Ion Number Density Research Articles

Adsorption and energy storage characteristics of ionic liquids in porous zeolite-templated carbon materials

The energy storage capacity of supercapacitors is closely related to the capacity of their electrode materials to adsorb electrolytes. Porous zeolite-templated carbon (ZTC) materials are a type of porous carbon material with a well-defined spatial structure and are thus promising electrode materials. This study utilizes molecular dynamics simulations to compare the ion number density and charge density distributions of the [EMI][BF4] ionic liquid for various ZTC materials, while also examining the ion adsorption characteristics for different electrode charges. Parameters such as the degree of confinement (DOC) and the charge compensation per carbon (CCpC) are introduced to represent the ion adsorption and charge storage capacity of the materials, with a higher DOC indicating a greater number of encapsulated ions and a higher CCpC indicating a more efficient charge storage. The findings suggest that materials with a larger pore size tend to exhibit increased ion adsorption. However, many CCpC adsorption sites that can store more charge are then found in positions with a smaller DOC. This work unveils the ion adsorption characteristics of ZTC materials in charged electrode and presents the differential capacitance curves of various materials, thereby providing a theoretical foundation for the utilization of ZTC materials as electrodes in supercapacitors.

Photoionization ion mobility analyzer for on-site measurement of exhaled acetone by coupling miniature thermoelectric cooling dehydration

The breath concentration of acetone holds significant clinical importance, the development of on-site and accurate analyzer for exhaled acetone is highly demanded. A photoionization ion mobility analyzer based on a low-pressure krypton discharge lamp has been developed for direct and rapid determination of the acetone concentration. The difficulty for sensitive measurement of acetone by vacuum ultraviolet photoionization was the strong absorption of water molecules in the breath air. An online dehydration device with a miniature thermoelectric cooling quartz trap has been developed, which was capable for reducing the relative humidity from over 90 % to below 1 %. The dehydration could enhance the signal intensity of acetone about 85 times. The response time of current thermoelectric cooling dehydration was only 1/20 of the Nafion tube dehydration. A limit of detection 0.02 ppmV and linear response up to 2.0 ppmV were achieved. The interferences from ammonia in exhaled breath was eliminated using a calibration method based on ion number density, achieving recoveries ranging from 90 % to 110 %. In the final, the variation trends of exhaled acetone level in healthy individuals following the ingestion of glucose under fasting conditions were carried out to demonstrate the potential application of the analyzer.

Construction of Kinetic Model of Vacuum Arc Magnetic Fluid Under External Magnetic Field

The external magnetic field is an important control method of vacuum arc at present. Because of its high efficiency and economy, it has become an important method to study the kinetic model of vacuum arc magnetic fluid. Therefore, the kinetic model of vacuum arc magnetic fluid under the external magnetic field is constructed. Firstly, the mass conservation equation, radial momentum conservation equation, axial momentum conservation equation, energy conservation equation, electromagnetic equations are analyzed. The boundary conditions of the dynamic model are cathode boundary, anode boundary and fluid wall boundary. The fluid dynamics calculation software FLUENT is used as the calculation platform, and its secondary development is carried out. Combining VC++self-programming and self-defined macro functions, according to the boundary conditions, the kinetic model of vacuum arc magnetic fluid under external magnetic field is solved, and the kinetic model analysis of vacuum arc magnetic fluid under external magnetic field is realized. Experimental analysis shows under the action of longitudinal magnetic field, the intensity of longitudinal magnetic field increases, the maximum point of ion rotation speed in the magnetic fluid of vacuum arc moves outward along the edge of vacuum arc, the number density of electrons gradually moves from the central axis to the radial direction, and the high density area increases first and then decreases; Under the action of transverse magnetic field, the intensity of transverse magnetic field increases, the ion pressure in vacuum arc magnetic fluid gradually shifts and increases, and the ion number density also increases.

Three-dimensional transient modeling and simulation of high-current multi-component vacuum arc under transverse magnetic field

This paper established a three-dimensional transient MHD model of a high-current multi-component vacuum arc under a transverse magnetic field (TMF) to simulate the dynamic characteristics of plasma parameters in the uniform motion mode of a contracted arc under lower TMF. The model considered the ionization–recombination process among the multi-components and used the P1 model to calculate the thermal radiation losses. The simulation results show that the ion number density of The TMF arc is on the order 1024 m−3, and when the plasma temperature reaches 4.3 eV, the effects of thermal radiation cannot be ignored. The majority of the plasma from the cathode and anode undergo acceleration and then deceleration before finally intersecting at the center of the arc, creating an extreme value of the density and the pressure, where a large amount of kinetic energy is converted into internal energy. The arc will be bent and deflected under the action of the ampere force, and the deflection of Cu3+ is especially obvious. The TMF affects the collision strength of the jet in the intersection area and, thus, affects the ion density, in which the change of Cu2+ is dominant. The ionization–recombination process of ions is mainly determined by the electron temperature, which is affected by the arc current. As the current decreases, Cu1+ increases and Cu2+ and Cu3+ decrease, and the change in ionization rate is the main reason for the change in the proportion of each ionic component; the heat flux density to the anode and cathode is on the order of 1010 W/m2, which heats the front of the arc and ensures the stable movement of the arc. Meanwhile, due to the high ion number density, the ion heat flux accounts for the main part of the heat flux, and the anode exhibits a higher proportion of ion heat flux.

Dust particle surface potential in an argon-helium plasma using the (r,q)-distribution function

Abstract In this paper, the dust particle surface potential for argon-helium plasma is evaluated analytically and numerically in the context of negatively charged dust particles by employing a power-law r , q -distribution function. Recent studies have reported the argon-helium plasma and conducted a brief theoretical and experimental survey. To deepen our understanding further, this study aims to analyze the argon-helium plasma comprehensively using the same pattern but with the r , q -distribution function. For this purpose, the current balance equations are derived for electron, helium and argon ions, when these charge species attain the quasineutrality condition. We numerically examined the currents of plasma species for a broad range of effective distribution function parameters r and q . It is revealed that the surface potential of dust particles is significantly affected by the parameters r and q , helium ion-to-electron temperature ratio, argon ion-to-electron temperature ratio, and helium ion to argon ion number density ratio. By incorporating the multi-ion (argon-helium) species, the significance of low-temperature non-Maxwellian dusty (complex) plasma is briefly examined.

Analytical modeling of nucleation and growth of graphene layers on CNT array and its application in field emission of electrons

Carbon Nanotube (CNT) arrays and graphene have undergone several investigations to achieve efficient field emission (FE) owing to CNT’s remarkable large aspect ratio and graphene’s exceptional FE stability. However, when dense CNT arrays and planar graphene layers were used as field emitters, their field enhancement factor reduced dramatically. Therefore, in this paper, we numerically analyze the growth of a dense CNT array with planar graphene layers (PGLs) on top, resulting in a CNT-PGL hybrid and the associated field enhancement factor. The growth of the CNT array is investigated using Plasma Enhanced Chemical Vapor Deposition (PECVD) chamber in C2H2/NH3 environment with variable C2H2 flow, Ni catalyst film thickness, and substrate temperature followed by PGL precipitation on its top at an optimized cooling rate and Ni film thickness. The analytical model developed accounts for the number density of ions and neutrals, various surface elementary processes on catalyst film, CNT array growth, and PGLs precipitation. According to our investigation, the average growth rate of CNTs increases and then decreases with increasing C2H2 flow rate and catalyst film thickness. CNTs grow at a faster rate when the substrate temperature increases. Furthermore, as the chamber temperature is lowered from 750 °C to 250 °C in N2 environment and Ni film thickness grows, the number of the graphene layers increases. The field enhancement factors for the CNT array and hybrid are then calculated based on the optimal parameter values. The average height of the nanotubes, their spacing from one another, and the penetration of the electric field due to graphene coverage are considered while computing the field enhancement factor. It has been found that adding planar graphene layers to densely packed CNTs can raise its field enhancement factor. The results obtained match the current experimental observations quite well.

Two-dimensional investigation of characteristic parameters and their gradients for the self-generated electric and magnetic fields of laser-induced zirconium plasma

Two-dimensional diagnosis of laser-induced zirconium (Zr) plasma has been experimentally performed using the time-of-flight method by employing Faraday cups in addition to electric and magnetic probes. The characteristic parameters of laser-induced Zr plasma have been evaluated as a function of different laser irradiances ranging from 4.5 to 11.7 GW cm−2 at different axial positions of 1–4 cm with a fixed radial distance of 2 cm. A well-supporting correlation between the plume parameters and the laser-plasma-produced spontaneous electric and magnetic (E and B) fields was established. The measurements of the characteristic parameters and spontaneously induced fields were observed to have an increasing trend with the increasing laser irradiance. However, when increasing the spatial distance in both the axial and radial directions, the plasma parameters (electron/ion number density, temperature and kinetic energy) did not show either continuously increasing or decreasing trends due to various kinetic and dynamic processes during the spatial evolution of the plume. However, the E and B fields were observed to be always diffusing away from the target. The radial component of electron number densities remained higher than the axial number density component, whereas the axial ion number density at all laser irradiances and axial distances remained higher than the radial ion number density. The higher axial self-generated electric field (SGEF) values than radial SGEF values are correlated with the effective charge-separation mechanism of electrons and ions. The generation of a self-generated magnetic field is observed dominantly in the radial direction at increasing laser irradiance as compared to the axial one due to the deflection of fast-moving electrons and the persistence of two-electron temperature on the radial axis.

Effect of trapping of electrons and positrons on the evolution of shock wave in magnetized plasma: A complex trapped K-dV burgers’ equation

Our research demonstrates that positive and negative ions, along with trapped electrons and positrons, propagate as small-amplitude electrostatic shock waves in a magnetized collisions-less plasma. The trapped Korteweg-de Vries Burger's (T-KdVB) equation was derived by the widely recognized standard reductive perturbation technique (RPT), employing two separate scales of standard coordinates. The study examines the impact of temperature ratio on the shock wave characteristics of positive and negative ions, as well as positrons with electrons. The analysis and discussion focus on the impacts of negative ion number densities, as well as the number densities of electrons and positrons. The T-KdVB equations are responsible for governing rarefactive shock waves. Additionally, it is important to acknowledge that nonlinearity and dissipation play a key role in controlling the amplitude of the shock.

Improving the Sensitivity and Linear Range of Photoionization Ion Mobility Spectrometry via Confining the Ion Recombination and Space Charge Effects Assisted by Theoretical Modeling.

Photoionization (PI) is an efficient ionization source for ion mobility spectrometry (IMS) and mass spectrometry. Its hyphenation with IMS (PI-IMS) has been employed in various on-site analysis scenarios targeting a wide range of compounds. However, the signal intensity and linear dynamic range of PI-IMS at ambient pressure usually do not follow the Beer-Lambert law predictions, and the factors causing that negative deviation remain unclear. In this work, a variable pressure PI-IMS system was developed to examine the ion loss effects from factors like ion recombination and space charge by varying its working pressure from 1 to 0.1 bar. Assisted by theoretical modeling, it was found that ion recombination could contribute up to 90% of signal intensity loss for ambient pressure PI-IMS setups. Lowering the pressure and increasing the electric field in PI-IMS helped suppress the ion recombination process and thus an optimal pressure Poptimal appeared for best signal intensity, despite the decreased net ion number density and the increased space charge effect. A simplified theoretical equation taking ion recombination as the primary ion loss factor was derived to link Poptimal with analyte concentration and electric field in PI-IMS, enabling a swift optimization of the PI-IMS performance. For example, compared to ambient pressure, PI-IMS at a Poptimal of 0.4 bar provided a signal intensity increment of more than 400% for 0.716 ppmv toluene and also expanded the linear dynamic range by more than two times. Revealing factors influencing the PI-IMS response would also benefit the applications of other chemical ionization sources in IMS or mass spectrometry (MS).

Effect of Interlayer Spaces and Interfacial Structures on High-Performance MXene/Ionic Liquid Supercapacitors: A Molecular Dynamics Simulation.

The combination of high-capacitance MXenes and wide-electrochemical-window ionic liquids (ILs) has exhibited bright prospects in supercapacitors. Several strategies, such as surficial functionalization and interlayer spacing tuning, have been used to enhance the electrochemical performance of supercapacitors. However, the lack of theoretical guidance on these strategies, including the effects of the microenvironment in the interlayer of confined ILs, hindered the further exploration of such devices. Herein, we performed molecular dynamics simulations to comprehensively investigate the effects of the interlayer space and surface terminations of MXene electrodes on capacity. The results show that the electrical double layer (EDL) structure was found to form on the interface between the MXene electrode and ILs electrolyte by analyzing the ion number density and charge density in the nanometer confined spaces. Under the same potential, the -OH terminations significantly impact the ion orientation in the EDL, particularly near the electrode surface, where cations tend to align vertically, allowing the retention of more cations at the electrode surfaces. Interestingly, such an orientation distribution was decisively from the hydrogen bonds expressed by O-H···O between the -OH termination of MXene and -OH groups of ILs. The differential capacitances of the supercapacitors were calculated by the surficial electron density, and it showed that the capacitance is a nearly one-quarter increase in the 14 Å interlayer spacing compared with that of 10 Å under an applied potential of 2 V. At the same time, the Ti3C2(OH)2 electrode had a higher differential capacitance than the Ti3C2O2 electrode, which possibly originates from the stronger hydrogen bonds to contribute to the vertical aggregation of the cations. Our results highlighted the roles of the interlayer spacing distance and surface terminations of the MXene on the performance of the type of supercapacitor.

Multi-ion magnetized sheath properties with non-extensive electron distribution

Magnetized plasma sheath plays an important role in semiconductor processing, material surface modification, film deposition, etc. In plasma experiments and discharge applications, multi-ion plasma consisting of more than two kinds of ions often exists. For a long range interacting plasma system, non-Maxwellian electrons can be described by the non-extensive distribution of Tsallis. In this work, a fluid model with one-dimensional spatial coordinates and three-dimensional velocity coordinates is established for the multi-ion plasma sheath. It is assumed that the electron velocity in the sheath follows a non-extensive distribution, and the background helium ions and different kinds of impurity ions are magnetized in a magnetic field with a certain tilt angle. The effects of non-extensive parameters, impurity ions and oblique magnetic field on the number density, velocity, wall potential and kinetic energy of ions in the multi-ion magnetic sheath are investigated by numerical simulation. The results show that in the helium-hydrogen or helium-argon mixed plasma sheath, the ionic velocity along the vertical wall direction decreases with the increase of the non-extensive parameters, the number density of ions and electrons in the sheath, the sheath thickness , and the kinetic energy of ions at the wall decrease. When the concentration of impurity ions increases, the kinetic energy of ions on the wall is independent of the type of ions. With the increase of magnetic field intensity, the number density of helium ions and the velocity along the vertical wall fluctuate along the sheath edge, and the fluctuation amplitude increases with the decrease of non-extensive parameters, while the heavy ions have no obvious fluctuation. In addition, the effects of the types and concentrations of impurity ions on the related properties of the sheath are also analyzed. With the increase of the magnetic field intensity, the number density and the velocity along the vertical wall direction fluctuate at the sheath edge, and the fluctuation amplitude increases with the decrease of the non-extensive parameter, whereas there are no significant fluctuations for heavy ions. In addition, when impurity ions are heavy ions, the absolute value of wall potential increases with the increase of impurity ion concentration and the decrease of non-extensibility parameters, and the kinetic energy of background ions increases at the wall surface. When the impurity ion is a light ion, the absolute value of the wall potential decreases with the increase of the impurity ion concentration and the decrease of the non-extensibility parameter, and the kinetic energy of the background ion at the wall decreases.

Non-equilibrium steady states of electrolyte interfaces

The non-equilibrium steady states of a semi-infinite quasi-one-dimensional univalent binary electrolyte solution, characterised by non-vanishing electric currents, are investigated by means of Poisson-Nernst-Planck (PNP) theory. Exact analytical expressions of the electric field, the charge density and the number density are derived, which depend on the electric current density as a parameter. From a non-equilibrium version of the Grahame equation, which relates the total space charge per cross-sectional area and the corresponding contribution of the electric potential drop, the current-dependent differential capacitance of the diffuse layer is derived. In the limit of vanishing electric current these results reduce to those within Gouy-Chapman theory. It is shown that improperly chosen boundary conditions lead to non-equilibrium steady state solutions of the PNP equations with negative ion number densities. A necessary and sufficient criterion on surface conductivity constitutive relations is formulated which allows one to detect such unphysical solutions.

Electrochemical properties of a novel EDLC derived from plasticized biopolymer based electrolytes with valuable energy density close to NiMH batteries

This study introduces a novel system of solid electrolytes for electrical double-layer capacitors (EDLCs) utilizing biopolymer electrolytes with high energy density comparable to NiMH batteries. To prepare the electrolytes, a proton-conducting plasticized chitosan: poly(2-oxazoline) (POZ) with good film-forming properties was fabricated using a solution casting technique, and ammonium trifluoromethanesulfonate (NH4CF3SO3) salt was employed as a proton provider. Various glycerol concentrations were incorporated into the chitosan:POZ: NH4CF3SO3 system to enhance the ionic conductivity and fully transparent films were obtained. The impedance technique was utilized to determine the conductivity and measure the diffusion coefficient, mobility, and number density of ions. The electrochemical measurements, including linear sweep voltammetry (LSV) and cyclic voltammetry (CV), validated the high performance of the system. The EDLC was examined using galvanostatic charge-discharge (GCD) equipment, and the results revealed an energy density of 43 Wh/kg, specific capacitance of 300 F/g, and power density of 1800 W/kg over 500 cycles. These findings suggest that it is plausible to develop EDLCs that resemble batteries, making them a more desirable energy storage option for the industry.

Influence of Crustal Magnetic Fields on Horizontal Plasma Transport and Ion Escape on Mars

Owing to its unevenly distributed crustal fields, Mars acts as a unique obstacle to the solar wind. In the presence of the crustal fields, the transport of the planetary ions on the dayside ionosphere exhibits north–south asymmetry. Additionally, the heavy-ion loss in the magnetotail is affected by the crustal fields. In this paper, a three-dimensional multispecies magnetohydrodynamic model is employed to simulate Mars–solar wind interactions. Numerical results indicate that the meridional transport is dominant in most areas on the dayside ionosphere. In the presence of the crustal fields, the meridional transport on the southern hemisphere (southward transport) is reduced by more than 70% above the strong crustal sources, and the zonal velocity shows local changes inside strong and weak crustal field regions. These effects result in an increase or decrease in the number density of the heavy ions reaching the terminator, thereby influencing the thickness of the ionosphere. Decreased southward velocity leads to a reduction in the heavy-ion loss on the southern magnetotail. The radial outward flux is reduced by more than 30% for O2 + and CO2 + and by 10% for O+. This study shows that in addition to the zonal transport, the meridional transport is important for the day-to-night transport on the dayside of Mars. Collectively, the horizontal plasma transport, controlled by crustal fields, is associated with the altered ionosphere structure and reduced heavy-ion loss in the magnetotail.

The Long‐Term Flux of the Solar Wind Suprathermal Ions That Precipitate on the Lunar Surface

AbstractSolar wind ions weather the optical, physical, and chemical properties of the lunar surface. While the solar wind ion number density is dominated by the thermal population, the study of suprathermal ions is important to understand weathering effects that may develop at depth larger than the penetration depth of the bulk solar wind. Possible manifestations of suprathermal ion weathering include the creation of thick amorphous rims, contamination of isotopic ratios at depth, and alteration of the optical reflectance at infrared wavelengths. Furthermore, while the thermal population forms a beam parallel to the ecliptic plane, suprathermal ions may have a large northward or southward velocity component and can therefore directly access and weather the lunar polar regions, including the interiors of the Permanently Shadowed Regions (PSRs). In this article, we constrain the long‐term properties of the solar wind suprathermal ions using 17 years of observations by the SupraThermal Ion Composition Spectrometer onboard the Wind spacecraft (Wind‐STICS). We find that the 17‐year omnidirectional energy spectra of protons, helium ions, and oxygen ions observed by Wind‐STICS are in excellent agreement with the 11‐month estimates published by Mewaldt et al. (2001, https://doi.org/10.1063/1.1433995) and Mewaldt et al. (2007, https://doi.org/10.1007/978-0-387-74184-0_32). This agreement validates the conclusions of Nénon and Poppe (2020, https://doi.org/10.3847/PSJ/abbe0c) who proposed that suprathermal ions heavier than helium may increase the rate of amorphous rim formation in lunar samples by 50%. Furthermore, the Wind‐STICS observations of out‐of‐ecliptic ions reveal that the lunar PSRs are weathered by the same flux of >15 keV/nucleon as anywhere else on the lunar surface.

A linear parameters study of ion cyclotron emission using drift ring beam distribution

Ion Cyclotron Emission (ICE) holds great potential as a diagnostic tool for fast ions in fusion devices. The theory of Magnetoacoustic Cyclotron Instability (MCI), as an emission mechanism for ICE, states that MCI is driven by a velocity distribution of fast ions that approximates to a drift ring beam. In this study, the influence of key parameters (velocity spread of the fast ions, number density ratio, and instability propagation angle) on the linear MCI is systematically investigated using the linear kinetic dispersion relation solver BO (Xie 2019 Comput. Phys. Commun. 244 343). The computational spectra region considered extends up to 40 times the ion cyclotron frequency. By examining the influence of these key parameters on MCI, several novel results have been obtained. In the case of MCI excited by super-Alfvénic fast ions (where the unique perpendicular speed of fast ion is greater than the perpendicular phase velocity of the fast Alfvén waves), the parallel velocity spread significantly affects the bandwidth of harmonics and the continuous spectrum, while the perpendicular velocity spread has a decisive effect on the MCI growth rate. As the velocity spread increases, the linear relationship between the MCI growth rate and the square root of the number density ratio transitions to a linear relationship between the MCI growth rate and the number density ratio. This finding provides a linear perspective explanation for the observed linear relation between fast ion number density and ICE intensity in JET. Furthermore, high harmonics are more sensitive to changes in propagation angle than low harmonics because a decrease in the propagation angle alters the dispersion relation of the fast Alfvén wave. In the case of MCI excited by sub-Alfvénic fast ions (where the unique perpendicular speed of fast ion is less than the perpendicular phase velocity of the fast Alfvén waves), a significant growth rate increase occurs at high harmonics due to the transition of sub-Alfvénic fast ions to super-Alfvénic fast ions. Similarly, for MCI excited by greatly sub-Alfvénic fast ions (where the unique perpendicular speed of fast ion is far less than the perpendicular phase velocity of the fast Alfvén waves), the growth rate at high harmonics also experiences a drastic increase compared to the low harmonic, thereby expanding the parameter range of the velocity spread.

Ion transport in thermally responsive pectin film

The ionic conductivity of CaCl2-crosslinked pectin was found to exhibit a record-high temperature response, suggesting its potential applications in wearable devices and infrared sensors [R. Di Giacomo et al., Sci. Rob. 2, eaai9251 (2017)]. However, little was known about its ion conduction mechanisms and the origin of its high-temperature sensitivity. In this study, we perform controlled experiments and identify calcium ions as the dominant current carriers. By analyzing infrared spectra at different temperatures, we find that the temperature response is due to changes in ion mobility, rather than variations in ion number density. We compare measurements and modeling results of nine different multivalent ions and find a positive correlation between their temperature responses and their binding energy to pectin. While these findings are fundamental in nature, they provide relevant guidance for the future design of temperature-sensitive polymers and other materials for organic electronics.

Measurement of Ion Energy Distribution Function of Fast Plasma Flow Driven by Plasma Focus Device Using Retarding Field Energy Analyzer

To understand the mechanism of particle acceleration in collisionless shocks, generating a collisionless plasma flowing through dilute gas is required. We have proposed a compact plasma focus (CPF) device to generate collisionless plasma by using pulsed-power discharge. To discuss a particle acceleration process in collisionless shocks, it is necessary to evaluate an ion energy distribution function (IEDF) of the plasma. In this study, we measured the IEDF of the plasma flow using a retarding field energy analyzer (RFA). The experimental results measured by the RFA showed that ions with a few eV are dominant in the plasma flow generated by the CPF device. The IEDF could be fitted with the shifted Maxwellian distribution. The plasma parameters were estimated to be the ion number density ni = 4.6+−00..28 × 1019 m−3, the ion temperature Ti = 0.8+−00..64 eV, and the drift velocity vd = 11+−03..55 km/s. The estimated velocity approximately agreed with the result of a time-of-flight method calculated by the ion current waveform.

The magnetic field design of a solenoid for the cold-cathode Penning ion source of a miniature neutron tube

A high-yield and beam-stable neutron tube can be applied in many fields. It is of great significance to the optimal external magnetic field intensity of the cold-cathode Penning ion source (PIS) and precisely controls the movement of deuterium (D), tritium (T) ions and electrons in the source of the neutron tubes. A cold-cathode PIS is designed based on the solenoidal magnetic field to obtain better uniformity of the magnetic field and higher yield of the neutron tube. The degree of magnetic field uniformity among the magnetic block, double magnetic rings and solenoidal ion sources is compared using finite element simulation methods. Using drift diffusion approximation and a magnetic field coupling method, the plasma distribution of hydrogen and the relationship between plasma density and magnetic field intensity at 0.06 Pa pressure and a solenoid magnetic field are obtained. The results show that the solenoidal ion source has the most uniform magnetic field distribution. The optimum magnetic field strength of about 0.1 T is obtained in the ion source at an excitation voltage of 1 V. The maximum average number density of monatomic hydrogen ions (H+) is 1 × 108 m−3, and an ion-beam current of about 14.51 μA is formed under the −5000 V extraction field. The study of the solenoidal magnetic field contributes to the understanding of the particle dynamics within the PIS and provides a reference for the further improvement of the source performance of the neutron tube in the future.

Fluid-chemical modeling of the near-cathode sheath formation process in a high current broken in DC air circuit breaker

When the contacts of a medium-voltage DC air circuit breaker (DCCB) are separated, the energy distribution of the arc is determined by the formation process of the near-electrode sheath. Therefore, the voltage drop through the near-electrode sheath is an important means to build up the arc voltage, which directly determines the current-limiting performance of the DCCB. A numerical model to describe the near-electrode sheath formation process can provide insight into the physical mechanism of the arc formation, and thus provide a method for arc energy regulation. In this work, we establish a two-dimensional axisymmetric time-varying model of a medium-voltage DCCB arc when interrupted by high current based on a fluid-chemical model involving 16 kinds of species and 46 collision reactions. The transient distributions of electron number density, positive and negative ion number density, net space charge density, axial electric field, axial potential between electrodes, and near-cathode sheath are obtained from the numerical model. The computational results show that the electron density in the arc column increases, then decreases, and then stabilizes during the near-cathode sheath formation process, and the arc column’s diameter gradually becomes wider. The 11.14 V–12.33 V drops along the 17 μm space charge layer away from the cathode (65.5 kV/m–72.5 kV/m) when the current varies from 20 kA–80 kA. The homogeneous external magnetic field has little effect on the distribution of particles in the near-cathode sheath core, but the electron number density at the near-cathode sheath periphery can increase as the magnetic field increases and the homogeneous external magnetic field will lead to arc diffusion. The validity of the numerical model can be proven by comparison with the experiment.