Three classes of giant magnetoresistance Co(1 nm)/Cu(2.1 nm) multilayers were sputter grown with different microstructures in respect to grain size and interface roughness, depending on deposition conditions. Magnetization and current in-plane giant-magnetoresistance (GMR) isothermal loops reveal an unusually high increase of coercivity from 280 down to 5 K. In addition, a systematic variation was observed in the temperature dependence of the indirect exchange coupling as the Co–Cu layering is modified in the three classes of Co/Cu multilayers. Specifically, the temperature dependence of the saturation (switching) field in the GMR-loops, and the indirect coupling strength, vary as (T/T0)/sinh(T/T0) whereas the spin-blocking temperature T0 is found equal to 84(4), 96(11), and 105(10) K for class A, B, and C multilayers, respectively. These results indicate that the desirable low hysteresis appears in the GMR loops at room temperature because the spin structure becomes unstable above the obtained T0 due to domain wall fluctuations. Such magnetic fluctuations define a short–range order state above T0 that depends on Co–Cu intermixing and geometric factors of the grains.
Read full abstract