The Archean East Indian cratonic margin was affected by the Kerguelen plume (KP) ∼117Ma, causing flood-basalt eruptions of the Rajmahal–Bengal–Sylhet Traps (RBST). The RBST cover ∼one million km2 in and around the Bengal Basin as alkalic–ultrabasic intrusives in the west and Sikkim in the north, and Sylhet basalts and alkalic–carbonatitic–ultramafic complexes in the Shillong plateau – Mikir hills farther east of the Rajmahal–Bengal Traps. We provide new Nd–Sr–Pb-isotopic and trace element data on 21 unreported discrete lava flows of the Rajmahal Traps, 56 alkalic–carbonatitic–mafic–ultramafic rocks from four alkalic complexes, and three dikes from the Gondwana Bokaro coalfields, all belonging to the RBST. The data allow geochemical correlation of the RBST with some contemporaneous Kerguelen Plateau basalts and KP-related volcanics in the southern Indian Ocean. Specifically, the new data show similarity with previous data of Rajmahal group I–II basalts, Sylhet Traps, Bunbury basalts, and lavas from the southern Kerguelen Plateau, indicating a relatively primitive KP source, estimated as: εNd(I)=+2, 87Sr/86Sr(I)=0.7046, with a nearly flat time-integrated rare earth element (REE) pattern. We model the origin of the uncontaminated RBST basalts by ∼18% batch melting with a 2× chondritic KP source in the spinel-peridotite stability depths of 60–70km in the mantle. The new geochemical data similar to the Rajmahal group II basalts indicate a light REE enriched average source at εNd(I)=−5, 87Sr/86Sr(I)=0.7069. Our geochemical modeling indicates these lavas assimilated granulites of the Eastern Ghats, reducing the thickness of the continental Indian lithosphere. Lack of an asthenospheric MORB component in the RBST province is indicated by various trace element ratios as well as the Nd-Sr isotopic ratios.Three alkalic complexes, Sung, Samchampi, and Barpung in NE India, and one in Sikkim to the north are of two groups: carbonatites, pyroxenites, lamproites, nephelinites, sovites, melteigite in the first group and syenites and ijolites in the second. The Nd–Sr–Pb-isotopic and trace element geochemistry of the first group of carbonatitic–ultrabasic rocks are consistent with similar data of the RBST lavas of the present and previous studies, and are modeled as derived from a relatively primitive carbonated garnet peridotite source in the KP. In contrast, the syenites and ijolites of the second group show a wide range of Nd–Sr–Pb isotopic compositions, modeled by low-degree melts of an ancient recycled carbonated eclogite also in the KP. The KP thus reflects heterogeneities in the lower mantle-derived plume with carbonated components yielding ultrabasic melts at greater depths with low-degree melting, followed by rise of the plume at shallower depths causing tholeiitic flood basalt volcanism. Collectively, these data imply a zone of influence of the plate-motion-reconstructed KP head for ∼1000km around the Bengal Basin, as represented by the widely scattered and diverse rock types of the RBST.