Aerosol Indirect Effect Research Articles

Entrainment Makes Pollution More Likely to Weaken Deep Convective Updrafts Than Invigorate Them

AbstractAre the results of aerosol invigoration studies that neglect entrainment valid for diluted deep convective clouds? We address this question by applying an entraining parcel model to soundings from tropical and midlatitude convective environments, wherein pollution is assumed to increase parcel condensate retention. Invigoration of 5%–10% and <2% is possible in undiluted tropical and midlatitude parcels respectively when freezing is rapid. This occurs because the positive buoyancy contribution from freezing is larger than the negative buoyancy contribution from condensate loading, leading to positive net condensate contribution to buoyancy. However, aerosol‐induced weakening is more likely when realistic entrainment rates occur because water losses from entrainment more substantially reduce the latent heating relative to the loading contribution. This leads to larger net negative buoyancy contribution from condensates in polluted than in clean entraining parcels. Our results demonstrate that accounting for entrainment is critical in conceptual models of aerosol indirect effects in deep convection.

Transported aerosols regulate the pre-monsoon rainfall over north-east India: a WRF-Chem modelling study

Abstract. The study differentiates and quantifies the impacts of aerosols emitted locally within the north-east (NE) India region and those transported from outside this region to ascertain whether local or transported aerosols are more impactful in influencing this region's rainfall during the pre-monsoon season (March–April–May). Due to the existence of a declining pre-monsoon rainfall trend in NE India, the study also quantified the role of different aerosol effects in radiative forcing (RF) and rainfall. The study has been carried out using the WRF-Chem model by comparing simulation scenarios where emissions were turned on and off within and outside the NE region. The impact of all emissions as a whole and black carbon (BC) specifically was studied. Results show that aerosols transported primarily from the Indo-Gangetic Plain (IGP) were responsible for 93.98 % of the PM10 mass over NE India's atmosphere and 64.18 % of near-surface PM10 concentration. Transported aerosols contributed >50 % of BC, organic carbon, sulfate, nitrate, ammonium and dust aerosol concentration and are hence a major contributor to air pollution. Hence, the aerosol effects were much greater with transported aerosols. An indirect aerosol effect was found to be the major effect and more impactful, with transported aerosols that dominated both rainfall and RF and suppressed rainfall more significantly than the direct and semi-direct effect. However, the increase in direct radiative effects with an increase in transported BC counteracted the rainfall suppression caused by relevant processes of other aerosol effects. Thus, this study shows atmospheric transport to be an important process for this region, as transported emissions, specifically from the IGP, were also found to have greater control over the region's rainfall. Thus, emission control policies implemented in the IGP will reduce air pollution as well as the climatic impacts of aerosols over the NE India region.

Aerosol Indirect Effects on Water Vapor in the UTLS of Typhoon Saomai (2006)

AbstractThe evolution of landfalling Typhoon Saomai (2006) is simulated using the Weather Research and Forecasting model with spectral bin microphysics scheme, showing tropical cyclone (TC) could vertically transport water vapor from troposphere to upper troposphere and lower stratosphere (UTLS). Three aerosol sensitivity experiments are conducted to explore the indirect effects of aerosol served as cloud condensation nuclei (CCN) on overshooting convection (OTC) and water vapor content in UTLS, namely MAR (maritime), MIX (semi‐continental) and CON (continental). Results revealed that CON simulation with high initial aerosol concentration showing invigorated convection at the periphery of the TC, which interfered with the reformation of TC eyewall, leading to TC weakening finally. In addition, CON simulated the least water content in UTLS through suppressing the number of convection overshooting the tropopause level. Most overshooting events take place during TC developing stage in the eyewall region before landfall. Higher levels of CCN concentration could lead to decreased number of OTC in TC, consistently reduced the water vapor content in UTLS. CON and MIX experiments simulated respectively 21.9% (16.2%) and 9.96% (1.5%) less OTC (water vapor content in UTLS) than MAR simulation. Water vapor content in UTLS is affected by the interaction of OTC and ice‐phase microphysics. The interesting point is that the CCN sensitivity experiments show that water vapor content in UTLS of a TC is sensitive to the CCN concentration in the boundary layer.

Aerosol indirect effects on orographic clouds and precipitation

The sensitivity of warm orographic cloud development to aerosol indirect effects was investigated through aerosol-aware Weather Research and Forecast model simulations contrasting aerosol-cloud-precipitation interactions using the default (generic) aerosol and regional aerosol measurements from the Integrated Precipitation and Hydrology Experiment in the Southern Appalachian Mountains for three rainfall events: 1) enhanced local convection; 2) a frontal system, and 3) a tropical system. Using the regional aerosol activation spectrum yields higher number of drops than using the default, smaller cloud droplets and delayed rainfall onset under weak synoptic forcing conditions. Evaluation against aircraft measurements in isolated convective clouds reveals that while the model microphysics falls short of reproducing the vertical structure of nonprecipitating clouds, the liquid water content, and the concentration of cloud droplets near cloud base are in keeping with observations. The simulated cloud vertical structure shows the regional signature of orographic enhancement over the mountains vis-a-vis the adjacent plains. In the inner region, valley-ridge circulations organize the spatial patterns of cloudiness under weak synoptic forcing. The formation of early afternoon low-level clouds over the ridges in the summertime reflects the aerosol indirect effect. By contrast, for large-scale systems with strong and sustained moisture convergence at low levels (frontal and tropical systems), mechanically forced rainfall efficiency is enhanced, there is no delay in the onset of precipitation, and the aerosol indirect effect is negligible. This study shows that the impact of aerosol-cloud-precipitation interactions on the spatial variability of orographic rainfall is conditional on weather regime.

Assessing the Aerosols, Clouds and Their Relationship Over the Northern Bay of Bengal Using a Global Climate Model

AbstractComprehensive evaluation of aerosol‐cloud interactions (ACI) simulated by climate models using observations is crucial for advancing model development. Here, we use Moderate Resolution Imaging Spectroradiometer (MODIS) data to evaluate aerosol and cloud properties obtained from Community Atmosphere Model 5 (CAM5) over northern Bay of Bengal during winter season. We conduct simulations for default model setup as well as for prescribed, and nudged meteorology using Goddard Earth Observing System (GEOS5) reanalysis dataset in order to study the impact of meteorological parameters on simulated ACI. CAM5 captures the spatial variability of cloud optical depth (τc), cloud droplet number concentration (Nc), and liquid water path (LWP), although the values are overestimated in the model. Default model strongly simulates observed negative cloud effective radius (re)‐Nc susceptibility but fails to reproduce the observed positive LWP‐Nc susceptibility possibly due to evaporative cooling of the large number of smaller droplets. Compared to default and prescribed meteorology simulations, nudging specific humidity (Q) at 6‐hr relaxation time scale leads to a positive LWP‐Nc susceptibility, and an overall improved simulation of aerosol indirect effects. Increasing the relaxation time scale beyond 6‐hr degrade the simulation of indirect effects suggesting high sensitivity of indirect effects to Q and serious deficiencies in Q simulated by the model. Improvement in simulation of aerosol and cloud characteristics are also noted when winds (UV) are nudged but it worsens some of the simulated ACI sensitivities due to increased transport of absorbing aerosols over the study region and a dominant semi‐direct effect in the model.

Aerosol radiative feedback enhances particulate pollution over India: A process understanding

In this study, we investigate the role of aerosol direct radiative feedback on regional meteorological changes and subsequent distribution of air pollutant with the focus on particulate matter PM2.5 and ozone (O3) over India. WRF-Chem simulations have been applied for Baseline case with both aerosol direct and indirect effects and another simulation including only aerosol indirect effects. The aerosol direct radiative feedback on the meteorology and air quality were investigated by taking the differences between these two simulations. A comprehensive model evaluation showed the model had the capacity to reproduce the observations and well captured the temporal and spatial variation in meteorological and aerosol fields. We found that the reduction in incoming shortwave solar radiation, temperature at 2 m and planetary boundary layer height annually and across all the season due to aerosol radiation interaction (ARI). The concentration of PM2.5 and gaseous precursors like SO2 and NO2 showed enhancements, while O3 concentration mostly showed a reduction. Spatial and annual average PM2.5 concentration was increased by +6%, SO2 concentration was increased by +1.4%, NO2 concentration was increased by +3.4%, and O3 concentration was reduced by −1.4%. Largest regional increases of 40% in particulate pollution induced by ARI occurred over north-western Indian region. The increase in PM2.5 concentration was highly related to stabilisation induced through meteorological variables and increases in primary aerosol concentration. The decrease in O3 concentration was highly related increases in NO2 and SO2 concentration. In the most polluted regions of India, ARI significantly enhance surface-level particulate pollution and related premature mortality, of particular concern considering likely future increasing trends. This study highlights the importance of inclusion and better representations of ARI and for implementing effective mitigation plans.

Aerosol-cloud-precipitation interaction during some convective events over southwestern Iran using the WRF model

Four convective precipitation events in southwestern Iran are examined in this study using the aerosol-aware bulk microphysical scheme implemented in the Weather Research and Forecasting (WRF) model. Two simulations were conducted for each of the events, which included the control and polluted simulations. In the control simulation, the concentration of aerosols in the current climate is considered, while the concentration of aerosols was increased by a factor of 5 at all grid points in the polluted simulation. The aim of this research is to evaluate the effects of aerosols on cloud microphysics and precipitation. During the convective events, southerly to southwesterly warm and dry winds dominated, causing a substantial transport of aerosols and humidity. Relatively high values of planetary boundary-layer height (PBLH) are simulated in the polluted simulations, which indicate a higher convective activity and more efficient transport of aerosols and moisture in the vertical. Also, the convective available potential energy (CAPE) increases in polluted simulations, implying that an increase in the concentration of aerosols is associated with more favorable thermodynamic conditions for convection. In all simulations, the reflection of shortwave radiation by clouds increases, indicating that the first indirect effect of aerosols plays a key role in the energy budget of the Earth. On the other hand, an increase in the concentration of aerosols only slightly influences longwave radiation. Altitudes of the lifting condensation level (LCL) and the level of free convection (LFC) increase in all polluted compared to control simulations. This indicates that the air parcel needs to rise to a higher altitude to get saturated. The impact of an increase in the concentration of aerosols on cloud development is substantial in a simulation that contains a higher convergence of vertical moisture flux and stronger winds over the region. The convergence of the vertical moisture flux in the three simulations indicates that more water vapor is available in these simulations to be condensed on aerosols, which increases the cloud water content. Thus, the number density of cloud droplets is higher in the polluted compared to control simulations. The altitude of the maximum mass density of cloud droplets is nearly the same in the simulation (between 3 and 6 km). Due to higher specific humidity in these altitudes, higher water vapor can be condensed on condensation nuclei. An increase in ice and snow, which indicates a higher lifting of droplets to the freezing level, is seen in the simulations with the negative convergence of vertical moisture flux. This indicates that these regions may help the large-scale collection of moisture and its lifting. In simulations with a divergence of moisture in the northern and the whole domain, the cloud water content decreases. In simulations with a higher moisture difference, there is higher precipitation in the polluted compared to control simulations because, in the humid atmosphere, there is enough water vapor to be condensed on aerosols, which leads to the formation of larger cloud droplets. Thus, the collision of cloud droplets is more efficient, and precipitation increases. In addition, due to a lower cloud base, there is less chance for the evaporation and melting of precipitation.

Examination of aerosol indirect effects during cirrus cloud evolution

Abstract. Aerosols affect cirrus formation and evolution, yet quantification of these effects remain difficult based on in situ observations due to the complexity of nucleation mechanisms and large variabilities in ice microphysical properties. This work employed a method to distinguish five evolution phases of cirrus clouds based on in situ aircraft-based observations from seven U.S. National Science Foundation (NSF) and five NASA flight campaigns. Both homogeneous and heterogeneous nucleation were captured in the 1 Hz aircraft observations, inferred from the distributions of relative humidity in the nucleation phase. Using linear regressions to quantify the correlations between cirrus microphysical properties and aerosol number concentrations, we found that ice water content (IWC) and ice crystal number concentration (Ni) show strong positive correlations with larger aerosols (>500 nm) in the nucleation phase, indicating strong contributions of heterogeneous nucleation when ice crystals first start to nucleate. For the later growth phase, IWC and Ni show similar positive correlations with larger and smaller (i.e., >100 nm) aerosols, possibly due to fewer remaining ice-nucleating particles in the later growth phase that allows more homogeneous nucleation to occur. Both 200 m and 100 km observations were compared with the nudged simulations from the National Center for Atmospheric Research (NCAR) Community Atmosphere Model version 6 (CAM6). Simulated aerosol indirect effects are weaker than the observations for both larger and smaller aerosols for in situ cirrus, while the simulated aerosol indirect effects are closer to observations in convective cirrus. The results also indicate that simulations overestimate homogeneous freezing, underestimate heterogeneous nucleation and underestimate the continuous formation and growth of ice crystals as cirrus clouds evolve. Observations show positive correlations of IWC, Ni and ice crystal mean diameter (Di) with respect to Na in both the Northern and Southern Hemisphere (NH and SH), while the simulations show negative correlations in the SH. The observations also show higher increases of IWC and Ni in the SH under the same increase of Na than those shown in the NH, indicating higher sensitivity of cirrus microphysical properties to increases of Na in the SH than the NH. The simulations underestimate IWC by a factor of 3–30 in the early/later growth phase, indicating that the low bias of simulated IWC was due to insufficient continuous ice particle formation and growth. Such a hypothesis is consistent with the model biases of lower frequencies of ice supersaturation and lower vertical velocity standard deviation in the early/later growth phases. Overall, these findings show that aircraft observations can capture both heterogeneous and homogeneous nucleation, and their contributions vary as cirrus clouds evolve. Future model development is also recommended to evaluate and improve the representation of water vapor and vertical velocity on the sub-grid scale to resolve the insufficient ice particle formation and growth after the initial nucleation event.

Aerosol activation characteristics and prediction at the central European ACTRIS research station of Melpitz, Germany

Abstract. Understanding aerosol particle activation is essential for evaluating aerosol indirect effects (AIEs) on climate. Long-term measurements of aerosol particle activation help to understand the AIEs and narrow down the uncertainties of AIEs simulation. However, they are still scarce. In this study, more than 4 years of comprehensive aerosol measurements were utilized at the central European research station of Melpitz, Germany, to gain insight into the aerosol particle activation and provide recommendations on improving the prediction of number concentration of cloud condensation nuclei (CCN, NCCN). (1) The overall CCN activation characteristics at Melpitz are provided. As supersaturation (SS) increases from 0.1 % to 0.7 %, the median NCCN increases from 399 to 2144 cm−3, which represents 10 % to 48 % of the total particle number concentration with a diameter range of 10–800 nm, while the median hygroscopicity factor (κ) and critical diameter (Dc) decrease from 0.27 to 0.19 and from 176 to 54 nm, respectively. (2) Aerosol particle activation is highly variable across seasons, especially at low-SS conditions. At SS=0.1 %, the median NCCN and activation ratio (AR) in winter are 1.6 and 2.3 times higher than the summer values, respectively. (3) Both κ and the mixing state are size-dependent. As the particle diameter (Dp) increases, κ increases at Dp of ∼40 to 100 nm and almost stays constant at Dp of 100 to 200 nm, whereas the degree of the external mixture keeps decreasing at Dp of ∼40 to 200 nm. The relationships of κ vs. Dp and degree of mixing vs. Dp were both fitted well by a power-law function. (4) Size-resolved κ improves the NCCN prediction. We recommend applying the κ–Dp power-law fit for NCCN prediction at Melpitz, which performs better than using the constant κ of 0.3 and the κ derived from particle chemical compositions and much better than using the NCCN (AR) vs. SS relationships. The κ–Dp power-law fit measured at Melpitz could be applied to predict NCCN for other rural regions. For the purpose of improving the prediction of NCCN, long-term monodisperse CCN measurements are still needed to obtain the κ–Dp relationships for different regions and their seasonal variations.

CCN Spectral Modality Compared to Droplet Spectra and Drizzle in RICO Cumuli

AbstractRain in Cumulus over the Ocean (RICO) warm cloud microphysics and drizzle comparisons with cloud condensation nuclei (CCN) spectra displayed similarities with earlier analyses of low‐altitude Ice in Clouds Experiment‐Tropical (ICE‐T) warm maritime cumuli. These comparisons of high‐resolution CCN spectra measured at 100 m altitude with cloud and drizzle measurements were consistent within three altitude bands between 600 and 3,700 m. For both projects, clouds associated with bimodal CCN (accumulation mode dominant) displayed more drizzle than clouds associated with unimodal CCN (Aitken mode dominant). Higher concentrations in clouds associated with bimodal CCN than clouds associated with unimodal CCN extended throughout the ranges of 3 drizzle drop probes (260X, 2DC, and 2DP) between 60 and 5,200 μm diameter. Ratios of drizzle drop concentrations in clouds associated with bimodal CCN to those in clouds associated with unimodal CCN were as much as an order of magnitude. Confirmation of a relationship between CCN modality and cloud droplet spectra found in ICE‐T was often obscured in RICO by drizzle effects on droplet spectra. There was also an association between cloudiness and CCN bimodality that is consistent with clouds as a source of accumulation mode particles. These consistent results now found in two warm maritime small low‐altitude cumulus cloud experiments show that CCN bimodality could inhibit the indirect aerosol effect (IAE), especially second IAE (cloud lifetime) in warm maritime cumuli. These RICO and ICE‐T observations in maritime cumuli are opposite of the results in the Marine Stratus/Stratocumulus Experiment, which indicated that CCN bimodality could enhance both IAE.

Radiative effects and feedbacks of anthropogenic aerosols on boundary layer meteorology and fine particulate matter during the COVID-19 lockdown over China

The COVID-19 epidemic has exerted significant impacts on human health, social and economic activities, air quality and atmospheric chemistry, and potentially on climate change. In this study, an online coupled regional climate–chemistry–aerosol model (RIEMS-Chem) was applied to explore the direct, indirect, and feedback effects of anthropogenic aerosols on radiation, boundary layer meteorology, and fine particulate matter during the COVID-19 lockdown period from 23 January to 8 April 2020 over China. Model performance was validated against a variety of observations for meteorological variables, PM2.5 and its chemical components, aerosol optical properties, as well as shortwave radiation flux, which demonstrated that RIEMS-Chem was able to reproduce the spatial distribution and temporal variation of the above variables reasonably well. During the study period, direct radiative effect (DRE) of anthropogenic aerosols was stronger than indirect radiative effect (IRE) in most regions north of the Yangtze River, whereas IRE dominated over DRE in the Yangtze River regions and South China. In North China, DRE induced larger changes in meteorology and PM2.5 than those induced by IRE, whereas in South China, the changes by IRE were remarkably larger than those by DRE. Emission reduction alone during the COVID-19 lockdown reduced PM2.5 concentration by approximately 32 % on average over East China. As a result, DRE at the surface was weakened by 15 %, whereas IRE changed little over East China, leading to a decrease in total radiative effect (TRE) by approximately 7 % in terms of domain average. The DRE-induced changes in meteorology and PM2.5 were weakened due to emission reduction, whereas the IRE-induced changes were almost the same between the cases with and without emission reductions. By aerosol radiative and feedback effects, the COVID-19 emission reductions resulted in 0.06 °C and 0.04 °C surface warming, 1.6 and 4.0 μg m−3 PM2.5 decrease, 0.4 and 1.3 mm precipitation increase during the lockdown period in 2020 in terms of domain average over North China and South China, respectively, whereas the lockdown caused negligible changes on average over East Asia.

Increased aerosols can reverse Twomey effect in water clouds through radiative pathway

Aerosols play important roles in modulations of cloud properties and hydrological cycle by decreasing the size of cloud droplets with the increase of aerosols under the condition of fixed liquid water path, which is known as the first aerosol indirect effect or Twomey-effect or microphysical effect. Using high-quality aerosol data from surface observations and statistically decoupling the influence of meteorological factors, we show that highly loaded aerosols can counter this microphysical effect through the radiative effect to result both the decrease and increase of cloud droplet size depending on liquid water path in water clouds. The radiative effect due to increased aerosols reduces the moisture content, but increases the atmospheric stability at higher altitudes, generating conditions favorable for cloud top entrainment and cloud droplet coalescence. Such radiatively driven cloud droplet coalescence process is relatively stronger in thicker clouds to counter relatively weaker microphysical effect, resulting the increase of cloud droplet size with the increase of aerosol loading; and vice-versa in thinner clouds. Overall, the study suggests the prevalence of both negative and positive relationships between cloud droplet size and aerosol loading in highly polluted regions.

Stronger Response to the Aerosol Indirect Effect Due To Cooling in Remote Regions.

It is often assumed that effective radiative forcings, regardless of forcing agent, are additive in the temperature change. Using climate model simulations with abruptly applied aerosol forcing we find that the temperature response per unit forcing is larger if induced by aerosol-cloud interactions than directly by aerosols. The spatial patterns of forcing and temperature change show that aerosol-cloud interactions induce cooling over remote oceans in the extratropics, whereas the effect of increased emissions is localized around the emission sources primarily over tropical land. The results are consistent with ideas of how the patterns of sea surface temperature impact radiative feedbacks, and a large forcing efficacy of aerosol-cloud interactions could help explain previously observed intermodel spread in the response to aerosols.

Impact of urban aerosols on the cloud condensation activity using a clustering model

The indirect effect of aerosols on climate through aerosol-cloud-interactions is still highly uncertain and limits our ability to assess anthropogenic climate change. The foundation of this uncertainty is in the number of cloud condensation nuclei (CCN), which itself mainly stems from uncertainty in aerosol sources and how particles evolve to become effective CCN. We analyze particle number size distribution (PNSD) and CCN measurements from an urban site in a two-step method: (1) we use an unsupervised clustering model to classify the main aerosol categories and processes occurring in the urban atmosphere and (2) we explore the influence of the identified aerosol populations on the CCN properties. According to the physical properties of each cluster, its diurnal timing, and additional air quality parameters, the clusters are grouped into five main aerosol categories: nucleation, growth, traffic, aged traffic, and urban background. The results show that, despite aged traffic and urban background categories are those with lower total particle number concentrations (Ntot) these categories are the most efficient sources in terms of contribution to the overall CCN budget with activation fractions (AF) around 0.5 at 0.75 % supersaturation (SS). By contrast, road traffic is an important aerosol source with the highest frequency of occurrence (32 %) and relatively high Ntot, however, its impact in the CCN activity is very limited likely due to lower particle mean diameter and hydrophobic chemical composition. Similarly, nucleation and growth categories, associated to new particle formation (NPF) events, present large Ntot with large frequency of occurrence (22 % and 28 %, respectively) but the CCN concentration for these categories is about half of the CCN concentration observed for the aged traffic category, which is associated with their small size. Overall, our results show that direct influence of traffic emissions on the CCN budget is limited, however, when these particles undergo ageing processes, they have a significant influence on the CCN concentrations and may be an important CCN source. Thus, aged traffic particles could be transported to other environments where clouds form, triggering a plausible indirect effect of traffic emissions on aerosol-cloud interactions and consequently contributing to climate change.

Exacerbation of Indian Summer Monsoon Breaks by the Indirect Effect of Regional Dust Aerosols

AbstractEvaluation of century‐long simulations of the Community Earth System Model (CESM) reveals model fidelity in capturing characteristics of aerosols, clouds, convection, rainfall and circulation over India associated with the active/break phase with wetter/drier than average rainfall within the summer monsoon season. During the breaks, aerosols build up over central India due to desert dust transported from the west by anomalous circulation, the trapping of dust emissions from the Thar‐desert and the increased aerosol lifetime in dry conditions. Break spells exhibit reduced cloud effective radius and enhanced lower atmospheric warming over central India as potential evidence for the indirect effect induced by dust aerosols. Consistently, break spells intensify in CESM simulation with increased loading of dust aerosols. The indirect effect of dust aerosols in warming the atmosphere and exacerbating the severity of breaks is conspicuous in simulations forced with the indirect effect of aerosols alone, both for present‐day and pre‐industrial periods.

Study on the Parameters of Ice Clouds Based on 1.5 µm Micropulse Polarization Lidar

Dust aerosols can participate in the heterogeneous nucleation process as effective ice nucleation particles, thus changing the physical properties of clouds. In this paper, we used an eye-safe 1550 nm micropulse polarization single photon lidar combined with meteorological stations, HYSPLIT backward trajectory analysis, ERA5 reanalysis data, CALIPSO, Himawari-8 and Terra-MODIS satellite data to compare the difference in cloud characteristics between dust and clean cirrus cases in Jinan from 26–29 March 2022. The study found that the aerosol affected the cloud effective radius, and the cloud top temperature impacted the properties of depolarization of dust ice clouds. According to the statistical results of the upper and lower quartiles, the depolarization ratio (DPR) range of dust cirrus on 26 March was 0.46–0.49, a similar range to the clean cirrus, while that of dust cirrus on 27 March was 0.54–0.59, which seemed much larger. Different height and temperature conditions lead to differences in the habits of ice crystals in clouds, thus changing the DPR. However, the range of the DPR between clean cirrus and dust cirrus showed no obvious difference, as the former was 0.43–0.53 and the latter was 0.46–0.59. Under the condition of higher aerosol loading, the lidar range-corrected signal (RCS) of cirrus clouds was stronger, and the cloud effective radius was 48 μm, larger than that of clean cirrus (32 μm). This may be the effect of dust on the microphysical properties of clouds. This study discusses the indirect effects of dust aerosols on cirrus clouds and the underlying mechanisms from the perspectives of microphysics and optics, which can provide more references for urban air pollution processes and aerosol-cloud interactions.

The dominant role of aerosol-cloud interactions in aerosol-boundary layer feedback: Case studies in three megacities in China

Interactions between aerosols and meteorology have received increasing attention in recent decades. Through interactions with radiation, aerosols involve in thermodynamic processes and cause cloud adjustment, referred to as the direct and semi-direct effects respectively. They also involve in cloud microphysical processes by severing as cloud condensation nuclei or ice nuclei, referred to as indirect effect. Aerosol direct effect is found to potentially exacerbate air quality by stabilizing the planetary boundary layer (PBL). However, their impacts through the interaction with clouds, including semi-direct and indirect effect remain unclear. In this study, we conducted model simulations to evaluate the direct, semi-direct and indirect effects of aerosols in PBL structure and surface PM2.5 concentration during three heavy haze events under overcast conditions. Overall, the aerosol-PBL feedback results in a 22%–36% decrease of PBL height and 5%–28% increase of PM2.5 concentration. The indirect effect always has the largest impact on PBL and PM2.5 pollution, accounting for 59%–84% of the changes. The semi-direct effect is the weakest on average, although it can exceed the direct effect at certain times and locations. Black carbon aerosols play the vital role in both the direct and semi-direct effects. Our findings promote the understanding of heavy haze formation, and highlight the dominant role of aerosol-cloud interaction in the feedback process of aerosols to PBL structure and air quality.

Impact of Inclusion of the Indirect Effects of Sulfate Aerosol on Radiation and Cloudiness in the INMCM Model

Impact of Inclusion of the Indirect Effects of Sulfate Aerosol on Radiation and Cloudiness in the INMCM Model

Polar Aerosol Vertical Structures and Characteristics Observed with a High Spectral Resolution Lidar at the ARM NSA Observatory

Aerosol vertical distributions impact both the direct and indirect radiative effects of aerosols. High Spectra Resolution Lidar (HSRL) separates between atmospheric molecular signals and aerosol particle signals and therefore can provide reliable measurements of aerosol properties. Six years of HSRL measurements between 2014 and 2019 from the Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) North Slope of Alaska (NSA) atmospheric observatory at Utqiaġvik are used to statistically analyze Arctic aerosol vertical distributions. The annual cycle of aerosol vertical distributions in terms of aerosol particulate backscatter coefficient (βp), lidar scattering ratio (SR), and aerosol particulate depolarization ratio (δp) profiles at the wavelength of 532 nm shows that Arctic Haze events are prevalent in later winter and spring at the NSA site. Mineral dust is frequently presented in strong aerosol layers in the spring, fall, and winter seasons. Over the summer season, the NSA site has large aerosol loadings that are dominated by small spherical aerosol particles.

Aerosol-cloud interaction in water clouds observed using ground-based, in-situ, and satellite-based observations over an Indian continental region

The impact of atmospheric aerosols on climate by acting as cloud condensation nuclei is very complex and unable to capture completely by climate models. In this study, an observational approach to estimate the aerosol-cloud interaction (ACI) in water clouds is presented using a combination of ground-based, in-situ balloon-borne, and satellite-based measurements of nearly 7 years over an Indian region. Aerosol and cloud optical depths (AOD and COD retrieved from lidar) are the aerosol and cloud proxies, respectively, used for estimating ACI by constraining liquid water path (LWP retrieved from radiosonde) and background meteorological conditions. Seasonal variations of the occurrence of water clouds detected from backscattered lidar signals using the wavelet covariance transform method are identical to those obtained from radiosonde observations. The ACI analysis shows that the correlation between AOD and COD is highest near the cloud base and it decreases as the height above the cloud base increases for all the LWP values ranging from 30 to 150 g/m2. The calculated ACIτ parameter is within the theoretical limit. The highest correlation value near the cloud base are observed at the LWP bin of 60 to 90 g/m2. ACI at the cloud base shows a decreasing pattern as the cloud base temperature decreases for LWP values of 30 to 60 g/m2 whereas different patterns for all other LWPs. High ACI is observed when the wind direction at the cloud base is northeasterly and low ACI when it is southeasterly and southwesterly. This result supports the observation of the high occurrence of water clouds during winter followed by the post-monsoon season and low occurrence during monsoon and pre-monsoon seasons over the observational site. Thus, the estimated ACI is in accordance with the theoretical concept of aerosol indirect effect i.e. the polluted atmospheric condition leads to clouds with more cloud fraction and cloud optical depth.