A stochastic technique based upon the Serpent code is used along with the JEFF-3.3 nuclear data library consistently including their covariance, to adjust fast, non-resonant ENDF-6 format data for U-235 and Pu-239, and this in conjunction with the Asymptotic Generalized Linear Least-Squares (AGLLS) assimilation methodology. The current investigations are focused on simple, well documented critical systems such as Godiva and Jezebel exhibiting much stronger sensitivities of the assimilated parameters to this nuclear data. Correspondingly, the assimilation database consists of effective multiplication factors along with ratios of fission reaction rates per atom for Pu-239 and U-235 which are spectral indices measured at core center.By not identifying the fission cross-section of U-235 with a standard, we find that this data set should be decreased between 2 keV and 2.2 MeV; in relative terms by maximum 5.9 % occurring in the energy range between 41 keV and 67 keV which is less than two standard deviations (σ) of 6.6 %, obtained from the covariance files of the JEFF-3.3 library. Whereas ν¯ needs to be increased by up to ∼ 0.3 %, corresponding to half a σ. Also to reduce is the elastic scattering P1 cross-section between 111 keV and 10 MeV with a stronger decrease amounting to 12.7 % in the range 2.2 MeV-3.7 MeV.For the capture cross-section, we find a decrease of maximum 3 % between 111 keV and 3.7 MeV, in which case the one-σ limit is about 10 %.For Pu-239, the results of the adjustment study also indicate a reduction of the elastic scattering P1 cross-section in the same energy range as for U-235, however by only 5.7 %. The fission and inelastic scattering cross-section changes are much smaller than 1 %; as opposed to U-235, ν¯ is to decrease, and this by less than 0.5 % corresponding to one σ. The additionally proposed fission spectrum change not exceeding the one-σ limit somewhat shifts the median emission energy to a lower value. Differently from U-235, the adjustment of the capture cross-section is an increase of maximum 1.8 % in the range 2.2 MeV-3.7 MeV, which is well below the one-σ limit of the JEFF-3.3 library.