lunar samples to infer a conservative lower bound iron condensation efficiency of M dust,Fe/ M tot,Fe ≳ 4 × 10 −4 for the supernova which apparently produced these species 2–3 Myr ago.

IRON-60 HETEROGENEITY AND INCOMPLETE ISOTOPE MIXING IN THE EARLY SOLAR SYSTEM

Short-lived radionuclides (e.g., 26Al, 53Mn, 60Fe, 182Hf) are widely used to refine the chronology of the early solar system. They provide chronological information, however, only if they were homogeneously distributed in the source region of the objects under scrutiny at the time of their formation. With the high level of precision now achieved on isotopic measurements, very short time intervals can in principle be resolved and a precise evaluation of the initial homogeneity degree becomes increasingly crucial. High-precision nickel isotope data for differentiated meteorites (angrites, ureilites) and chondritic (CB) components allow us to test the initial distribution of radioactive 60Fe and stable Ni isotopes. Although these meteorites appear to have formed nearly contemporaneously, they yield variable initial 60Fe/56Fe ratios. Besides, the CB metal nodules and ureilite silicates show nucleosynthetic anomalies. The new data presented here do not confirm the recently inferred late injection of 60Fe into the protoplanetary disk. Instead, live 60Fe was present, but heterogeneously distributed, from the start of the solar system, revealing an incomplete mixing of material from various nucleosynthetic sources and restricting the use of the 60Fe-60Ni system as a chronometer.

60Fe: A Heat Source for Planetary Differentiation from a Nearby Supernova Explosion

From a sample of the Semarkona (LL 3.0) ordinary chondrite we report the in situ discovery of 60Ni isotopic anomalies attributable to the decay of short-lived 60Fe (half-life 1.5 Myr) in the mineral phases troilite (FeS) and magnetite (Fe3O4). The troilite shows a 60Ni excesses of up to ~100 parts per thousand (‰) relative to its solar isotopic abundance. A positive correlation between 60Ni excesses and 56Fe/58Ni ratios provides evidence for live 60Fe in the early solar system. The inferred 60Fe/56Fe ratio of (0.92 ± 0.24) × 10-6 is the highest measured in any meteorite sample so far. This ratio is higher than predictions for production within asymptotic giant branch stars, but falls within the range expected for a Type II supernova source. This result is strongly suggestive of injection of freshly synthesized 60Fe into the nascent solar nebula by a nearby supernova explosion. Such a high abundance of 60Fe will exclude irradiation with solar energetic particles as the sole mechanism responsible for the production of short-lived radionuclides. It further shows that the decay of 60Fe was an important heat source for early planetary melting and differentiation and for keeping asteroids thermally active for much longer than would be possible from the decay of 26Al alone.

Deep‐Ocean Crusts as Telescopes: Using Live Radioisotopes to Probe Supernova Nucleosynthesis

Live 60Fe has recently been detected in a deep-ocean ferromanganese crust, isolated in layers dating from about 3 Myr ago. Since 60Fe has a mean life of 2.2 Myr, a near-Earth supernova is the only likely source for such a signal, and we explore here the consequences of a supernova origin. We combine the 60Fe data with several supernova nucleosynthesis models to calculate the supernova distance as a function of progenitor mass, finding an allowed range of 15-120 pc. We also predict the signals expected for several other radioisotopes, which are independent of the supernova distance. Species likely to be present near or above background levels are 10Be, 26Al, 53Mn, 182Hf and 244Pu. Of these, 182Hf and 244Pu are nearly background-free, presenting the best opportunities to provide strong confirmation of the supernova origin of the 60Fe signal, and to demonstrate that at least some supernovae are the source for the r-process. The accuracies of our predictions are hampered by large uncertainties in the predicted 60Fe yields for supernovae of different masses, so the new crust data motivate a redoubled theoretical attack on this problem.

Evidence for live 60Fe in meteorites

We report a preliminary in situ finding of 60Ni isotopic anomalies, attributed to the decay of short-lived 60Fe (half-life 1.5 Ma), in Fe-sulfides and pyroxene in the Chervony Kut eucrite and in the Semarkona (LL3.0) ordinary chondrite using the new state-of-the-art NanoSIMS technique at MPI in Mainz. In Semarkona, troilites (FeS) show 60Ni excesses of up to 46 ± 15‰ (2σ). A positive correlation between 60Ni excesses and 56Fe/ 58Ni ratios provides evidence for live 60Fe in the early solar system. The inferred 60Fe/ 56Fe ratio of (7.3 ± 2.6) × 10 −7 is much higher than previously estimated for the initial solar system value. In terms of a chronological interpretation, this corresponds to one half-life of 60Fe. In Chervony Kut, two pyrrhotite {Fe (1−x)S} types (abundant Pyr-1 crystals and rare Pyr-2 veins) and pyroxene {(Mg,Fe)SiO 3} grains show 60Ni excesses. The delta- 60Ni varies from 22 ± 16‰ (2σ) in Pyr-1 to an extremely high value of 1775 ± 250‰ in Pyr-2 veins. No clear correlation is seen between the 60Ni excess and the Fe/Ni ratio, which does not allow a plausible explanation for the extreme excess encountered in Pyr-2. More meticulous analyses are underway in order to confirm this preliminary finding.

Live radioisotopes as signatures of nearby supernovae

Nearby (≲1 kpc) supernovae were almost certainly common in earth’s geological history. Such events allow the direct study of their freshly synthesized live radioisotopes, opening new windows onto supernovae. Very close supernovae (within a few tens of pc) may deposit radioisotopes directly on the earth. Recent high-sensitivity accelerator mass spectrometry measurements of deep-ocean samples find live 60Fe at levels that greatly exceed background, suggesting an explosion occurred within 30 pc during the last 5 Myr. Somewhat more distant – but also more frequent – supernovae leave observable signatures of radioisotopes whose decay includes γ-ray line emission. In particular, a large, old supernova remnant was recently discovered at ∼100 pc, and appears to contain 26Al. If confirmed, this would be the first detection of 26Al in a single remnant, and would be a new probe of supernova nucleosynthesis and astrophysics.

60Fe in eucrites

Additional evidence for the existence in the early solar system of live 60Fe has been found in the basaltic achondrite Juvinas. The relative abundance of 60Fe/ 56Fe of x0223C; 4 × 10 −10 at the time of meteorite solidification is one order of magnitude lower than that previously observed for the eucrite Chervony Kut. This difference corresponds to a ∼ 4.7 Ma time interval between closure of the 60Fe- 60Ni isotopic system in the two meteorites. The factor two higher initial 60Ni/ 58Ni ratio in Juvinas is consistent with this time difference and a common bulk Fe/Ni ratio in the two meteorites. Using the 60Fe- 60Ni isotope system as a chronometer various models for the evolution of the eucrite parent body of different degrees of complexity are discussed. Regardless of the detailed differences between these models a short time interval of only a few million years between planetary differentiation and basaltic crust formation is indicated.