Huguangyan Maar Lake Research Articles

Major Holocene cryptotephras layers identified from Jeju Island, Republic of Korea: Implications for regional volcanic eruptions and environmental changes

Cryptotephras recorded in sediments are valuable isochrons with which to reconstruct volcanic eruptive history and synchronize environmental changes across large regions. Here we identify four cryptotephras from Jeju Island, Republic of Korea, that constitute tie-points linking palaeoenvironmental records of tropical to mid-latitude east Asia. A cryptotephra of unknown source with trachytic glass compositions at around 2700 cal a BP (named M263a) can be correlated with the HGY263 recorded in the Huguangyan Maar lake in southern China, and SG14–0433 recorded in Suigetsu lake in central Japan. Another population of glass shards with basaltic andesitic to trachybasaltic composition (named M263b) represents the first cryptotephra record of a Jeju eruption. A rhyolitic cryptotephra at ∼7384 cal a BP (H53) can be correlated with the ∼7.3 ka Kikai-Akahoya eruption (specifically, the K-Ah tephra) from Kikai caldera, southern Kyushu, Japan. The cryptotephra coincides with a marked change in aquatic algae communities in Jeju sediments, possibly signifying a climate response to the eruption. Additionally, cryptotephra layers at ∼6948 cal a BP (H22) in the Hanon Maar Lake and ∼ 1030 cal a BP (M125) in Mulyoungari wetland exhibit similar glass compositions to those of the K-Ah tephra, which suggests they are the product of unknown eruptions from Kikai or a neighboring volcano. Given the widespread distributions of K-Ah and M263a tephra across east Asia, Jeju sediments can be precisely synchronized with those high-resolution sediments from southern China and Japan, providing two Holocene marker horizons for palaeoenvironmental comparisons across east Asia. Our work shows great promise for the improved chronological constraints and inter-site linkages for palaeoenvironmental sequences in the region through the application of tephrochronology.

Centennial Records of Microplastics in Lake Cores in Huguangyan Maar Lake, China.

Microplastic records from lake cores can reconstruct the plastic pollution history. However, the associations between anthropogenic activities and microplastic accumulation are not well understood. Huguangyan Maar Lake (HML) is a deep-enclosed lake without inlets and outlets, where the sedimentary environment is ideal for preserving a stable and historical microplastic record. Microplastic (size: 10-500 μm) characteristics in the HML core were identified using the Laser Direct Infrared Imaging system. The earliest detectable microplastics appeared unit in 1955 (1.1 items g-1). The microplastic abundance ranged from n.d. to 615.2 items g-1 in 1955-2019 with an average of 134.9 items g-1. The abundance declined slightly during the 1970s and then increased rapidly after China's Reform and Opening Up in 1978. Sixteen polymer types were detectable, with polyethylene and polypropylene dominating, accounting for 23.5 and 23.3% of the total abundance, and the size at 10-100 μm accounted for 80%. Socioeconomic factors dominated the microplastic accumulation based on the random forest modeling, and the contributions of GDP per capita, plastic-related industry yield, and total crop yield were, respectively, 13.9, 35.1, and 9.3% between 1955-2019. The total crop yield contribution further increased by 1.7% after 1978. Coarse sediment particles increased with soil erosion exacerbated microplastics discharging into the sediment.

Source appointment of δ13C in sediments of a maar lake in southern China: Implications of fossil fuel CO2 emissions

Stable carbon isotopes (δ13C) in lake sediments can record changes in CO2 emissions from fossil fuels (FFs) combustion; however, the exact proportion of δ13C changes caused by FFs combustion remains unclear. Here, taking the Huguangyan Maar Lake (HGY) located in low latitude with high intensity of human activities in southern China as an example, we used the MixSIAR Bayesian stable isotope mixing model to trace the source change of δ13C in the HGY sediments over the past 130 years. The δ13C value, ranging from −20.23‰ to −24.29‰, with an average of −22.39 ± 1.5‰, displayed a continuous downward trend from the bottom to top throughout the core, with the fastest decline occurring between 1950AD and 1996AD. Quantitative source appointment indicates that the contribution of FFs sources to δ13C depletion in the HGY sediments has increased nearly three-fold over the past 130 years, from 18.6% to 67.8%, which may be related to the Suess Effect of the 13C-depleted FFs burning. The increase in δ13C in HGY sediments in the past decade was consistent with the increase in δ13C–CO2 emitted by global fossil-fuel consumption, and was also related to the decrease in fossil fuels consumption caused by China's Clean Air Act. This study demonstrates that the isotope traceability model is helpful for source appointment of δ13C in lake sediments and that the δ13C in maar lake sediments can be used to trace CO2 emissions from global FFs combustion. This therefore provides new insights on the carbon cycle during the Anthropocene.

Millennial and suborbital-scale El Niño/Southern Oscillation control of climate variability in southern China over the past 70 ka

Hydroclimatic changes in East Asia on suborbital and millennial time scales have been shown to be highly uncertain. The El Niño-Southern Oscillation (ENSO) activity plays a key role in precipitation in low-latitude East Asia on interannual and interdecadal time scales. However, there remained some ambiguity about their connection on millennial and suborbital time scales. This study comprehensively explored the multifaceted relationships between ENSO activities, suborbital and millennial-scale drought events, and hydroclimatic variations within the Huguangyan Maar Lake (HML) region during the past 70 ka. Four suborbital-scale dry and wet hydroclimatic phases interspersed with ten millennial-scale extreme dry intervals were revealed by the ratio of hematite and goethite (Hem/Goe). These stages and intervals unexpectedly coupled with the zonal sea surface temperature (ΔSST) of the tropical Pacific Ocean, underscored the complex spatial and temporal dynamics of ENSO impacts. We propose the “glacial-El Niño-arid” and “interglacial-La Niña-humid” hydroclimate patterns on the suborbital scale. While on the millennial-scale, La Niña-like fluctuations during the persistent cold period (16–40 ka) increased the frequency and intensity of droughts in low-latitude East Asia, which was in stark contrast to the wet climate in northern China. The dynamic relationship underpins a millennia-spanning La Niña-drought pattern, elucidating the intertwined nature of ENSO dynamics and hydroclimatic variability on both sub-orbital and millennial scales. The above findings can be attributed to changes in the location and intensity of the Western Pacific subtropical high (WPSH) over southern China induced by persistent mean ENSO-like states in the tropical Pacific. This also indicates that the hydroclimate in low-latitude East Asia is more sensitive to variations in tropical ENSO compared to northern China.

Climate-vegetation-erosion interactions revealed by the sediments of Huguangyan Maar Lake, southern China

Soil erosion is a serious environmental problem in the red soil region of southern China, yet little is known about the factors responsible and their specific effects on long-term soil erosion dynamics in this region. We addressed this issue via a study of the sediments of Huguangyan Maar Lake (HML), a crater lake in southern China. Our results confirm that the sediments in HML are mainly derived from the erosional input of weathering products of wall rocks, via catchment runoff. Having established the provenance of the HML sediments, the sediment accumulation rate, mass accumulation rate, and geochemical element fluxes were used to reconstruct soil erosion processes in the HML catchment over the past ∼1400 years. The potential drivers of soil erosion were explored, and regional comparisons were made to evaluate the representativeness of this study. The results show that: 1) Higher precipitation before ∼830 CE, coupled with a lower level of human activity, promoted increased vegetation coverage which reduced the rate of soil erosion. 2) Lower precipitation during 830 CE–1390 CE reduced the rate of soil loss. 3) Abundant precipitation was the main cause of the more intense soil erosion during 1390 CE–1878 CE, which may have been exacerbated by the reduced vegetation cover caused by intensive human activity. 4) During 1878 CE–2019 CE, the vegetation cover gradually recovered under the combined effects of vegetation restoration and higher precipitation, which reduced the rate of soil erosion within the HML catchment. Compared to the Chinese Loess Plateau, the erosion level in the HML catchment was relatively low during the period of intensive human activities. Overall, our results contribute to an improving understanding of the driving mechanisms of soil erosion, and they provide a guide for soil conservation measures in southern China.

Coupled temperature variations in the Huguangyan Maar Lake between high and low latitude

Coupled temperature variations in the Huguangyan Maar Lake between high and low latitude

Thermoluminescence of Natural Quartz Grains Beside Huguangyan Maar Lake

In order to study the relationship between the thermoluminescence (TL) properties of natural quartz crystals and the irradiation history, the TL test of quartz particles was carried out on volcanic ash near Huguangyan Maar Lake in Zhanjiang City. The TL glow curve and dose response of quartz were measured. The parameters of TL traps are calculated, and the activation energies corresponding to the TL peaks of 260, 310 and 365 °C of quartz grains are 1.34, 1.44 and 1.51eV, respectively. The peak position of the TL glow curve changes mildly with the increase of irradiation dose of quartz particles, indicating that the energy of a TL trap is not a single value, but an energy distribution; in the range of 355 °C to 375°C, the TL sensitivity changes greatly with the increase of the historical irradiation dose.

Sedimentary records of polycyclic aromatic hydrocarbons from three enclosed lakes in China: Response to energy structure and economic development

Historical polycyclic aromatic hydrocarbon (PAH) pollution was explored through the sedimentary records of three lakes: Huguangyan Maar Lake (HGY) in South China, Mayinghai Lake (MYH) in North China, and Sihailongwan Lake (SHLW) in Northeast China. In these three lakes, the PAH concentrations in sediments are still rising, showing the different trend to lakes in developed countries. PAH pollution in South China occurred from 1850, much earlier than the increases since 1980 observed in North and Northeast China. The temporal trends of PAH concentrations in lake sediments are highly correlated with local economic development. Spatially, although the region where HGY is located has the highest gross domestic product, higher fluxes of PAHs were found in MYH sediments, indicating that atmospheric PAH pollution in North China might be more serious, and that PAH pollution is not fully correlated with economic development. Source analysis suggested that the PAHs in lake sediments are mainly derived from oil leaks, coal and biomass combustion, vehicle emissions, and diagenesis. Positive matrix factorization (PMF) model revealed that the contribution of vehicle emissions and coal combustion to PAHs has increased significantly in the past 40 years. Benzo(a)pyrene equivalent (BaPE) in the surface sediments of MYH and SHLW were similar and higher than in HGY. In HGY, vehicle emissions posed the highest toxic risk, followed by coal combustion. However, in MYH, the toxicity risk of vehicle emissions was close to that of coal and biomass combustion due to the highly developed coal industry in Shanxi Province. In SHLW, the contribution of fossil fuel combustion to BaPE was significantly higher than that of biomass combustion. This study provides important information for understanding PAH pollution affected by anthropogenic activities in the Anthropocene and provides a scientific basis for formulating PAH pollution control strategies.

Meltwater Pulse1A Triggered an Extreme Cooling Event: Evidence From Southern China

AbstractMeltwater Pulse 1A injection into the North Atlantic coincided with the Bølling warming event, despite climate model simulations indicating that the Meltwater Pulse 1A should have inevitably lead to an extreme cooling in the northern hemisphere. However, so far no cooling event has been found in paleoclimate records responding to Meltwater Pulse 1A. Here we reconstruct winter temperature based on sedimentary diatoms from Huguangyan Maar Lake in tropical China. The results show that winter temperature dropped by at least 6°C within ∼100 years at 14.8 ± 0.02 ka BP, coeval with the onset of Meltwater Pulse 1A, within dating uncertainty. We argue that Meltwater Pulse 1A weakened the Atlantic Meridional Overturning Circulation (AMOC), resulting in abrupt severe cooling in the Northern Hemisphere that caused a severe winter temperature drop in East Asia by strengthening the winter monsoon. We propose that extreme cooling in winter temperature triggered the Bølling warming by stopping the freshwater release from the ice‐sheet, triggering the AMOC to recover quickly and causing the Bølling event as an overshoot under gradual forcing.

Record of heavy metals in Huguangyan Maar Lake sediments: Response to anthropogenic atmospheric pollution in Southern China

The historical atmospheric heavy metal pollution of southern China over the past 200 years was explored by analyzing radiometric dating, heavy metals, and Pb isotopes from a sediment core in Huguangyan Maar Lake. Zn, Cd, Sb, Tl, and Pb in the lake are closely related to anthropogenic activities, while Cr and Ni are mainly derived from the weathering of basalt surrounding the lake. Atmospheric Zn, Cd, Sb, and Tl increased rapidly after 1980, consistent with the local industrial development. The increase of atmospheric Pb in southern China occurred earlier than in other regions of China, with the increase after 1850. War and the use of leaded gasoline were the main causes for the rapid increase in atmospheric Pb during 1910–1950. From 1950 to 2000, the input of Pb from anthropogenic activities decreased gradually due to the stable social environment. After 2000, atmospheric Pb continued to rise due to continued industrial development. The three-end-member model of Pb isotopes indicates that coal combustion is the main source of current atmospheric Pb. The proportion of Pb derived from vehicle exhaust emissions reached a peak in the 1960s, then gradually decreased and further reduced with the ban on leaded gasoline after 2000. These results are important in identifying the sources of atmospheric heavy metal pollution and in formulating pollution control strategies.

Four widespread East Asian tephra marker horizons during early MIS 3: ∼60–50 ka tephrostratigraphy of Huguangyan Maar Lake southern China

Tephra layers from explosive eruptions can provide valuable isochronous marker horizons for paleoenvironmental studies across large regions. East Asia and Southeast Asia are host to more than half of the Earth's subaerial volcanoes, and tephras from these volcanoes offer significant numbers of widely distributed marker layers. However, the integrated tephrostratigraphic framework of this region is less refined because only limited (crypto-) tephra sequences have been established. In this study, we present a cryptotephra sequence covering the period ∼60–50 ka in East Asia from a lacustrine sediment from Huguangyan Maar Lake, southern China. Four cryptotephra layers were identified, one of which can be correlated with the ∼53.8 ka Unnan eruption (SUn) of Sambe volcano, Japan. This tephra provides a critical isochronous marker horizon for linking paleoenvironmental records from central Japan to southern China, illustrating a consistent environmental shift during early MIS 3 across this region. The three other tephras cannot be correlated with known eruptions, but glass geochemical compositions suggest that they may be from Japan or surrounding areas, implying that they too may be widely distributed around East Asia. Importantly, two of them feature at the start of MIS 3, and thus can be potentially be used to establish the synchroneity of the onset of MIS 3 around East Asia, overcoming challenges that presently hinder the dating of early MIS 3 in this region.

Magnetic properties of the surface sediments from the Huguangyan Maar Lake in tropical Southern China and the sediment source identification

ABSTRACTDeciphering the source(s) of sediment deposited in Hugunagyan Lake in South China using magnetic properties will advance our understanding of the evolution of East Asian monsoon systems. However, the source of magnetic minerals in the surface sediments of this lake is unknown, still needing further exploration. Due to simple hydrological systems, the Hugunagyan Lake provides a unique record for investigating the magnetic property of sediments and surface processes. In this study, based on the magnetic properties of 43 surface sediment, 12 surface soil, and 7 volcanic rock samples from the catchment, we demonstrate that the magnetic minerals in sediments were dominated by fine super paramagnetic magnetic particles, with coexistence of pseudo‐single‐domain states minerals. There are no signatures showing the presence of biogenic and authigenic magnetite. The magnetic properties of surface sediments display significant differences between the potential sources of aeolian dust from the loess in North China and modern surface soils in Central Asia, suggesting that the magnetic minerals mainly originate from the weathered materials in the catchment, and there are no further signals of winter monsoon‐driven aeolian dust input.

Dissolved organic carbon concentration and its seasonal variation in the Huguangyan Maar Lake of Southern China

Dissolved organic carbon concentration and its seasonal variation in the Huguangyan Maar Lake of Southern China

Multidecadal‐ to Centennial‐Scale 10Be Variations in Holocene Sediments of Huguangyan Maar Lake, South China

AbstractWe report a new high‐resolution Holocene 10Be record from Huguangyan Maar Lake in subtropical‐tropical South China, aimed to detect the atmospheric 10Be production signal in low‐latitude regions. After minimizing climatic effects by regression analyses between 10Be concentration and climatic proxies from the same archive, we successfully distinguished variations in geomagnetic field intensity and solar activity using 2,000‐year low‐ and high‐pass filtering, respectively, of the residual 10Be record (a proxy of the atmospheric 10Be production rate). The resulting 10Be‐derived record of geomagnetic field intensity is generally comparable with geomagnetic models, and the solar‐modulated 10Be signal shows significant correlations with solar activity proxies. The preservation of 10Be production signal in the sediments of this low‐latitude maar lake highlights the largely unexplored potential as well as limitations of 10Be as a tool to reconstruct variations in solar activity and geomagnetic field intensity.

Paleomagnetic Secular Variation and Relative Paleointensity During the Holocene in South China—Huguangyan Maar Lake Revisited

AbstractThe scarcity of reliable paleomagnetic secular variation (PSV) records from East Asia especially from low‐latitude regions impedes better understanding of global PSV mechanisms. Here we report on a radiocarbon‐dated Holocene PSV record from a composite ~6.7‐m‐long core collected from the high‐sedimentation‐rate Huguangyan Maar Lake (HML) in subtropical‐tropical South China. Rock magnetic results demonstrate that the natural remanent magnetization resides in single‐domain magnetite. Alternating field demagnetization experiments at 1‐cm spacing on u‐channel samples reveal six distinct inclination highs at ~7,500 BCE, ~5,100 BCE, ~4,600 BCE, ~3,600–3,400 BCE, ~1,600–1,200 BCE, and 600–800 CE; three inclination lows at ~4,800 BCE, ~600–300 BCE, and ~1,000–1,300 CE; and three eastward declination trends at ~3,600–3,200 BCE, ~2,600–2,400 BCE, and 400 BCE to 200 CE. The similarity between the HML PSV record and other independently dated records from East Asia and geomagnetic field models corroborates the robustness of our age model and Holocene PSV record. Strikingly, centennial‐ to millennial‐scale PSV features of the HML are comparable, within age uncertainties, with other Holocene records from Europe, North America, and Canada, suggesting that such directional patterns are likely to be hemispheric in scale. Although relative paleointensity data of HML are affected by environmental factors (e.g., organic matter diagenesis), the record still provides a regionally important new PSV reference curve whose conspicuous features may serve as stratigraphic markers for East Asian paleorecords.

Microbial diversity in Huguangyan Maar Lake of China revealed by high–throughput sequencing

Huguangyan Maar Lake is a typical maar lake in the southeast of China. It is well preserved and not disturbed by anthropogenic activities. In this study, microbial community structures in sediment and water samples from Huguangyan Maar Lake were investigated using a high–throughput sequencing method. We found significant differences between the microbial community compositions of the water and the sediment. The sediment samples contained more diverse Bacteria and Archaea than did the water samples. Actinobacteria, Betaproteobacteria, Cyanobacteria, and Deltaproteobacteria predominated in the water samples while Deltaproteobacteria, Anaerolineae, Nitrospira, and Dehalococcoidia were the major bacterial groups in the sediment. As for Archaea, Woesearchaeota (DHVEG–6), unclassified Archaea, and Deep Sea Euryarchaeotic Group were detected at higher abundances in the water, whereas the Miscellaneous Crenarchaeotic Group, Thermoplasmata, and Methanomicrobia were significantly more abundant in the sediment. Interactions between Bacteria and Archaea were common in both the water column and the sediment. The concentrations of major nutrients ( $$\text{NO}_3^-$$ , $$\text{PO}_4^{3-}$$ , $$\text{SiO}_3^{2-}$$ and $$\text{NH}_4^+$$ ) shaped the microbial population structures in the water. At the higher phylogenetic levels including phylum and class, many of the dominant groups were those that were also abundant in other lakes; however, novel microbial populations (unclassified) were often seen at the lower phylogenetic levels. Our study lays a foundation for examining microbial biogeochemical cycling in sequestered lakes or reservoirs.

Experiment and interpretation of geomorphological detection by multi-beam sonar in Huguang-yan Maar Lake

The Huguangyan Maar Lake is caused by a volcanic eruption. The original sediments at the bottom of the lake are natural yearbooks for the evolution of the earth’s climate and environment. A multi-beam sonar technique is used to scan the full coverage on the lake surface to get fine samples of echoes form the lake bottom. The information of the bathymetric data of the lake bottom is accurately described and the results of three-dimensional geomorphology imaging are given. The results show that the lake is divided into two parts, east and west, by a north-south underwater volcanic wall, and the maximum depth of water is over 22 meters. We apply a texture feature extraction method based on multi-scale fractal dimension to describe the characteristics of the sediments and roughness. Multi-scale fractal dimensions algorithm is used to extract waveform characteristics of depth samples in different directions. General distribution of sediment at the bottom of the lake is distinguished by the width of multi-scale fractal spectrum. The results obtained can be helpful for the estimation of the physical properties of sediments.

Spatiotemporal evolution of C3/C4 vegetation and its controlling factors in southern China since the last glacial maximum

To date, few research have been reported on the evolution of C3/C4 vegetation in southern China, and the main mechanism influencing the evolution of C3/C4 vegetation is unclear. That makes it difficult for researchers to understand the competition mechanism of C3 and C4 plants under different climate environments and its relationship with the climate factors. It is also not conducive for researchers to assess the influence of future climate change on regional C3/C4 vegetation. Exactly, C3/C4 vegetation change in the regional-scale will have a significant impact on the global carbon cycle and agricultural production. Therefore, it is especially important to reconstruct the evolutionary history of C3/C4 vegetation in southern China and clarify the influencing mechanism of climate change. In this study, we systematically analyzed stable carbon isotope ( δ 13C) of the long-chain n -alkanes in sediment samples from eight lakes and four peat profiles in southern China, to reconstruct the spatiotemporal evolution of C3/C4 vegetation in these regions since the Last Glacial Maximum (LGM) and to investigate the climate factors that affect the C4 plant abundance change in the research area. The integrated long-chain n -alkane (C27–C33) stable carbon isotope results of samples from Zhanjiang Huguangyan Maar Lake, Xingyun Lake, Lugu Lake and Dingnan peat showed that, from the LGM to the Early Holocene, C4 plant relative abundance exhibited a gradually increasing trend from 21% to 34%. In the Middle Holocene, the C4 plant abundance significantly declined and reached a lowest value of 10%. In space, the C4 plant abundance generally exhibited a gradually declining trend from south to north in the LGM and the Early Holocene, while it showed an opposite trend in the Holocene Climate Optimum (6.0 cal ka BP). It reflected that the main influencing factor on C4 plants spatial distribution was changing from temperature to precipitation. This study indicated that temperature was the dominant factor affecting C4 plant distribution in southern China, however, when the temperature condition was appropriate, an increase in precipitation (especially more spring precipitation) would reduce the competitive advantages of C4 plants. Therefore, the combination of temperature and seasonal precipitation was the important factor that determines the C3/C4 vegetation proportion change in the southern China. Under the premise that the temperature will rise and precipitation will increase in the future, the reduction of a competitive advantage for the C4 plants could affect agricultural production in China.

Spatial and temporal distributions of nutrients and their influencing factors in the Huguangyan Maar Lake

Spatial and temporal distributions of nutrients and their influencing factors in the Huguangyan Maar Lake

Huguangyan Maar Lake (SE China): A solid record of atmospheric mercury pollution history in a non-remote region

Mercury is a highly toxic metal that can cause harm to environment and human health. As atmospheric deposition is the main source of total Hg input to aquatic system in remote and pristine regions, almost all the studies on atmospheric Hg pollution history concentrated in these areas, while the studies in non-remote areas are much limited, especially for the long history records. In this study, Huguangyan Maar Lake, an undisturbed lake system at low altitude in China, was selected to reconstruct the atmospheric mercury pollution history. Variation patterns of TOC, Hg and non-residual Sr in the sediment core indicated that, compared to the direct atmospheric Hg deposition, the effect of either Hg scavenging from water column by algae or the catchment inputs of previously deposited Hg on the Hg accumulation in the lake sediment was limited. The sediment Hg content in Huguangyan Lake was mainly controlled by the atmospheric Hg deposition, and thus accurately reflected the atmospheric Hg pollution history. The Hga (Hg content from atmospheric deposition) in Huguangyan Lake presented a comparable variation pattern to that in remote sites. It had the same variation trend as the global atmospheric Hg before 1950 CE, which could be attributed to the Industrial Revolution. After that, it was mainly controlled by Hg emissions from Asian countries. The variation of Hga also indicated that atmospheric Hg deposition accelerated significantly since 2000 CE. This study, along with other investigations in remote sites in China, showed that the sediment Hg in Huguangyan Lake responded to the atmospheric Hg pollution more sensitively than in the alpine regions. It should be noted that, the more intensive acceleration of Hg deposition in Huguangyan Lake may imply that the South of China suffered from much more serious atmospheric Hg pollution than previous studies revealed.