Laser Polarization Direction Research Articles

Ellipticity of the harmonic emission from graphene irradiated by a linearly polarized laser

We investigate the high-order harmonic generation in graphene irradiated by a linearly polarized intense laser, addressing the ellipticity or polarization properties of the harmonics. We exploit time-dependent density functional theory to calculate the harmonic spectra for a laser wavelength of 4770 nm and an intensity of 1.7 $\mathrm{TW}/{\mathrm{cm}}^{2}$, and our numerical results can qualitatively reproduce recent experimental data. Our simulations also reveal that the harmonic ellipticity depends on both the harmonic order and the orientation angle between the graphene symmetric axis and the laser polarization direction. It can reach 0.68 for the ninth-order harmonic at the orientation angle of ${20}^{\ensuremath{\circ}}$. To understand the mechanism of the high ellipticity, we develop a two-band model based on the tight-binding approximation. We may explain the ellipticity of high-order harmonic generation by investigating the transition dipole moments in the two-band model. Our theory further predicts a sensitive dependence of the harmonic ellipticity on the laser intensity for various laser wavelengths.

Orientation dependence of high-order harmonic generation in graphene

We investigate the orientation dependence of high-order harmonic generation (HHG) in graphene by solving the semiconductor Bloch equations. The tight-binding approximation including up to the third-nearest-neighbor atoms is used to model the graphene. Our simulations show that the orientation dependence of HHG shows different patterns for different harmonics. With increasing the laser intensity, these patterns become similar except for a double-peak structure shown in lower-order harmonics. The double-peak structure appears at high laser intensity due to the contribution of the harmonic perpendicular to the laser polarization direction. The harmonic yield is decomposed as the contributions of the nearest-neighbor interaction, the second-nearest-neighbor interaction, and the third-nearest-neighbor interaction. Our results show that the harmonic yields are mainly contributed by the nearest-neighbor interaction, but the third-nearest-neighbor interaction also plays an important role and modifies the orientation dependence.

Fabrication of high-aspect-ratio grooves with high surface quality by using femtosecond laser

PurposeThe purpose of this study is to fabricate high-aspect-ratio grooves with high surface quality by femtosecond laser (FS) to improve the machinability of silicon carbide (SiC) and optimize the process parameters in micromechanical applications.Design/methodology/approachFour contrast experiments are reported to characterize the FS laser grooving process for SiC with polarization direction, crystal orientation, multi-pass scanning and z layer feed, respectively. The effects of different experimental conditions on the groove characteristics, material removal rate (MRR), aspect ratio, heat affected zone (HAZ) and surface roughness Ra are analyzed.FindingsThe influence of increasing laser fluence and multi-scanning pass on the groove depth is greater than on the groove width. The MRR, aspect ratio, HAZ and Ra increased with the increase of laser fluence and multi-scanning pass. The direction of laser polarization affects the direction of hot electron injection but has little effect on the material characteristics. FS laser ablation is an isotropic process and there is no obvious change in different crystal orientations. The z-layer feed can significantly increase the groove width and depth and reduce HAZ and Ra. The maximum aspect ratio of 82.67% was fabricated.Originality/valueThe results contribute to the understanding of the removal mechanism and reduce the friction of the microfluidic device and improve the flowability in the FS laser ablation of SiC. This paper provides suggestions for the selection of suitable process parameters and provides a wider possibility for the application of micro-texture on SiC.

Extreme Sub-Wavelength Structure Formation from Mid-IR Femtosecond Laser Interaction with Silicon.

Mid-infrared (MIR) wavelengths (2–10 m) open up a new paradigm for femtosecond laser–solid interactions. On a fundamental level, compared to the ubiquitous near-IR (NIR) or visible (VIS) laser interactions, MIR photon energies render semiconductors to behave like high bandgap materials, while driving conduction band electrons harder due to the scaling of the ponderomotive energy. From an applications perspective, many VIS/NIR opaque materials are transparent for MIR. This allows sub-surface modifications for waveguide writing while simultaneously extending interactions to higher order processes. Here, we present the formation of an extreme sub-wavelength structure formation (∼) on a single crystal silicon surface by a 3600 nm MIR femtosecond laser with a pulse duration of 200 fs. The 50–100 nm linear structures were aligned parallel to the laser polarization direction with a quasi-periodicity of 700 nm. The dependence of the structure on the native oxide, laser pulse number, and polarization were studied. The properties of the structures were studied using scanning electron microscopy (SEM), atomic force microscopy (AFM), cross-sectional transmission electron-microscopy (CS-TEM), electron diffraction (ED), and energy-dispersive X-ray spectroscopy (EDX). As traditional models for the formation of laser induced periodic surface structure do not explain this structure formation, new theoretical efforts are needed.

Multi-dimensional kinetic simulations of laser radiation absorption and electron acceleration in inhomogeneous underdense plasma

The sub-relativistic laser beam interaction with an underdense plasma is investigated via two-dimensional (2D) numerical simulations with respect to the laser polarization direction. Different parametric instabilities dominate the interaction depending on the propagation direction of the daughter waves in the simulation plane with respect to the laser field polarization and laser propagation direction. In the plane containing the laser electric field (p-polarization) the interaction is dominated by the two-plasmon decay instability and the beating of large amplitude electron plasma waves produces periodic ion density perturbations suppressing stimulated Raman scattering in the quarter critical density zone. A stronger absorption and heating of hot electrons is observed in the case where laser polarization is perpendicular to the simulation plane (s-polarization). Furthermore, by comparing a plane laser wave with a narrow beamlet, the effect of the initial transverse laser profile is proven to play an important role in exciting the filamentation instability, which competes with stimulated Brillouin scattering and affects the laser absorption and hot electron generation. A dedicated three-dimensional simulation indicates that a 2D simulation with p-polarization produces a more reliable results while the case of s-polarization overestimates the laser absorption and hot electron generation.

Influence of polarization directions of the IR+XUV two-color laser fields on angle-resolved photoelectron energy spectrum.

By employing the frequency-domain theory, we investigate the influence of polarization directions on angle-resolved photoelectron energy spectrum in the above-threshold ionization (ATI) process of atoms exposed to the IR+XUV two-color laser fields, which shows the multiplateau structures. When the ionized electron is emitted along the IR laser's polarization direction, the width of each plateau keeps a certain energy range, and the jet structures and main lobes are determined by both the emission angle relative to the polarization direction of the XUV laser field and the number of the XUV photons absorbed by the electron. While when the ionized electron is emitted along the XUV laser's polarization direction, the width of each plateau depends on the polarization direction of the IR laser field, and the angular distribution of the ionized electron exhibits the isotropic characteristics. These results show that the ATI spectrum may be effectively controlled by changing the angle between the two laser fields' polarization directions.

Understanding the plasmon-enhanced photothermal effect of a polarized laser on metal nanowires

Improving photothermal efficiency can reduce the melting threshold of metal nanowires. The photothermal efficiency of a polarized laser to Cu nanowires was investigated by numerical simulation and experiment. Our simulation results reveal that the photothermal efficiency of a polarized laser depends on the intensity and distribution area of surface plasmons excited by the laser. As the angle between the polarization direction of the incident laser and the long axis of the Cu nanowire increases, the laser-excited surface plasmons shift from both ends to the sidewall of the Cu nanowire. Such a distribution of surface plasmons was confirmed by the melting behavior of Cu nanowires irradiated by a 450 nm polarized laser. Increasing the laser wavelength will enhance the intensity of the surface plasmons but reduce the distribution area of the surface plasmons. As a result, a higher photothermal efficiency was achieved using a laser with a polarization direction perpendicular to the long axis of the Cu nanowire and a wavelength less than 550 nm. Due to the higher photothermal efficiency, the melting threshold of Cu nanowire irradiated by a laser with polarization perpendicular to the long axis of the Cu nanowire is 32 mW, which is around 20% lower that of Cu nanowire irradiated by a laser with polarization parallel to the long axis of the Cu nanowire.

Unusual Polarization Relation between Single-Mode Lasing Emission and Excitation Laser from an Evanescent-Wave Pumped Micro-Cavity Laser

Using a fiber of that is 125 μm in diameter in rhodamine 6G ethanol solution, controllable multi- and single-whispering-gallery-mode (WGM) optofluidic lasers based on evanescent-wave-coupled gain are both available. With multi-mode WGM emission, lasing emission with almost pure TM (transverse magnetic) or almost TE (transverse electric) modes can be obtained when the pump laser has an electric field parallel (perpendicular) to the fiber axis, i.e., the polarization direction of output laser is the same as that of the pump laser. On the other hand, when the laser emission is single-mode, the TE output laser always emerges firstly above lasing threshold, then keeps TE mode while the pump laser’s intensity increases with polarization direction perpendicular to the fiber axis; on the contrary, TE emission will dwindle relatively, while the TM emission emerges and dominates the spectra, when the pump laser’s intensity increases with polarization parallel to the fiber axis. Our work proves that controlling the leakage of the evanescent wave from high-Q microcavities is crucial for both modes of lasing emission and its polarization.

Creation of azimuthally and radially directed laser-induced periodic structures on large tantalum surface

The formation of well-controlled nano/micrometer-sized structures on metallic surfaces enables the modification of their optical and wetting properties. Forming such structures on the surface of biocompatible materials, in particular, can expand their applications in various areas of science and technology. Here we present results on covering tantalum (Ta), a biocompatible material, with complex nanosized structures comprising azimuthally- and radially-directed laser-induced periodic surface structures (LIPSS) by rotating the metallic sample with respect to the polarization direction of the irradiating laser pulses. For the first time, we use a high-repetition rate (150 kHz) fiber-based laser with 37 fs ablating pulses and a central wavelength of 1030 nm to form ripples that are directed both parallel and perpendicular to the laser polarization direction on the surface of Ta. Rotating the target during ablation led to forming two distinct zones of structures. The first zone, around the circumference of the target, consisted of both high- and low-spatial-frequency LIPSS, while in the second zone, at the center of the target, was covered by nanoparticles redeposition. We demonstrate how the formation of such complex structures significantly alters the optical reflectance and wetting characteristics of Ta.

Terahertz optics-driven phase transition in two-dimensional multiferroics

Displacive martensitic phase transition is potentially promising in semiconductor-based data storage applications with fast switching speed. In addition to traditional phase transition materials, the recently discovered two-dimensional ferroic materials are receiving a lot of attention owing to their fast ferroic switching dynamics, which could tremendously boost data storage density and enhance read/write speed. In this study, we propose that a terahertz laser with an intermediate intensity and selected frequency can trigger ferroic order switching in two-dimensional multiferroics, which is a damage-free noncontacting approach. Through first-principles calculations, we theoretically and computationally investigate optically induced electronic, phononic, and mechanical responses of two experimentally fabricated multiferroic (with both ferroelastic and ferroelectric) materials, β-GeSe and α-SnTe monolayer. We show that the relative stability of different orientation variants can be effectively manipulated via the polarization direction of the terahertz laser, which is selectively and strongly coupled with the transverse optical phonon modes. The transition from one orientation variant to another can be barrierless, indicating ultrafast transition kinetics and the conventional nucleation-growth phase transition process can be avoidable.

Near-field imaging of femtosecond propagating surface plasmon and regulation of excitation efficiency

Near-field imaging and active control of excitation efficiency of femtosecond propagating surface plasmon (fs-PSP) are the prerequisites for its application. Here, we perform near-field imaging of fs-PSP excited at the trench etched on silver nano-film by using photoemission electron microscopy (PEEM). As an excellent near-field microscopy technique of in situ imaging with a high spatial resolution (< 20 nm), it needs neither molecular reporters nor scanning probes as required in nonlinear fluorescence microscopy in nonlinear fluorescence microscopy or scanning near-field optical microscopy, both of which may potentially bias PSP derived from such measurements. The period of the interference patterns induced by the incident femtosecond laser and the laser-induced fs-PSP and the wavelength of fs-PSP in a range of 720–900 nm of the incident laser wavelength are systematically measured. The fringe period of the interference pattern between fs-PSP and the incident laser is a range of 5.9–7.7 µm, and the wavelength of fs-PSP is in a range of 700–879 nm. The experimental results are consistent with the theoretical simulation results. Furthermore, we demonstrate that the excitation efficiency of fs-PSP can be actively controlled by adjusting the polarization direction of the incident laser in the femtosecond pump-probe experiments. Specifically, it is found that when the incident laser is polarized to 0° (p-polarization light), the excitation efficiency of PSP reaches a maximum value, and when the incident light is polarized to 90° (s-polarization light), the excitation efficiency of fs-PSP is the lowest. Unlike the simulation result by the finite difference time domain (FDTD) method, a plateau area of the intensity of the photoemission signal with the polarization direction of the incident laser appears in the femtosecond pump-probe experiment. This phenomenon is attributed to the background noise of the detection laser that masks the change of the fs-PSP excitation efficiency. In a word, this research realizes the experimental measurement of the basic parameters of fs-PSP and the manipulation of fs-PSP excitation efficiency by adjusting the polarization angle of the incident laser. This research lays a foundation for realizing the engineering manipulation of fs-PSP excitation efficiency and optimizing the performance of plasmonic devices.

Polarization Characteristics of the Near-Field Distribution of One-Dimensional Subwavelength Gratings

To improve the anti-laser damage performance of one-dimensional (1D) subwavelength gratings (SWGs), this paper proposes to reasonably reduce the peak electric field at the grating ridges to further reduce the laser damage caused by the electric field contribution. Based on Maxwell’s equations, the equations for solving the field intensity of the near-field distribution of the dielectric materials are derived. The numerical simulation theoretical model is described. A 1064 nm laser in the –y direction irradiates the geometric surfaces under two perpendicular polarization directions: perpendicular to the grating ridges (transverse magnetic wave (TM) or x-polarization) and parallel to the grating ridges (transverse electric wave (TE) or z-polarization). We discuss the effects of the profile shape, structural parameters and refractive index of the material on the near-field distribution at the 1D SWG ridges by using a finite element method (FEM). The near-field distribution is sensitive to the x- and z-polarization of incident light. The near-field distribution of the 1D SWGs for TM waves is modulated by the surface, whereas that for TE waves is similar to the distribution of the bare substrate. The results show that the near-field distribution of 1D SWGs greatly depends on the laser polarization direction.

Interference effect in high order harmonic generation by aligned O<sub>2</sub>

High order harmonic generation (HHG) is an important phenomenon when atoms or molecules interact with an intense laser field. It can be used to generate ultrashort laser source, and can also be used to investigate the atomic and molecular dynamics and obtain the electric structure information of molecules. All these require to understand in depth the mechanism of HHG. There are complicated interference effects in HHG spectra of molecules due to multiple re-collision atomic centers in the molecule. In this paper, spectra of aligned O<sub>2</sub> molecule in linearly polarized laser field is investigated by using the Lewenstein' s model. The dependence of the spectrum on the angle θ between the nuclear axis of the molecule and the laser polarization direction is obtained. It is shown that the maximum yield of HHG occurs at <i>θ</i> of 45°, which is in consistence with the experimental result. In addition, it is found that there exists a minimum value in the HHG spectrum for any given value of<i> θ</i>. The harmonic order corresponding to the minimum increases with <i>θ</i> increasing. It is found that the minimum comes from the coherent superposition of contributions from two channels. One channel refers to that the ionized electron from one atomic center, subjected to the electric field of the laser, moves back to its parent atomic center and there it combines with the molecule and emits harmonics; while the other channel is that the ionized electron generated from one atomic center move back to the other atomic center to complete the combination and emission of harmonics. The angle <i>θ-</i>dependent phase difference between contributions from these two channels is calculated and the harmonic order corresponding to the minimum value is obtained. Finally, the reason why the yield of HHG is low for the case of the molecular axis parallel to the laser polarization direction is different from that for the case of the molecular axis perpendicular to the polarization direction. For the parallel case, the contributions to HHG from the two channels are both small so that the amplitude of their coherent superposition is small. While for the perpendicular case, the individual contribution from each channel is not small but their destructive interference leads to small yield in harmonicspectrum.

Femtosecond Laser-Induced Periodic Surface Structures on Different Tilted Metal Surfaces.

Laser-induced periodic surface structures (LIPSS) are used for the precision surface treatment of 3D components. However, with LIPSS, the non-normal incident angle between the irradiated laser beam and the specimen surface occurs. This study investigated LIPSS on four different metals (SUS 304, Ti, Al, and Cu), processed on a tilted surface by an s-polarized femtosecond fiber laser. A rotated low spatial frequency LIPSS (LSFL) was obtained on SUS 304 and Ti materials by the line scanning process. However, LSFL on Cu and Al materials was still perpendicular to the laser polarization. The reason for the rotated and un-rotated LSFL on tilted metal surfaces was presented. The electron-phonon coupling factor and thermal conductivity properties might induce rotational LSFL on tilted SUS 304 and Ti surfaces. When fabricating LSFL on an inclined plane, a calibration model between the LSFL orientation and inclined plane angle must be established. Hence, the laser polarization direction must be controlled to obtain suitable LSFL characteristics on a 3D surface.

20 kHz dual-plane stereo-PIV measurements on a swirling flame using a two-legged burst-mode laser.

Dual-plane stereoscopic particle image velocimetry (PIV) is capable of quantifying the flow field in terms of three-component (3C) flow vectors and 3C vorticity vectors simultaneously. Here, we present a test rig to carry out the 20 kHz dual-plane stereo PIV measurements on a premixed swirling flame by using a two-legged burst-mode laser. Other than the traditional methods employing the laser polarization direction and the two-color separation methods, two same-color laser sheets with a 100 ns delay were adopted to separate the imaging processes for the two pairs of cameras using the image straddling method. Each laser sheet with the same wavelength of 532 nm has a pulse cyclic frequency of 20 kHz within each burst generated by the high-repetition-rate burst-mode laser. 3C velocity vectors of a swirling flame were obtained based on the sequential particle images for each laser sheet. In spite of non-perfect simultaneous flow measurements on the two spatially separated laser sheets, the velocity error caused by the 100 ns delay on top of a 50 μs duration, which was used for the velocity vector calculation, is negligible. This short-delay separation method significantly simplifies the experimental setup for dual-plane stereo PIV measurements, especially for low-speed flows.

Angular Trapping of Spherical Janus Particles

AbstractDeveloping angular trapping methods, which enable optical tweezers to rotate a micronsized bead, is of great importance for studies of biomacromolecules in a wide range of torque‐generation processes. Here a novel controlled angular trapping method based on model composite Janus particles is reported, which consist of two hemispheres made of polystyrene and poly(methyl methacrylate). Through computational and experimental studies, the feasibility to control the rotation of a Janus particle in a linearly polarized laser trap is demonstrated. The results show that the Janus particle aligned its two hemispheres interface parallel to the laser propagation direction and polarization direction. The rotational state of the particle can be directly visualized by using a camera. The rotation of the Janus particle in the laser trap can be fully controlled in real time by controlling the laser polarization direction. The newly developed angular trapping technique has the great advantage of easy implementation and real‐time controllability. Considering the easy chemical preparation of Janus particles and implementation of the angular trapping, this novel method has the potential of becoming a general angular trapping method. It is anticipated that this new method will significantly broaden the availability of angular trapping in the biophysics community.

Photoinduced tunable birefringence and dichroism in silver nanogratings

Silver nanogratings are anisotropic plasmonic nanostructures with potential application in optical components due to their large birefringence and dichroism. We induced linear birefringence and linear dichroism in subwavelength Ag-AgCl films by irradiating with a single low-power linearly polarized laser beam. The laser beam aligns silver nanoparticles in the direction of laser polarization and forms nanograting. We used Stokes parameters to determine linear birefringence and linear dichroism in silver aligned nanostructures. The values of linear dichroism and linear birefringence in silver nanogratings are controllable through manipulating the spatial period of nanogratings. The dispersion characteristic of dichroism and birefringence is also investigated.

Distribution of laser shot-noise energy delivered to a levitated nanoparticle

This paper quantifies the rate at which laser shot noise energy is delivered to a nanoparticle for the various scenarios commonly encountered in levitated optomechanics. While previous articles have the same form and dependencies, the proportionality constants often differ in the literature. This paper resolves these discrepancies. The rate at which energy is delivered to an optically trapped particle's respective degrees of freedom depends on the radiation pattern of scattered light as well as the direction of laser propagation. For a traveling plane wave with linearly polarized light, in the Rayleigh regime this leads the translational shot noise heating rate to be proportional to $1/10$ of the total rate in the laser polarization direction, $7/10$ in the laser propagation direction, and $2/10$ in the direction perpendicular to both. Analytical expressions for the shot noise heating rate are provided in the Rayleigh limit as well as numerical calculations for particles in the Mie regime for silica and diamond. For completeness, numerical calculations of the shot noise heating for silica Mie particles at the focus of a strongly focused laser beam are calculated for varying numerical aperture and common laser wavelengths. Both numerical calculations show that the Rayleigh expression generally gives an overestimate of the shot noise heating especially for larger radii, but is still a good approximation even for incident focal fields. The exception to the relative decrease is when a Mie resonance is reached which was found for diamond. Lastly, Rayleigh expressions for the rotational shot noise heating for a symmetric top-like particle for linear, elliptically, and unpolarized light are also provided.

Theoretical Exploration of Terahertz Single-Photon Detection and Imaging by Nonlinear Optical Frequency Up-Conversion

Terahertz single-photon detection and imaging have attracted full attention recently. Nonlinear optical frequency up-conversion is a promising technique that can be expected to satisfy this demand thanks to its high sensitivity and fast response. In this paper, theoretical analysis and numerical calculations based on the organic salt 4′-dimethylamino-N-methyl-4-stilbazolium tosylate (DAST) crystal were performed to show that the optimization of the detection of terahertz is different from that of the generation of terahertz, including the use of difference-frequency generation (DFG) technique, the larger thickness of the crystal, and especially the selection of the polarization direction of the pumping laser. For two different polarization configurations, the photons of the up-converted signal light both can be amplified compared with the number of incident terahertz photons under some optimal designs of the nonlinear frequency conversion process. Therefore, terahertz single-photon detection can be realized with single-photon detectors (SPDs) or even possibly with ordinary avalanche photodiodes (APDs). Furthermore, for terahertz single-photon imaging, the frequency up-conversion with the pumping laser polarized along b-axis of DAST crystal has a better performance, which is rarely used in terahertz generation.

Asymmetric enhancement of N2+ lasing in intense, birefringence-modulating elliptical laser fields.

We experimentally demonstrate an asymmetric enhancement of the N2+ lasing at 391 nm for the transition between the B2Σu+ (v = 0) and X2Σg+ (v" = 0) states in an intense laser field with the ellipticity, ε, modulated by a 7-order quarter-wave plate (7-QWP). It is found that when the 7-QWP is rotated from α = 0 to 90°, where α is the angle between the polarization direction of the input laser and the slow axis of the 7-QWP, the intensity of the 391-nm lasing is optimized at ε ∼ 0.3 with α∼ 10°-20° and 70°-80° respectively, but the optimization intensity at α∼ 10°-20° is about 4 times smaller than that at α∼ 70°-80°. We interpret the asymmetric enhancement based on a post-ionization coupling model, in which the birefringence of the 7-QWP induces an opposite change in the relative amplitudes of the ordinary (Eo) and extraordinary (Ee) electric components under the two conditions, so that the same temporal separation of Eo and Ee leads to a remarkably different coupling strength for the population transfer from the X2Σg+ (v "=0) to A2Πu (v '=2) states.