AbstractThe possibility of using metals from mining activity as tracers for identifying stream sediment sources is explored. Sampling of monthly bed sediment yield and of the spatial and temporal variation in Pb concentration was undertaken in a 1·02 km2 catchment, and estimates of the sediment contribution from different stream reaches are calculated. The method has considerable limitations, for metal concentrations are notably dependent on sediment size, season, source availability, and the chemical mobility of the metal used. In most natural streams these must preclude the use of pollutants for simple sediment source identification.