Large Number Of Photons Research Articles

Unconventional photon blockade via two-photon absorption

The unconventional photon blockade, which relies on the physical mechanism of quantum interference, is primarily investigated using a general master equation, where a weak nonlinearity must be presented in the system to achieve photon antibunching. In this study, we explore the unconventional photon blockade using an alternative master equation known as the two-photon absorption master equation, which is derived from the system and environment interaction via two-photon absorption. Specifically, we find that the unconventional photon blockade can be triggered in two-coupled cavities, where each cavity interacts with a two-photon absorption environment. Different from unconventional photon blockade via the general master equation, we show that the two-photon absorption acts as the weak nonlinearity, and this photon blockade corresponds to a large average photon number. To derive optimal conditions for achieving this blockade, we propose a non-Hermitian Hamiltonian method to describe the mode loss caused by the two-photon absorption. In addition, we highlight the distinctions between our proposal and other approaches for generating single-photon states based on two-photon absorption.

Vector irradiance modelling in a seawater column for assessing the detection capabilities of an oil-in-water emulsion

The possibility of tracking oil pollution in the sea has been an issue that has been analysed for a long time, and the use of light interactions with the sea polluted with various forms of oil has been the subject of numerous studies. This paper presents the results of the Monte Carlo simulations of the fate of a large number of virtual photons to demonstrate changes in the downwelling vector irradiance and upwelling vector irradiance in oil-free seawater and analogously seawater column polluted with an oil-in-water emulsion. The analyses were carried out for eight wavelengths ranging from 412 to 676 nm, upon the assumption of an oil concentration of 10 ppm, taking into account the data of absorption and scattering properties of the southern Baltic Sea. The most favourable combination of wavelengths for the detection of an oil-in-water emulsion was 555/412 for all tested depths.

Population Fluctuation Mechanism of the Super‐Thermal Photon Statistic of Quantum LEDs with Collective Effects

AbstractThe analytical procedure is developed for the calculation of the quantum second‐order autocorrelation function of a small super‐radiant LED, where the field, polarisation, and population of the active medium cannot be eliminated adiabatically. The Langevin force, which describes the effect of population fluctuations on the LED polarisation and preserves the operator commutation relations, is found. It is demonstrated that the super‐thermal photon statistics with of a small quantum LED with large photon number fluctuations, emitter‐field coupling, bad cavity, and operating in the limit , is the result of a combined effect of the spontaneous emission, collective effects and population fluctuations. Analytical expressions for and are derived.

Antibunched N-photon bundles from dark states assisted by ac Stark shift

In this paper, we propose an interesting scheme to generate antibunched N-photon bundles from dark states by using a single-atom cavity quantum electrodynamics system. The dispersive coupling between the atom and cavity introduces a Stark shift to one of the ground states, while the resonant coupling, along with a control field, forms a coherent N-excitation dark state assisted by the shift. Consequently, super-Rabi oscillation is established between the vacuum state and the N-excitation dark state when a probe field weakly couples to two ground states, enabling antibunched N-photon bundle emission within long-lived atomic coherence. As a byproduct, the generated high-efficiency single-photon source with a large mean photon number and high fidelity is of great value in quantum information processing.

Effects of measurement power on state discrimination and dynamics in a circuit-QED experiment

We explore the effects of driving a cavity at a large photon number in a circuit-QED experiment where the “matterlike” part corresponds to a unique Andreev level in a superconducting weak link. The three many-body states of the weak link, corresponding to the occupation of the Andreev level by 0, 1, or 2 quasiparticles, lead to different cavity frequency shifts. We show how the nonlinearity inherited by the cavity from its coupling to the weak link affects the state discrimination and the photon number calibration. Both effects require treating the evolution of the driven system beyond the dispersive limit. In addition, we observe how transition rates between the circuit states (quantum and parity jumps) are affected by the microwave power, and compare the measurements with a theory accounting for the “dressing” of the Andreev states by the cavity. Published by the American Physical Society 2024

Effect of photons and electrons on the over-response of optical fiber X-ray sensors

Optical fiber X-ray sensors are prone to over-response compared to ionization chambers (ICs) when used to measure the percentage depth dose (PDD) curves and off axis ratio (OAR) curves. Investigating this phenomenon is crucial for the successful adoption of these sensors in clinical radiotherapy. Compared with ion chambers and other water equivalent dosimeters, the fiber X-ray sensors using high Zeff scintillators (Gd2O2S:Tb) have generally higher mass attenuation coefficients. In this case, the response of scintillators to photons needs to be considered. In this article, a Monte-Carlo (MC) software package BEAMnrc was used to simulate the distribution of photon and electron fluxes in a clinical based water phantom, besides the energy deposition of air and Gd2O2S:Tb in varying energy was also simulated. The distribution of the photon and electron fluxes in the horizontal (radial) direction at a fixed 10 cm water depth was studied, as well as the fluxes in the vertical (depth) direction. An embedded-structure fiber X-ray sensor was used for the experimental measurements. The simulation results indicate that, in the horizontal direction, there are many photons remain outside the radiation field. In the vertical direction, as the size of the radiation field increases, the maximum point of the photon flux shifts towards a deeper water depth. These behavior of photon flux is consistent with the fiber X-ray sensors measurement. However, the maximum point of the electron flux remains unchanged in the vertical direction. In the horizontal direction, the electron flux decreases rapidly, and this scenario is similar to the case when using the ion chamber. Results of analyzing the spectra inside and outside the radiation field show that there is a large number of photons with energy below 0.2 MeV outside the radiation field, and the proportion of these low-energy photons is greater than 60 %. The findings indicate that the fiber X-ray sensors' over-response can be primarily attributed to the lower energy scattered photons.

Ionizing terahertz waves with 260 MV/cm from scalable optical rectification.

Terahertz (THz) waves, known as non-ionizing radiation owing to their low photon energies, can actually ionize atoms and molecules when a sufficiently large number of THz photons are concentrated in time and space. Here, we demonstrate the generation of ionizing, multicycle, 15-THz waves emitted from large-area lithium niobate crystals via phase-matched optical rectification of 150-terawatt laser pulses. A complete characterization of the generated THz waves in energy, pulse duration, and focal spot size shows that the field strength can reach up to 260 megavolts per centimeter. In particular, a single-shot THz interferometer is employed to measure the THz pulse duration and spectrum with complementary numerical simulations. Such intense THz pulses are irradiated onto various solid targets to demonstrate THz-induced tunneling ionization and plasma formation. This study also discusses the potential of nonperturbative THz-driven ionization in gases, which will open up new opportunities, including nonlinear and relativistic THz physics in plasma.

Photocatalytic Deposition of Au Nanoparticles on Ti3C2Tx MXene Substrates for Surface-Enhanced Raman Scattering.

Surface-enhanced Raman scattering (SERS) is a promising technique for sensitive detection. The design and optimization of plasma-enhanced structures for SERS applications is an interesting challenge. In this study, we found that the SERS activity of MXene (Ti3C2Tx) can be improved by adding Au nanoparticles (NPs) in a simple photoreduction process. Fluoride-salt-etched MXene was deposited by drop-casting on a glass slide, and Au NPs were formed by the photocatalytic growth of gold(III) chloride trihydrate solutions under ultraviolet (UV) irradiation. The Au-MXene substrate formed by Au NPs anchored on the Ti3C2Tx sheet produced significant SERS through the synergistic effect of chemical and electromagnetic mechanisms. The structure and size of the Au-decorated MXene depended on the reaction time. When the MXene films were irradiated with a large number of UV photons, the size of the Au NPs increased. Hot spots were formed in the nanoscale gaps between the Au NPs, and the abundant surface functional groups of the MXene effectively adsorbed and interacted with the probe molecules. Simultaneously, as a SERS substrate, the proposed Au-MXene composite exhibited a wider linear range of 10-4-10-9 mol/L for detecting carbendazim. In addition, the enhancement factor of the optimized SERS substrate Au-MXene was 1.39 × 106, and its relative standard deviation was less than 13%. This study provides a new concept for extending experimental strategies to further improve the performance of SERS.

Photon blockade with high photon occupation via cavity electromagnetically induced transparency

Photon blockade (PB) is one of the effective methods to generate single-photon sources. In general, both the PB effect with the significant sub-Poissonian statistics and a large mean photon number are desired to guarantee the brightness and the purity of single-photon sources. Here, we propose to obtain the PB effect at the cavity dark-state polariton (DSP) using a cavity Λ-type electromagnetically induced transparency (EIT) system with and without the two-photon dissipation (TPD). In the Raman resonance case, the PB effect at the DSP could by realized by using the TPD process in the weak or intermediate coupling regime, which accompanies with near unity transmission, i.e., very high photon occupation. In the slightly detuned Raman resonance case, the excited state is induced into the components of the DSP, and the atomic dissipation path is added into the two-photon excitation paths. Thus, the PB effect at the DSP can be obtained due to the quantum destructive interference (QDI) in the strong coupling regime, which can be further enhanced using the TPD process. Due to the slight detuning, the PB effect still remains high photon occupation and has highly tunability. This work provides an alternative way to manipulate the photon statistics by the PB effect and has potential applications in generating single-photon sources with high brightness and purity.

Programmable multiphoton quantum interference in a single spatial mode.

The interference of nonclassical states of light enables quantum-enhanced applications reaching from metrology to computation. Most commonly, the polarization or spatial location of single photons are used as addressable degrees of freedom for turning these applications into praxis. However, the scale-up for the processing of a large number of photons of these architectures is very resource-demanding due to the rapidly increasing number of components, such as optical elements, photon sources, and detectors. Here, we demonstrate a resource-efficient architecture for multiphoton processing based on time-bin encoding in a single spatial mode. We use an efficient quantum dot single-photon source and a fast programmable time-bin interferometer to observe the interference of up to eight photons in 16 modes, all recorded only with one detector, thus considerably reducing the physical overhead previously needed for achieving equivalent tasks. Our results can form the basis for a future universal photonics quantum processor operating in a single spatial mode.

Two-photon absorption cross sections of pulsed entangled beams.

Entangled two-photon absorption (ETPA) could form the basis of nonlinear quantum spectroscopy at very low photon fluxes, since, at sufficiently low photon fluxes, ETPA scales linearly with the photon flux. When different pairs start to overlap temporally, accidental coincidences are thought to give rise to a "classical" quadratic scaling that dominates the signal at large photon fluxes and, thus, recovers a supposedly classical regime, where any quantum advantage is thought to be lost. Here, we scrutinize this assumption and demonstrate that quantum-enhanced absorption cross sections can persist even for very large photon numbers. To this end, we use a minimal model for quantum light, which can interpolate continuously between the entangled pair and a high-photon-flux limit, to analytically derive ETPA cross sections and the intensity crossover regime. We investigate the interplay between spectral and spatial degrees of freedom and how linewidth broadening of the sample impacts the experimentally achievable enhancement.

Photonic quantum metrology with variational quantum optical nonlinearities

Photonic quantum metrology harnesses quantum states of light, such as NOON or twin-Fock states, to measure unknown parameters beyond classical precision limits. Current protocols suffer from two severe limitations that preclude their scalability: the exponential decrease in fidelities (or probabilities) when generating states with large photon numbers due to gate errors and the increased sensitivity of such states to noise. Here, we develop a deterministic protocol combining quantum optical nonlinearities and variational quantum algorithms that provides a substantial improvement on both fronts. First, we show how the variational protocol can generate metrologically relevant states with a small number of operations which do not significantly depend on photon number, resulting in exponential improvements in fidelities when gate errors are considered. Second, we show that such states offer a better robustness to noise compared to other states in the literature. Since our protocol harnesses interactions already appearing in state-of-the-art setups, such as cavity QED, we expect that it will lead to more scalable photonic quantum metrology in the near future. Published by the American Physical Society 2024

Stabilizer Subsystem Decompositions for Single- and Multimode Gottesman-Kitaev-Preskill Codes

The Gottesman-Kitaev-Preskill (GKP) error-correcting code encodes a finite-dimensional logical space in one or more bosonic modes, and has recently been demonstrated in trapped ions and superconducting microwave cavities. In this work we introduce a new subsystem decomposition for GKP codes that we call the stabilizer subsystem decomposition, analogous to the usual approach to quantum stabilizer codes. The decomposition has the defining property that a partial trace over the nonlogical stabilizer subsystem is equivalent to an ideal decoding of the logical state, distinguishing it from previous GKP subsystem decompositions. We describe how to decompose arbitrary states across the subsystem decomposition using a set of transformations that move between the decompositions of different GKP codes. Besides providing a convenient theoretical view on GKP codes, such a decomposition is also of practical use. We use the stabilizer subsystem decomposition to efficiently simulate noise acting on single-mode GKP codes, and in contrast to more conventional Fock basis simulations, we are able to consider essentially arbitrarily large photon numbers for realistic noise channels, such as loss and dephasing. Published by the American Physical Society 2024

Quantitative bounds to propagation of quantum correlations in many-body systems

We investigate how much information about a quantum system can be simultaneously communicated to independent observers, by establishing quantitative limits to bipartite quantum correlations in many-body systems. As recently reported in Girolami et al. (2022) [16], bounds on quantum discord and entanglement of formation between a single quantum system and its environment, e.g., a large number of photons, dictate that independent observers which monitor environment fragments inevitably acquire only classical information about the system. Here, we corroborate and generalize those findings. First, we calculate continuity bounds of quantum discord, which establish how much states with a small amount of quantum correlations deviate from being embeddings of classical probability distributions. Also, we demonstrate a universally valid upper bound to the bipartite entanglement of formation between an arbitrary pair of components of a many-body quantum system. The results confirm that proliferation of classical information in the Universe suppresses quantum correlations.

Broadband Spectroscopy and Interferometry with Undetected Photons at Strong Parametric Amplification

AbstractNonlinear interferometry with entangled photons allows for characterizing a sample without detecting the photons interacting with it. This method enables highly sensitive optical sensing in the wavelength regions where efficient detectors are still under development. Recently, nonlinear interferometry has been applied to interferometric measurement techniques with broadband light sources, such as Fourier‐transform infrared spectroscopy and infrared optical coherence tomography. However, they have been demonstrated with photon pairs produced through spontaneous parametric down‐conversion (SPDC) at a low parametric gain, where the average number of photons per mode is much smaller than one. The regime of high‐gain SPDC offers several important advantages, such as the amplification of light after its interaction with the sample and a large number of photons per mode at the interferometer output. This work presents broadband spectroscopy and high‐resolution optical coherence tomography with undetected photons generated via high‐gain SPDC in an aperiodically poled lithium niobate crystal. To prove the principle, reflective Fourier‐transform near‐infrared spectroscopy with a spectral bandwidth of 17 THz and optical coherence tomography with an axial resolution of 11 µm are demonstrated.

Strong single-photon to two-photon bundles emission in spin-1 Jaynes–Cummings model

High-quality special nonclassical states beyond the strong single atom-cavity coupling regime are fundamental elements in quantum information science. Here, we study strong single-photon blockade to two-photon bundles emission in a single spin-1 atom coupled to an optical cavity by constructing a spin-1 Jaynes–Cummings model (JCM). By tuning the quadratic Zeeman shift, the energy-spectrum anharmonicity can be significantly enhanced, leading to a remarkable increase in the dressed-state splitting of the well-resolved n-photon resonance. The mechanism, which benefits from the internal degrees of freedom in high-spin systems, compensates for the strong coupling condition required by the multi-photon blockade, thereby facilitating the experimental feasibility of engineering special nonclassical states beyond the strong-coupling limit. It is shown that the photon emission from the spin-1 JCM demonstrates high-quality single photon and two-photon bundles with large steady-state photon numbers in the cavity-driven and atom-pump cases, respectively. In particular, compared to the two-level two-photon JCM, the antibunching amplitude of the three-order correlation function for two-photon bundles in the spin-1 JCM is enhanced by 3 orders of magnitude. More interestingly, a multimode transducer, enabling a transition from strong single-photon blockade to two-photon bundles and super-Poissonian photon emission, is achieved and highly controllable by the light-cavity detuning in the presence of both atom and cavity driven fields. This study based on the high-spin JCM broadens the scope of engineering special nonclassical quantum states beyond the standard two-level JCM. Our proposal not only opens up a new avenue for generating high-quality n-photon sources but also provides versatile applications in quantum networks and metrology.

Three-dimensional irradiance and temperature distributions resulting from transdermal application of laser light to human knee-A numerical approach.

The use of light for therapeutic applications requires light-absorption by cellular chromophores at the target tissues and the subsequent photobiomodulation (PBM) of cellular biochemical processes. For transdermal deep tissue light therapy (tDTLT) to be clinically effective, a sufficiently large number of photons must reach and be absorbed at the targeted deep tissue sites. Thus, delivering safe and effective tDTLT requires understanding the physics of light propagation in tissue. This study simulates laser light propagation in an anatomically accurate human knee model to assess the light transmittance and light absorption-driven thermal changes for eight commonly used laser therapy wavelengths (600-1200 nm) at multiple skin-applied irradiances (W cm-2 ) with continuous wave (CW) exposures. It shows that of the simulated parameters, 2.38 W cm-2 (30 W, 20 mm beam radius) of 1064 nm light generated the least tissue heating -4°C at skin surface, after 30 s of CW irradiation, and the highest overall transmission-approximately 3%, to the innermost muscle tissue.

Classical Emulation of Bright Quantum States

AbstractThe way to emulate classically a number of fundamental quantum mechanical experiments is shown, such as Hong‐Ou‐Mandel interference, phase measurements with NOON states and specifically structured “revivals” in Jaynes‐Cummings model using coherent states with large number of photons. It is also shown that certain classes of bright non‐classical states can be efficiently emulated by our technique independently of the average photon number of these states.

Scattershot multiboson correlation sampling with random photonic inner-mode multiplexing

Multiphoton interference is an essential phenomenon at the very heart not only of fundamental quantum optics and applications in quantum information processing and sensing but also of demonstrations of quantum computational supremacy in boson sampling experiments relying only on linear optical interferometers. However, scalable boson sampling experiments with either photon number states or squeezed states are challenged by the need to generate a large number of photons with fixed temporal and frequency spectra from one experimental run to another. Unfortunately, even the well-established standard multiplexing techniques employed to generate photons with fixed spectral properties are affected by the detrimental effects of losses, spectral distorsions and reduction in purity. Here, we employ sampling correlation measurements in the photonic inner modes, time and frequency, at the interferometer input and output to ensure the occurrence of multiphoton interference even with pure states of input photons with random spectral overlap from one sample to another. Indeed, by introducing a random multiplexing technique where photons are generated with random inner-mode parameters, it is possible to substantially enhance the probability to successfully generate samples and overcome the typical drawbacks in standard multiplexing. We also demonstrate the classical hardness of the resulting problem of scattershot multiboson correlation sampling based on this technique. Therefore, these results not only shed new light in the computational complexity of multiboson interference but also allow us to enhance the experimental scalability of boson sampling schemes. Furthermore, this research provides a new exciting route toward future demonstrations of quantum computational supremacy with scalable experimental resources as well as future applications in quantum information processing and sensing beyond boson sampling.

Algorithm of quantum engineering of large-amplitude high-fidelity Schrödinger cat states

We present an algorithm of quantum engineering of large-amplitude ge 5 high-fidelity ge 0.99 even/odd Schrödinger cat states (SCSs) using a single mode squeezed vacuum (SMSV) state as resource. Set of k beam splitters (BSs) with arbitrary transmittance and reflectance coefficients sequentially following each other acts as a hub that redirects a multiphoton state into the measuring modes simultaneously measured by photon number resolving (PNR) detectors. We show that the multiphoton state splitting guarantees significant increase of the success probability of the SCSs generator compared to its implementation in a single PNR detector version and imposes less requirements on ideal PNR detectors. We prove that the fidelity of the output SCSs and its success probability are in conflict with each other (which can be quantified) in a scheme with ineffective PNR detectors, especially when subtracting large (say, 100) number of photons, i.e., increasing the fidelity to perfect values leads to a sharp decrease in the success probability. In general, the strategy of subtracting up to 20 photons from initial SMSV in setup with two BSs is acceptable for achieving sufficiently high values of the fidelity and success probability at the output of the generator of the SCSs of amplitude le 3 with two inefficient PNR detectors.