Karlsruhe Tritium Neutrino Research Articles

Multi‐Photon 3D Laser Micro‐Printed Plastic Scintillators for Applications in Low‐Energy Particle Physics

AbstractPlastic scintillators are inexpensive to manufacture and therefore a popular alternative to inorganic crystalline scintillators. For many applications, their advantages outweigh their lower light yield. Additionally, it is easier to structure plastic scintillators with well‐developed processing techniques which is of growing relevance in modern applications. One technique to structure plastic material is 3D printing, with noteworthy recent advances in one‐photon‐based approaches. However, some applications require high spatial resolution and optically smooth surfaces, which can be achieved by multi‐photon 3D laser micro‐printing. One application example is the improvement of sensitivity of the Karlsruhe Tritium Neutrino (KATRIN) experiment. This improvement can be realized by printing a 3D scintillator structure as an active transverse energy filter directly onto the detector. Herein, the first two‐photon printable plastic scintillator providing a printing resolution in the micrometer regime is presented. Using the benefits of two‐photon grayscale lithography, optical‐grade surfaces are achieved. The light output is estimated to be 930 photons MeV−1. A prototype structure printed directly on a single‐photon avalanche diode array is demonstrated.

Constraining the mass-spectra in the presence of a light sterile neutrino from absolute mass-related observables

The framework of three-flavor neutrino oscillation is a well-established phenomenon, but results from the short-baseline experiments, such as the Liquid Scintillator Neutrino Detector (LSND) and MiniBooster Neutrino Experiment (MiniBooNE), hint at the potential existence of an additional light neutrino state characterized by a mass-squared difference of approximately 1 eV2. The new neutrino state is devoid of all Standard Model (SM) interactions, commonly referred to as a “sterile” state. In addition, a sterile neutrino with a mass-squared difference of 10−2 eV2 has been proposed to improve the tension between the results obtained from the Tokai to Kamioka (T2K) and the NuMI Off-axis νe Appearance (NOνA) experiments. Further, the nonobservation of the predicted upturn in the solar neutrino spectra below 8 MeV can be explained by postulating an extra light sterile neutrino state with a mass-squared difference around 10−5 eV2. The hypothesis of an additional light sterile neutrino state introduces four distinct mass spectra depending on the sign of the mass-squared difference. In this paper, we discuss the implications of the above scenarios on the observables that depend on the absolute mass of the neutrinos; namely, the sum of the light neutrino masses (Σ) from cosmology, the effective mass of the electron neutrino from beta decay (mβ), and the effective Majorana mass (mββ) from neutrinoless double beta decay. We show that some scenarios can be disfavored by the current constraints of the above variables. The implications for projected sensitivity of Karlsruhe Tritium Neutrino Experiment (KATRIN) and future experiments like Project-8, next Enriched Xenon Observatory (nEXO) are discussed. Published by the American Physical Society 2024

Development of a silicon drift detector array to search for keV-scale sterile neutrinos with the KATRIN experiment

Sterile neutrinos in the keV mass range present a viable candidate for dark matter. They can be detected through single β -decay, where they cause small spectral distortions. The Karlsruhe Tritium Neutrino (KATRIN) experiment aims to search for keV-scale sterile neutrinos with high sensitivity. To achieve this, the KATRIN beamline will be equipped with a novel multi-pixel silicon drift detector focal plane array named TRISTAN. In this study, we present the performance of a TRISTAN detector module, a component of the eventual 9-module system. Our investigation encompasses spectroscopic aspects such as noise performance, energy resolution, linearity, and stability.

A thermionic electron gun to characterize silicon drift detectors with electrons

The TRISTAN detector is a new detector for electron spectroscopy at the Karlsruhe Tritium Neutrino (KATRIN) experiment. The semiconductor detector utilizes the silicon drift detector technology and will enable the precise measurement of the entire tritium β-decay electron spectrum. Thus, a significant fraction of the parameter space of potential neutrino mass eigenstates in the keV-mass regime can be probed. We developed a custom electron gun based on the effect of thermionic emission to characterize the TRISTAN detector modules with mono-energetic electrons before installation into the KATRIN beamline. The electron gun provides an electron beam with up to 25 keV kinetic energy and an electron rate in the order of 105 electrons per second. This manuscript gives an overview of the design and commissioning of the electron gun. In addition, we will shortly discuss a first measurement with the electron gun to characterize the electron response of the TRISTAN detector.

Improved treatment of the T2\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$_2$$\\end{document} molecular final-states uncertainties for the KATRIN neutrino-mass measurement

The KArlsruhe TRItium Neutrino experiment (KATRIN) aims to determine the effective mass of the electron antineutrino via a high-precision measurement of the tritium β\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\\upbeta $$\\end{document}-decay spectrum in its end-point region. The target neutrino-mass sensitivity of 0.2eV/c2\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$${0.2}~\ ext {eV}/\ ext {c}^2$$\\end{document} at 90% CL can only be achieved in the case of high statistics and good control of the systematic uncertainties. One key systematic effect originates from the calculation of the molecular final states of T2\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$_2$$\\end{document}β\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\\upbeta $$\\end{document} decay. In the first neutrino-mass analyses of KATRIN the contribution of the uncertainty of the molecular final-states distribution (FSD) was estimated via a conservative phenomenological approach to be 2×10-2eV2/c4.\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$2 \ imes 10^{-2}~\ ext {eV}^{2}/\ ext {c}^{4}.$$\\end{document} In this work a new procedure is presented for estimating the FSD-related uncertainties by considering the details of the final-states calculation, i.e. the uncertainties of constants, parameters, and functions used in the calculation as well as its convergence itself as a function of the basis-set size used in expanding the molecular wave functions. The calculated uncertainties are directly propagated into the experimental observable, the squared neutrino mass mν2,\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$m_\ u ^2,$$\\end{document} and thus have to be determined individually for each experimental configuration. For the experimental conditions of the first KATRIN measurement campaign the new procedure is presented in detail, allowing for the application of this procedure to other experiments. This specific calculation leads to a constraint of the FSD-related uncertainty of 1.3×10-3eV2/c4,\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$1.3 \ imes 10^{-3}~\ ext {eV}^{2}/\ ext {c}^{4},$$\\end{document} well below the design limit of 7.5×10-3eV2/c4\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$7.5 \ imes 10^{-3}~\ ext {eV}^{2}/\ ext {c}^{4}$$\\end{document} for any individual systematic contribution.

Penning-trap measurement of the Q value of electron capture in 163Ho for the determination of the electron neutrino mass

The investigation of the absolute scale of the effective neutrino mass remains challenging due to the exclusively weak interaction of neutrinos with all known particles in the standard model of particle physics. At present, the most precise and least-model-dependent upper limit on the electron antineutrino mass is set by the Karlsruhe Tritium Neutrino Experiment (KATRIN) from the analysis of the tritium β-decay. Another promising approach is the electron capture in 163Ho, which is under investigation using microcalorimetry by the Electron Capture in Holmium (ECHo) and HOLMES collaborations. An independently measured Q value for this process is vital for the assessment of systematic uncertainties in the neutrino mass determination. Here we report a direct, independent determination of this Q value by measuring the free-space cyclotron frequency ratio of highly charged ions of 163Ho and 163Dy in the Penning-trap experiment PENTATRAP. Combining this ratio with atomic physics calculations of the electronic binding energies yields a Q value of 2,863.2 ± 0.6 eV c−2, which represents a more than 50-fold improvement over the state of the art. This will enable the determination of the electron neutrino mass on a sub-electronvolt level from the analysis of the electron capture in 163Ho.

In Situ Tritium Decontamination of the KATRIN Rear Wall Using an Ultraviolet/Ozone Treatment

The KArlsruhe TRItium Neutrino (KATRIN) collaboration aims to determine the neutrino mass with a sensitivity of 0.2 eV/c2 (90% confidence level). This will be achieved by probing the end-point region of the β-electron spectrum of gaseous tritium with an electrostatic spectrometer. A gold-coated stainless steel disk defines the reference potential for high-precision neutrino mass measurement, and it terminates the β-electron flux as the physical boundary of the tritium source. This so-called rear wall is exposed to tritium, which leads to adsorption and absorption. This in turn leads to systematic uncertainties for the neutrino mass measurements that need to be understood and mitigated. In maintenance phases, during which the gaseous tritium source was emptied (<10−5 of nominal gas density), the activity that accumulated on the rear wall during normal operation was monitored using beta-induced X-ray spectrometry (BIXS) and direct observation of emitted β electrons with a silicon detector. Dependency of the observed activity increase on the integral tritium throughput was investigated and found to converge from limited exponential growth to continuous linear growth. This paper gives an overview of the results that were obtained using several methods of in situ decontamination of the rear wall while continuously monitoring the activity. The decontamination methods included heating during continuous evacuation; flushing the system with nitrogen, deuterium, or air with residual humidity at different pressures; and illumination of the rear wall with ultraviolet (UV) light. These well-known methods led to only a small ( ≈ 15%) decrease in the observed activity. However, a decrease of the surface activity by three orders of magnitude in less than 1 week was achieved by combination of different methods using UV light, a heated surface, and a low (5 to 100 mbar) pressure of air inside the chamber, leading to the production of highly reactive ozone. This proved to be by far the most efficient method, drastically reducing the contribution of the rear wall surface activity to the β spectrum of the gaseous source.

Four Years of Tritium Operation of the KATRIN Experiment at TLK

The Karlsruhe Tritium Neutrino (KATRIN) experiment measures the tritium β-spectrum close to the maximum decay energy to achieve the value of the electron-antineutrino mass with a sensitivity of 0.2 eV/c2 (90% confidence level). Since only a small fraction of the decay electrons carries nearly all the energy, a high luminous tritium source, with its supporting infrastructure facilities, is necessary. Since the start of the tritium operation of KATRIN back in May 2018, more than 600 days of 24/7 measuring campaigns with a total tritium throughput of ≈18.1 kg and a tritium concentration >95% have been conducted. Despite several technical issues occurring during the run time, the necessary reliable supply of tritium was provided. This contribution will give an overview of the current operational conditions of the Tritium Laboratory Karlsruhe tritium facilities involved, as well as the relevant technical, analytical, and administrative procedures implemented. Furthermore, an analysis will be given for system and component malfunctions in the tritium loop as well as the associated actions for problem-solving and repair. In addition, an end-of-life investigation for the component failure will be presented.

Operation modes of the KATRIN experiment Tritium Loop System using 83mKr

The KArlsruhe TRItium Neutrino (KATRIN) experiment aims to search for the effective electron antineutrino mass with a sensitivity of 0.2 eV (90 % C.L.).In order to achieve this goal, KATRIN measurement phases focusing on the neutrino mass search are alternated with phases of investigations of systematic effects.During these phases, metastable 83mKr is used as a calibration source.The monoenergetic conversion electrons emitted accompanying the decay of 83mKr allow a direct access to the starting conditions of β-electrons produced inside the windowless gaseous tritium source (WGTS) of KATRIN.To make use of 83mKr in the WGTS, the Tritium Loop System, which provides a stable flow of tritium to the WGTS, needs to be operated in special modes.This paper focuses on the technical implementation of these modes and their performance with regard to the achievable 83mKr-rates, gas densities, and gas compositions inside the WGTS.

Characterization of the KATRIN cryogenic pumping section

The KArlsruhe TRItium Neutrino (KATRIN) experiment aims to determine the effective anti-electron neutrino mass with a sensitivity of 0.2eV/c2 by using the kinematics of tritium β-decay. It is crucial to have a high signal rate which is achieved by a windowless gaseous tritium source producing 1011β-electrons per second. These are guided adiabatically to the spectrometer section where their energy is analyzed. In order to maintain a low background rate below 0.01cps, one essential criteria is to permanently reduce the flow of neutral tritium molecules between the source and the spectrometer section by at least 14 orders of magnitude. A differential pumping section downstream from the source reduces the tritium flow by seven orders of magnitude, while at least another factor of 107 is achieved by the cryogenic pumping section where tritium molecules are adsorbed on an approximately 3K cold argon frost layer. In this paper, the results of the cryogenic pumping section commissioning measurements using deuterium are discussed. The cryogenic pumping section surpasses the requirement for the flow reduction of 107 by more than one order of magnitude. These results verify the predictions of previously published simulations.

KATRIN: status and prospects for the neutrino mass and beyond

The Karlsruhe Tritium Neutrino (KATRIN) experiment is designed to measure a high-precision integral spectrum of the endpoint region of T2 β decay, with the primary goal of probing the absolute mass scale of the neutrino. After a first tritium commissioning campaign in 2018, the experiment has been regularly running since 2019, and in its first two measurement campaigns has already achieved a sub-eV sensitivity. After 1000 days of data-taking, KATRIN’s design sensitivity is 0.2 eV at the 90% confidence level. In this white paper we describe the current status of KATRIN; explore prospects for measuring the neutrino mass and other physics observables, including sterile neutrinos and other beyond-Standard-Model hypotheses; and discuss research-and-development projects that may further improve the KATRIN sensitivity.

Characterization measurements of the TRISTAN multi-pixel silicon drift detector

Sterile neutrinos are a minimal extension of the standard model of particle physics. A laboratory-based approach to search for this particle is via tritium β-decay, where a sterile neutrino would cause a kink-like spectral distortion. The Karlsruhe Tritium Neutrino (KATRIN) experiment extended by a multi-pixel Silicon Drift Detector system has the potential to reach an unprecedented sensitivity to the keV-scale sterile neutrino in a lab-based experiment. The new detector system combines good spectroscopic performance with a high rate capability. In this work, we report about the characterization of charge-sharing between pixels and the commissioning of a 47-pixel prototype detector in a MAC-E filter.

Wideband precision stabilization of the -18.6kV retarding voltage for the KATRIN spectrometer

The Karlsruhe Tritium Neutrino Experiment (KATRIN) measures the effective electron anti-neutrino mass with an unprecedented design sensitivity of 0.2 eV (90 % C.L.). In this experiment, the energy spectrum of beta electrons near the tritium decay endpoint is analyzed with a highly accurate spectrometer. To reach the KATRIN sensitivity target, the retarding voltage of this spectrometer must be stable to the ppm (1 × 10-6) level and well known on various time scales (μs up to months), for values around -18.6 kV. A custom-designed high-voltage regulation system mitigates the impact of interference sources in the absence of a closed electric shield around the large spectrometer vessel. In this article, we describe the regulation system and its integration into the KATRIN setup. Independent monitoring methods demonstrate a stability within 2 ppm, exceeding KATRIN's specifications.

Fast and precise model calculation for KATRIN using a neural network

We present a fast and precise method to approximate the physics model of the Karlsruhe Tritium Neutrino (KATRIN) experiment using a neural network. KATRIN is designed to measure the effective electron anti-neutrino mass m_nu using the kinematics of upbeta -decay with a sensitivity of 200 meV at 90% confidence level. To achieve this goal, a highly accurate model prediction with relative errors below the 10^{-4}-level is required. Using the regular numerical model for the analysis of the final KATRIN dataset is computationally extremely costly or requires approximations to decrease the computation time. Our solution to reduce the computational requirements is to train a neural network to learn the predicted upbeta -spectrum and its dependence on all relevant input parameters. This results in a speed-up of the calculation by about three orders of magnitude, while meeting the stringent accuracy requirements of KATRIN.

Forward Beam Monitor for the KATRIN experiment

The KArlsruhe TRItium Neutrino (KATRIN) experiment aims to measure the neutrino mass with a sensitivity of 0.2 eV (90 % CL). This will be achieved by a precision measurement of the endpoint region of the β-electron spectrum of tritium decay. The β-electrons are produced in the Windowless Gaseous Tritium Source (WGTS) and guided magnetically through the beamline. In order to accurately extract the neutrino mass the source activity is required to be stable and known to a high precision. The WGTS therefore undergoes constant extensive monitoring from several measurement systems. The Forward Beam Monitor (FBM) is one such monitoring system. The FBM system comprises a complex mechanical setup capable of inserting a detector board into the KATRIN beamline with a positioning precision of better than 0.3 mm. The electron flux density at that position is on the order of 106 s-1 mm-2. The detector board contains two silicon detector chips of p-i-n diode type which can measure the β-electron flux from the source with a precision of 0.1 % within 60 s with an energy resolution of FWHM = 2 keV. The unique challenge in developing the FBM arises from its designated operating environment inside the Cryogenic Pumping Section which is a potentially tritium contaminated ultra-high vacuum chamber at cryogenic temperatures in the presence of a 1 T strong magnetic field. Each of these parameters do strongly limit the choice of possible materials which e.g. caused difficulties in detector noise reduction, heat dissipation and lubrication. In order to completely remove the FBM from the beam tube a 2 m long traveling distance into the beamline is needed demanding a robust as well as highly precise moving mechanism.

Direct neutrino-mass measurement with sub-electronvolt sensitivity

Since the discovery of neutrino oscillations, we know that neutrinos have non-zero mass. However, the absolute neutrino-mass scale remains unknown. Here we report the upper limits on effective electron anti-neutrino mass, mν, from the second physics run of the Karlsruhe Tritium Neutrino experiment. In this experiment, mν is probed via a high-precision measurement of the tritium β-decay spectrum close to its endpoint. This method is independent of any cosmological model and does not rely on assumptions whether the neutrino is a Dirac or Majorana particle. By increasing the source activity and reducing the background with respect to the first physics campaign, we reached a sensitivity on mν of 0.7 eV c–2 at a 90% confidence level (CL). The best fit to the spectral data yields {{mbox{}}}{m}_{nu }^{2}{{mbox{}}} = (0.26 ± 0.34) eV2 c–4, resulting in an upper limit of mν < 0.9 eV c–2 at 90% CL. By combining this result with the first neutrino-mass campaign, we find an upper limit of mν < 0.8 eV c–2 at 90% CL.

The design, construction, and commissioning of the KATRIN experiment

The KArlsruhe TRItium Neutrino (KATRIN) experiment, which aims to make a direct and model-independent determination of the absolute neutrino mass scale, is a complex experiment with many components.More than 15 years ago, we published a technical design report (TDR) [1] to describe the hardware design and requirements to achieve our sensitivity goal of 0.2 eV at 90% C.L. on the neutrino mass.Since then there has been considerable progress, culminating in the publication of first neutrino mass results with the entire beamline operating [2].In this paper, we document the current state of all completed beamline components (as of the first neutrino mass measurement campaign), demonstrate our ability to reliably and stably control them over long times, and present details on their respective commissioning campaigns.

Analysis methods for the first KATRIN neutrino-mass measurement

We report on the data set, data handling, and detailed analysis techniques of the first neutrino-mass measurement by the Karlsruhe Tritium Neutrino (KATRIN) experiment, which probes the absolute neutrino-mass scale via the $\beta$-decay kinematics of molecular tritium. The source is highly pure, cryogenic T$_2$ gas. The $\beta$ electrons are guided along magnetic field lines toward a high-resolution, integrating spectrometer for energy analysis. A silicon detector counts $\beta$ electrons above the energy threshold of the spectrometer, so that a scan of the thresholds produces a precise measurement of the high-energy spectral tail. After detailed theoretical studies, simulations, and commissioning measurements, extending from the molecular final-state distribution to inelastic scattering in the source to subtleties of the electromagnetic fields, our independent, blind analyses allow us to set an upper limit of 1.1 eV on the neutrino-mass scale at a 90\% confidence level. This first result, based on a few weeks of running at a reduced source intensity and dominated by statistical uncertainty, improves on prior limits by nearly a factor of two. This result establishes an analysis framework for future KATRIN measurements, and provides important input to both particle theory and cosmology.

Kilogram scale throughput performance of the KATRIN tritium handling system

The Karlsruhe Tritium Neutrino (KATRIN) experiment aims to determine the effective mass of the electron antineutrino by investigating the tritium β-spectrum close to the energetic endpoint. To achieve this, there are stringent and challenging requirements on the stability of the gaseous tritium source. The tritium loop system has the task to provide the <0.1 % stabilized flow rate of tritium gas into the KATRIN source with a throughput of 40 g/day and a tritium purity>95 %. KATRIN started full tritium operation in early 2019. This paper focusses on the observed radiochemical effects and confirms that non-negligible quantities during initial tritium operation have to be expected.

Characterization of silicon drift detectors with electrons for the TRISTAN project

Sterile neutrinos are a minimal extension of the standard model of particle physics. A promising model-independent way to search for sterile neutrinos is via high-precision β-spectroscopy. The Karlsruhe tritium neutrino (KATRIN) experiment, equipped with a novel multi-pixel silicon drift detector focal plane array and read-out system, named the TRISTAN detector, has the potential to supersede the sensitivity of previous laboratory-based searches. In this work we present the characterization of the first silicon drift detector prototypes with electrons and we investigate the impact of uncertainties of the detector’s response to electrons on the final sterile neutrino sensitivity.