Intense X-ray Source Research Articles

Generation of attosecond gigawatt soft x-ray pulses through coherent Thomson backscattering.

Collision between relativistic electron sheets and counterpropagating laser pulses is recognized as a promising way to produce intense attosecond x rays through coherent Thomson backscattering (TBS). In a double-layer scheme, the electrons in an ultrathin solid foil are first pushed out by an intense laser driver and then interact with the laser reflected off a second foil to form a high-density relativistic electron sheet with vanishing transverse momentum. However, the repulsion between these concentrated electrons can increase the thickness of the layer, reducing both its density and subsequently the coherent TBS. Here, we present a systematic study on the evolution of the flying electron layer and find that its resulting thickness is determined by the interplay between the intrinsic space-charge expansion and the velocity compression induced by the drive laser. How the laser driver, the target areal density, the reflector, and the collision laser intensity affect the properties of the produced x rays is explored. Multidimensional particle-in-cell simulations indicate that employing this scheme in the nonlinear regime has the potential to stably produce soft x rays with several gigawatt peak power in hundreds of terawatt ultrafast laser facilities. The pulse duration can be tuned to tens of attoseconds. This compact and intense attosecond x-ray source may have broad applications in attosecond science.

X-ray computed tomography of the periodically moving object

X-ray computed tomography is a standard method of non-destructive testing of a wide range of static objects. In recent years, time-dependent tomography has been on the rise, for which it is necessary to acquire a series of tomographic data covering the event of interest. For slower processes, conventional laboratory X-ray computed tomography (CT) scanners can be used, while when events are faster, a very intense X-ray source is usually required. For high resolution requirements, the need for an intense X-ray source leads to the use of a synchrotron. An exception is tomographic tracking of periodic events. As will be shown, for these, a good quality reconstruction can be achieved even in the case of a relatively low-intensity X-ray source. To avoid blurring of the individual X-ray images by the motion of the object, the exposure time must be reasonably short. At motion rates of units of Hz, this time cannot be longer than tens of ms, this requirement naturally leads to low data statistics. Sufficient statistics is achieved by integrating images taken at an identical position of the moving object. A key requirement of such an approach is the precise synchronization of all active components of the system. The imaging detector must be capable of taking images on demand by hardware triggering with the capability of adequately short exposures. The ability of the CT system to investigate periodically moving objects will be demonstrated on the object oscillating harmonically at 3.81 Hz.

A fully dynamical description of time-resolved resonant inelastic X-ray scattering of pyrazine.

Recent advancements in ultrashort and intense X-ray sources have enabled the utilisation of resonant inelastic X-ray scattering (RIXS) as a probing technique for monitoring photoinduced dynamics in molecular systems. To account for dynamic phenomena like non-adiabatic transitions across the relevant electronic state manifold, a time-dependent framework is crucial. Here, we introduce a fully time-dependent approach for calculating transient RIXS spectra using wavepacket dynamics simulations, alongside an explicit treatment of the X-ray probe pulse that surpasses Kramers-Heisenberg-Dirac constraints. Our analysis of pyrazine at the nitrogen K-edge underscores the importance of considering nuclear motion effects in all electronic states involved in the transient RIXS process. As a result, we propose a numerically exact approach to computationally support and predict cutting-edge time-resolved RIXS experiments.

Proposal for Observing XUV-Induced Rabi Oscillation Using Superfluorescent Emission.

Intense x-ray and extreme ultraviolet (XUV) light sources have been available for decades, however, due to weak nonlinear interaction in the XUV photon energy range, observation of Rabi oscillation induced by XUV pulse remains a very challenging experimental task. Here we suggest a scheme where photoionization of a He medium by an intense XUV pump pulse is followed by a strong population inversion and Rabi oscillation at the He^{+}(1s-3p) transition and is accompanied by superfluorescence (SF) of the 7.56eV pulse at the He^{+}(3p-2s) transition. Our numerical simulations show that the Rabi oscillation at the He^{+}(1s-3p) transition induced by an XUV pulse with photon energy 48.36eV results in significant signatures in the SF spectra, allowing us to identify and characterize the XUV induced Rabi-oscillatory regime. The proposed scheme provides a sensitive tool to monitor and control ultrafast nonlinear dynamics in atoms and molecules triggered by intense XUV.

UV Photoelectron Spectroscopy of Aqueous Solutions.

ConspectusKnowledge of the electronic structure of an aqueous solution is a prerequisite to understanding its chemical and biological reactivity and its response to light. One of the most direct ways of determining electronic structure is to use photoelectron spectroscopy to measure electron binding energies. Initially, photoelectron spectroscopy was restricted to the gas or solid phases due to the requirement for high vacuum to minimize inelastic scattering of the emitted electrons. The introduction of liquid-jets and their combination with intense X-ray sources at synchrotrons in the late 1990s expanded the scope of photoelectron spectroscopy to include liquids. Liquid-jet photoelectron spectroscopy is now an active research field involving a growing number of research groups. A limitation of X-ray photoelectron spectroscopy of aqueous solutions is the requirement to use solutes with reasonably high concentrations in order to obtain photoelectron spectra with adequate signal-to-noise after subtracting the spectrum of water. This has excluded most studies of organic molecules, which tend to be only weakly soluble. A solution to this problem is to use resonance-enhanced photoelectron spectroscopy with ultraviolet (UV) light pulses (hν ≲ 6 eV). However, the development of UV liquid-jet photoelectron spectroscopy has been hampered by a lack of quantitative understanding of inelastic scattering of low kinetic energy electrons (≲5 eV) and the impact on spectral lineshapes and positions.In this Account, we describe the key steps involved in the measurement of UV photoelectron spectra of aqueous solutions: photoionization/detachment, electron transport of low kinetic energy electrons through the conduction band, transmission through the water-vacuum interface, and transport through the spectrometer. We also explain the steps we take to record accurate UV photoelectron spectra of liquids with excellent signal-to-noise. We then describe how we have combined Monte Carlo simulations of electron scattering and spectral inversion with molecular dynamics simulations of depth profiles of organic solutes in aqueous solution to develop an efficient and widely applicable method for retrieving true UV photoelectron spectra of aqueous solutions. The huge potential of our experimental and spectral retrieval methods is illustrated using three examples. The first is a measurement of the vertical detachment energy of the green fluorescent protein chromophore, a sparingly soluble organic anion whose electronic structure underpins its fluorescence and photooxidation properties. The second is a measurement of the vertical ionization energy of liquid water, which has been the subject of discussion since the first X-ray photoelectron spectroscopy measurement in 1997. The third is a UV photoelectron spectroscopy study of the vertical ionization energy of aqueous phenol which demonstrates the possibility of retrieving true photoelectron spectra from measurements with contributions from components with different concentration profiles.

High granularity resistive Micromegas for high particle rates environment

The new era of particle physics experiments is moving towards new upgrades of present accelerators (Large Hadron Collider at CERN) and the design of high energy (tens/hundreds TeV scale) and very high intensity new particle accelerators (FCC-ee/hh, EIC, Muon Collider). Cost effective, high efficiency particle detection in a high background and high radiation environment is fundamental to accomplish their physics program. We present a new high granularity resistive Micromegas detector capable to ensure full efficient and stable operation and a good tracking capabilities up to particle fluxes of 10 MHz/cm2. A summary of the detector performances, measured by mean of high intensity X-ray, muon and pion sources, is reported, together with most recent results from test beam activities.

Precise wavefront characterization of x-ray optical elements using a laboratory source.

Improvements in x-ray optics critically depend on the measurement of their optical performance. The knowledge of wavefront aberrations, for example, can be used to improve the fabrication of optical elements or to design phase correctors to compensate for these errors. At present, the characterization of such optics is made using intense x-ray sources, such as synchrotrons. However, the limited access to these facilities can substantially slow down the development process. Improvements in the brightness of lab-based x-ray micro-sources in combination with the development of new metrology methods, particularly ptychographic x-ray speckle tracking, enable characterization of x-ray optics in the lab with a precision and sensitivity not possible before. Here, we present a laboratory setup that utilizes a commercially available x-ray source and can be used to characterize different types of x-ray optics. The setup is used in our laboratory on a routine basis to characterize multilayer Laue lenses of high numerical aperture and other optical elements. This typically includes measurements of the wavefront distortions, optimum operating photon energy, and focal length of the lens. To check the sensitivity and accuracy of this laboratory setup, we compared the results to those obtained at the synchrotron and saw no significant difference. To illustrate the feedback of measurements on performance, we demonstrated the correction of the phase errors of a particular multilayer Laue lens using a 3D printed compound refractive phase plate.

The upgraded ALICE TPC

A large Time Projection Chamber (TPC) is the main device for tracking and particle identification in the ALICE experiment at the Large Hadron Collider (LHC) at CERN. In the upcoming Run 3, the LHC will deliver lead beams colliding at an interaction rate of up to 50kHz. In order to read out all minimum bias events in Pb–Pb collisions, the TPC was upgraded with an amplification stage based on Gas Electron Multipliers (GEM) and new front-end electronics. With the new amplification stage, a trigger-less operation of the TPC becomes possible, resulting in a continuous readout without dead time.The exchange of the readout chambers and front-end electronics took place in a dedicated clean room in 2019/20. The upgraded TPC was then moved back to its designated position at the interaction point 2 of the LHC and an extensive commissioning programme was carried out. It includes, inter alia, noise studies, measurements of laser tracks, irradiation of the TPC with an intense X-ray source, the flushing of radioactive 83mKr into the active volume and the operation during the first proton–proton collisions provided by the LHC. During these measurements, the TPC operated at nominal conditions and the continuous readout capability was tested successfully.

Ab initio reconstruction from one-dimensional crystal diffraction data.

Filamentary and rod-like assemblies are ubiquitous in biological systems, and single such assemblies can form one-dimensional (1D) crystals. New, intense X-ray sources, such as X-ray free-electron lasers, make it feasible to measure diffraction data from single 1D crystals. Such experiments would present some advantages, since cylindrical averaging of the diffraction data in conventional fiber diffraction analysis is avoided, there is coherent signal amplification relative to single-particle imaging, and the diffraction data are oversampled compared with those from a 3D crystal so that the phase problem is better determined than for a 3D crystal [Millane (2017). Acta Cryst. A73, 140-150]. Phasing of 1D crystal diffraction data is examined, by simulation, using an iterative projection algorithm. Ab initio phasing is feasible with realistic noise levels and little envelope information is required if a shrink-wrap algorithm is also incorporated. Some practical aspects of the proposed experiments are explored.

Incoherent ultrarelativistic channeling particle scattering by electrons

The problem of high-energy charged particle motion in the field of atomic strings and planes of oriented crystals, widely applied to control large accelerator beams and generate intense gamma radiation, is addressed. Following the previously developed theory of channeled particles incoherent scattering by crystal atom nuclei, we consider here the same by crystal atom electrons. The theory developed takes into consideration all the effects of momentum transfer between fast particles and electrons of atoms in a crystal in the range from the nuclear radius up to the many inter-atomic distances. The theory also includes the temperature-dependent Debye – Waller factor, as well as both the atomic form factors and scattering function, evaluated with the detail consideration of atomic structure. All the modifications of electron scattering in crystals are reduced to the value of the effective minimum momentum transfer, which by an order of value exceeds that one, related with the Bethe – Bloch mean atomic energy. Substituting this quantity to the expression for the mean square of the scattering angle of a classically moving particle makes it possible to compare the scattering by electrons and nuclei, while its joint use with the Rutherford cross section allows for the correct simulations of the planar channeling of positively charged particles in the thickest crystals, supposed to be used for the beam extraction from high energy accelerators, measurement of electromagnetic characteristics of short-living particles and development of intense narrow-band X-ray and gamma radiation sources based on crystal undulators.

X-ray third-order nonlinear asymmetric diffraction in the transmission geometry

For high intensity x-ray sources, the investigations of the nonlinear x-ray effects become essential. The x-ray third-order nonlinear asymmetric transmission case dynamical diffraction is investigated theoretically in perfect crystals. The three essential input parameters are taken into account: the deviation from the Bragg exact orientation, the asymmetry angle of reflecting atomic planes and the intensity of incident wave. The third-order nonlinear equations for the asymmetrical dynamical diffraction and two integrals of motion are presented. The exact solutions for the wave amplitudes, presented via Jacobi elliptic functions, have been found. The solutions are periodic functions of the depth. It is shown that the behavior of the waves inside the crystal is determined by the sign of a combined parameter, which includes the three input parameters, mentioned above. The regions, where this parameter is positive, negative or zero, are found. For positive values, the energy is concentrated both in the transmitted and diffracted waves while for the negative values, the energy is concentrated mainly in the transmitted beam. It is found that when this combined parameter is zero, the amplitudes are elementary periodic or non-periodic functions. For the periodic solutions, the nonlinear Pendellösung effect takes place, i.e. the transmitted and diffracted waves periodically exchange with their energies. For the period, called an extinction length, an exact expression is found. It is shown that for large values of the asymmetry factor, the observation of the nonlinear diffraction effects can be realized for sufficiently low intensities of the incident wave. The obtained results can be used for experimental investigation of the nonlinear Bragg diffraction and for preparation of high intensity x-ray beams with given parameters. The expression for the nonlinear extinction length allows to estimate the third-order nonlinear susceptibilities of crystals by measuring the extinction length in experiments.

Implosion mediated gas-puff hybrid X-pinch

Imploding gas-puff z-pinches are efficient sources of intense x-rays. However, the unpredictable size, number, and location of hot spots along the pinch axis make them unsuitable for applications such as point-projection radiography. Crossed wire or hybrid X-pinches, on the other hand, provide small, localized sources but require fast current rise times and must be reloaded after each pulse. In this Letter, we present the first experimental demonstration of an implosion mediated gas-puff hybrid x-pinch in which an annular gas-puff implosion is shaped and focused onto a pair of conical electrodes separated by a small gap. This setup produces an intense x-ray source with controllable timing that can be operated with or without a central wire. Because the gas-puff implosion time determines the formation of the pinch, this configuration can continue to operate efficiently as a point x-ray source for longer current pulses than conventional x-pinches.

The ThomX ICS source

ThomX is a new generation Compact Compton Source. It is currently commissioned by and at the IJCLab (Laboratoire de physique des 2 infinis - Irène Joliot-Curie (UMR9012)) at Orsay. The first beam is expected at the begining of 2021. The aim of ThomX is to demonstrate the characteristics of an intense and Compact (lab-size) X-ray source based on Compton Scattering. The performances are mostly driven by the laser optical system which is above the state of the art of stored laser power. Proof of principle of various X-ray techniques will be performed thanks to the versatile ThomX beamline. Firstly, this article presents the machine description. Secondly, the issues and limits of the laser system are discussed. Then, the ThomX beamline is described and the machine status conclude the ThomX presentation. Finally, the expected performances for the next years and the possible experiments that can be made with this new machine are detailed.

Monitoring shot-to-shot variations of soft x-ray sources using aluminum foils.

We report a straightforward beam splitter in the soft x-ray spectral range using a thin oxidized aluminum foil. As it allows us to monitor reliably shot-to-shot variations in energy and in energy distribution, this beam splitter is of high interest for the simultaneous use of diagnostics for soft x-rays sources. We measure a transmission of 0.5 and a reflectivity of 0.018 at 22.5° of incidence with a soft x-ray laser working at 32.8 nm. These values are in good agreement with the theory. As the theory predicts a reflectivity and a transmission of both 12% at 52.5° of incidence for 32.8 nm, it can also be useful for experiments that require the division and recombination of a beam, for instance, interferometry or pump-probe technique with an intense soft x-ray source.

Dual-Energy X-ray Medical Imaging with Inverse Compton Sources: A Simulation Study

It has been long recognized that dual-energy imaging could help to enhance the detectability of lesions in diagnostic radiology, by removing the contrast of surrounding tissues. Furthermore, X-ray attenuation is material specific and information about the object constituents can be extracted for tissue characterisation, i.e., to assess whether lesions represent a malignant or benign process. However, a true separation between the low and high energy components is not possible with conventional sources because of their broad X-ray spectrum, and the artifacts produced in the subtracted image can be only partially removed. Finally, dose issues have also prevented so far the application of dual-energy techniques within the clinical context. Very recently, a new intense and monochromatic X-ray source was proposed to fill the gap between a synchrotron radiation facility and the standard X-ray tube. Indeed, inverse Compton scattering (ICS) sources, which are based on the interaction of a powerful laser beam and a bright beam of relativistic electrons, are among the most promising innovative sources of monochromatic X and gamma radiation. In this contribution, we review the main features that allow an ICS source to meet the requirements of a medical imaging application. Specific examples of K-edge subtraction are then provided, to show the potential of ICS in clinical applications that require intravenous injection of a contrast medium.

Enhanced brightness of a laser-driven x-ray and particle source by microstructured surfaces of silicon targets

The production of intense x-ray and particle sources is one of the most remarkable aspects of high energy laser interaction with a solid target. Wide application of these laser-driven secondary sources requires a high yield, which is partially limited by the amount of laser energy absorbed by the target. Here, we report on the enhancement of laser absorption and x-ray and particle flux by target surface modifications. In comparison to targets with flat front surfaces, our experiments show exceptional laser-to-target performance for our novel cone-shaped silicon microstructures. The structures are manufactured via laser-induced surface structuring. Spectral and spatial studies of reflectance and x-ray generation reveal significant increases of the silicon Kα line and a boost of the overall x-ray intensity, while the amount of reflected light decreases. Also, the proton and electron yields are enhanced, but both temperatures remain comparable to those of flat foil targets. We support the experimental findings with 2D particle in cell simulations to identify the mechanisms responsible for the strong enhancement. Our results demonstrate how custom surface structures can be used to engineer high power laser-plasma sources for future applications.

Study of stability in a liner-on-target gas puff Z-pinch as a function of pre-embedded axial magnetic field

Gas puff Z-pinches are intense sources of X-rays and neutrons but are highly susceptible to the magneto-Rayleigh-Taylor instability (MRTI). MRTI mitigation is critical for optimal and reproducible yields, motivating significant attention toward various potential mitigation mechanisms. One such approach is the external application of an axial magnetic field, which will be discussed here in the context of recent experiments on the Zebra generator (1 MA, 100 ns) at the University of Nevada, Reno. In these experiments, an annular Kr gas liner is imploded onto an on-axis deuterium target with a pre-embedded axial magnetic field Bz0 ranging from 0 to 0.3 T. The effect of Bz0 on the stability of the Kr liner is evaluated with measurements of plasma radius, overall instability amplitude, and dominant instability wavelength at different times obtained from time-gated extreme ultraviolet pinhole images. It was observed that the external axial magnetic field does not affect the implosion velocity significantly and that it reduces the overall instability amplitude and the presence of short-wavelength modes, indicating improved pinch stability and reproducibility. For the highest applied Bz0=0.3 T, the stagnation radius measured via visible streak images was found to increase. These findings are consistent with experiments reported in the literature, but here, the Bz0 required for stability, Bz0=0.13 Ipk/R0 (where Ipk is the driver peak current and R0 is the initial radius), is lower. This could be attributed to the smaller load geometry, both radially and axially. Consistent with other experiments, the cause of decreased convergence cannot be explained by the additional axial magnetic pressure and remains an open question.

Peakaboo: Advanced software for the interpretation of X-ray fluorescence spectra from synchrotrons and other intense X-ray sources

Abstract Peakaboo is a platform for the analysis of full spectrum synchrotron X-ray fluorescence (XRF) map data. It offers robust, automated fitting of XRF spectral peaks, increasing the sensitivity to trace chemical elements. Large arrays of spectral data can also be processed into element maps to define spatial relationships. The modifications to Peakaboo introduced since 2017 are particularly designed to help new users to become rapidly competent in the handling of complex XRF spectra. Some of the most important innovations of the software are described below. Finally, we share examples of its application in Earth and Environmental Sciences.

High-Power Ultrashort Pulse Lasers to Pump Plasma-Based Soft X-Ray Lasers

High-energy ultrashort pulse optical lasers operating at high repetition rate are required to drive intense compact coherent soft X-ray sources, including soft X-ray lasers, for applications in nanoscience and nanotechnology, material studies, and high field science. This paper reviews two types of high-power solid-state laser systems developed at Colorado State University to pump compact, high repetition rate, and plasma-based soft X-ray lasers. One is a flashlamp-pumped, petawatt-class Ti:sapphire chirped-pulse amplification laser that generates 0.85 PW pulses of 30 fs duration at 3.3 Hz repetition rate. Using a fraction of the output energy from this laser, we have demonstrated gain-saturated, compact, repetitive lasers down to 6.85 nm in Ni-like Gd and have observed gain in shorter wavelength transitions, down to 5.85 nm in Ni-like Dy. The second type of pump laser is an all diode-pumped chirped-pulse amplification system based on cryogenically cooled Yb:YAG active mirror amplifiers that produces 1 J pulses of picosecond duration at 500 Hz repetition rate. These compact diode-pumped laser systems have enabled new advances in high-average-power tabletop soft X-ray lasers that include 100 Hz demonstrations at wavelengths ranging from 10.9 to 18.9 nm, as well long duration operation at these high repetition rates for periods up to one hour. These and other recent results that include the operation of an 18.9 nm laser Ni-like Mo laser at 400 Hz repetition rate open a path to compact kilohertz repetition rate soft X-ray lasers.

Improvement of harmonic spectra from superposition of initial state driven by homogeneous and inhomogeneous combined field

A larger harmonic cutoff with a higher harmonic yield is a necessary requirement for producing intense ultrashort extreme ultraviolet (XUV) and X-ray sources. In this paper, we present a potential method to improve the harmonic cutoff and harmonic yield from the superposition of initial states in the He atom driven by the low-intensity homogeneous and inhomogeneous combined field. The results can be separated into two parts, that is, (i) the extension of harmonic cutoff via the optimization of three-color homogeneous and inhomogeneous field (covering the carrier envelope phase, delay time, intensity ratio, and inhomogeneous effect); and (ii) the enhancement of harmonic yield via the superposition of ground state and excited state as the initial state. Consequently, a water window harmonic plateau with an intensity enhancement of six orders of magnitude can be obtained. Moreover, the harmonic plateau is contributed by a single harmonic emission peak. Finally, through the Fourier transformation of some selected harmonics on the spectral continuum, a number of sub-50 as water window attosecond pulses with the intensity enhancement of six orders of magnitude can be obtained.