Pump Laser Research Articles

Self-injection-locked second-harmonic generation at 532 nm in high-Q Fabry-Perot micro-cavities

Based on the combination of DFB laser self-injection-locking (SIL) and external-cavity frequency-doubling, we have successfully demonstrated, for the first time to our knowledge, the self-injection-locked second-harmonic generation (SHG) at 532 nm by adopting the high-Q Fabry-Perot (FP) micro-cavities. With the DFB incident pump power of 79 mW at 1064 nm, the maximum output SHG power of 20.7 mW at 532 nm was achieved from the 11 mm long plane-concave FP external-cavity of 0.12 mL volume with the 10 mm long PPLN crystal. The corresponding output SHG efficiency of 26.2 % and the Q-factor of 56.5 M both exceeded all known SIL-SHG results reported, and the SIL SHG output power was one order of magnitude higher than the previous maximum of over 2 mW. The reliable SIL has been realized by utilizing the natural birefringence of the intracavity nonlinear crystal to provide laser feedback, and the intrinsic linewidth of the SIL pump laser at 1064 nm was about 30 Hz. Moreover, by replacing the PPLN crystal with the LN and KTP crystals, the output SHG power of 6.1 mW and 2.7 mW at 532 nm were respectively obtained with the Q-factors of 29.3 M and 27.6 M. Our new SIL-SHG design with the high-Q FP micro-cavity paves the way to a new type of the field-deployable ultra-narrow-linewidth visible and near-visible lasers of low size, weight, and power (SWaP).

21.8 W acetylene-filled hollow-core anti-resonant fiberamplified spontaneous emission source at 3.1 µm.

We report a 20-W-level acetylene-filled nested hollow-core anti-resonant fiber (nested HC-ARF) amplified spontaneous emission (ASE) source at 3.1 µm. A 1535 nm hundred-watt wavelength tunable single-frequency fiber laser with a high signal-to-noise ratio and narrow linewidth is built for pumping acetylene molecules. Simultaneously, a homemade 120 µm core diameter eight-tube nested HC-ARF is used as a gas chamber to obtain high pump laser coupling efficiency. The mid-infrared (mid-IR) ASE source output power of 21.8 W is achieved at 3.1 µm through the low-pressure acetylene gas-filled nested HC-ARF, and the slope efficiency is 25.1%. In addition, the ASE source features an excellent beam quality of Mx 2 = 1.16 and My 2 = 1.13. To the best of our knowledge, for the first time, it is a record output power for such mid-infrared ASE sources while maintaining excellent beam quality. This work provides a new way to achieve high-power mid-infrared emission.

Optical Amplification at 1.5µm in ErIII Coordination Polymer-Doped Waveguides Based on Intramolecular Energy Transfer.

9,9-bis (diphenylphosphorylphenyl) fluorene (FDPO) and dibenzotetrathienoacene (DBTTA), are synthesized as the neutral and anionic ligands, respectively, to prepare the ErIII coordination polymer [Er(DBTTA)3(FDPO)]n. Based on the intramolecular energy transfer, optical gains at 1.5µm are demonstrated in [Er(DBTTA)3(FDPO)]n-doped polymer waveguides under excitations of low-power light-emitting diodes (LEDs) instead of laser pumping. A ligand-sensitization scheme between organic ligands and Er3+ ions under an excitation of an ultraviolet (UV) LED is established. Relative gains of 10.5 and 8.5dBcm-1 are achieved at 1.53 and 1.55µm, respectively, on a 1-cm-long SU-8 channel waveguide with a cross-section of 2×3µm2 and a 1.5-µm-thick [Er(DBTTA)3(FDPO)]n-doped polymethylmethacrylate (PMMA) as upper cladding. The ErIII coordination polymer [Er(DBTTA)3(FDPO)]n can be conveniently integrated with various low-loss inorganic waveguides to compensate for optical losses in the C-band window. Moreover, by relying on the intramolecular energy transfer and UV LED top-pumping technology, it is easy to achieve coupling packaging of erbium-doped waveguide amplifiers (EDWAs) with pump sources in planar photonic integrated chips, effectively reducing the commercial costs.

Tunable band-stop fiber filter based on laser-induced graphene metamaterial in THz frequency.

As an important device in the application of terahertz (THz) technology, a THz filter has broad application prospects in the fields of THz communication, imaging, and sensing. In this paper, a THz filter based on grating structure laser-induced graphene (LIG)/ side polishing terahertz fiber composite structure is proposed. In the experiment, we achieved the maximum Q factor of 23.83 at the central resonant frequency of 0.715 THz. By modifying the grating structure, a tunable operational span of 269 GHz was achieved, along with a tunable range of 21 GHz through laser stimulation. In testing, we found that LIG materials prepared with circular filling are more sensitive to relatively high-power pump lasers, while LIG samples prepared with line filling exhibit better linear response to laser power. Furthermore, the compact and highly integrated nature of the device suggests its broad potential utility in the realm of THz frequency selection.

Random lasing using laser generated and modified silver nanoparticles

The authors report incoherent random laser action in systems where the optical feedback is provided by multiple scattering generated by different classes of silver nanoparticles in the colloidal state, having plasmon resonances at different frequencies. They found improved performance of triangular silver nanoplates as compared to nanospheres, with a threshold as low as 1 mJ/cm2 and a 5 times lower optimal silver concentration, due to plasmonic enhancement effects and tuning of the plasmon resonance. The nanoparticles were also tested for stability against illumination by the pump laser, as the onset of pulsed laser melting is comparable to random laser threshold in terms of pump fluence, severely limiting the range of operation of nanoparticles with main plasmon resonance close to the pump wavelength. The optimal approach to choose plasmonic nanoparticles for random lasing must, therefore, take the stability aspect into serious consideration as well as the plasmonic enhancement of random lasing.

Low-noise short-wavelength pumped frequency downconversion for quantum frequency converters

We present a highly efficient low-noise quantum frequency converter from the visible range to telecom wavelengths, combining a pump laser at intermediate frequency resonantly enhanced in an actively stabilized cavity with a monocrystalline bulk crystal. A demonstrator for photons emitted by nitrogen-vacancy-center qubits achieves 43% external efficiency with a noise photon rate per wavelength (frequency) band of 2 s−1/pm(17 s−1/GHz) – reducing the noise by two orders of magnitude compared with current devices based on periodically poled crystals with waveguides. With its tunable output wavelength, this device enables the generation of indistinguishable telecom photons from different network nodes and is, as such, a crucial component for a future quantum internet based on optical fiber.

Vibrational coherences in half-broadband 2D electronic spectroscopy: Spectral filtering to identify excited state displacements.

Vibrational coherences in ultrafast pump-probe (PP) and 2D electronic spectroscopy (2DES) provide insights into the excited state dynamics of molecules. Femtosecond coherence spectra and 2D beat maps yield information about displacements of excited state surfaces for key vibrational modes. Half-broadband 2DES uses a PP configuration with a white light continuum probe to extend the detection range and resolve vibrational coherences in the excited state absorption (ESA). However, the interpretation of these spectra is difficult as they are strongly dependent on the spectrum of the pump laser and the relative displacement of the excited states along the vibrational coordinates. We demonstrate the impact of these convoluting factors for a model based upon cresyl violet. A careful consideration of the position of the pump spectrum can be a powerful tool in resolving the ESA coherences to gain insights into excited state displacements. This paper also highlights the need for caution in considering the spectral window of the pulse when interpreting these spectra.

Simulation of the synergistic effect of multiple operation parameters on cavity soliton in nonlinear fiber resonator

All optical soliton communication is a new generation of ultra-long distance and ultra-high speed optical fiber communication technology. Optical cavity solitons (CSs), whose pulse property is unique, have shown great potentials in optical soliton communication systems. Here, a theoretical model of nonlinear fiber resonator for CS generation is proposed. The effect of pump laser and resonant cavity parameters on the CS pulse performance is detailedly investigated and deeply analysed. Furthermore, the synergistic effect of continuous wave (CW) pump laser power and pump pulse peak power, and the synergistic effect of dispersion condition, fiber nonlinear coefficient and fiber length on the generation and property of CS pulse are respectively discussed and summarized. Finally, the launch conditions and parameter variation tolerances of cavity soliton in nonlinear fiber resonant cavity have been successfully generalized. These results can provide important instruction to the experimental generation and optimization of CS pulse.

Strong frequency correlation and anticorrelation between a Raman laser and its pump laser for positive and negative dispersions

Strong frequency correlation and anticorrelation between a Raman laser and its pump laser for positive and negative dispersions

Selective cooling and squeezing in a lossy optomechanical closed loop embodying an exceptional surface

A closed-loop, lossy optomechanical system consisting of one optical and two degenerate mechanical resonators is computationally investigated. This system constitutes an elementary synthetic plaquette derived from the loop phase of the intercoupling coefficients. In examining a specific quantum attribute, we delve into the control of quadrature variances within the resonator selected through the plaquette phase. An amplitude modulation is additionally applied to the cavity-pumping laser to incorporate mechanical squeezing. Our numerical analysis relies on the integration-free computation of steady-state covariances for cooling and the Floquet technique for squeezing. We provide physical insights into how non-Hermiticity plays a crucial role in enhancing cooling and squeezing in proximity to exceptional points. This enhancement is associated with the behavior of complex eigenvalue loci as a function of the intermechanical coupling rate. Additionally, we demonstrate that the parameter space embodies an exceptional surface, ensuring the robustness of exceptional point singularities under experimental parameter variations. However, the pump laser detuning breaks away from the exceptional surface unless it resides on the red-sideband by an amount sufficiently close to the mechanical resonance frequency. Finally, we show that this disparate parametric character entitles frequency-dependent cooling and squeezing, which is of technological importance.

Active offset-frequency control of optical frequency comb via sum-frequency mixing of passively mode-locked laser and continuous-wave laser

We propose a method for actively controlling the frequency of an optical frequency comb (OFC) using sum-frequency generation (SFG) with a nonlinear crystal. For the first time, OFC generation was experimentally demonstrated via sum-frequency mixing of a narrowband continuous wave (CW) laser and a passively mode-locked fiber laser. By adjusting the optical frequency of the CW laser, we successfully controlled the offset-frequency of the SFG-OFC, which was mapped from the OFC of the pulse pump laser. Furthermore, by comparing the spectral widths of the SFG-OFC modes generated from two CW lasers with different spectral widths, we confirmed that the spectral characteristics of the SFG-OFC modes depended on the spectral features of the CW laser.

2.1–2.2 μm wavelength-tunable cascade gain modulation Raman fiber laser

We present a theoretical and experimental analysis of a mid-infrared wavelength-tunable cascade gain modulation Raman fiber laser. Our simulation model incorporates the Generalized Nonlinear Schrödinger Equation with the fiber Bragg grating transmission functions. Utilizing the pulse tracking method, we investigate and analyze the impact of pump pulse width and Raman gain fiber length on the first and second order Raman laser thresholds. Additionally, we exhibit the evolution process of the pulse and optical spectrum at a constant pump pulse energy. Furthermore, we present the output pulse width and energy, and the Raman laser center wavelength as a function of the pump pulse energy. Subsequently, using the optimal theoretical values of pump pulse width and Raman gain fiber length, we experimentally achieve the gain modulation Raman fiber laser. With a 1990 nm laser pumping, the Raman laser can produce a 2172 nm laser with a pulse width of 1.25 µs and a single pulse energy of approximately 400 nJ. When tuning the pump laser wavelength from 1950 nm to 2030 nm, the gain modulation Raman laser wavelength can vary from 2130 nm to 2215 nm. Importantly, our experimental results closely align with the theoretical predictions. This study provides valuable insights for the investigation of gain modulation Raman fiber lasers.

Real-time measurement of pump beam polarization through the transmitted light intensity in a polarized alkali metal vapor cell.

A laser beam with left-/right-handed circular polarization is generally used to create the oriented atomic spins for precision measurements in a spin-exchange relaxation-free (SERF) co-magnetometer. The fluctuation of laser polarization interferes with the spin polarization of alkali metal atoms, leading to the system performance degradation. Here, we report a method for real-time polarization state measurement by using the transmitted light intensity of the pump beam passing through the vapor cell. Based on the principle of circular dichroism, the optical absorption model of polarized alkali metal atoms is established. The simulation results of the transmittance of the pump laser with different polarization states through the alkali metal vapor cell are given and verified by experiments. The experimental results show that the circularly polarized beam has the weakest absorption, while the linearly polarized laser beam is absorbed the strongest. The achieved measurement accuracy stands at an impressive 98.83 %. This work provides a simple and easy-to-use way to measure the polarization state of the laser beam used in the vapor cell devices, particularly the microfabricated prototypes with limited space.

The laser pump X-ray probe system at LISA P08 PETRA III.

Understanding and controlling the structure and function of liquid interfaces is a constant challenge in biology, nanoscience and nanotechnology, with applications ranging from molecular electronics to controlled drug release. X-ray reflectivity and grazing incidence diffraction provide invaluable probes for studying the atomic scale structure at liquid-air interfaces. The new time-resolved laser system at the LISA liquid diffractometer situated at beamline P08 at the PETRA III synchrotron radiation source in Hamburg provides a laser pump with X-ray probe. The femtosecond laser combined with the LISA diffractometer allows unique opportunities to investigate photo-induced structural changes at liquid interfaces on the pico- and nanosecond time scales with pump-probe techniques. A time resolution of 38 ps has been achieved and verified with Bi. First experiments include laser-induced effects on salt solutions and liquid mercury surfaces with static and varied time scales measurements showing the proof of concept for investigations at liquid surfaces.

Demonstration of standing cavity Brillouin random fiber lasers using double fiber Bragg grating arrays.

Bidirectional feedback by fiber Bragg grating arrays (FBGAs) reduced the loss of the cavity and increased stimulated Brillouin scattering (SBS) gain by bi-directional Stokes wave through FBGA associated Rayleigh feedback of the pump wave. As a result, the Q value of the Brillouin random fiber laser (BRFL) increased significantly, which leads to narrow linewidth. This is different from the ring configuration with unidirectional SBS gain versus dual SBS gain of the same fiber length. Highly efficient use of the SBS gain fiber for coherent SBS amplification suppressed thermal noise associated Stokes wave. Such an efficient SBS laser is realized by a standing cavity BRFL based on double FBGAs. Multiple scattering of light traveling in strong scattering FBGAs enables light localization and the generation of high-Q reflection peaks. Coherent SBS amplification with high Q help to reduce laser relative intensity noise (RIN) and laser linewidth. Experimental results demonstrate that the BRFL supports localized modes by increasing the scattering strength of the FBGA random feedback, resulting in long lifetime and single-frequency emission with 20 dB noise floor reduction. The BRFL with a 1 km Brillouin gain fiber exhibits lower RIN and narrower linewidth than that with a 10 km Brillouin gain fiber due to the stronger gain competition of more modes in the longer cavity length. The optimized standing caivty BRFL with 1 km gain fiber leads to 3.5 kHz linewidth versus 40 kHz from the pump laser. These findings provide experimental evidence that double FBGAs offer a unique setting to control mode dynamics, realizing low-noise single-frequency lasing.

Demonstration of Optical Gain at 1535 nm Based on ErIII Complex‐Doped Polymer Waveguides Under Light‐Emitting Diode Excitation

AbstractA near‐infrared luminescent complex Er(DBTTA)3(DBFDPO) [where DBTTA = dibenzotetrathienoacene; DBFDPO = 4,6‐bis (diphenylphosphoryl) dibenzofuran] is synthesized. Based on the intramolecular energy transfer between organic ligands and Er3+ ions, optical gains at 1535 nm are demonstrated in Er(DBTTA)3(DBFDPO)‐doped polymer waveguides under the excitation of light‐emitting diodes (LEDs) instead of laser pumping. Relative gains of 6.4, 8.2, and 10.6 dB are obtained in 1 cm long waveguides with cross‐sectional dimensions of 6 × 4, 4 × 4, and 2 × 3 µm2 respectively, using the vertical top‐pumping mode of a 365 nm LED with 462 mW. Incorporating an ≈100 nm thick aluminum reflector grown under the lower cladding, enhanced the optical gain to 11.6 dB cm−1 in a waveguide with a cross‐section of 4 × 4 µm2, and an internal gain of ≈7.4 dB cm−1 is achieved. By relying on the intramolecular energy transfer and LED top‐pumping technology, the upconversion luminescence of Er3+ ions and thermal damage to polymer waveguides caused by the high power density of laser pumping can be effectively reduced. The complex Er(DBTTA)3(DBFDPO)‐doped polymer can be spin‐coated on different types of waveguides to compensate for optical losses at 1.5 µm and is expected to have a critical role in planar photonic integration.

Free-space laser emission from Nd:YAG elliptical microdisks.

The utilization of deformed microcavities, such as elliptical microdisks, has been widely acknowledged as an effective solution for achieving free-space emission in microcavity lasers. However, the deformations introduced in the microcavity structure tend to decrease the quality factor (Q factor), resulting in weakened output intensity. To address this issue, one potential approach is to employ highly efficient laser gain media that can compensate for the negative impact of the structure on the output intensity. In this study, we employed the exceptional laser crystal material Nd:YAG as the laser gain medium and successfully fabricated an elliptical microdisk laser with a major semiaxis of 15 µm and an eccentricity ratio of 0.15. By utilizing an 808 nm laser for pumping, we were able to achieve free-space laser emission with a slope efficiency of 1.7% and a remarkable maximum output power of 58 µW. This work contributes toward the advancement of the application of deformation microcavity lasers.

Magnetic field mapping along a NV-rich nanodiamond-doped fiber

Integration of NV−-rich diamond with optical fibers enables guiding quantum information on the spin state of the NV− color center. Diamond-functionalized optical fiber sensors have been demonstrated with impressive sub-nanotesla magnetic field sensitivities over localized magnetic field sources, but their potential for distributed sensing remains unexplored. The volumetric incorporation of diamonds into the optical fiber core allows developing fibers sensitive to the magnetic field over their entire length. Theoretically, this makes distributed optical readout of small magnetic fields possible, but does not answer questions on the addressing of the spatial coordinate, i.e., the location of the field source, nor on the performance of a sensor where the NV− fluorescence is detected at one end, thereby integrating over color centers experiencing different field strength and microwave perturbation. Here, we demonstrate distributed magnetic field measurements using a step-index fiber with the optical core volumetrically functionalized with NV− diamonds. A microwave antenna on a translation stage is scanned along a 13 cm long section of a straight fiber. The NV− fluorescence is collected at the fiber's far end relative to the laser pump input end. Optically detected magnetic resonance spectra were recorded at the fiber output for every step of the antenna travel, revealing the magnetic field evolution along the fiber and indicating the magnetic field source location. The longitudinal distribution of the magnetic field along the fiber is detected with high accuracy. The simplicity of the demonstrated sensor would be useful for, e.g., magnetic-field mapping of photonics- and/or spintronics-based integrated circuits.

Investigation of the sensitization effect of Yb3+ in Yb, Er co-doped Sr5(PO4)3F transparent ceramics: From single-band red upconversion to temperature sensing behavior

Lanthanide-ion-doped red upconversion (UC) fluorescent materials with excellent signal-to-noise ratio, stability, and red-green luminous intensity ratio have proven of tremendous research importance for biomedical, three-dimensional (3D) displays, sensors, and other sectors. In this study, xYb, 1Er: Sr5(PO4)3F (S-FAP) (x=0–5 at%) transparent ceramics with outstanding optical quality were fabricated by hot pressing the co-precipitation powder with high sintering activity. The energy dispersive X-ray (EDX) results showed that the trivalent lanthanide ions were evenly doped into the S-FAP ceramic lattice. Increased Yb3+ doping considerably restricted the growth of ceramic grain size, which should be attributable to a decrease in sintering activity under high Yb doping conditions. The co-doping of Yb3+ successfully resulted in a significant improvement in up/down conversion efficiency via effective energy transfer mechanisms and the optimization of the electron population at the energy level of red-green emission. Furthermore, single-band red upconversion luminescence with the greatest red-green upconversion luminescence integral intensity ratio of 125.74 was discovered under 980 nm laser pumping at room temperature. The energy transition process involved in the phenomenon of the up-conversion luminescence intensity shift of red-green emission has been thoroughly examined. Finally, the noncontact optical thermometric ability based on fluorescence intensity ratio (FIR) technology showed that the maximum absolute sensitivity (Sa) of the 5Yb1Er sample in the temperature range of 320–556 K is 1.1×10−3 K−1, implying the possible use of Yb/Er-doped S-FAP transparent ceramics in the field of optical thermometers.

Orthogonally polarized dual-wavelength Pr:LiGdF4 lasers in the green range

We demonstrate a diode-pumped continuous-wave tunable orthogonally polarized dual-wavelength Pr:LiGdF4 laser in the green range. The excellent mode matching between the pump and green lasers is achieved under the consideration of thermally induced effects. We analyze the condition of gain-to-loss balance via an uncoated glass etalon to achieve the dual-wavelength operation. At an absorbed pump power of 17.9 W, a dual-wavelength laser operating at 546 nm in π-polarization and 538 nm in σ-polarization with 1.72 W of average output power was obtained. Orthogonally polarized dual-wavelength laser operation at shorter- or longer-wavelength pairs with lower average output power could also be realized for other output-coupling transmissions. To the best of our knowledge, this is the first work realizing orthogonally polarized dual-wavelength operation in Pr:LiGdF4 lasers.