Inelastic Cross Sections Research Articles

Reevaluation of the cosmic antideuteron flux from cosmic-ray interactions and from exotic sources

Cosmic-ray antideuterons could be a key for the discovery of exotic phenomena in our Galaxy, such as dark-matter annihilations or primordial black hole evaporation. Unfortunately the theoretical predictions of the antideuteron flux at Earth are plagued with uncertainties from the mechanism of antideuteron production and propagation in the Galaxy. We present the most up-to-date calculation of the antideuteron fluxes from cosmic-ray collisions with the interstellar medium and from exotic processes. We include for the first time the antideuteron inelastic interaction cross section recently measured by the ALICE collaboration to account for the loss of antideuterons during propagation. In order to bracket the uncertainty in the expected fluxes, we consider several state-of-the-art models of antideuteron production and of cosmic-ray propagation.

A novel formulation of the unintegrated gluon distribution for DIS

We provide a semi-classical description of the inclusive gluon mediated Deep Inelastic Scattering cross section in a way that accounts for the leading powers in both the Regge and Bjorken limits. Our approach thus allows a systematic matching of small and moderate xBj regimes of gluon proton structure functions. We find a new unintegrated gluon distribution with an explicit dependence on the longitudinal momentum fraction x which entirely spans both the dipole operator and the gluonic Parton Distribution Function. Computing this gauge invariant gluon operator on the lattice could allow to probe the energy dependence of the saturation scale from first principles.

Hadron Production Measurements at NA61/SHINE for Precise Determination of Accelerator Neutrino Fluxes

The total systematic uncertainty of the neutrino flux in accelerator-based neutrino experiments is dominated by the Monte Carlo modeling of hadronic interactions. Direct hadron production measurements for T2K and Fermilab neutrino experiments, MINERvA, NOvA and DUNE, are being performed at the NA61/SHINE spectrometer at CERN's Super Proton Synchrotron. Crucial for improving neutrino flux predictions, hadron yields, inelastic and production cross sections are obtained at NA61/SHINE where interactions of various hadron beams with thin and thick (replica) targets are reproduced. Recently obtained results will be reported. An extension of NA61/SHINE's programme of hadron production measurements for neutrino experiments is planned beyond 2020.

HeH+ Collisions with H2: Rotationally Inelastic Cross Sections and Rate Coefficients from Quantum Dynamics at Interstellar Temperatures.

We report for the first time an accurate ab initio potential energy surface for the HeH+–H2 system in four dimensions (4D) treating both diatomic species as rigid rotors. The computed ab initio potential energy point values are fitted using an artificial neural network method and used in quantum close coupling calculations for different initial states of both rotors, in their ground electronic states, over a range of collision energies. The state-to-state cross section results are used to compute the rate coefficients over a range of temperatures relevant to interstellar conditions. By comparing the four dimensional quantum results with those obtained by a reduced-dimensions approach that treats the H2 molecule as an averaged, nonrotating target, it is shown that the reduced dimensionality results are in good accord with the four dimensional results as long as the HeH+ molecule is not initially rotationally excited. By further comparing the present rate coefficients with those for HeH+–H and for HeH+–He, we demonstrate that H2 molecules are the most effective collision partners in inducing rotational excitation in HeH+ cation at interstellar temperatures. The rotationally inelastic rates involving o-H2 and p-H2 excitations are also obtained and they turn out to be, as in previous systems, orders of magnitude smaller than those involving the cation. The results for the H2 molecular partner clearly indicate its large energy-transfer efficiency to the HeH+ system, thereby confirming its expected importance within the kinetics networks involving HeH+ in interstellar environments.

A Theoretical Study of Scattering of Electrons and Positrons by CO2 Molecule

This article presents a theoretical investigation of the differential, integrated, elastic, inelastic, total, momentum-transfer, and viscosity cross-sections, along with the total ionization cross-section, for elastically scattered electrons and positrons from a carbon dioxide (CO2) molecule in the incident energy range of 1 eV ≤Ei≤ 1 MeV. In addition, for the first time, we report the spin polarization of e±−CO2 scattering systems. The independent atom model (IAM) with screening correction (IAMS) using a complex optical potential was employed to solve the Dirac relativistic equation in partial-wave analysis. The comparison of our results with the available experimental data and other theoretical predictions shows a reasonable agreement in the intermediate- and high-energy regions.

Competing ionization and dissociation in the H$$_{2}$$ gerade system

A numerically solvable two-dimensional (2D) model, employed by the authors to study the dissociative recombination of H$_2^+$ in the ungerade symmetry [Phys. Rev. A $\mathbf{98}$, 062706 (2018)], is extended to describe the collision process in the gerade symmetry of H$_2$. In this symmetry the ionization and dissociation processes are driven primarily by the direct, curve-crossing mechanism. The model is represented by a set of three coupled electronic channels in 2D, in the space of $s,p,d$ partial waves of the colliding electron. We demonstrate that the Born-Oppenheimer properties of the H$_2$ molecule in the relevant range of internuclear distances can be described by such a model. The molecular rotational degrees of freedom are accounted for by the rotational frame transformation. The numerical solution of the model is discussed and the resulting rovibrationally inelastic and dissociative recombination cross sections are compared with the available data.

Investigation of rotational (de-)excitation of cyanic acid (HOCN) by collision with He atoms

ABSTRACT The rotational inelastic (de-)excitation of the cyanic acid (HOCN) molecule by collision with helium (He) atoms is studied. A new three-dimensional potential energy surface (3D-PES) for the HOCN−He van der Waals system is given. Explicitly correlated coupled cluster approach with single, double and perturbative triple excitation (CCSD(T)-F12a) in conjunction with augmented-correlation consistent-polarized valence triple zeta (aVTZ) Gaussian basis set is adopted to generate the ab initio 3D-PES. A global minimum with a well depth of 87.59 cm−1 localized at R = 5.9 bohr, θ= 76°, ϕ = 90° is found. Rotational inelastic cross-sections relevant to the 21 first rotational levels (up to $J_{K_aK_c}=8_{08}$) are investigated for total energy up to 550 cm−1 using coupled-states approach. Thermal rate coefficients are obtained for temperatures ranging between 0 and 90 K. |ΔJ| = 1 with |ΔKa| = |ΔKc| = 0 processes are found to be the predominant ones.

Atomic site occupancy of alloying elements and Laves phase stability in γ-γ′ Co-base superalloys

The atomic site occupancy of alloying elements in the ZrCo2 and HfCo2 based Laves phases formed in the Co-9Al-9W-2Zr and Co-9Al-9W-2Hf alloys was experimentally determined by the combined techniques of energy-dispersive X-ray spectroscopy mapping with atomic resolution and the atom location by channeling enhanced microanalysis (ALCHEMI) method. The results show that both Al and W occupy the Zr site in the C15 and the Hf site in the C36 crystal structure. The atomic locations of Al and W were further confirmed by comparing calculated inelastic cross-sections with experimental ALCHEMI results. Using the determined atomic site occupancies of alloying elements, special quasirandom structure solid solution models with 192 atoms were constructed and employed in first-principles calculations. It is found theoretically that the energy of formation of the C15 structure is always lower than that of the C36 structure at 0 K in both ZrCo2 and HfCo2 phases, no matter whether Al and W are incorporated or not. However, further ab initio molecular dynamics simulations suggest that lattice vibration at finite temperature contributes significantly to the phase stability, stabilizing the C36 structure compared to the C15 type for the (Hf, Al, W)Co2 phase at finite temperature, which fits well with the experimental findings.

Cross sections and transport coefficients for electrons in C2H6O and its mixtures with Ar and Ne

In this paper, we show and discuss a set of cross sections for electron collisions with dimethyl ether (DME, C2H6O) obtained by the standard swarm analysis of experimental data for drift velocities and ionization coefficients measured in pure DME and its mixtures with Ar and Ne by E. Oettinger and coworkers. While the existing cross section set gave relatively good predictions for drift velocities, it proved necessary to modify the inelastic cross sections in order to achieve a better agreement with drift velocities in gas mixtures and a good agreement for the ionization coefficient. Furthermore, the derived set of cross sections was used to calculate the electron transport and rate coefficients under the influence of a constant electric field and crossed electric and magnetic DC and RF orthogonal configuration fields. The effect of the magnitude and frequency of the fields on electron transport was studied separately. Our work has resulted in a database of collision and transport data which can be used in modeling of both DC and RF discharges and plasma applications containing pure DME and its mixtures.Graphical abstract

Elastic and Inelastic Cross Sections for Low-Energy Electron Collisions with ClF Molecule Using the R-Matrix Method

The ClF molecule belongs to an interhalogen family and is important in laser physics and condensed phase molecular dynamics. The elastic and excitation scattering cross sections are obtained in a fixed nuclei approximation using the UKRmol+ codes based on R-matrix formalism. The scattering calculations were performed in the static-exchange (SE), static-exchange-plus-polarisation (SEP), and close-coupling (CC) models. Three CC models with different target states were employed, namely, the 1-state, 5-states, and 12-states. In the CC model, the target states were represented by configuration interaction (CI) wavefunctions. A good agreement of dipole and quadrupole moments of the ground state was obtained with the experimental values, which indicates a good representation of the target modelling. The study predicted the existence of a shape resonance in the SE, SEP, and 5-states CC models. This resonance vanished in the 12-states CC model. The excitation cross sections from ground to the lowest two excited states were also reported. The elastic differential and momentum transfer cross sections were obtained in the 12-states CC models. The contribution of long-range interactions to elastic scattering was included via Born closure approach. The quantities like collision frequencies and rate coefficients were also presented over a wide range of electron temperatures. The ionization cross sections were computed using the binary-encounter-Bethe (BEB) model. The results were reported in C2v point group representation.

Improvements in the particle and heavy-ion transport code system (PHITS) for simulating neutron-response functions and detection efficiencies of a liquid organic scintillator

ABSTRACT In this study, we simulated the neutron-response functions and detection efficiencies of a liquid organic scintillator using the particle and heavy-ion transport code system (PHITS). We incorporated the algorithm and database of the neutron-response simulation code SCINFUL–QMD into PHITS. Then, we updated the total, elastic, and inelastic cross-section data of the hydrogen and carbon nuclei for neutrons and developed a new scorer to analyze the light outputs from a scintillator. The calculation results of the neutron-response functions and the detection efficiencies were compared with results of SCINFUL–QMD, the previous PHITS with the new scorer, and the reported measurements. It was found that the improved PHITS successfully reproduced the results calculated by SCINFUL–QMD, except for around 150 MeV where a discontinuity in the detection-efficiency curve was observed in the SCINFUL–QMD values. Our results showed better agreement with the measured data than the results of the previous PHITS. The uncertainties of the detection efficiencies calculated by PHITS using the present extensions were estimated to be approximately 15% for neutrons in the energy region below 100 MeV.

Near-threshold scaling of resonant inelastic collisions at ultralow temperatures

We show that the cross sections for a broad range of resonant {\it inelastic} processes accompanied by excitation exchange (such as spin-exchange, F\"orster resonant, or angular momentum exchange) exhibit an unconventional near-threshold scaling $E^{\Delta m_{12}}$, where $E$ is the collision energy, $\Delta m_{12}=m_1'+m_2'-m_1-m_2$, and $m_i$ and $m_i'$ are the initial and final angular momentum projections of the colliding species ($i=1,\,2$). In particular, the inelastic cross sections for $\Delta m_{12}=0$ transitions display an unconventional $E^0$ scaling similar to that of elastic cross sections, and their rates vanish as $T^{\Delta m_{12}+1/2}$. For collisions dominated by even partial waves (such as those of identical bosons in the same internal state) the scaling is modified to $\sigma_\text{inel}\propto E^{\Delta m_{12} +1} $ if $\Delta m_{12}$ is odd. We present accurate quantum scattering calculations that illustrate these modified threshold laws for resonant spin exchange in ultracold Rb+Rb and O$_2$+O$_2$ collisions. Our results illustrate that the threshold scaling of collision cross sections is determined only by the energetics of the underlying process (resonant vs. exothermic) rather than by whether the internal states of colliding particles is changed in the collision.

TOTEM, recent experimental review

The TOTEM (TOTal cross section, Elastic scattering and diffraction dissociation Measurement at the LHC) experiment, located at the interaction point 5 of the LHC, has measured the total, elastic and inelastic proton-proton crosssections, using a luminosity independent method, based on the optical theorem, in a center-of-mass energy range from 2.76 to 13 TeV. The elastic scattering was investigated in a wide range of the squared four-momentum transfer |t| allowing study of the Coulomb-nuclear interference region down to |t| ∼ 8 × 10−4 GeV2. This made possible the first measurement of the ρ parameter at √s = 13 TeV, ρ being the ratio between the real and the imaginary part of the nuclear elastic scattering amplitude at t = 0. This measurement, combined with the total crosssection results, led to the exclusion of all the models classified and published by the COMPETE Collaboration. The results obtained by TOTEM are indeed compatible with predictions of a colourless 3-gluon bound state exchange in the t-channel of proton-proton elastic scattering, as postulated by alternative theoretical models both in the Regge-like framework and in the modern QCD framework. This result has been confirmed, with a significance of 5.4σ, also by the comparison with the pp data measured by the D0 collaboration at Fermilab. In this contribution the TOTEM experiment results will be described, along with the actual experiment status, the future physics program for the LHC Run 3.

Understanding how minority relativistic electron populations may dominate charge state balance and radiative cooling of a post-thermal quench tokamak plasma

Minority relativistic electron populations can occur in a range of complex plasmas. Of specific interest is when runaway electrons form among the presence of high-atomic-number ion species in a tokamak plasma discharge. It has been recently demonstrated that ion charge state distributions and radiation losses at low bulk electron temperatures can be dominated by relativistic electrons, even though their density is orders of magnitude lower. This was attributed to the relativistic enhancement of electron impact inelastic cross sections. In this work, we provide a closer inspection of the atomic physics underpinning this effect. We also demonstrate the consequences of runaway enhanced scattering on post-disruption tokamak fusion discharges with neon and argon impurities present. Effects on charge state distributions, radiation and spectral characteristics, and reduced-order modeling considerations are discussed.

К вопросу о методе перепроекцирования для неупругих процессов в атомных столкновениях в рамках подхода Борна — Оппенгеймера

The paper provides a detailed description of the reprojection method for the exact solution of the nonadiabatic nuclear dynamics within the Born–Oppenheimer formalism. In particular, it discusses the asymptotic behaviour of a state-to-state transition probability when a nonadiabatic radial coupling for this transition has a nonzero asymptotic value—a fundamental feature of the Born–Oppenheimer approach. It is known that the conventional Born–Oppenheimer approach leads to divergency of inelastic cross sections and inelastic rate coefficients, while the reprojection method provides convergences. The article describes physical background of the reprojection method.

Measurement of the EMC effect in light and heavy nuclei

Inclusive electron scattering from nuclear targets has been measured to extract the nuclear dependence of the inelastic cross section in Hall C at the Thomas Jefferson National Accelerator facility. Results are presented for 2H, 3He, 4He, 9B, 12C, 63Cu and 197Au at an incident electron beam energy of 5.77 GeV for a range of momentum transfer from Q^2 = 2 to 7 (GeV/c)^2. These data improve the precision of the existing measurements of the EMC effect in the nuclear targets at large x, and allow for more detailed examinations of the A dependence of the EMC effect.

O18+Se76 elastic and inelastic scattering at 275 MeV

Background: An accurate description of the initial and final state interactions in the O18+Se76 collision is demanded by the NUMEN project. The study of single and double charge exchange nuclear reactions is the main purpose for NUMEN, since these can be used as tools to provide experimentally driven information about nuclear matrix elements of interest in the context of neutrinoless double-β decay. To date, the details of the optical potentials and nuclear response to isospin operators for many of the projectile-target systems proposed for the NUMEN double charge exchange studies are poorly known. The O18+Se76 case, here under study, is particularly relevant due to its connection with the Ge76 neutrinoless double-β decay. Purpose: In this work the authors want to characterize the initial-state interaction for the O18+Se76 reactions at 275 MeV incident energy determining the optical potential and evaluating the effect of couplings with the inelastic scattering on the elastic channel. Methods: The angular distributions of differential cross section were measured in the angular region between 4∘ and 22∘ in the center-of-mass reference frame. The cross sections were compared with theoretical calculations, that adopt different optical potentials. Coupling effects on the elastic channel were determined into the coupled channels formalism. Results: The excitation energy spectrum of the colliding nuclei and the cross section angular distributions were measured with satisfactory energy resolution. The elastic scattering cross section is not well reproduced in the full angular range explored when the optical model approach is adopted. A good agreement is found using coupled channel calculations. The initial state interaction for the O18+Se76 nuclear reactions at 275 MeV is determined. Conclusions: Coupled channels effects are crucial to obtain a good description of the measured elastic and inelastic channels cross sections, even at large transferred momenta where the optical model approach fails in reproducing the experimental data. The role of channel coupling could be relevant also in the analysis of other open reaction channels in the same collision and should be accounted for in double charge exchange analyses as well.Received 19 December 2020Revised 6 October 2021Accepted 10 November 2021DOI:https://doi.org/10.1103/PhysRevC.104.054610©2021 American Physical SocietyPhysics Subject Headings (PhySH)Research AreasDirect reactionsLow & intermediate energy heavy-ion reactionsNuclear reactionsNuclear structure & decaysNucleon-nucleon interactionsTransfer reactionsProperties59 ≤ A ≤ 896 ≤ A ≤ 19TechniquesCollective modelsNuclear data analysis & compilationNuclear reaction analysisOptical, coupled-channel & distorted wave modelsSpectrometers & spectroscopic techniquesNuclear Physics

Differential Condensation of Methane Isotopologues Leading to Isotopic Enrichment under Non-equilibrium Gas-Surface Collision Conditions.

We examine the initial differential sticking probability of CH4 and CD4 on CH4 and CD4 ices under nonequilibrium flow conditions using a combination of experimental methods and numerical simulations. The experimental methods include time-resolved in situ reflection–absorption infrared spectroscopy (RAIRS) for monitoring on-surface gaseous condensation and complementary King and Wells mass spectrometry techniques for monitoring sticking probabilities that provide confirmatory results via a second independent measurement method. Seeded supersonic beams are employed so that the entrained CH4 and CD4 have the same incident velocity but different kinetic energies and momenta. We found that as the incident velocity of CH4 and CD4 increases, the sticking probabilities for both molecules on a CH4 condensed film decrease systematically, but that preferential sticking and condensation occur for CD4. These observations differ when condensed CD4 is used as the target interface, indicating that the film’s phonon and rovibrational densities of states, and collisional energy transfer cross sections, have a role in differential energy accommodation between isotopically substituted incident species. Lastly, we employed a mixed incident supersonic beam composed of both CH4 and CD4 in a 3:1 ratio and measured the condensate composition as well as the sticking probability. When doing so, we see the same effect in the condensed mixed film, supporting an isotopic enrichment of the heavier isotope. We propose that enhanced multi-phonon interactions and inelastic cross sections between the incident CD4 projectile and the CH4 film allow for more efficacious gas–surface energy transfer. VENUS code MD simulations show the same sticking probability differences between isotopologues as observed in the gas–surface scattering experiments. Ongoing analyses of these trajectories will provide additional insights into energy and momentum transfer between the incident species and the interface. These results offer a new route for isotope enrichment via preferential condensation of heavier isotopes and isotopologues during gas–surface collisions under specifically selected substrate, gas-mixture, and incident velocity conditions. They also yield valuable insights into gaseous condensation under non-equilibrium conditions such as occur in aircraft flight in low-temperature environments. Moreover, these results can help to explain the increased abundance of deuterium in solar system planets and can be incorporated into astrophysical models of interstellar icy dust grain surface processes.

Theoretical study of the HCS+–H2 van der Waals complex: potential energy surface, rovibrational bound states, and rotationally inelastic collisional cross sections

An accurate ground-state intermolecular potential energy surface (PES) was calculated for the HCS–H complex. The surface was constructed from 3023 ab initio energies, computed with explicitly correlated coupled-cluster theory, CCSD(T)-F12b, with extrapolation to the complete basis set limit (VTZ-F12/VQZ-F12). The new 4D PES was used to compute rovibrational energies, rotational constants, and close-coupling quantum scattering calculations at low collision energies. A symmetry-adapted Lanczos algorithm was used to variationally compute the low-lying rovibrational bound states. Rotational constants for states of two isomers were determined from the energy levels and reported in hopes of motivating experiments. The rotationally inelastic state-to-state cross sections of HCS by collision with para- and ortho-H were computed and compared, and trends and propensities are discussed.

Correspondence between isoscalar monopole strengths and $\alpha$ inelastic cross sections on 24Mg

Abstract The correspondence between the isoscalar monopole (IS0) transition strengths and $\alpha$ inelastic cross sections, the $B({\rm IS0})$–$(\alpha,\alpha')$ correspondence, is investigated for $^{24}$Mg($\alpha,\alpha'$) at 130 and 386 MeV. We adopt a microscopic coupled-channel reaction framework to link structural inputs, diagonal and transition densities, for $^{24}$Mg obtained with antisymmetrized molecular dynamics to the ($\alpha,\alpha'$) cross sections. We aim at clarifying how the $B({\rm IS0})$–$(\alpha,\alpha')$ correspondence is affected by the nuclear distortion, the in-medium modification to the nucleon–nucleon effective interaction in the scattering process, and the coupled-channel effect. It is found that these effects are significant and the explanation of the $B({\rm IS0})$–$(\alpha,\alpha')$ correspondence in the plane wave limit with the long-wavelength approximation, which is often used, makes no sense. Nevertheless, the $B({\rm IS0})$–$(\alpha,\alpha')$ correspondence tends to remain because of a strong constraint on the transition densities between the ground state and the $0^+$ excited states. The correspondence is found to hold at 386 MeV with an error of about 20%–30%, while it is seriously compromised at 130 MeV, mainly by the strong nuclear distortion. It is also found that when a $0^+$ state that has a different structure from a simple $\alpha$ cluster state is considered, the $B({\rm IS0})$–$(\alpha,\alpha')$ correspondence becomes less valid. For a quantitative discussion on the $\alpha$ clustering in $0^+$ excited states of nuclei, a microscopic description of both the structure and reaction parts will be necessary.