Nowadays, research is mostly focused on developing luminous materials. Specifically, compounds based on inorganic phosphorus have found widespread use in a variety of applications, like radiation dosimetry, field emission displays (FEDs), cathode ray tubes (CRTs), lamp industries, and white light emitting diodes (WLEDs). In order to achieve white light emission, we successfully synthesized single-host K2NaAlF6 co-doped with Dy3+/Eu3+ in this study utilizing the pechini sol-gel approach. Under UV light, the synthesized samples' luminescence characteristics were examined. XRD analysis verified K2NaAlF6's phase purity. The phosphor materials have a tendency to aggregate, as seen by SEM pictures. The K2NaAlF6:Dy3+ doped phosphors showed good excitation at 349 nm in photoluminescence (PL) experiments, with strong emission bands at 489 nm (blue) and 576 nm (yellow). Strong orange emissions were seen for K2NaAlF6: Eu3+ doped phosphors at 595 nm and 614 nm, which correspond to the 5D0→7F1 and 5D0→7F2 transitions in Eu3+ ions. When these rare earths were co-doped, intense red, yellow, and blue emissions were produced. The Commission Internationale de l'Eclairage (CIE) coordinates were used to calculate the colour characteristics of the luminous produced samples. Consequently, these results imply that Dy3+/Eu3+ co-doped K2NaAlF6 phosphors, when stimulated by UV LEDs, could be appropriate for creating reddish-orange and warm white lighting systems.
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