Diamond crystals have garnered significant attention for applications in photonics, owing to their characteristics of ultra-high thermal conductivity, extremely broad spectral transmission range, and high Raman gain coefficient. These characteristics are particularly advantageous for the development of high-power, multi-wavelength lasers. In this work, we utilize single crystal diamond as a Raman gain medium, for intracavity wavelength-conversion of emission from a side-pumped, electro-optically Q-switched Nd:YAG module. Cascaded Raman conversion is demonstrated and dual-wavelength, pulsed laser emission at wavelengths of 1.2 μm (first-Stokes wavelength) and 1.5 μm (second-Stokes wavelength) is achieved (with a maximum combined pulse energy of 6.19 mJ). The relative ratio of output energy at the two Stokes orders could be varied by tuning the characteristics of the output coupling mirror and the length of the laser resonator. When operating at maximum pump power, the pulse width of the second-Stokes field was approximately half that of the first-Stokes field (second-Stokes ∼10 ns, first-Stokes ∼18 ns), resulting in maximum peak powers of 174 kW (at 1.2 μm) and 220 kW (at 1.5 μm). To the best of our knowledge, this is the highest reported peak power generated from a dual-wavelength, intracavity diamond Raman laser. This work highlights the diversity and utility of diamond as an effective wavelength-conversion component in high-power lasers, and stands as the current state-of-the-art in high pulse-energy, high peak-power, multi-wavelength intracavity Raman lasers.
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