Levitated Nanoparticles Research Articles

Simultaneous ground-state cooling of two levitated nanoparticles by coherent scattering

Simultaneous ground-state cooling of two levitated nanoparticles by coherent scattering

Fluctuating parametric drive of coupled classical oscillators can simulate dissipative qubits

We investigate a system composed of two coupled oscillators subject to stochastic fluctuations in its internal parameters. In particular, we answer the question whether the well-known classical analogy of the quantum dynamics of two-level systems (TLSs), i.e., qubits, provided by two coupled oscillators can be extended to simulate the dynamics of dissipative quantum systems. In the context of nanomechanics, the analogy in the dissipation-free case has already been tested in multiple experimental setups, e.g., doubly clamped or cantilever string resonators and optically levitated particles. A well-known result of this classical analogy is that the relaxation and decoherence times of the analog quantum system must be equal, i.e., T1=T2, in contrast to the general case of quantum TLSs. We show that this fundamentally quantum feature, i.e., T1≠T2, can be implemented as well in the aforementioned classical systems by adding stochastic fluctuations in their internal parameters. Moreover, we show that these stochastic contributions can be engineered in the control apparatus of those systems, discussing, in particular, the application of this theory to levitated nanoparticles and to nanostring resonators. Published by the American Physical Society 2024

Steady motional entanglement between two distant levitated nanoparticles

Quantum entanglement in macroscopic systems is not only essential for practical quantum information processing, but also valuable for the study of the boundary between quantum and the classical world. However, it is very challenging to achieve the steady remote entanglement between distant macroscopic systems. We consider two distant nanoparticles, both of which are optically trapped in two cavities. Based on the coherent scattering mechanism, we find that the ultrastrong optomechanical coupling between the cavity modes and the motion of the levitated nanoparticles could be achieved. The large and steady entanglement between the filtered output cavity modes and the motion of nanoparticles can be generated if the trapping laser is under the red sideband. Then through entanglement swapping, the steady motional entanglement between the distant nanoparticles can be realized. We numerically simulate and find that the two nanoparticles with 10 km distance can be entangled for the experimentally feasible parameters, even in room temperature environments. The generated continuous variable multipartite entanglement is the key to realizing the quantum enhanced sensor network and the sensitivity beyond the standard quantum limit.

Controlling Optomechanical Libration with the Degree of Polarization.

Control of the potential energy and free evolution lie at the heart of levitodynamics as key requirements for sensing, wave function expansion, and mechanical squeezing protocols. Here, we experimentally demonstrate versatile control over the optical potential governing the libration motion of a levitated anisotropic nanoparticle. This control is achieved by introducing the degree of polarization as a new tool for rotational levitodynamics. We demonstrate thermally driven free rotation of a levitated anisotropic scatterer around its short axis and we use the rotational degrees of freedom to probe the local spin of a strongly focused laser beam.

3D sympathetic cooling and detection of levitated nanoparticles

Cooling the center-of-mass motion of levitated nanoparticles provides a route to quantum experiments at mesoscopic scales. Here we demonstrate three-dimensional sympathetic cooling and detection of the center-of-mass motion of a levitated silica nanoparticle. The nanoparticle is electrostatically coupled to a feedback-cooled particle while both particles are trapped in the same Paul trap. We identify two regimes, based on the strength of the cooling: in the first regime, the sympathetically cooled particle thermalizes with the directly cooled one, while in the second regime, the sympathetically cooled particle reaches a minimum temperature. This result provides a route to efficiently cool and detect particles that cannot be illuminated with strong laser light, such as absorptive particles, and paves the way for controlling the motion of arrays of several trapped nanoparticles.

Tuneable Gaussian entanglement in levitated nanoparticle arrays

Optically levitated nanoparticles emerged as an interesting platform for probing fundamental physics. Quantum control of their motion (including potential shaping) predisposes them for emulating various physical systems and studying quantum phenomena with massive objects. Extending these capabilities to quantum many-body systems requires feasible strategies to couple and entangle nanoparticles directly or via an optical bus. We propose a variable, deterministic scheme to generate Gaussian entanglement in the motional steady state of levitated nanoparticles using coherent scattering. Coupling multiple nanoparticles to a common cavity mode allows cooling of a collective Bogoliubov mode; cooling multiple Bogoliubov modes (by trapping each nanoparticle in multiple tweezers, each scattering into a separate cavity mode) removes most thermal noise, leading to strong entanglement. Numerical simulations for three nanoparticles show great tuneability of entanglement with realistic experimental parameters. Our proposal paves the way towards complex motional quantum states for advanced quantum sensing protocols and many-body quantum simulations.

Scalable all-optical cold damping of levitated nanoparticles.

Motional control of levitated nanoparticles relies on either autonomous feedback via a cavity or measurement-based feedback via external forces. Recent demonstrations of the measurement-based ground-state cooling of a single nanoparticle employ linear velocity feedback, also called cold damping, and require the use of electrostatic forces on charged particles via external electrodes. Here we introduce an all-optical cold damping scheme based on the spatial modulation of trap position, which has the advantage of being scalable to multiple particles. The scheme relies on programmable optical tweezers to provide full independent control over the trap frequency and position of each tweezer. We show that the technique cools the centre-of-mass motion of particles along one axis down to 17 mK at a pressure of 2 × 10-6 mbar and demonstrate its scalability by simultaneously cooling the motion of two particles. Our work paves the way towards studying quantum interactions between particles; achieving three-dimensional quantum control of particle motion without cavity-based cooling, electrodes or charged particles; and probing multipartite entanglement in levitated optomechanical systems.

Dynamics of Nano-Particles Inside an Optical Cavity in the Quantum Regime

We investigate the optomechanical effect on a single nano-particle inside an optical cavity, by deriving the optical forces acting on the nano-particle by the cavity from quantum theory. We obtain the steady state of the system and found that the force contains three terms associated with the gradient force, the back-action force resulting from the intra-cavity photon energy change, as well as the reactive force associated with the coupling between the external field and the cavity. Moreover, we solve the dynamical system for a dielectric particle in a small mode volume cavity, which is characterized by a quasi-periodic pattern. These results are important for understanding the control of various types of levitated nano-particles through optomechanical coupling.

Tunable light-induced dipole-dipole interaction between optically levitated nanoparticles.

Arrays of optically trapped nanoparticles have emerged as a platform for the study of complex nonequilibrium phenomena. Analogous to atomic many-body systems, one of the crucial ingredients is the ability to precisely control the interactions between particles. However, the optical interactions studied thus far only provide conservative optical binding forces of limited tunability. In this work, we exploit the phase coherence between the optical fields that drive the light-induced dipole-dipole interaction to couple two nanoparticles. In addition, we effectively switch off the optical interaction and observe electrostatic coupling between charged particles. Our results provide a route to developing fully programmable many-body systems of interacting nanoparticles with tunable nonreciprocal interactions, which are instrumental for exploring entanglement and topological phases in arrays of levitated nanoparticles.

Imaging-based feedback cooling of a levitated nanoparticle.

Imaging-based detection of the motion of levitated nanoparticles complements a widely used interferometric detection method, providing a precise and robust way to estimate the position of the particle. Here, we demonstrate a camera-based feedback cooling scheme for a charged nanoparticle levitated in a linear Paul trap. The nanoparticle levitated in vacuum was imaged using a complementary metal-oxide semiconductor (CMOS) camera system. The images were processed in real-time with a microcontroller integrated with a CMOS image sensor. The phase-delayed position signal was fed back to one of the trap electrodes, resulting in cooling by velocity damping. Our study provides a simple and versatile approach applicable for the control of low-frequency mechanical oscillators.

A Chemical Nanoreactor Based on a Levitated Nanoparticle in Vacuum.

A single levitated nanoparticle is used as a nanoreactor for studying surface chemistry at the nanoscale. Optical levitation under controlled pressure, surrounding gas composition, and humidity provides extreme control over the nanoparticle, including dynamics, charge, and surface chemistry. Using a single nanoparticle avoids ensemble averages and allows studying how the presence of silanol groups at its surface affects the adsorption and desorption of water from the background gas with excellent spatial and temporal resolution. Herein, we demonstrate the potential of this versatile platform by studying the Zhuravlev model in silica particles. In contrast to standard methods, our system allowed the observation of an abrupt and irreversible change in scattering cross section, mass, and mechanical eigenfrequency during the dehydroxylation process, indicating changes in density, refractive index, and volume.

Mechanical Squeezing via Unstable Dynamics in a Microcavity.

We theoretically show that strong mechanical quantum squeezing in a linear optomechanical system can be rapidly generated through the dynamical instability reached in the far red-detuned and ultrastrong coupling regime. We show that this mechanism, which harnesses unstable multimode quantum dynamics, is particularly suited to levitated optomechanics, and we argue for its feasibility for the case of a levitated nanoparticle coupled to a microcavity via coherent scattering. We predict that for submillimeter-sized cavities the particle motion, initially thermal and well above its ground state, becomes mechanically squeezed by tens of decibels on a microsecond timescale. Our results bring forth optical microcavities in the unresolved sideband regime as powerful mechanical squeezers for levitated nanoparticles, and hence as key tools for quantum-enhanced inertial and force sensing.

Detailed fluctuation theorem bound for apparent violations of the second law.

The second law of thermodynamics is a statement about the statistics of the entropy production, 〈Σ〉≥0. For small systems, it is known that the entropy production is a random variable and negative values (Σ<0) might be observed in some experiments. This situation is sometimes called apparent violation of the second law. In this sense, how often is the second law violated? For a given average 〈Σ〉, we show that the strong detailed fluctuation theorem implies a lower tight bound for the apparent violations of the second law. As applications, we verify that the bound is satisfied for the entropy produced in the heat exchange problem between two reservoirs mediated by a bosonic mode in the weak-coupling approximation, a levitated nanoparticle, and a classical particle in a box.

On-chip optical levitation with a metalens in vacuum

Optical levitation of dielectric particles in vacuum is a powerful technique for precision measurements, testing fundamental physics, and quantum information science. Conventional optical tweezers require bulky optical components for trapping and detection. Here, we design and fabricate an ultrathin dielectric metalens with a high numerical aperture of 0.88 at 1064 nm in vacuum. It consists of 500-nm-thick silicon nano-antennas, which are compatible with an ultrahigh vacuum. We demonstrate optical levitation of nanoparticles in vacuum with a single metalens. The trapping frequency can be tuned by changing the laser power and polarization. We also transfer a levitated nanoparticle between two separated optical tweezers. Optical levitation with an ultrathin metalens in vacuum provides opportunities for a wide range of applications including on-chip sensing. Such metalenses will also be useful for trapping ultracold atoms and molecules.

Large Quantum Delocalization of a Levitated Nanoparticle Using Optimal Control: Applications for Force Sensing and Entangling via Weak Forces.

We propose to optimally control the harmonic potential of a levitated nanoparticle to quantum delocalize its center-of-mass motional state to a length scale orders of magnitude larger than the quantum zero-point motion. Using a bang-bang control of the harmonic potential, including the possibility of inverting it, the initial ground-state-cooled levitated nanoparticle coherently expands to large scales and then contracts to the initial state in a time-optimal way. We show that this fast loop protocol can be used to enhance force sensing as well as to dramatically boost the entangling rate of two weakly interacting nanoparticles. We parameterize the performance of the protocol, and therefore the macroscopic quantum regime that could be explored, as a function of displacement and frequency noise in the nanoparticle's center-of-mass motion. This noise analysis accounts for the sources of decoherence relevant to current experiments.

Theory of nanoparticle cooling by elliptic coherent scattering

Coherent scattering of an elliptically polarised tweezer into a cavity mode provides a promising platform for cooling levitated nanoparticles into their combined rotational and translational quantum regime [Phys. Rev. Lett. 126, 163603 (2021)]. This article presents the theory of how aspherical nanoparticles are affected by elliptically polarised laser beams, how two orthogonal cavity modes enable rotational and translational cooling, and how the resulting power spectra contain signatures of rotational non-linearities. We provide analytic expressions for the resulting trapping frequencies, opto-mechanical coupling strengths, cooling rates, and steady-state occupations and we study their dependence on the tweezer ellipticity.

Quantum electromechanics with levitated nanoparticles

Preparing and observing quantum states of nanoscale particles is a challenging task with great relevance for quantum technologies and tests of fundamental physics. In contrast to atomic systems with discrete transitions, nanoparticles exhibit a practically continuous absorption spectrum and thus their quantum dynamics cannot be easily manipulated. Here, we demonstrate that charged nanoscale dielectrics can be artificially endowed with a discrete level structure by coherently interfacing their rotational and translational motion with a superconducting qubit. We propose a pulsed scheme for the generation and read-out of motional quantum superpositions and entanglement between several levitated nanoparticles, providing an all-electric platform for networked hybrid quantum devices.

Stationary Gaussian entanglement between levitated nanoparticles

Coherent scattering of photons is a novel mechanism of optomechanical coupling for optically levitated nanoparticles promising strong, versatile interactions with light and between nanoparticles. We show that it allows efficient deterministic generation of Gaussian entanglement between two particles in separate tweezers. A combination of red- and blue-detuned tweezers brings a mechanical Bogoliubov mode to its ground state. An additional, dispersively coupled cavity mode can reduce noise in the orthogonal mode, resulting in strong entanglement as quantified by the logarithmic negativity and verifiable with the Duan criterion for realistic experimental parameters. Such an important resource for quantum sensing and quantum simulations is pivotal for current experiments and presents an important step towards optomechanics with multiple particles in the quantum regime.

Classical and quantum time crystals in a levitated nanoparticle without drive

Time crystal is defined as a phase of matter spontaneously exhibiting a periodicity in time. Previous studies focused on discrete quantum time crystals under periodic drive. Here, we propose a time crystal model based on a levitated charged nanoparticle in a static magnetic field without drive. Both the classical time crystal in thermal equilibrium and the quantum time crystal in the ground state can emerge in the spin rotational mode, under the strong magnetic field or the large charge-to-mass ratio limit. Besides, for the first time, the \emph{time polycrystal} is defined and naturally appears in this model. Our model paves a way for realizing time crystals in thermal equilibrium.

Optical levitation using broadband light

The ability to create dynamic, tailored optical potentials has become important across fields ranging from biology to quantum science. We demonstrate a method for the creation of arbitrary optical tweezer potentials using the broadband spectral profile of a superluminescent diode combined with the chromatic aberration of a lens. A tunable filter, typically used for ultrafast laser pulse shaping, allows us to manipulate the broad spectral profile and therefore the optical tweezer potentials formed by focusing of this light. We characterize these potentials by measuring the Brownian motion of levitated nanoparticles in vacuum and also demonstrate interferometric detection and feedback cooling of the particle’s motion. This simple and cost-effective technique will enable wide application and allow rapid modulation of the optical potential landscape in excess of megahertz frequencies.