Laser Acceleration Of Electrons Research Articles

Correlation of Laser-Accelerated Electron Energy with Electromagnetic Pulse Emission from Thin Metallic Targets

High-power pulsed lasers are used more and more as tools for particle acceleration. Characterization of the accelerated particles in real-time and monitoring of the electromagnetic pulses (EMPs) during particle acceleration are critical challenges in laser acceleration experiments. Here, we used the CETAL-PW laser facility at NILPRP for particle acceleration from different thin metallic targets, at laser intensities of the order of 3×1021 W/cm2. We investigated the dependence of EMP amplitude (EMPA) and the accelerated electrons’ maximal energy (AEME), on thickness, resistivity, and atomic number of the target. We have found a quasi-linear dependence between EMPA and AEME and propose an analytical model for the GHz EMP emission. The model considers the neutralization current flowing through the target stalk as the main source of the EMP in the GHz domain, the current being produced by the positive charge accumulated on the target after the electron’s acceleration from the rear side of a metallic target. The data presented here support the possibility of using EMP signals to characterize the laser-accelerated particles in a real-time non-invasive way.

Optimizing proton acceleration using hollow laser pulses and a double-layer target: effects of focal spot position and polarization

Abstract We study the influence of hollow laser pulse settings, specifically adjustments to the focal plane and the phase structure and polarization, on the acceleration of high-energy, low-divergence proton beams from a double-layer target using a feasible laser energy (~ 3.7 J). We investigate the laser's relativistic self-focusing dynamics in the near-critical plasma layer of the target and examine hot electron generation and proton acceleration using three-dimensional particle-in-cell (PIC) simulations. First, we vary the focal spot position of a tightly focused twisted driver, leading to distinct laser beam width evolution that impacts hot electron generation in the near-critical plasma, particularly in the transverse direction. The resulting proton beams differ in maximum longitudinal momentum (0.29-0.35 mi c) and transverse profile. The most efficient acceleration, with a cutoff energy of 40 MeV and ultra-low divergence (~25 mrad), occurs when the driver is focused at the center of the target.
Next, we modify the phase structure and polarization of the laser pulse, transitioning from a linearly polarized twisted beam to cylindrical vector beams with radial and azimuthal polarization, all exhibiting hollow, cylindrically symmetric intensity profiles. This change primarily affects the proton beam's maximum energies, influenced by the ultra-relativistic direct laser-accelerated (DLA) electrons, efficiently generated only by the radially polarized and twisted laser pulses. However, the bulk properties of the proton beam remain similar, as the relativistic mid-energy electrons (< 25 MeV), which sustain a strong sheath field, are the main contributors to proton acceleration in this setup.

COMPARATIVE ANALYSIS OF SIMULATION RESULTS OF DIELECTRIC LASER ACCELERATION OF NON-RELATIVISTIC ELECTRONS IN TRANSPARENT AND REFLECTIVE PERIODIC STRUCTURES

To support of our experimental studies on dielectric laser acceleration, numerical studies of laser acceleration of nonrelativistic electrons with the initial energy of 33.9 keV in transparent and reflective periodic structures are carried out. On the basis of computer simulations, the acceleration rates of electrons and the quality of their beams after acceleration in compact structures of different configurations were determined and compared. Prospective acceleration schemes are proposed, in particular with reflective periodic structures, which can provide higher rates of electron acceleration in periodic structures than in previously obtained studies.

Radiation-Driven Reactivity of Metal Ions in Molten Salts

Molten salts are proposed as liquid fuels or coolants in a new fleet of molten salt nuclear reactors that would have operational and safety advantages over present reactor systems. Under those conditions, the salt will be exposed to high radiation levels, and understanding the chemical effects of radiolysis on the molten salt fuel or coolant is essential to reliable, efficient and sustainable reactor operation. Building this understanding begins with identifying primary salt radiolysis products (solvated electrons (esolv –) and Cl2 •–) and characterizing their reactivities, for which we conduct high-temperature pulse radiolysis transient absorption spectroscopy at the BNL Laser-Electron Accelerator Facility. Here we report on the reaction kinetics of reactions of metal ions with esolv – and Cl2 •– in different molten salt compositions. Salt mixtures containing mono- and divalent cations are particularly interesting because of their tunable Lewis acidity-basicity that can be used to control the solubility and redox poise of dissolved metal ions in the reactor. Previously we showed how varying the MgCl2:KCl mixing ratio alters the absorption spectra of radiolytically-produced excess electrons, with increasing blue shifts related to the likely number of Mg2+ ions adjacent to the cavity electron. The strong blue shifts indicate significant changes in the electron’s energetics and reactivity that we now have probed by measuring reaction kinetics with metal ion electron acceptors. We observed that reaction rates of the solvated electron depend strongly on the composition of the salt. Reactivity trends among first-row transition metals in eutectic LiCl-KCl will be discussed. This work was supported as part of the Molten Salts in Extreme Environments Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science.

Electron Dynamics in a Relativistic Central Field Approach Associated with Laser Acceleration of Electrons

We perform 2D PIC simulations and observe different scenarios of electron trajectories trapped inside the bubble formed during the laser wakefield acceleration process (LWFA). The trajectories can close on the inside or on the outside of the bubble. The evolution of maximum energy of the injected electrons in both cases is evaluated. We propose an analytic approach based on a relativistic central field model for describing the attraction of electrons near the bubble edge and compare it with the simulations.

Mid-infrared dielectric laser acceleration in a silicon dual pillar structure.

Dielectric laser accelerators use near-infrared laser pulses to accelerate electrons at dielectric structures. Driving these devices with mid-infrared light should result in relaxed requirements on the electron beam, easier fabrication, higher damage threshold, and thus higher acceleration gradients. In this paper, we demonstrate dielectric laser acceleration of electrons driven with 10 μm light in a silicon dual pillar structure. We observe the acceleration of 27 keV electrons by 1.4 keV, corresponding to a 93 MeV/m acceleration gradient. The damage threshold of the structures of 3.3 ± 0.6 GV/m peak field is significantly higher than for near-infrared accelerators. The dual pillar acceleration structure itself even survived 5.2 ± 0.9 GV/m, the highest field strength we could achieve with the current system. This together with the larger structure acceptance bodes well for future dielectric laser accelerators driven with mid-infrared light.

High-brightness betatron emission from the interaction of a sub picosecond laser pulse with pre-ionized low-density polymer foam for ICF research

Direct laser acceleration (DLA) of electrons in plasmas of near-critical density (NCD) is a very advancing platform for high-energy PW-class lasers of moderate relativistic intensity supporting Inertial Confinement Fusion research. Experiments conducted at the PHELIX sub-PW Nd:glass laser demonstrated application-promising characteristics of DLA-based radiation and particle sources, such as ultra-high number, high directionality and high conversion efficiency. In this context, the bright synchrotron-like (betatron) radiation of DLA electrons, which arises from the interaction of a sub-ps PHELIX laser pulse with an intensity of 1019 W/cm2 with pre-ionized low-density polymer foam, was studied. The experimental results show that the betatron radiation produced by DLA electrons in NCD plasma is well directed with a half-angle of 100–200 mrad, yielding (3.4 ± 0.4)·1010 photons/keV/sr at 10 keV photon energy. The experimental photon fluence and the brilliance agree well with the particle-in-cell simulations. These results pave the way for innovative applications of the DLA regime using low-density pre-ionized foams in high energy density research.

All-optical source size and emittance measurements of laser-accelerated electron beams

Novel schemes for generating ultralow emittance electron beams have been developed in past years and promise compact particle sources with excellent beam quality suitable for future high-energy physics experiments and free-electron lasers. Recent theoretical work has proposed a laser-based method capable of resolving emittances in the sub 0.1 mm mrad regime by modulating the electron phase space ponderomotively. Here we present the first experimental demonstration of this scheme using a laser wakefield accelerator. The observed emittance and source size are consistent with published values. We also show calculations demonstrating that tight bounds on the upper limit for emittance and source size can be derived from the “laser-grating” method even in the presence of low signal to noise and uncertainty in laser-grating parameters. Published by the American Physical Society 2024

The influence of laser focusing conditions on the direct laser acceleration of electrons

Direct laser acceleration of electrons during a high-energy, picosecond laser interaction with an underdense plasma has been demonstrated to be substantially enhanced by controlling the laser focusing geometry. Experiments using the OMEGA EP facility measured electrons accelerated to maximum energies exceeding 120 times the ponderomotive energy under certain laser focusing, pulse energy, and plasma density conditions. Two-dimensional particle-in-cell simulations show that the laser focusing conditions alter the laser field evolution, channel fields generation, and electron oscillation, all of which contribute to the final electron energies. The optimal laser focusing condition occurs when the transverse oscillation amplitude of the accelerated electron in the channel fields matches the laser beam width, resulting in efficient energy gain. Through this observation, a simple model was developed to calculate the optimal laser focal spot size in more general conditions and is validated by experimental data.

Electron acceleration and x-ray generation from near-critical-density carbon nanotube foams driven by moderately relativistic lasers

Direct laser acceleration of electrons in near-critical-density (NCD) carbon nanotube foams (CNFs) has its advantages in the high-efficiency generation of relativistic electrons and broadband x-rays. Here, we report the first simultaneous measurement on the spectra of laser-driven electrons and x-rays from CNFs at moderately relativistic intensities of around 5×1019 W/cm2. The density and thickness of the CNFs were scanned in the experiments, indicating the optimized electron temperature of 5.5 MeV and x-ray critical energy of 5 keV. Two-dimensional particle-in-cell simulations confirm that the electrons, with a temperature significantly higher than the pondermotive scale, are directly accelerated by the laser along the NCD plasma channel, while the bright x-rays are emitted by these electrons through betatron radiation or Thomson backscattering inside the channel. The simultaneously generated electrons and x-rays, automatically synchronized with the femtosecond laser driver, are suitable for applications such as bi-modal radiography.

Direct Laser Acceleration in Underdense Plasmas with Multi-PW Lasers: A Path to High-Charge, GeV-Class Electron Bunches.

The direct laser acceleration (DLA) of electrons in underdense plasmas can provide hundreds of nC of electrons accelerated to near-GeV energies using currently available lasers. Here we demonstrate the key role of electron transverse displacement in the acceleration and use it to analytically predict the expected maximum electron energies. The energy scaling is shown to be in agreement with full-scale quasi-3D particle-in-cell simulations of a laser pulse propagating through a preformed guiding channel and can be directly used for optimizing DLA in near-future laser facilities. The strategy towards optimizing DLA through matched laser focusing is presented for a wide range of plasma densities paired with current and near-future laser technology. Electron energies in excess of 10GeV are accessible for lasers at I∼10^{21} W/cm^{2}.

Capillary discharge in the high repetition rate regime

Plasma discharge in the capillary is used to develop x-ray lasers, waveguides for high power laser pulses, and as active plasma lenses to focus high energy charged particle beams. Capillary discharges in the high repetition rate regime are of interest for applications that require large average values, such as luminosity and/or electric current of laser accelerated particles. In the present paper, we study the capillary discharge in the high repetition rate regime in connection with the ultrashort laser pulse guiding for laser electron acceleration. Using magnetohydrodynamic computer simulations and theoretical scaling, we investigate the filling of the capillary with the gas, the electric discharge development leading to outflow of the plasma from the capillary, and the recovery of gas distribution after the discharge end. In the next cycle, these processes are repeated. As a result, we found the characteristic cycle time, which determines the upper limit on the repetition rate allowed by the capillary parameters. In the case of the capillary discharges used for acceleration of sub-GeV electron beams, e.g., needed for compact free electron lasers, an upper limit on the repetition rate is approximately equal to 10 kHz. Published by the American Physical Society 2024

Characterization of bright betatron radiation generated by direct laser acceleration of electrons in plasma of near critical density

Directed x-rays produced in the interaction of sub-picosecond laser pulses of moderate relativistic intensity with plasma of near-critical density are investigated. Synchrotron-like (betatron) radiation occurs in the process of direct laser acceleration (DLA) of electrons in a relativistic laser channel when the electrons undergo transverse betatron oscillations in self-generated quasi-static electric and magnetic fields. In an experiment at the PHELIX laser system, high-current directed beams of DLA electrons with a mean energy ten times higher than the ponderomotive potential and maximum energy up to 100 MeV were measured at 1019 W/cm2 laser intensity. The spectrum of directed x-rays in the range of 5–60 keV was evaluated using two sets of Ross filters placed at 0° and 10° to the laser pulse propagation axis. The differential x-ray absorption method allowed for absolute measurements of the angular-dependent photon fluence. We report 1013 photons/sr with energies >5 keV measured at 0° to the laser axis and a brilliance of 1021 photons s−1 mm−2 mrad−2 (0.1%BW)−1. The angular distribution of the emission has an FWHM of 14°–16°. Thanks to the ultra-high photon fluence, point-like radiation source, and ultra-short emission time, DLA-based keV backlighters are promising for various applications in high-energy-density research with kilojoule petawatt-class laser facilities.

Electron energy gain due to a laser frequency modulation experienced by electron during betatron motion

Direct laser acceleration of electrons is an important energy deposition mechanism for laser-irradiated plasmas that is particularly effective at relativistic laser intensities in the presence of quasi-static laser-driven plasma electric and magnetic fields. These radial electric and azimuthal magnetic fields provide transverse electron confinement by inducing betatron oscillations of forward-moving electrons undergoing laser acceleration. Electrons are said to experience a betatron resonance when the frequency of betatron oscillations matches the average frequency of the laser field oscillations at the electron position. In this paper, we show that the modulation of the laser frequency as seen by an electron performing betatron oscillations can be another important mechanism for net energy gain that is qualitatively different from the betatron resonance. Specifically, we show that the frequency modulation experienced by the electron can lead to net energy gain in the regime where the laser field performs three oscillations per betatron oscillation. There is no net energy gain in this regime without the modulation because the energy gain is fully compensated by the energy loss. The modulation slows down the laser oscillation near transverse stopping points, increasing the time interval during which the electron gains energy and making it possible to achieve net energy gain.

THz transition radiation of electron bunches laser-accelerated in long-scale near-critical-density plasmas

Direct laser electron acceleration in near-critical density plasma produces collimated electron beams with high charge Q (up to µC). This regime could be of interest for high-energy THz radiation generation, as many of the mechanisms have a scaling ∝Q2 . In this work, we focus specifically on the challenges that arise during numerical investigations of transition radiation in such interactions. Detailed analytical calculations that include both the diffraction and decoherence effects of the characteristics of transition radiation in the THz range were conducted with the input parameters obtained from 3D particle-in-cell and hydrodynamic simulations. The calculated characteristics of THz radiation are in good agreement with the experimentally measured ones. Therefore, this approach can be used both to optimize the properties of THz radiation and to distinguish the transition radiation contribution if several mechanisms of THz radiation generation are considered.

Electron-positron generation by irradiating various metallic materials with laser-accelerated electrons

We examined electron–positron pair production in solid iron, zinc, tungsten, and lead targets irradiated by a laser-accelerated electron beam generated with a 100TW laser. These targets were assessed at the target thickness of 0.5, 1.25, and 2.0radiation lengths for each material. Using a 0.75-T-magnetic spectrometer, we measured the electron and positron yields and spectra, producing 3 × 108 positrons per shot with a peak leptonic density of 4 × 1012cm−3. These experimental results agree very well with Monte Carlo simulations conducted with the simulation code Geant4. Importantly, our findings show that normalizing the target thickness to each material’s radiation length results in consistent electron and positron yields across the materials, effectively reducing discrepancies due to material differences.

Mitigation of electromagnetic pulses interfering with Thomson parabola ion spectrometers at XG-III laser facility.

The Thomson parabola ion spectrometer is vulnerable to intense electromagnetic pulses (EMPs) generated by a high-power laser interacting with solid targets. A metal shielding cage with a circular aperture of 1mm diameter is designed to mitigate EMPs induced by a picosecond laser irradiating a copper target in an experiment where additionally an 8-ns delayed nanosecond laser is incident into an aluminum target at the XG-III laser facility. The implementation of the shielding cage reduces the maximum EMP amplitude inside the cage to 5.2 kV/m, and the simulation results indicate that the cage effectively shields electromagnetic waves. However, the laser-accelerated relativistic electrons which escaped the target potential accumulate charge on the surface of the cage, which is responsible for the detected EMPs within the cage. To further alleviate EMPs, a lead wall and an absorbing material (ECCOSORB AN-94) were added before the cage, significantly blocking the propagation of electrons. These findings provide valuable insights into EMP generation in large-scale laser infrastructures and serve as a foundation for electromagnetic shielding design.

Study of the isomeric yield ratio in the photoneutron reaction of natural holmium induced by laser-accelerated electron beams

Introduction: An accurate knowledge of the isomeric yield ratio (IR) induced by the photonuclear reaction is crucial to study the nuclear structure and reaction mechanisms. 165Ho is a good candidate for the investigation of the IR since the Ho target has a natural abundance of 100% and the residual nuclide has a good decay property.Methods: In this study, the photoneutron production of 164m, gHo induced by laser-accelerated electron beams is investigated experimentally. The γ-ray spectra of activated Ho foils are off-line detected. Since the direct transitions from the 164mHo are not successfully observed, we propose to extract the IRs of the 164m, gHo using only the photopeak counts from the ground-state decay.Results: The production yields of 164m, gHo are extracted to be (0.45 ± 0.10) × 106 and (1.48 ± 0.14) × 106 per laser shot, respectively. The resulting IR is obtained to be 0.30 ± 0.08 at the effective γ-ray energy of 12.65 MeV.Discussion: The present data, available experimental data, and TALYS calculations are then compared to examine the role of the excitation energy. It is found that besides the giant dipole resonance, the excitation energy effect also plays a key role in the determination of the IRs.

Excitation of an upper hybrid wave by Laguerre–Gaussian pulse in plasma with a density ramp and electron acceleration

In this paper, the excitation of an upper hybrid wave (UHW) by propagation of a Laguerre–Gaussian (LG) laser pulse in an exponential density ramp plasma has been investigated in relativistic regime. A uniform static magnetic field was externally applied perpendicular to the propagation of the laser. The spatiotemporal dynamics of laser pulse have been studied by two coupled differential equations obtained via the moment theory approach. The propagating laser pulse excites an electron plasma wave, which further interacts with the laser pulse in the presence of applied transverse magnetic field and generates an UHW. The excited UHW further traps the plasma electrons and accelerates them. It has been observed that the presence of density ramp affects the laser dynamics, excited UHW, and electron acceleration. The applied magnetic field and modes of LG laser have also shown significant effect on electron acceleration. Energy gain of the order of 400 MeV/mm has been obtained for electrons.

Laser-driven electrodynamic implosion of fast ions in a thin shell

Collision of laser-driven subrelativistic high-density ion flows provides a way to create extremely compressed ion conglomerates and study their properties. This paper presents a theoretical study of the electrodynamic implosion of ions inside a hollow spherical or cylindrical shell irradiated by femtosecond petawatt laser pulses. We propose to apply a very effective mechanism for ion acceleration in a self-consistent field with strong charge separation, based on the oscillation of laser-accelerated fast electrons in this field near the thin shell. Fast electrons are generated on the outer side of the shell under irradiation by the intense laser pulses. It is shown that ions, in particular protons, may be accelerated at the implosion stage to energies of tens and hundreds of MeV when a sub-micrometer shell is irradiated by femtosecond laser pulses with an intensity of 1021–1023 W cm−2.