Liquid Argon Scintillation Light Research Articles

Doping liquid argon with xenon in ProtoDUNE Single-Phase: effects on scintillation light

Doping of liquid argon TPCs (LArTPCs) with a small concentration of xenon is a technique for light-shifting and facilitates the detection of the liquid argon scintillation light. In this paper, we present the results of the first doping test ever performed in a kiloton-scale LArTPC. From February to May 2020, we carried out this special run in the single-phase DUNE Far Detector prototype (ProtoDUNE-SP) at CERN, featuring 720 t of total liquid argon mass with 410 t of fiducial mass. A 5.4 ppm nitrogen contamination was present during the xenon doping campaign. The goal of the run was to measure the light and charge response of the detector to the addition of xenon, up to a concentration of 18.8 ppm. The main purpose was to test the possibility for reduction of non-uniformities in light collection, caused by deployment of photon detectors only within the anode planes. Light collection was analysed as a function of the xenon concentration, by using the pre-existing photon detection system (PDS) of ProtoDUNE-SP and an additional smaller set-up installed specifically for this run. In this paper we first summarize our current understanding of the argon-xenon energy transfer process and the impact of the presence of nitrogen in argon with and without xenon dopant. We then describe the key elements of ProtoDUNE-SP and the injection method deployed. Two dedicated photon detectors were able to collect the light produced by xenon and the total light. The ratio of these components was measured to be about 0.65 as 18.8 ppm of xenon were injected. We performed studies of the collection efficiency as a function of the distance between tracks and light detectors, demonstrating enhanced uniformity of response for the anode-mounted PDS. We also show that xenon doping can substantially recover light losses due to contamination of the liquid argon by nitrogen.

A novel cryogenic VUV spectrofluorometer for the characterization of wavelength shifters

We present a novel cryogenic VUV spectrofluorometer designed to characterize wavelength shifters (WLS) crucial for experiments based on liquid argon (LAr) scintillation light detection. Wavelength shifters like 1,1,4,4-tetraphenyl-1,3-butadiene (TPB) or polyethylene naphthalate (PEN) are used in these experiments to shift the VUV scintillation light to the visible region. Precise knowledge of the optical properties of the WLS at liquid argon's temperature (87 K) and LAr scintillation wavelength (128 nm) is necessary to model and understand the detector response. The cryogenic VUV spectrofluorometer was commissioned to measure the emission spectra and relative wavelength shifting efficiency (WLSE) of samples between 300 K to 87 K for VUV (120 nm to 190 nm) and UV (310 nm) excitation. New mitigation techniques for surface effects on cold WLS were established. As part of this work, the TPB-based wavelength shifting reflector (WLSR) featured in the neutrinoless double-beta decay experiment LEGEND-200 was characterized. The WLSE was observed to increase by (54 ± 5) % from room temperature (RT) to 87 K. PEN installed in LEGEND-200 was also characterized, and a first measurement of the relative WLSE and emission spectrum at RT and 87 K is presented. The WLSE of amorphous PEN was found to be enhanced by at least (37 ± 4) % for excitation with 128 nm and by (52 ± 3) % for UV excitation at 87 K compared to RT.

Liquid argon light collection and veto modeling in GERDA Phase II

The ability to detect liquid argon scintillation light from within a densely packed high-purity germanium detector array allowed the Gerda experiment to reach an exceptionally low background rate in the search for neutrinoless double beta decay of {}^{76}Ge. Proper modeling of the light propagation throughout the experimental setup, from any origin in the liquid argon volume to its eventual detection by the novel light read-out system, provides insight into the rejection capability and is a necessary ingredient to obtain robust background predictions. In this paper, we present a model of the Gerda liquid argon veto, as obtained by Monte Carlo simulations and constrained by calibration data, and highlight its application for background decomposition.

Understanding the enhancement of scintillation light in xenon-doped liquid argon

Measuring the scintillation light in noble gases is an important detection technique in particle physics. Numerous rare event searches like neutrino beam experiments, neutrino-less double beta-decay, and dark matter searches use argon-based detectors. In liquid argon, the light yield can be enhanced by the addition of a small quantity of xenon, where ∼10−1000 ppm are added. The general enhancement mechanism and its pathway via an energy transfer between argon and xenon excimers is well known, however the importance of absorption of argon excimer emission by atomic xenon has not been fully appreciated. This absorption significantly reduces the light yield in commercially available argon (extracted from air) which contains trace amounts (∼ 0.1 ppm) of xenon. The addition of a small xenon dopant of ∼10 ppm recovers this lost light resulting in an increased light yield over un-doped argon of about a factor of two. In this paper we introduce a model for the light production in xenon doped argon, including absorption and re-emission, and compare it to the measured time dependence of light emission in xenon-doped argon.

Scintillation and optical properties of xenon-doped liquid argon

Liquid argon (LAr) is a common choice as detection medium in particle physics and rare-event searches. Challenges of LAr scintillation light detection include its short emission wavelength, long scintillation time and short attenuation length. The addition of small amounts of xenon to LAr is known to improve the scintillation and optical properties. We present a characterization campaign on xenon-doped liquid argon (XeDLAr) with target xenon concentrations ranging from 0 to 300 ppm by mass encompassing the measurement of the photoelectron yield Y, effective triplet lifetime τ 3 and effective attenuation length λ att. The measurements were conducted in the Subterranean Cryogenic ARgon Facility, Scarf, a 1 t (XeD)LAr test stand in the shallow underground laboratory (UGL) of TU-Munich. These three scintillation and optical parameters were observed simultaneously with a single setup, the Legend Liquid Argon Monitoring Apparatus, Llama. The actual xenon concentrations in the liquid and gaseous phases were determined with the Impurity DEtector For Investigation of Xenon, Idefix, a mass spectrometer setup, and successful doping was confirmed. At the highest dopant concentration we find a doubling of Y, a tenfold reduction of τ 3 to ∼90 ns and a tenfold increase of λ att to over 6 m.

Using 22Na and 83mKr to calibrate and study the properties of scintillation in xenon-doped liquid argon

We have measured the properties of scintillation light in liquid argon doped with xenon concentrations from 165 ppm to 10,010 ppm using a 22Na source. The energy transfer processes in the xenon-doped liquid argon are discussed in detail, and a new waveform model is established and used to fit the average waveform. The time profile of the scintillation photon in the xenon-doped liquid argon and of the TPB emission are presented. The quantities of xenon-doped are controlled by a Mass Flow Controller which is calibrated via a Redusial Gas Analyzer to ensure that the xenon concentration is accurate. In addition, a successful test of 83mKr as a calibration source has been implemented in the xenon-doped liquid argon detector for the first time. By comparing the light yield of the 22Na and 83mKr, it can be concluded that the scintillation efficiency is almost same over the range of 41.5 keV to 511 keV.

Design and implementation of the new scintillation light detection system of ICARUS T600

ICARUS T600 is the far detector of the Short Baseline Neutrino program at Fermilab (U.S.A.), which foresees three Liquid Argon Time Projection Chambers along the Booster Neutrino Beam line to search for LSND-like sterile neutrino signal. The T600 detector underwent a significant overhauling process at CERN, introducing new technological developments while maintaining the already achieved performances. The realization of a new liquid argon scintillation light detection system is a primary task of the detector overhaul. As the detector will be subject to a huge flux of cosmic rays, the light detection system should allow the 3D reconstruction of events contributing to the identification of neutrino interactions in the beam spill gate. The design and implementation of the new scintillation light detection system of ICARUS T600 is described.

A measurement of the group velocity of scintillation light in liquid argon

The propagation velocity of scintillation light in liquid argon vg at λ ∼ 128 nm wavelength, has been measured for the first time in a dedicated experimental setup at CERN. The obtained result 1/vg = 7.46 ± 0.08 ns/m, is then used to derive the value of the refractive index (n) and the Rayleigh scattering length (L) for liquid argon in the VUV region. For λ = 128 nm we found n= 1.358 ± 0.003 and L= 99.1 ± 2.3 cm. The measured values are of interest for a variety of experiments searching for rare events like neutrino and dark matter interactions. The derived quantities also represent key information for theoretical models describing the propagation of scintillation light in liquid argon.

Development of the Light Collection Module for the Liquid Argon Time Projection Chamber (LArTPC)

A modular liquid argon (LAr) Time Projection Chamber (TPC) with pixelated charge readout is considered as a part of the near-detector for the Deep Underground Neutrino Experiment (DUNE) [1]. Such a TPC is being developed by the ArgonCube collaboration [2]. To provide a trigger for the data acquisition (DAQ) of a neutrino event the LAr scintillation light detection is proposed. The light is a vacuum ultraviolet (UV) with 128 nm wavelength, thus, it is a challenge to register it. The main requirements imposed on the light detection system are a good performance at cryogenic temperatures, non-conductive materials, compact dimensions, and a detection efficiency at a level of percent. A Light Collection Module (LCM) as a candidate for the system has been developed at Joint Institute for Nuclear Research (JINR) in Dubna, Russia. The LCM is based on the wavelength-shifting (WLS) fibers that are coated with Tetraphenyl Butadiene (TPB) and read out by silicon photomultipliers (SiPM). Also at JINR, a full readout chain for the light detection system has been developed, consisting of the front-end electronics, power-supply for the SiPMs, and the DAQ. A cryogenic test setup has been built at JINR to study the performance of the LCM in LAr. A similar study was carried out in the laboratory for high energy physics of Bern University with highly purified LAr. These studies have shown that the photon detection efficiency (PDE) of the LCM for the LAr scintillation light is about 1–2%. Further tests in the ArgonCube prototype TPC will provide the real performance of the LCM system with a full readout chain.

Measurement of liquid argon scintillation light properties by means of an alpha source placed inside the CERN 10-PMT LAr detection system

A particle detection system that exploits the scintillation light produced by ionizing particles in liquid argon (LAr) has been assembled at CERN. The system is based on 10 large-area photomultiplier tubes (PMT) immersed in a 1500-liter dewar filled with liquid argon and equipped with an extendible feed-through and mechanical support for an alpha source (241Am). The position of the source can be changed with respect to the PMT plane in vertical and horizontal directions. Arrays of silicon photomultiplier (SiPM) photodetectors, integrated in the source support, are used for the data acquisition trigger and to define the t0 of the light generation. PMT and SiPM signals can be recorded at different distances and different positions allowing the measurement of some of the LAr scintillation light properties. The system was studied and characterized in detail, and physics results on LAr scintillation properties are expected soon.

First liquid argon test of the X-ARAPUCA

The X-ARAPUCA is a device for the detection of scintillation light in liquid argon and represents an evolution of the ARAPUCA design, with an increased collection efficiency and a simpler design. The first liquid argon test of an X-ARAPUCA prototype has been performed in the cryogenic facility of the Laboratáorio de Léptons da UNCIAMP and showed a detection efficiency of 3.5%± 0.5%, in line with the expectations from Monte Carlo simulations and extrapolations from measurements with standard ARAPUCAs.

First calorimetric energy reconstruction of beam events with ARAPUCA light detector in protoDUNE-SP

ProtoDUNE Single Phase at CERN is the large-scale prototype for the far detector of the future DUNE experiment. ProtoDUNE is in stable operation since Oct. 2018 at the CERN Neutrino Platform. Test beam data in the energy range of sub-GeV to a few GeV were collected in fall 2018 providing a set of key measurements. Particles (electrons, protons, pions, muons and kaons) are identified combining information from a set of beam-line detectors (Time of Flight, Cherenkov) and TPC reconstruction. Three different technologies are implemented in the protoDUNE photon detector system (PDS). Results from the response of ARAPUCA, one of the PDS components, are presented providing first calorimetric energy measurements of beam events from liquid argon scintillation light signals.

Calorimetry for low-energy electrons using charge and light in liquid argon

Precise calorimetric reconstruction of 5-50 MeV electrons in liquid argon time projection chambers (LArTPCs) will enable the study of astrophysical neutrinos in DUNE and could enhance the physics reach of oscillation analyses. Liquid argon scintillation light has the potential to improve energy reconstruction for low-energy electrons over charge-based measurements alone. Here we demonstrate light-augmented calorimetry for low-energy electrons in a single-phase LArTPC using a sample of Michel electrons from decays of stopping cosmic muons in the LArIAT experiment at Fermilab. Michel electron energy spectra are reconstructed using both a traditional charge-based approach as well as a more holistic approach that incorporates both charge and light. A maximum-likelihood fitter, using LArIAT's well-tuned simulation, is developed for combining these quantities to achieve optimal energy resolution. A sample of isolated electrons is simulated to better determine the energy resolution expected for astrophysical electron-neutrino charged-current interaction final states. In LArIAT, which has very low wire noise and an average light yield of 18 pe/MeV, an energy resolution of $\sigma/E \simeq 9.3\%/\sqrt{E} \oplus 1.3\%$ is achieved. Samples are then generated with varying wire noise levels and light yields to gauge the impact of light-augmented calorimetry in larger LArTPCs. At a charge-readout signal-to-noise of S/N $\simeq$ 30, for example, the energy resolution for electrons below 40 MeV is improved by $\approx$ 10%, $\approx$ 20%, and $\approx$ 40% over charge-only calorimetry for average light yields of 10 pe/MeV, 20 pe/MeV, and 100 pe/MeV, respectively.

Backgrounds in the DEAP-3600 Dark Matter Experiment

The DEAP-3600 experiment, located at SNOLAB, is searching for dark matter with a single phase liquid argon (LAr) target. For a background-free exposure of 3000 kg·yr, the projected sensitivity to the spin-independent WIMP-nucleon cross section at 100 GeV/c2 WIMP mass is 10−46 cm2.The experimental signature of dark matter interactions is keV-scale argon recoils producing 128 nm LAr scintillation photons which are wavelength shifted and observed by 255 PMTs. To reach the large background-free exposure, a combination of careful material selection, passive shielding, active vetoes, fiducialization and pulse shape discrimination (PSD) is used. The main concept of the background rejection in DEAP-3600 is the powerful PSD, employing the large difference between fast and slow components of LAr scintillation light. The designed background level of DEAP-3600 is less than 0.6 events in a 3000 kg·yr exposure. The experiment was filled in November 2016 and is currently taking dark matter search data.

Electromagnetic backgrounds and potassium-42 activity in the DEAP-3600 dark matter detector

The DEAP-3600 experiment is searching for WIMP dark matter with a 3.3 tonne single phase liquid argon (LAr) target, located 2.1 km underground at SNOLAB. The experimental signature of dark matter interactions is keV-scale $^{40}$Ar nuclear recoils (NR) producing 128 nm LAr scintillation photons observed by PMTs. The largest backgrounds in DEAP-3600 are electronic recoils (ER) induced by $\beta$ and $\gamma$-rays originating from internal and external radioactivity in the detector material. A background model of the ER interactions in DEAP-3600 was developed and is described in this work. The model is based on several components which are expected from radioisotopes in the LAr, from ex-situ material assay measurements, and from dedicated independent in-situ analyses. This prior information is used in a Bayesian fit of the ER components to a 247.2 d dataset to model the radioactivity in the surrounding detector materials. While excellent discrimination between ERs and NRs is reached with pulse shape discrimination, utilizing the large difference between fast and slow components of LAr scintillation light, detailed knowledge of the ER background and activity of detector components, sets valuable constraints on other key types of backgrounds in the detector: neutrons and alphas. In addition, the activity of $^{42}$Ar in LAr in DEAP-3600 is determined by measuring the daughter decay of $^{42}$K. This cosmogenically activated trace isotope is a relevant background at higher energies for other rare event searches using atmospheric argon e.g. DarkSide-20k, GERDA or LEGEND. The specific activity of $^{42}$Ar in the atmosphere is found to be $40.4 \pm 5.9$ $\mu$Bq/kg of argon.

ARAPUCA light trap for large liquid argon time projection chambers

ARAPUCA is a totally innovative device for liquid argon scintillation light detection. It is composed of a passive light collector and of active devices. The active devices are standard SiPMs that operate at liquid argon temperature, while the passive collector is a photon trap that allows the collection of light with extremely high efficiency. The total detection efficiency of the device can be tuned by modifying the ratio between the area of the active components (SiPM) and that of the optical window. Few arrays of ARAPUCAs will be installed inside the prototype of the Deep Underground Neutrino Experiment - protoDUNE - and their performances will be compared with those of more standard solutions based on guiding bars. The results of the most recent tests of ARAPUCAs in a liquid argon environment, which led to the actual design for the protoDUNE, will be reported together with the proposal of a photon detection system for the Deep Underground Neutrino Experiment based on ARAPUCAs combined with dielectric mirror foils coated by wavelength-shifter.

Scintillation light DAQ and trigger system for the ICARUS T600 experiment at fermilab

Abstract ICARUS T600 will operate at shallow depths as far detector for the Short Baseline Neutrino (SBN) program at FNAL taking data from the BNB and NuMI beams. The entire apparatus will be exposed to the huge cosmic background which can mimic genuine neutrino interactions. To distinguish the signals related to the neutrino beams from those induced by cosmic rays, the detector will be provided with a trigger system that will exploit the coincidence of the prompt signals from the liquid argon scintillation light, detected by 360 Photomultiplier Tubes (PMTs), with a beam gate window generated in correspondence to the expected arrival time of neutrinos in the T600.

Experimental study of the propagation of scintillation light in Liquid Argon

Properties of the propagation of scintillation light in liquid argon (LAr), at λ ∼ 128 nm wavelength, have been experimentally investigated in a dedicated setup at CERN. The speed of scintillation photons has been measured for the first time in this medium, refractive index and the Rayleigh scattering are being studied as well. Such measurement provides a key ingredient for the interpretation of data from the current and next generation large mass LAr detectors as those dedicated to the search for rare events such as neutrinos or Dark Matter. Furthermore the improvement on the understanding of the scintillation light propagation represent a benchmark for the multiple theoretical models and simulations for the next generation of detectors which are now based on still incomplete measurements and calculations. • Measurement of the scintillation light propagation speed in liquid argon. • Optical properties as refractive index and Rayleigh Scattering ( λ =128 nm) are derived. • Measurement of interest for LAr-based large scale future experimental setups. • Results can be used to improve current Monte Carlo simulations.

Test and characterization of 400 Hamamatsu R5912-MOD photomultiplier tubes for the ICARUS T600 detector

ICARUS T600 will be operated as far detector of the Short Baseline Neutrino program at Fermilab (U.S.A.), which foresees three liquid argon time projection chambers along the Booster Neutrino Beam line to search for a LSND-like sterile neutrino signal. The detector employs 360 photomultiplier tubes, Hamamatsu model R5912-MOD, suitable for cryogenic applications. A total of 400 PMTs were procured from Hamamatsu and tested at room temperature to evaluate the performance of the devices and their compliance to detect the liquid argon scintillation light in the T600 detector. Furthermore 60 units were also characterized at cryogenic temperature, in liquid argon bath, to evaluate any parameter variation which could affect the scintillation light detection. All the tested PMTs were found to comply with the requirements of ICARUS T600 and a subset of 360 specimens was selected for the final installation in the detector.

Surface background suppression in liquid argon dark matter detectors using a newly discovered time component of tetraphenyl-butadiene scintillation

Decays of radioisotopes on inner detector surfaces can pose a major background concern for the direct detection of dark matter. While these backgrounds are conventionally mitigated with position cuts, these cuts reduce the exposure of the detector by decreasing the sensitive mass, and uncertainty in position determination may make it impossible to adequately remove such events in certain detectors. In this paper, we provide a new technique for substantially reducing these surface backgrounds in liquid argon (LAr) detectors, independent of position cuts. These detectors typically use a coating of tetraphenyl-butadiene (TPB) on the inner surfaces as a wavelength shifter to convert vacuum ultraviolet (VUV) LAr scintillation light to the visible spectrum. We find that TPB scintillation contains a component with a previously unreported exceptionally long lifetime ($\sim$ms). We discovered that this component differs significantly in magnitude between alpha, beta, and VUV excitation, which enables the use of pulse shape discrimination to suppress surface backgrounds by more than a factor of $10^3$ with negligible loss of dark matter sensitivity. We also discuss how this technique can be extended beyond just LAr experiments.