Identical Photons Research Articles

Engineering quantum states from a spatially structured quantum eraser.

Quantum interference is a central resource in many quantum-enhanced tasks, from computation to communication. While usually occurring between identical photons, it can also be enabled by performing projective measurements that render the photons indistinguishable, a process known as quantum erasing. Structured light forms another hallmark of photonics, achieved by manipulating the degrees of freedom of light, and enables a multitude of applications in both classical and quantum regimes. By combining these ideas, we design and experimentally demonstrate a simple and robust scheme that tailors quantum interference to engineer photonic states with spatially structured coalescence along the transverse profile, a type of quantum mode with no classical counterpart. To achieve this, we locally tune the distinguishability of a photon pair by spatially structuring the polarization and creating a structured quantum eraser. We believe that these spatially engineered multiphoton quantum states may be of significance in fields such as quantum metrology, microscopy, and communication.

Tunable single-photon emitters in 2D materials.

Single-photon emitters (SPEs) hold the key to many quantum technologies including quantum computing. In particular, developing a scalable array of identical SPEs can play an important role in preparing single photons - crucial resources for computation - at a high rate, allowing to improve the computational capacity. Recently, different types of SPEs have been found in various 2D materials. Towards realizing scalable SPE arrays in 2D materials for quantum computation, it is required to develop tunable SPEs that can produce identical photons by precisely controlling emission properties. Here, we present a brief review of the recent progress on various tuning methods in different 2D materials. Firstly, we discuss the operation principle of different 2D SPEs along with their unique characteristics. Secondly, we introduce various dynamic strain engineering methods for tuning the emission wavelengths in 2D SPEs. We also present several electric field-induced wavelength tuning methods for 2D SPEs. Lastly, we discuss the outlook of dynamically tunable 2D SPEs towards scalable 2D SPE arrays for realizing practical quantum photonics applications.

Generation and characterization of polarization-entangled states using quantum dot single-photon sources

Single-photon sources based on semiconductor quantum dots find several applications in quantum information processing due to their high single-photon indistinguishability, on-demand generation, and low multiphoton emission. In this context, the generation of entangled photons represents a challenging task with a possible solution relying on the interference in probabilistic gates of identical photons emitted at different pulses from the same source. In this work, we implement this approach via a simple and compact design that generates entangled photon pairs in the polarization degree of freedom. We operate the proposed platform with single photons produced through two different pumping schemes, the resonant excited one and the longitudinal-acoustic phonon-assisted configuration. We then characterize the produced entangled two-photon states by developing a complete model taking into account relevant experimental parameters, such as the second-order correlation function, Hong–Ou–Mandel visibility, multiphoton emission and pump laser filtering. Our source shows long-term stability and high quality of the generated entangled states, thus constituting a reliable building block for optical quantum technologies.

Boson bunching is not maximized by indistinguishable particles

Boson bunching is among the most remarkable features of quantum physics. A celebrated example in optics is the Hong–Ou–Mandel effect, where the bunching of two photons arises from a destructive quantum interference between the trajectories where they both either cross a beamsplitter or are reflected. This effect takes its roots in the indistinguishability of identical photons. Hence, it is generally admitted—and experimentally verified—that bunching vanishes as soon as photons can be distinguished, for example, when they occupy distinct time bins or have different polarizations. Here we disprove this alleged straightforward link between indistinguishability and bunching by exploiting a recent finding in the theory of matrix permanents. We exhibit a family of optical circuits such that the bunching of photons into two modes can be substantially boosted by making them partially distinguishable via an appropriate polarization pattern. This boosting effect is already visible in a seven-photon interferometric process, making the observation of this phenomenon within reach of current photonic technology. This unexpected behaviour questions our understanding of multiparticle interference in the grey zone between indistinguishable bosons and classical particles. A common belief about boson bunching—fully indistinguishable bosons exhibit the utmost bunching—is theoretically disproved with seven photons of distinct polarization in a seven-mode interferometric process. Enhanced bunching could thus be observed with partially distinguishable photons.

Multiple Tin-Vacancy Centers in Diamond with Nearly Identical Photon Frequency and Linewidth

Tin-vacancy (Sn-$V$) centers in diamond, which possess good optical and spin properties, are a promising system for constructing quantum network nodes. Tin atoms are heavy, though, and generating photons with identical wavelength and linewidth from multiple Sn-$V$ emitters is challenging, due to the strain in the diamond host material. This study shows that multiple Sn-$V$ centers, formed deep within bulk diamond by ion implantation and high-temperature annealing, emit nearly identical photons. This leads to two-photon interference from distant centers, an important step toward building quantum network nodes.

Perfect splitting of a two-photon pulse

We employ a cascaded system approach to numerically simulate the interaction of photon pulses with a two-level scatterer in a chiral waveguide QED setup and show that the scattering of a two-photon pulse may lead to the predominant population of only two output wave packet modes in an entangled state, $|2,0\ensuremath{\rangle}--|0,2\ensuremath{\rangle}$. In a complementary wave-packet basis, this is a product state of two orthogonal single-photon wave packets. Operating this process in reverse allows a perfect merging of distinguishable single-photon wave packets into a single-mode pulse carrying two identical photons.

Possibilities of Multiphoton Microscopy in Semiconductor Nanomaterials Research

Multiphoton microscopy is the method using nonlinear optical effect which is two-photon absorption. It occurs when two identical photons are absorbed simultaneously. The photon energy should be around two times smaller than the photon energy for one-photon absorption. Thus, the excitation irradiation wavelength for multiphoton microscopy should be twice that for conventional confocal microscopy. Nowadays, multiphoton microscopy is widely used for biological research, but it is possible to apply this for non-biological materials studying, particularly, for solid-state materials and structures. Low-wavelength laser irradiation deep penetration, focusing and optical signal analysis possibility provides essential new challenges solving of hierarchical "smart" nanoparticles synthesis for target drug delivery, theranostics etc. In this paper we give an answer of some most popular questions about multiphoton microscopy. Nature and aspects of the multiphoton microscopy method were described. Advantages of this method in comparison with confocal microscopy method were shown. Multiphoton microscopy gives the best image contrast and the less photodamage and photobleaching of biological samples, and provides an opportunity of three-dimensional imaging of the biomaterials as well as the solid-state materials. Additionally, capabilities of this method for solid-state materials research were demonstrated by the porous silicon samples example. Also, multiphoton microscopy images of biological objects were shown.

Simulation of thermal fragility of vacuum squeezing in two photon lossy cavity

In this research, squeezing fragility due to thermal bath, in quantum squeezed state generation, is simulated. For this purpose, single mode dissipative cavity with non-zero second-order susceptibility is used. Cavity nonlinear medium is driving by laser pump with known frequency, and pairs of identical photons are created, with one-half frequency of driving pump. This process known as degenerate parametric down conversion. In the absence of any dissipation, simulation shows linear time dependent squeezing parameter, which is in agreement with theoretical results. In two photon loss of cavity in contact with cold reservoir, competition between gain and two photon loss, results in stable squeezing of initial vacuum, in steady state of system. At the end, has been shown that, non-zero thermal reservoir, omits the squeezing and leads the final cavity field to the thermal mixture of Fock states.

Distillation of Indistinguishable Photons.

A reliable source of identical (indistinguishable) photons is a prerequisite for exploiting interference effects, which is a necessary component for linear optical based quantum computing, and applications thereof such as Boson sampling. Generally speaking, the degree of distinguishability will determine the efficacy of the particular approach, for example by limiting the fidelity of constructed resource states, or reducing the complexity of an optical circuits output distribution. It is therefore of great practical relevance to engineer heralded sources of highly pure and indistinguishable photons. Inspired by magic state distillation, we present a protocol using standard linear optics which can be used to increase the indistinguishability of a photon source, to arbitrary accuracy. In particular, in the asymptotic limit of small error ε, to reduce the error to ε^{'}<ε requires O((ε/ε^{'})^{2}) photons. We demonstrate the scheme is robust to detection and control errors in the optical components, and discuss the effect of other error sources.

Entangling three identical particles via spatial overlap.

Quantum correlations between identical particles are at the heart of quantum technologies. Several studies with two identical particles have shown that the spatial overlap and indistinguishability between the particles are necessary for generating bipartite entanglement. On the other hand, researches on the extension to more than two-particle systems are limited by the practical difficulty to control multiple identical particles in laboratories. In this work, we propose schemes to generate two fundamental classes of genuine tripartite entanglement, i.e., GHZ and W classes, which are experimentally demonstrated using linear optics with three identical photons. We also show that the tripartite entanglement class decays from the genuine entanglement to the full separability as the particles become more distinguishable from each other. Our results support the prediction that particle indistinguishability is a fundamental element for entangling identical particles.

Quantum interference of identical photons from remote GaAs quantum dots

Photonic quantum technology provides a viable route to quantum communication1,2, quantum simulation3 and quantum information processing4. Recent progress has seen the realization of boson sampling using 20 single photons3 and quantum key distribution over hundreds of kilometres2. Scaling the complexity requires architectures containing multiple photon sources, photon counters and a large number of indistinguishable single photons. Semiconductor quantum dots are bright and fast sources of coherent single photons5-9. For applications, a roadblock is the poor quantum coherence on interfering single photons created by independent quantum dots10,11. Here we demonstrate two-photon interference with near-unity visibility (93.0 ± 0.8)% using photons from two completely separate GaAs quantum dots. The experiment retains all the emission into the zero phonon line-only the weak phonon sideband is rejected; temporal post-selection is not employed. By exploiting quantum interference, we demonstrate a photonic controlled-not circuit and an entanglement with fidelity of (85.0 ± 1.0)% between photons of different origins. The two-photon interference visibility is high enough that the entanglement fidelity is well above the classical threshold. The high mutual coherence of the photons stems from high-quality materials, diode structure and relatively large quantum dot size. Our results establish a platform-GaAs quantum dots-for creating coherent single photons in a scalable way.

How to administer an antidote to Schrödinger’s cat

In his 1935 Gedankenexperiment, Erwin Schrödinger imagined a box with a cat and a poisonous substance which has a 50% probability of being released, based on the decay of a radioactive atom. As such, the life of the cat and the state of the poison become entangled, and the fate of the cat is determined upon opening the box. We present an experimental technique that keeps the cat alive on any account. This method relies on the time-resolved Hong–Ou–Mandel effect: two long, identical photons impinging on a beam splitter always bunch in either of the outputs. Interpreting the first photon detection as the state of the poison, the second photon is identified as the state of the cat. Even after the collapse of the first photon’s state, we show their fates are intertwined through quantum interference. We demonstrate this by a sudden phase change between the inputs, administered conditionally on the outcome of the first detection, which steers the second photon to a pre-defined output and ensures that the cat is always observed alive.

Enhanced Emission from Bright Excitons in Asymmetrically Strained Colloidal CdSe/CdxZn1-xSe Quantum Dots.

Colloidal CdSe quantum dots (QDs) designed with a high degree of asymmetric internal strain have recently been shown to host a number of desirable optical properties including subthermal room-temperature line widths, suppressed spectral diffusion, and high photoluminescence (PL) quantum yields. It remains an open question, however, whether they are well-suited for applications requiring emission of identical single photons. Here we measure the low-temperature PL dynamics and the polarization-resolved fluorescence line narrowing spectra from ensembles of these strained QDs. Our spectroscopy reveals the radiative recombination rates of bright and dark excitons, the relaxation rate between the two, and the energy spectra of the quantized acoustic phonons in the QDs that can contribute to relaxation processes. In comparison to conventional colloidal CdSe/ZnS core/shell QDs, we find that in asymmetrically strained CdSe QDs over six times more light is emitted directly by the bright exciton. These results are therefore encouraging for the prospects of chemically synthesized colloidal QDs as emitters of single indistinguishable photons.

Scalable integrated single-photon source.

Photonic qubits are key enablers for quantum information processing deployable across a distributed quantum network. An on-demand and truly scalable source of indistinguishable single photons is the essential component enabling high-fidelity photonic quantum operations. A main challenge is to overcome noise and decoherence processes to reach the steep benchmarks on generation efficiency and photon indistinguishability required for scaling up the source. We report on the realization of a deterministic single-photon source featuring near-unity indistinguishability using a quantum dot in an "on-chip" planar nanophotonic waveguide circuit. The device produces long strings of >100 single photons without any observable decrease in the mutual indistinguishability between photons. A total generation rate of 122 million photons per second is achieved, corresponding to an on-chip source efficiency of 84%. These specifications of the single-photon source are benchmarked for boson sampling and found to enable scaling into the regime of quantum advantage.

Theory of HOM interference on coupled waveguides.

It is well known that the Hong-Ou-Mandel (HOM) effect can be realized on beam splitters (BSs) in the form of coupled waveguides. It is believed that in this case, the theory is similar to HOM interference on conventional BSs. In this work, it is shown that if a BS is used in the form of a coupled waveguide, the theory of HOM interference can differ significantly from the known one. It is shown that even in the case of completely identical photons, the visibility of V can essentially differ from unity. The developed theory must be taken into account in quantum optical schemes, where BSs are represented mainly as coupled waveguides.

Photon-mediated entanglement scheme between a ZnO semiconductor defect and a trapped Yb ion

We propose an optical scheme to generate an entangled state between a trapped ion and a solid state donor qubit through which-path erasure of identical photons emitted from the two systems. The proposed scheme leverages the similar transition frequencies between In donor bound excitons in ZnO and the P21/2 to S21/2 transition in Yb+. The lifetime of the relevant ionic state is longer than that of the ZnO system by a factor of 6, leading to a mismatch in the temporal profiles of emitted photons. A detuned cavity-assisted Raman scheme weakly excites the donor with a shaped laser pulse to generate photons with a 0.99 temporal overlap to the Yb+ emission and partially shift the emission of the defect toward the Yb+ transition. The remaining photon shift is accomplished via the dc Stark effect. We show that an entanglement rate of 2.1×104 s−1 and an entanglement fidelity of 94% can be attained using a weak excitation scheme with reasonable parameters.

Bohmian-Based Approach to Gauss-Maxwell Beams

Usual Gaussian beams are particular scalar solutions to the paraxial Helmholtz equation, which neglect the vector nature of light. In order to overcome this inconvenience, Simon et al. (J. Opt. Soc. Am. A 1986, 3, 536–540) found a paraxial solution to Maxwell’s equation in vacuum, which includes polarization in a natural way, though still preserving the spatial Gaussianity of the beams. In this regard, it seems that these solutions, known as Gauss-Maxwell beams, are particularly appropriate and a natural tool in optical problems dealing with Gaussian beams acted or manipulated by polarizers. In this work, inspired in the Bohmian picture of quantum mechanics, a hydrodynamic-type extension of such a formulation is provided and discussed, complementing the notion of electromagnetic field with that of (electromagnetic) flow or streamline. In this regard, the method proposed has the advantage that the rays obtained from it render a bona fide description of the spatial distribution of electromagnetic energy, since they are in compliance with the local space changes undergone by the time-averaged Poynting vector. This feature confers the approach a potential interest in the analysis and description of single-photon experiments, because of the direct connection between these rays and the average flow exhibited by swarms of identical photons (regardless of the particular motion, if any, that these entities might have), at least in the case of Gaussian input beams. In order to illustrate the approach, here it is applied to two common scenarios, namely the diffraction undergone by a single Gauss-Maxwell beam and the interference produced by a coherent superposition of two of such beams.

A Bayesian validation approach to practical boson sampling

Boson sampling is a promising candidate for demonstrating quantum supremacy. The validation that involves judging whether a quantum setup outputs photons following the boson sampling model is an essential task in the experiments. However, the current validation methods may result in an incorrect conclusion being reached in realistic experiments, in which no ideally identical photons exist. Accordingly, this study proposes a slope-based approach, which is an extended Bayesian validation, to model the degree of photon indistinguishability. Through numerical simulations and performance evaluations, we demonstrate that the proposed approach can correctly validate boson sampling against the distribution of classical particles. In addition to offering a useful approach for validation, our research indicates that physicists should pay more attention to the quality of photon indistinguishability in boson sampling experiments.

Hong-Ou-Mandel interferometry on a biphoton beat note

Hong-Ou-Mandel interference, the fact that identical photons that arrive simultaneously on different input ports of a beam splitter bunch into a common output port, can be used to measure optical delays between different paths. It is generally assumed that great precision in the measurement requires that photons contain many frequencies, i.e., a large bandwidth. Here we challenge this “well-known” assumption and show that the use of two well-separated frequencies embedded in a quantum entangled state (discrete color entanglement) suffices to achieve great precision. We determine optimum working points using a Fisher Information analysis and demonstrate the experimental feasibility of this approach by detecting thermally-induced delays in an optical fiber. These results may significantly facilitate the use of quantum interference for quantum sensing, by avoiding some stringent conditions such as the requirement for large bandwidth signals.

Creating photonic GHZ and W states via quantum walk

We propose schemes for preparing W and GHZ photonic states entangled in polarization via quantum walks, where the trajectory exchanging of identical photons plus postselection induces the coupling between their polarization degrees of freedom. Being different from the polarization beam splitter-based approach, the indistinguishability of identical photons provides an alternative for coupling photons, which is more phase stable and may induce richer actions than the traditional polarization beam splitter on input photons. Our schemes demonstrate that this new coupling mechanism for photons is originated from the fact that trajectory-exchanging operation plus postselection can extract entangled states from the initially product states, and this new coupling mechanism may find considerable potential applications in both quantum communication and quantum computation.