Lasing In Air Research Articles

Bidirectional Cascaded Superfluorescent Lasing in Air Enabled by Resonant Third Harmonic Photon Exchange from Nitrogen to Argon.

Cavity-free lasing in atmospheric air has stimulated intense research toward a fundamental understanding of underlying physical mechanisms. In this Letter, we identify a new mechanism-a third-harmonic photon mediated resonant energy transfer pathway leading to population inversion in argon via an initial three-photon excitation of nitrogen molecules irradiated by intense 261nm pulses-that enables bidirectional two-color cascaded lasing in atmospheric air. By making pump-probe measurements, we conclusively show that such cascaded lasing results from superfluorescence rather than amplified spontaneous emission. Such cascaded lasing with the capability of producing bidirectional multicolor coherent pulses opens additional possibilities for remote sensing applications.

Fluorescence and lasing of neutral nitrogen molecules inside femtosecond laser filaments in air: mechanism and applications.

High power femtosecond laser pulses launched in air undergo nonlinear filamentary propagation, featuring a bright and thin plasma channel in air with its length much longer than the Rayleigh length of the laser beam. During this nonlinear propagation process, the laser pulses experience rich and complex spatial and temporal transformations. With its applications ranging from supercontinuum generation, laser pulse compression, remote sensing to triggering of lightning, the underlying physical mechanism of filamentation has been intensively studied. In this review, we will focus on the fluorescence and cavity-free lasing effect of the plasma filaments in air. The different mechanisms underlying the fluorescence of the excited neutral nitrogen molecules will be throughly examined and it is concluded that the electron collision excitation is the dominant channel for the formation of the excited nitrogen molecules. The recently discovered "air lasing" effect, a cavity-free bidirectional lasing emission emitted by the filaments, will be introduced and its main properties will be emphasized. The applications of the fluorescence and lasing effect of the neutral nitrogen molecules will be introduced, with two examples on spectroscopy and detection of electric field. Finally, we discuss the quenching effect of the lasing effect in atmosphere and the mechanisms responsible will be analyzed. An outlook for the achievement of backward lasing in air will be briefly presented.

Extremely enhanced N2+ lasing in a filamentary plasma grating in ambient air.

Cavity-free air lasing offers a promising route towards the realization of atmospheric lasers for various applications such as remote sensing and standoff spectroscopy; however, achieving efficient generation and control of air lasing in ambient air is still a challenge. Here we show the experimental realization of a giant lasing enhancement by three to four orders of magnitude in ambient air for the self-seeded N2+ lasing at 428 nm, assigned to the B2Σu+(ν'=0) and X2Σg+(ν''=1) emission, by modulating the spatiotemporal overlap of ultrashort near-infrared control-pump pulses in a filamentary plasma grating; meanwhile, the spontaneous emission from the same transition is only enhanced by three to four times. We find that this enhancement is sensitive to the relative polarization and interference time of the two pulses, and reveal that the formation of the plasma grating induces different population variations in the B2Σu+(ν'=0) and X2Σg+(ν''=1) levels, resulting in an enormous population inversion between the two levels, thereby a higher gain for the giant enhancement of N2+ lasing in ambient air.

Remote Lasing in Humid Air from Atomic Hydrogen

Over the last few years, air lasing has emerged as an attractive topic in standoff detection research. However, existing approaches have relied on the major species of air as the gain medium. This work presents the first experimental demonstration of an air laser based on water vapor, a minor constituent of air. The approach relies on photodissociation of water vapor molecules followed by two-photon pumping of the constituent hydrogen atoms to produce lasing on the well-known Balmer-alpha line. This hydrogen laser is characterized in both the forward as well as return direction, and this paper discusses the effect of some parameters, including the presence and type of buffer gas, as well as the pump beam focusing. It is found that most of these results can be explained in terms of their influence on the gain of the stimulated emission process. This method can be potentially applied to other hydrogen-containing molecules and offers a promising approach for standoff detection of trace species.

Analytical study of the spiky feature in a two-photon driven lossy ladder system

There has been an experimental report (Traverso et al 2012 Proc. Natl Acad. Sci. USA 109 15185) that oxygen lasing in ambient air exhibits a spiky feature. We theoretically explore a ladder-type three-level atomic system driven by a two-photon resonant pump pulse in a lossy medium, which corresponds to that oxygen experiment. We study the Maxwell–Bloch equations both numerically and analytically and discover that a long pump field brings competition between two mechanisms of coherent pumping and coherent emission, leading to the spiky emission, which cannot be produced using a short pump. The results indicate that atomic coherence occurs in the experiment. Our study provides a clear understanding of the oxygen experiment using a nanosecond pump laser and could lead to the potential application of this oxygen lasing in future experiments.

A Breakthrough for Remote Lasing in Air

A scheme using two pump wavelengths in the infrared and ultraviolet produces more efficient laserlike emission in air, which could benefit remote sensing applications.

Self-seeded lasing in ionized air pumped by 800 nm femtosecond laser pulses

We report on the lasing in air and pure nitrogen gas pumped by a single 800 nm femtosecond laser pulse. Depending on gas pressure, incident laser power and beam convergence, different lasing lines are observed in the forward direction with rapid change of their relative intensities. The lines are attributed to transitions between vibrational and rotational levels of the first negative band of the singly charged nitrogen molecule-ion. We show that self-seeding plays an important role in the observed intensity changes.

On-chip microlasers for biomolecular detection via highly localized deposition of a multifunctional phospholipid ink

We report on a novel approach to realize on-chip microlasers, by applying highly localized and material-saving surface functionalization of passive photonic whispering gallery mode microresonators. We apply dip-pen nanolithography on a true three-dimensional structure. We coat solely the light-guiding circumference of pre-fabricated poly(methyl methacrylate) resonators with a multifunctional molecular ink. The functionalization is performed in one single fabrication step and simultaneously provides optical gain as well as molecular binding selectivity. This allows for a direct and flexible realization of on-chip microlasers, which can be utilized as biosensors in optofluidic lab-on-a-chip applications. In a proof-of-concept we show how this highly localized molecule deposition suffices for low-threshold lasing in air and water, and demonstrate the capability of the ink-lasers as biosensors in a biotin-streptavidin binding experiment.

Remote lasing in air by recombination and electron impact excitation of molecular nitrogen

We analyze and simulate the physical mechanisms for a remote atmospheric lasing configuration which utilizes a combination of an ultrashort pulse laser to form a plasma filament of seed electrons, and a heater beam to heat the seed electrons. Nitrogen molecules are excited by electron impact and recombination processes to induce lasing in the ultraviolet. Recombination excitation, thermal excitation, gain, and saturation are analyzed and simulated. The lasing gain is sufficiently high to reach saturation within the length of the plasma filament. A remotely generated ultraviolet source may have applications for standoff detection of biological and chemical agents.

Backward lasing in air

Backward lasing in air

Backward lasing in air

Backward lasing in air

High-Gain Backward Lasing in Air

The compelling need for standoff detection of hazardous gases and vapor indicators of explosives has motivated the development of a remotely pumped, high-gain air laser that produces lasing in the backward direction and can sample the air as the beam returns. We demonstrate that high gain can be achieved in the near-infrared region by pumping with a focused ultraviolet laser. The pumping mechanism is simultaneous resonant two-photon dissociation of molecular oxygen and resonant two-photon pumping of the atomic oxygen fragments. The high gain from the millimeter-length focal zone leads to equally strong lasing in the forward and backward directions. Further backward amplification is achieved with the use of earlier laser spark dissociation. Low-divergence backward air lasing provides possibilities for remote detection.

Nanoslot laser

We propose and demonstrate photonic crystal nanolaser with a nanoslot. Using high-aspect etching process, we succeed in fabricating a 30-nm-wide nanoslot device and room temperature lasing in both air and liquids. As an index sensor, it exhibits a high sensitivity of 410 nm per refractive index unit, as well as low temperature dependence in water. These behaviors and theoretical analysis suggest that the mode is strongly localized in the nanoslot. This device will be effective for enhancing light-matter interaction in cavity quantum electro dynamics, nonlinear optics, and biosensing.

Air ultraviolet laser excited by high-power microwave pulses

Lasing in atmospheric air excited by high-power nanosecond microwave pulses was observed and investigated. Stimulated emission was observed as a result of transitions in N2 at wavelengths λ = 315.8, 337.1, and 357.7 nm and resonator-free amplification of spontaneous radiation. The forward and backward laser fluxes differed by a factor exceeding 10 demonstrating that a traveling wave configuration was established. The optimal air pressure was 38 Torr. In principle, it should be possible to construct a laser using free–localized discharge in air excited by crossing laser beams.