In this paper, the global smooth solution of Cauchy's problem of incompressible, resistive, viscous Hall-magnetohydrodynamics (Hall-MHD) is studied. By exploring the nonlinear structure of Hall-MHD equations, a class of large initial data is constructed, which can be arbitrarily large in $H^3(\mathbb{R}^3)$. Our result may also be considered as the extension of work of Lei-Lin-Zhou from the second-order semi-linear equations to the second-order quasilinear equations, because the Hall term elevates the Hall-MHD system to the quasilinear level.