Incoherent Mechanism Research Articles

An incoherent feed-forward loop involving bHLH transcription factors, Auxin and CYCLIN-Ds regulates style radial symmetry establishment in Arabidopsis.

The bilateral-to-radial symmetry transition occurring during the development of the Arabidopsis thaliana female reproductive organ (gynoecium) is a crucial biological process linked to plant fertilization and seed production. Despite its significance, the cellular mechanisms governing the establishment and breaking of radial symmetry at the gynoecium apex (style) remain unknown. To fill this gap, we employed quantitative confocal imaging coupled with MorphoGraphX analysis, in vivo and in vitro transcriptional experiments, and genetic analysis encompassing mutants in two bHLH transcription factors necessary and sufficient to promote transition to radial symmetry, SPATULA (SPT) and INDEHISCENT (IND). Here, we show that defects in style morphogenesis correlate with defects in cell-division orientation and rate. We showed that the SPT-mediated accumulation of auxin in the medial-apical cells undergoing symmetry transition is required to maintain cell-division-oriented perpendicular to the direction of organ growth (anticlinal, transversal cell division). In addition, SPT and IND promote the expression of specific core cell-cycle regulators, CYCLIN-D1;1 (CYC-D1;1) and CYC-D3;3, to support progression through the G1 phase of the cell cycle. This transcriptional regulation is repressed by auxin, thus forming an incoherent feed-forward loop mechanism. We propose that this mechanism fine-tunes cell division rate and orientation with the morphogenic signal provided by auxin, during patterning of radial symmetry at the style.

Distributions of easy axes and reversal processes in patterned MRAM arrays

The distribution of the easy-axes in an array of MRAM cells is a vital parameter to understand the switching and characteristics of the devices. By measuring the coercivity as a function of applied-field angle, and remaining close to the perpendicular orientation, a classic Stoner-Wohlfarth approximation has been applied to the resulting variation to determine the standard deviation, sigma , of a Gaussian distribution of the orientation of the easy-magnetisation directions. In this work we have compared MRAM arrays with nominal cells sizes of 20 nm and 60 nm and a range of free layer thicknesses. We have found that a smaller diameter cell will have a wider switching-field distribution with a standard deviation sigma = {9.5}^{circ }. The MRAM arrays consist of pillars produced by etching a multilayer thin film. This value of sigma is dominated by pillar uniformity and edge effects controlling the reversal, reinforcing the need for ever-improving etch processes. This is compared to larger pillars, with distributions as low as sigma = {5.5}^{circ }. Furthermore we found that the distribution broadens from sigma = {5.5}^{circ } to sigma = {8.5}^{circ } with free layer thickness in larger pillars and that thinner films had a more uniform easy-axis orientation. For the 20 nm pillars the non-uniform size distribution of the pillars, with a large and unknown error in the free-layer volume, was highlighted as it was found that the activation volume for the reversal of the free layer 930 nm^3 was larger than the nominal physical volume of the free layer. However for the 60 nm pillars, the activation volume was measured to be equal to one fifth of their physical volume. This implies that the smaller pillars effectively reverse as one entity while the larger pillars reverse via an incoherent mechanism of nucleation and propagation.

(Invited) Two-color soliton meta-atoms and molecules

We present a detailed overview of the physics of two-color soliton molecules in nonlinear waveguides, i.e. bound states of localized optical pulses which are held together due to an incoherent interaction mechanism. The mutual confinement, or trapping, of the subpulses, which leads to a stable propagation of the pulse compound, is enabled by the nonlinear Kerr effect. Special attention is paid to the description of the binding mechanism in terms of attractive potential wells, induced by the refractive index changes of the subpulses, exerted on one another through cross-phase modulation. Specifically, we discuss nonlinear-photonics meta atoms, given by pulse compounds consisting of a strong trapping pulse and a weak trapped pulse, for which trapped states of low intensity are determined by a Schr\"odinger-type eigenproblem. We discuss the rich dynamical behavior of such meta-atoms, demonstrating that an increase of the group-velocity mismatch of both subpulses leads to an ionization-like trapping-to-escape transition. We further demonstrate that if both constituent pulses are of similar amplitude, molecule-like bound-states are formed. We show that z-periodic amplitude variations permit a coupling of these pulse compound to dispersive waves, resulting in the resonant emission of Kushi-comb-like multi-frequency radiation.

Thermally activated motion of cold excitons in conjugated polymers

AbstractThermally activated migration of localized cold excitons were investigated in archetypal conjugated polymers; trans‐polyacetylene, polythiophene, and poly(p‐phenylene vinylene). Room temperature thermal energy has been found to provide sufficient energy to avail substantial mobility for excitons. A simple undistorted but displaced harmonic oscillator model has been assumed to predict the activation energy for exciton hopping between identical sites in perfectly planar conjugated chains, promoted by vibrational modes with Bu symmetry. The activation energies of exciton hopping has been found to increase in the order of trans‐polyacetylene (6.4 meV), polythiophene (29.5 meV), and poly(p‐phenylene vinylene) (147.4 meV). A rough Monte‐Carlo simulation based on incoherent hopping mechanism reveals excitons can displace in an average of 2.17 nm in polythiophene whereas those distances are much smaller in poly(p‐phenylene vinylene) (0.24 nm) and trans‐polyacetylene (0.37 nm). The simulation results partially explain why polythiophene based polymers are better suited for organic photovoltaic applications whereas poly(p‐phenylene vinylene) are more appropriate for organic light emitting diode applications.

Toward Optimizing and Understanding Reversible Hyperpolarization of Lactate Esters Relayed from para-Hydrogen.

The SABRE-Relay hyperpolarization method is used to enhance the 1H and 13C NMR signals of lactate esters, which find use in a wide range of medical, pharmaceutical, and food science applications. This is achieved by the indirect relay of magnetization from para-hydrogen, a spin isomer of dihydrogen, to OH-containing lactate esters via a SABRE-hyperpolarized NH intermediary. This delivers 1H and 13C NMR signal enhancements as high as 245- and 985-fold, respectively, which makes the lactate esters far more detectable using NMR. DFT-calculated J-couplings and spin dynamics simulations indicate that, while polarization can be transferred from the lactate OH to other 1H nuclei via the J-coupling network, incoherent mechanisms are needed to polarize the 13C nuclei at the 6.5 mT transfer field used. The resulting sensitivity boost is predicted to be of great benefit for the NMR detection and quantification of low concentrations (<mM) of lactate esters and could provide a useful precursor for the production of hyperpolarized lactate, a key metabolite.

Computational 3D microscopy with optical coherence refraction tomography.

Optical coherence tomography (OCT) has seen widespread success as an in vivo clinical diagnostic 3D imaging modality, impacting areas including ophthalmology, cardiology, and gastroenterology. Despite its many advantages, such as high sensitivity, speed, and depth penetration, OCT suffers from several shortcomings that ultimately limit its utility as a 3D microscopy tool, such as its pervasive coherent speckle noise and poor lateral resolution required to maintain millimeter-scale imaging depths. Here, we present 3D optical coherence refraction tomography (OCRT), a computational extension of OCT which synthesizes an incoherent contrast mechanism by combining multiple OCT volumes, acquired across two rotation axes, to form a resolution-enhanced, speckle-reduced, refraction-corrected 3D reconstruction. Our label-free computational 3D microscope features a novel optical design incorporating a parabolic mirror to enable the capture of 5D plenoptic datasets, consisting of millimetric 3D fields of view over up to ±75° without moving the sample. We demonstrate that 3D OCRT reveals 3D features unobserved by conventional OCT in fruit fly, zebrafish, and mouse samples.

Large field-of-view non-invasive imaging through scattering layers using fluctuating random illumination

Non-invasive optical imaging techniques are essential diagnostic tools in many fields. Although various recent methods have been proposed to utilize and control light in multiple scattering media, non-invasive optical imaging through and inside scattering layers across a large field of view remains elusive due to the physical limits set by the optical memory effect, especially without wavefront shaping techniques. Here, we demonstrate an approach that enables non-invasive fluorescence imaging behind scattering layers with field-of-views extending well beyond the optical memory effect. The method consists in demixing the speckle patterns emitted by a fluorescent object under variable unknown random illumination, using matrix factorization and a novel fingerprint-based reconstruction. Experimental validation shows the efficiency and robustness of the method with various fluorescent samples, covering a field of view up to three times the optical memory effect range. Our non-invasive imaging technique is simple, neither requires a spatial light modulator nor a guide star, and can be generalized to a wide range of incoherent contrast mechanisms and illumination schemes.

Exchange scattering on ultrafast timescales in a ferromagnetic two-sublattice system

We investigate ultrafast spin dynamics due to exchange, electron–phonon and Elliott–Yafet spin-flip scattering in a model with a simple band structure and ferromagnetically coupled electronic sublattices (or more generally, subsystems). We show that this incoherent model of electronic dynamics leads to sublattice magnetization changes in opposite directions after ultrashort-pulse excitation. This prominent feature on an ultrafast timescale is related to a transfer of energy and angular momentum between the subsystems due to exchange scattering. Our calculations illustrate a possible incoherent mechanism that works in addition to the coherent optically induced spin transfer mechanism.

Peculiar Radio–X-Ray Relationship in Active Stars

Abstract The empirical relationship between the nonthermal 5 GHz radio luminosity and the soft X-ray luminosity of active stellar coronae, canonically called the Güdel–Benz relationship, has been a cornerstone of stellar radio astronomy, as it explicitly ties the radio emission to the coronal heating mechanisms. The relationship extends from microflares on the Sun to the coronae of the most active stars suggesting that active coronae are heated by a flare-like process. The relationship is thought to originate from a consistent partition of the available flare energy into relativistic charges, which emit in the radio-band via the incoherent gyrosynchrotron mechanism, and heating of the bulk coronal plasma, which emits in the X-ray band via the Bremsstrahlung mechanism. Consequently, coherent emission from stellar and substellar objects is not expected to adhere to this empirical relationship, as it is observed in ultracool dwarf stars and brown dwarfs. Here we report a population of radio-detected chromospherically active stars that surprisingly follow the Güdel–Benz relationship despite their radio emission being classified as coherent emission by virtue of its high circularly polarized fraction and high brightness temperature. Our results prompt a reexamination of the physics behind the Güdel–Benz relationship, its implication for the mechanism of coronal heating and particle acceleration in active stars, and the phenomenological connection between solar and stellar flares.

Common Origin of Quasi-Periodic Pulsations in Microwave and Decimetric Solar Radio Bursts

We analyse quasi-periodic pulsations (QPP) detected in the microwave and decimeter radio emission of the SOL2017-09-05T07:04 solar flare, using simultaneous observations by the Siberian Radioheliograph 48 (SRH-48, 4-8 GHz) and Mingantu Spectral Radioheliograph (MUSER-I, 0.4-2 GHz). The microwave emission was broadband with a typical gyrosynchrotron spectrum, while a quasi-periodic enhancement of the decimetric emission appeared in a narrow spectral band (500-700 MHz), consistent with the coherent plasma emission mechanism. The periodicity that we found in microwaves is about 30 s, coming from a compact loop-like source with a typical height of about 31 Mm. The decimetric emission demonstrated a periodicity about 6 s. We suggested a qualitative scenario linking the QPPs observed in both incoherent and coherent spectral bands and their generation mechanisms. The properties of the QPPs found in the microwave signal are typical for perturbations of the flare loop by the standing sausage mode of a fast magnetohydrodynamic (MHD) wave. Our analysis indicated that this sausage-oscillating flare loop was the primary source of oscillations in the discussed event. The suggested scenario is that a fundamental sausage harmonic is the dominant cause for the observed QPPs in the microwave emission. The initiation of oscillations in the decimetric emission is caused by the third sausage harmonic via periodic and nonlinear triggering of the acceleration processes in the current sheets, formed at the interface between the sausage-oscillating flare loop and the external coronal loop that extended to higher altitudes. Our results demonstrate the possible role of MHD wave processes in the release and transport of energy during solar flares, linking coherent and incoherent radio emission mechanisms.

Relaxation of Plasma Excitations in Two-Dimensional Electron Systems

An investigation is performed of the relaxation of plasma excitations in two-dimensional electron systems (2D-ESes) in GaAs/AlGaAs heterostructures. The effect radiational and incoherent collisional relaxation mechanisms have on the linewidth of cyclotron magnetoplasma resonance (CR) is studied. CR arises as a pure resonance that does not hybridize with dimensional magnetoplasma excitations. It is shown how magnetoplasma resonances form a CR’s fine structure due to the interaction between coherent radiative and incoherent collisional mechanisms of two-dimensional plasma relaxation. A comparative analysis is performed of the dependences of cyclotron and transport periods of relaxation on both the temperature and electron density of 2D-ESes. It is demonstrated that the period of cyclotron relaxation could exceed that of transport at low electron densities.

Radio Measurements of the Magnetic Field in the Solar Chromosphere and the Corona

The structure of the upper solar atmosphere, on all observable scales, is intimately governed by the magnetic field. The same holds for a variety of solar phenomena that constitute solar activity, from tiny transient brightening to huge Coronal Mass Ejections. Due to inherent difficulties in measuring magnetic field effects on atoms (Zeeman and Hanle effects) in the corona, radio methods sensitive to electrons are of primary importance in obtaining quantitative information about its magnetic field. In this review we explore these methods and point out their advantages and limitations. After a brief presentation of the magneto-ionic theory of wave propagation in cold, collisionless plasmas, we discuss how the magnetic field affects the radio emission produced by incoherent emission mechanisms (free-free, gyroresonance, and gyrosynchrotron processes) and give examples of measurements of magnetic filed parameters in the quiet sun, active regions and radio CMEs. We proceed by discussing how the inversion of the sense of circular polarization can be used to measure the field above active regions. Subsequently we pass to coherent emission mechanisms and present results of measurements from fiber bursts, zebra patterns, and type II burst emission. We close this review with a discussion of the variation of the magnetic field, deduced by radio measurements, from the low corona up to ~ 10 solar radii and with some thoughts about future work.

Single-pixel fluorescent diffraction tomography.

Optical diffraction tomography (ODT) is an indispensable tool for studying objects in three dimensions. Until now, ODT has been limited to coherent light because spatial phase information is required to solve the inverse scattering problem. We introduce a method that enables ODT to be applied to imaging incoherent contrast mechanisms such as fluorescent emission. Our strategy mimics the coherent scattering process with two spatially coherent illumination beams. The interferometric illumination pattern encodes spatial phase in temporal variations of the fluorescent emission, thereby allowing incoherent fluorescent emission to mimic the behavior of coherent illumination. The temporal variations permit recovery of the spatial distribution of fluorescent emission with an inverse scattering model. Simulations and experiments demonstrate isotropic resolution in the 3D reconstruction of a fluorescent object.

Large Increase in the Dielectric Constant and Partial Loss of Coherence Increases Tunneling Rates across Molecular Wires.

Although the dielectric behavior of monolayers is important in a large range of applications, its role in charge transport studies involving molecular junctions is largely ignored. This paper describes a large increase in the relative static dielectric constant (εr) by simply increasing the thickness of well-organized monolayers of oligoglycine and oligo(ethylene glycol) from 7 up to 14. The resulting large capacitance of 3.5-5.1 μF/cm2 is thickness-independent, which is highly attractive for field-effect transistor applications. This increase of εr results in a linear increase of the thermal activation energy by a factor of 6, which suggests that the mechanism of charge transport gradually changes from coherent to (partially) incoherent tunneling. The comparisons of oligoglycine (which readily forms hydrogen bonds with neighboring molecules) and methyl terminated oligo(ethylene glycol) (which lacks hydrogen bond donors) monolayers, kinetic isotope effects, and relative humidity-dependent measurements all indicate the importance of strong hydrogen bonds involving ionic species and strongly bonded water in the unusual dielectric behavior and the incoherent tunneling mechanism. This partial loss of coherence of the charge carriers can explain the unusually small tunneling decay coefficients across long molecular wires, and the length-dependent increase of εr of monolayers opens up interesting new applications.

Coherence-assisted electron diffusion across the multi-heme protein-based bacterial nanowire

Biological electron transfer (ET) is one of the most studied biochemical processes due to its immense importance in biology. For many years, biological ET was explained using the classical incoherent transport mechanism, i.e. sequential hopping. One of the relatively recent major observations in this field is long-range extracellular ET (EET), where some bacteria were shown to mediate electrons for extremely long distances on the micrometer length scales across individual nanowires. This fascinating finding has resulted in several suggested mechanisms that might explain this intriguing EET. More recently, the structure of a conductive G. sulfurreducens nanowire has been solved, which showed a highly ordered quasi-1D wire of a hexaheme cytochrome protein, named OmcS. Based on this new structure, we suggest here several electron diffusion models for EET, involving either purely hopping or several degrees of mixed hopping and coherent transport, in which the coherent part is due to a local rigidification of the protein structure, associated with a decrease in the local reorganization energy. The effect is demonstrated for two closely packed heme sites as well as for longer chains containing up to several dozens porphyrins. We show that the pure hopping model probably cannot explain the reported conductivity values of the G. sulfurreducens nanowire using conventional values of reorganization energy and electronic coupling. On the other hand, we show that for a wide range of the latter energy values, the mixed hopping-coherent model results in superior electron diffusion compared to the pure hopping model, and especially for long-range coherent transport, involving multiple porphyrin sites.

Transition between coherent and incoherent chirping mechanisms in electron-positron pair creation

We examine the effect of a frequency-chirped external force field on the final energy that has been absorbed by two classical mechanical oscillators, by quantum mechanical two- and three-level systems, and by electron-positron pairs that were created from the quantum field theoretical Dirac vacuum. By comparing the final dynamical responses to the original force field with that associated with the corresponding time-reversed field, we can test the sensitivity of each of these five systems to the temporal phase information contained in the field. We predict that the linear oscillator, the two-level atom, and the pair-creation process triggered by a spatially homogeneous field are remarkably immune to this phase, whereas the quartic oscillator, the three-level atom, or the pair-creation process caused by a space-time field absorb the provided energy differently depending on the temporal details of the external field.

Properties of M Dwarf Flares at Millimeter Wavelengths

Abstract We report on two millimeter flares detected by the Atacama Large Millimeter/submillimeter Array at 220 GHz from AU Mic, a nearby M dwarf. The larger flare had a duration of only ∼35 s, with peak L R = 2 × 1015 erg s−1 Hz−1, and lower limit on linear polarization of . We examine the characteristics common to these new AU Mic events and those from Proxima Cen previously reported in MacGregor et al.—namely short durations, negative spectral indices, and significant linear polarization—to provide new diagnostics of conditions in outer stellar atmospheres and details of stellar flare particle acceleration. The event rates (∼20 and 4 events days−1 for AU Mic and Proxima Cen, respectively) suggest that millimeter flares occur commonly but have been undetected until now. Analysis of the flare observing frequency and consideration of possible incoherent emission mechanisms confirms the presence of MeV electrons in the stellar atmosphere occurring as part of the flare process. The spectral indices point to a hard distribution of electrons. The short durations and lack of pronounced exponential decay in the light curve are consistent with formation in a simple magnetic loop, with radio emission predominating from directly precipitating electrons. We consider the possibility of both synchrotron and gyrosynchrotron emission mechanisms, although synchrotron is favored given the linear polarization signal. This would imply that the emission must be occurring in a low density environment of only modest magnetic field strength. A deeper understanding of this newly discovered and apparently common stellar flare mechanism awaits more observations with better-studied flare components at other wavelengths.

Testing the Radiation Pattern of Meteor Radio Afterglow

AbstractRadio emission from meteors or meteor radio afterglows (MRAs) was first detected using the all‐sky imaging capabilities of the first station of the Long Wavelength Array (LWA1). In this work, we use the recently commissioned LWA Sevilleta (LWA‐SV) station along with the LWA1 to carry out coordinated observations. The combined all‐sky observations with LWA1 and LWA‐SV have coobserved 32 MRAs and 21 transmitter reflections from meteors (meteor scatter events), which are believed to be specular reflections from overdense trails. The flux density of the events observed by each station was measured from the all‐sky images. Triangulating the angular direction of events from each station gave the physical location and the distance of the event to each station. The luminosity of the events in each station was calculated using the flux distance relation for an isotropic source. The luminosity distribution for MRAs and meteor scatter events observed by each station shows a clear distinction between these two types of events as the ratio of luminosities is closer to unity for MRAs than the meteor scatter events. Furthermore, we find that MRAs follow an isotropic radiation pattern. This suggests, either a complete incoherent emission mechanism or an incoherent addition of coherently emitting small regions within the meteor trail.

Energy Fluctuations Induced Quantum Decoherence and Exciton Localization in Singlet Fission

Both quantum coherent and incoherent mechanisms have been revealed in singlet exciton fission. Also, in some systems, both mechanisms may concurrently operate. However, the comprehensive picture is...

Noninvasive light focusing in scattering media using speckle variance optimization

Optical imaging deep inside scattering media remains a fundamental problem in bio-imaging. While wavefront shaping has been shown to allow focusing of coherent light at depth, achieving it non-invasively remains a challenge. Various feedback mechanisms, in particular acoustic or non-linear fluorescence-based, have been put forward for this purpose. Non-invasive focusing at depth on fluorescent objects with linear excitation is, however, still unresolved. Here we report a simple method for focusing inside a scattering medium in an epi-detection geometry with a linear signal: optimizing the spatial variance of low contrast speckle patterns emitted by a set of fluorescent sources. Experimentally, we demonstrate robust and efficient focusing of scattered light on a single source, and show that this variance optimization method is formally equivalent to previous optimization strategies based on two-photon fluorescence. Our technique should generalize to a large variety of incoherent contrast mechanisms and holds interesting prospects for deep bio-imaging.