Laser-driven Ion Beams Research Articles

Optimization of laser-driven quantum beam generation and the applications with artificial intelligence

We have investigated space and astrophysical phenomena in nonrelativistic laboratory plasmas with long high-power lasers, such as collisionless shocks and magnetic reconnections, and have been exploring relativistic regimes with intense short pulse lasers, such as energetic ion acceleration using large-area suspended graphene. Increasing the intensity and repetition rate of the intense lasers, we have to handle large amounts of data from the experiments as well as the control parameters of laser beamlines. Artificial intelligence (AI) such as machine learning and neural networks may play essential roles in optimizing the laser and target conditions for efficient laser ion acceleration. Implementing AI into the laser system in mind, as the first step, we are introducing machine learning in ion etch pit analyses detected on plastic nuclear track detectors. Convolutional neural networks allow us to analyze big ion etch pit data with high precision and recall. We introduce one of the applications of laser-driven ion beams using AI to reconstruct vector electric and magnetic fields in laser-produced turbulent plasmas in three dimensions.

Scientific programme at the Laser Laboratory for Acceleration and Applications

In recent years, laser-driven accelerators have emerged as a promising technology for the development of compact and cost-effective sources of high-energy particles and radiation. Here, we introduce our research programme at the Laser Laboratory for Acceleration and Applications, which focusses on high-power laser systems, development of high-repetition rate targetry, and biomedical applications of laser-based accelerators. Our recent results include the generation of high-energy proton and ion beams through laser-plasma acceleration, which have potential applications in materials activation for medical imaging. We have also investigated the feasibility of using laser-driven X-rays and ion beams for radiobiological research, including FLASH therapy and hadron therapy.

Energy-chirp compensation of laser-driven ion beams enabled by structured targets

We show using 3D simulations that the challenge of generating dense mono-energetic laser-driven ion beams with low angular divergence can be overcome by utilizing structured targets with a relativistically transparent channel and an overdense wall. In contrast to a uniform target that produces a chirped ion beam, the target structure facilitates formation of a dense electron bunch whose longitudinal electric field reverses the energy chirp. This approach works in conjunction with existing acceleration mechanisms, augmenting the ion spectra. For example, our 3D simulations predict a significant improvement for a 2 PW laser pulse with a peak intensity of $5 \times 10^{22}$ W/cm$^2$. The simulations show a mono-energetic proton peak in a highly desirable energy range of 200 MeV with an unprecedented charge of several nC and relatively low divergence that is below 10$^{\circ}$.

Analyzing the filamentation of MeV-range proton bunches in a laser-driven ion beamline and optimizing their peak intensity

In this article, we report on the latest investigations and achievements in proton beam shaping with our laser-driven ion beamline at GSI Helmholtzzentrum f\"ur Schwerionenforschung GmbH. This beamline was realized within the framework of the Laser Ion Generation, Handling, and Transport (LIGHT) collaboration to study the combination of laser-driven ion beams with conventional accelerator components. At its current state, the ions are accelerated by the high-power laser PHELIX via target normal sheath acceleration, and two pulsed high-magnetic solenoids are used for energy selection, transport, and transverse focusing. In between the two solenoids, there is a rf cavity that gives the LIGHT beamline the capability to longitudinally manipulate and temporally compress ion bunches to sub-nanosecond durations. To get optimal results, the rf cavity has to be synchronized with the PHELIX laser and therefore a reliable measurement of the temporal ion beam profile is necessary. In the past, these measurements showed unexpected correlations between the temporal beam profile and the phase as well as the electric field strength of the cavity. In this article, we present a numerical simulation of the beam transport through the LIGHT beamline which explains this behavior by a beam filamentation. We also report on our latest experimental campaigns, in which we combined transverse and longitudinal focusing for the first time. This led to proton bunches with a peak intensity of $(3.28\ifmmode\pm\else\textpm\fi{}0.24)\ifmmode\times\else\texttimes\fi{}{10}^{8}\text{ }\text{ }\mathrm{protons}/({\mathrm{ns}\text{ }\mathrm{mm}}^{2})$ at a central energy of ($7.72\ifmmode\pm\else\textpm\fi{}0.14$) MeV. The intensity refers to a circle with a diameter of ($1.38\ifmmode\pm\else\textpm\fi{}0.02$) mm that encloses 50% of the protons in the focal spot at the end of the beamline. The temporal bunch width at this position was ($742\ifmmode\pm\else\textpm\fi{}40$) ps (FWHM).

Characteristics of laminar ion beams accelerated via a few-joule laser pulse

Laser-driven carbon ion beams from a carbon foil target via a 2.5-J laser pulse are investigated with three-dimensional particle-in-cell simulations. An ion bunch with a narrow energy range exhibits a thin shell shape with a certain diameter. The ion cloud has a layered structure of these ion bunches with different energies. The divergences of the ion bunch in the laser inclination direction and perpendicular to it are different in an oblique incidence laser. In addition, theoretical formulas for the radius of the generated ion beam and the energy spectrum are derived, and they are shown to be in good agreement with the simulation results.

Polarimetry for 3He Ion Beams from Laser–Plasma Interactions

We present a compact polarimeter for 3He ions with special emphasis on the analysis of short-pulsed beams accelerated during laser–plasma interactions. We discuss the specific boundary conditions for the polarimeter, such as the properties of laser-driven ion beams, the selection of the polarization-sensitive reaction in the polarimeter, the representation of the analyzing-power contour map, the choice of the detector material used for particle identification, as well as the production procedure of the required deuterated foil-targets. The assembled polarimeter has been tested using a tandem accelerator delivering unpolarized 3He ion beams, demonstrating good performance in the few-MeV range. The statistical accuracy and the deduced figure-of-merit of the polarimetry are discussed, including the count-rate requirement and the lower limit of accuracy for beam-polarization measurements at a laser-based ion source.

Online charge measurement for petawatt laser-driven ion acceleration.

Laser-driven ion beams have gained considerable attention for their potential use in multidisciplinary research and technology. Preclinical studies into their radiobiological effectiveness have established the prospect of using laser-driven ion beams for radiotherapy. In particular, research into the beneficial effects of ultrahigh instantaneous dose rates is enabled by the high ion bunch charge and uniquely short bunch lengths present for laser-driven ion beams. Such studies require reliable, online dosimetry methods to monitor the bunch charge for every laser shot to ensure that the prescribed dose is accurately applied to the biological sample. In this paper, we present the first successful use of an Integrating Current Transformer (ICT) for laser-driven ion accelerators. This is a noninvasive diagnostic to measure the charge of the accelerated ion bunch. It enables online estimates of the applied dose in radiobiological experiments and facilitates ion beam tuning, in particular, optimization of the laser ion source, and alignment of the proton transport beamline. We present the ICT implementation and the correlation with other diagnostics, such as radiochromic films, a Thomson parabola spectrometer, and a scintillator.

Temperature evolution of dense gold and diamond heated by energetic laser-driven aluminum ions

Recent studies have shown that energetic laser-driven ions with some energy spread can heat small solid-density samples uniformly. The balance among the energy losses of the ions with different kinetic energies results in uniform heating. Although heating with an energetic laser-driven ion beam is completed within a nanosecond and is often considered sufficiently fast, it is not instantaneous. Here we present a theoretical study of the temporal evolution of the temperature of solid-density gold and diamond samples heated by a quasimonoenergetic aluminum ion beam. We calculate the temporal evolution of the predicted temperatures of the samples using the available stopping power data and the SESAME equation-of-state tables. We find that the temperature distribution is initially very uniform, which becomes less uniform during the heating process. Then, the temperature uniformity gradually improves, and a good temperature uniformity is obtained toward the end of the heating process.

Laser-driven neutron source and nuclear resonance absorption imaging at ILE, Osaka University: review.

Here, we present an overview on the recent progress in the development of the laser-driven neutron source (LDNS) and nuclear resonance absorption (NRA) imaging at the Institute of Laser Engineering (ILE), Osaka University. The LDNS is unique because the number of neutrons per micro pulse is very large, and the source size and the pulse width are small. Consequently, extensive research and development of LDNSs is going on around the world. In this paper, a typical neutron generation process by the laser-driven ion beam, called the pitcher-catcher scheme, is described. The characteristics of the LDNS are compared with those of the accelerator-driven neutron source (ADNS), and unique application of the LDNS, such as NRA imaging, is presented. In the LDNS, NRA imaging is possible with a relatively short beam line in comparison with that of the ADNS since the neutron pulse width and the source size of the LDNS are small. Future prospects in research and development of NRA imaging with the LDNS at ILE Osaka University are also described.

Assessment of the reliability of deconvolution procedures for RCF spectroscopy of laser-driven ion beams

Laser-driven ion beams are defined by a number of unique features, including a large spread in energy. A stack configuration of radiochromic films (RCF) can be utilized to characterize such beams through measurements of their energy spectra. A spectroscopic procedure is reported that allows the proton energy density within each active layer of a radiochromic film (RCF) stack to be retrieved. This is based upon on a deconvolution algorithm developed through Geant4 Monte Carlo simulations to correct the contributions of energy depositions within a given film layer. Through Monte Carlo calculations, the spectrum retrieved from a simulated film stack can be retrieved and compared with a known energy spectrum, providing an examination of the efficacy of this tool. Application of the developed deconvolution procedure thus offers the potential to correctly reconstruct the incident energy spectrum of a laser-driven proton and ion beam from a stack of irradiated RCF.

Manipulating the Laser-Driven Proton Bunch with Plasma Wakefield

With the advantages of short duration and extreme brightness, laser proton accelerators (LPAs) show great potential in many fields for industrial, medical, and research applications. However, the quality of current laser-driven proton beams, such as the broad energy spread and large divergence angle, is still a challenge. We use numerical simulations to study the propagation of such proton bunches in the plasma. Results show the bunch will excite the wakefield and modulate itself. Although a small number of particles at the head of the bunch cannot be manipulated by the wakefield, the total energy spread is reduced. Moreover, while reducing the longitudinal energy spread, the wakefield will also pinch the beam in the transverse direction. The space charge effect of the bunch is completely offset by the wakefield, and the transverse momentum of the bunch decreases as the bunch transports in the plasma. For laser-driven ion beams, our study provides a novel idea about the optimization of these beams.

Handling and dosimetry of laser-driven ion beams for applications

Handling and dosimetry of laser-driven ion beams for applications

Dosimetric Optimization of a Laser-Driven Irradiation Facility Using the G4-ELIMED Application

ELIMED has been developed and installed at ELI beamlines as a part of the ELIMAIA beamline to transport, monitor, and use laser-driven ion beams suitable for multidisciplinary applications, including biomedical ones. This paper aims to investigate the feasibility to perform radiobiological experiments using laser-accelerated proton beams with intermediate energies (up to 30 MeV). To reach this goal, we simulate a proton source based on experimental data like the ones expected to be available in the first phase of ELIMED commissioning by using the G4-ELIMED application (an application based on the Geant4 toolkit that simulates the full ELIMED beamline). This allows the study of transmission efficiency and the final characteristics of the proton beam at the sample irradiation point. The Energy Selector System is used as an active energy modulator to obtain the desired beam features in a relatively short irradiation time (around 6 min). Furthermore, we demonstrate the capability of the beamline to filter out other ion contaminants, typically co-accelerated in a laser-plasma environment. These results can be considered as a detailed feasibility study for the use of ELIMED for various user applications such as radiobiological experiments with ultrahigh dose rate proton beams.

Generation and stopping of laser-driven two-component ion beam

The generation and stopping of a laser-driven two-component ion beam are investigated by three-dimensional particle-in-cell simulation and an extended stopping model. It is found that a two-component ion beam with the tunable composition ratio can be obtained from the two-species-ions sandwich target interacting with a relativistic laser pulse. When the generated proton beam mixed with a certain portion of carbon ions is transporting in fully ionized dense plasma, the beam stopping power is significantly enhanced compared to a pure proton beam. The maximum penetration depth is sharply reduced, and the Bragg peak with a higher magnitude appears earlier at the end of their paths, which is beneficial for achieving more localized energy deposition. The effect of heavy ion mixing on proton beam driven fast ignition is also discussed. A simple theoretical model is established, indicating that the required ignition time is relatively delayed for a heavy-ion doping case. For a small hot-spot size, it is possible to achieve the fusion ignition for a low mixed ratio. However, it is difficult to maintain a high fuel temperature due to the growing energy loss originating from mechanical work and thermal conduction.

Improving laser-accelerated proton beam divergence by electric and magnetic fields induced in flat channel-like targets

Improving parameters of laser-driven proton and ion beams becomes one of the most important goals in the field of laser acceleration in order to fulfill requirements of foreseen applications. This work presents parametric 2D and 3D particle-in-cell simulations of various target designs in order to reduce proton beam divergence without significant drop in maximum energies or in proton number. The optimal target design proved to be a channel-like target which produces not only a long-lasting focusing transverse electric field in contrast to a flat foil, but also a magnetic quadrupole with strong octupole component inside the guiding channel. A combination of both electric and magnetic features results in a strong proton beam divergence reduction, accompanied by a higher uniformity of the beam, which is studied as a function of proton energy.

Laser-driven acceleration of ion beams for high-gain inertial confinement fusion

Inertial confinement fusion (ICF) is currently one of the two main paths towards an energy source based on thermonuclear fusion. A promising ICF option is ion fast ignition (IFI), in which the ignition of nuclear fuel is initiated by an intense laser-driven ion beam. This paper presents the results of systematic numerical (particle-in-cell) studies of the properties of laser-driven carbon ion beams produced under conditions relevant for IFI, and the feasibility of achieving beam parameters required for fuel ignition is discussed. It was found that a 1 ps 200 kJ infrared laser driver is capable of producing ion beams with parameters required for IFI, even with a simple non-optimised target, but only at small distances (⩽0.1 mm) from the target. At such distances, the beam intensity and fluence exceeds 5 × 1021 W cm−2 and 2 GJ cm−2, respectively, while the beam energy approaches 30 kJ. The ion beam parameters can be significantly improved by carefully selecting the target thickness and shape. However, even with an optimised target, achieving the beam parameters required for IFI is possible only at distances from the target below 0.5 mm. The ion acceleration is accompanied by the emission of powerful (⩾50 PW) pulses of short-wavelength synchrotron radiation which are the source of significant ion energy losses and may pose a threat to the fusion infrastructure. In addition to ICF, the extremely intense ion beams demonstrated in the paper can be a unique research tool for research in nuclear physics, high energy-density physics or materials science.

Ion species discrimination method by linear energy transfer measurement in Fujifilm BAS-SR imaging plate.

We have developed a novel discrimination methodology to identify ions in multispecies beams with similar charge-to-mass ratios, but different atomic numbers. After an initial separation by charge-to-mass ratios using co-linear electric and magnetic fields, individual ions can be discriminated by considering the linear energy transfer of ions irradiating a stimulable phosphor plate (Fujifilm imaging plate) by comparison with the Monte Carlo calculation. We apply the method to energetic multispecies laser-driven ion beams and use it to identify silver ions produced by the interaction between a high contrast, high intensity laser pulse; and a sub-micrometer silver foil target. We also show that this method can be used to calibrate the imaging plate for arbitrary ion species in the range of Z ≥ 6 with dE/dx > 0.1 MeV/μm without requiring individual calibration.

Proton acceleration through a charged cavity created by ultraintense laser pulse

The potential of laser-driven ion beam applications is limited by high quality requirements. The excellent “point-source” characteristics of the laser accelerated proton beam in a broad energy range were found by using proton radiographs of a mesh. The “virtual source” of protons, the point where the proton trajectories are converging and form a waist, gradually decreases and moves asymptotically to the target with increasing particles' energy. Computer simulations confirmed that the beam profile at the center is fully conserved, the virtual source of higher energy protons gradually moves closer to the target, and if the particle energy is further increased, the virtual source will be located on the target front surface (for portions above 13 MeV, in this case) with a size comparable to the laser spot size. The laser ponderomotive force pushes the electrons deep into the target creating a bipolar charge structure, i.e., an electron cavity and spike which produces strong accelerating field, realizing a point-size source of accelerated protons. This behavior has not previously been predicted. These results contribute to the development of next generation laser-accelerators suitable for many applications.

A new energy spectrum reconstruction method for time-of-flight diagnostics of high-energy laser-driven protons.

The Time-of-Flight (TOF) technique coupled with semiconductorlike detectors, as silicon carbide and diamond, is one of the most promising diagnostic methods for high-energy, high repetition rate, laser-accelerated ions allowing a full on-line beam spectral characterization. A new analysis method for reconstructing the energy spectrum of high-energy laser-driven ion beams from TOF signals is hereby presented and discussed. The proposed method takes into account the detector's working principle, through the accurate calculation of the energy loss in the detector active layer, using Monte Carlo simulations. The analysis method was validated against well-established diagnostics, such as the Thomson parabola spectrometer, during an experimental campaign carried out at the Rutherford Appleton Laboratory (UK) with the high-energy laser-driven protons accelerated by the VULCAN Petawatt laser.

Superintense Laser-driven Ion Beam Analysis

Ion beam analysis techniques are among the most powerful tools for advanced materials characterization. Despite their growing relevance in a widening number of fields, most ion beam analysis facilities still rely on the oldest accelerator technologies, with severe limitations in terms of portability and flexibility. In this work we thoroughly address the potential of superintense laser-driven proton sources for this application. We develop a complete analytical and numerical framework suitable to describe laser-driven ion beam analysis, exemplifying the approach for Proton Induced X-ray/Gamma-ray emission, a technique of widespread interest. This allows us to propose a realistic design for a compact, versatile ion beam analysis facility based on this novel concept. These results can pave the way for ground-breaking developments in the field of hadron-based advanced materials characterization.