Abstract. In this study, which is the third part of the HaloCam series after Forster et al. (2017, 2020), we present a novel technique to retrieve quantitative information about ice crystal optical and microphysical properties using ground-based imaging observations of halo displays. Comparing HaloCam's calibrated RGB images of 22 and 46∘ halo observations against a lookup table of simulated radiances, this technique allows the retrieval of the sizes and shapes of randomly oriented crystals as well as the fraction of smooth and rough ice crystals for cirrus clouds. We analyzed 4400 HaloCam images between September 2015 and November 2016 showing a visible 22∘ halo. The optical properties of hexagonal 8-element aggregates of columns with a mean ice crystal effective radius of about 20 µm and a mixture of 37 % smooth and 63 % rough crystals on average best match the HaloCam observations. Implemented on different sites, HaloCam in combination with the machine-learning-based halo detection algorithm HaloForest can provide a consistent dataset for climatological studies of ice crystal properties representing typical cirrus clouds. Representative ice crystal optical properties are required for remote sensing of cirrus clouds as well as climate modeling. Since ground-based passive imaging observations provide information about the forward scattering part of the ice crystal optical properties, the results of this work ideally complement the results of satellite-based and airborne studies.
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