High-dimensional Orbital Angular Momentum Research Articles

On-demand orbital angular momentum comb from a digital laser

Photonic orbital angular momentum (OAM) carried by phase-structured vortex light is an important and promising resource for the ever-increasing demand towards high-capacity data information due to its intrinsic unlimited dimensionality. Large superpositions of OAM are easy to be produced, but on-demand generation of arbitrary OAM spectra such as an OAM comb similar to a frequency comb is still a challenge; especially, the on-demand OAM comb and arbitrary multi-OAM modes have not yet been realized at the source. Here we report a versatile at-source strategy for developing a flexibly and dynamically switchable on-demand digital OAM comb laser for the first time, to our knowledge, by controlling the phase degree of freedom itself rather than any proxy. For this aim, we present a crucial design idea that a nested ring cavity configuration is composed of a degenerate cavity embedded into a stable ring cavity and a pair of conjugate two-fold symmetric multi-spiral-phase digital holographic mirrors loaded onto reflective phase-only spatial light modulators. In the nested ring cavity, the stable ring cavity and the degenerate cavity meet the requirements of high spatial coherence and supporting any transverse mode, respectively. The paired conjugate holographic mirrors located in mutual object and image planes circumvent the competing issue among different OAM modes and control the number and chirality of modes in OAM combs with ease. Our strategy has also universality as it has the ability of encoding OAM spectra with arbitrary distribution. The realization of a dynamic on-demand multi-OAM-mode laser is an important progress in the infancy of multi-OAM-mode sources. Our idea provides a promising solution for development of emerging high-dimensional technologies; in the future, there will be increasing opportunities in the fundamentals and applications of high-dimensional OAM modes, and beyond. Our strategy not only contributes to the development of new laser technology, but also provides a toolbox for both linear and nonlinear generation of the multiple OAM modes at the source.

Polarization-controlled generation of multiple orbital angular momentum modes

By concurrently manipulating the degrees of freedom associated with polarization and orbital angular momentum (OAM), a variety of vector fields can be generated, which exhibit unique characteristics and have found extensive application in both classical and quantum optics. However, the OAM dimensions in these fields have been predominantly confined to two. Different from high-order OAM with a large topological charge, broadening the OAM dimensions beyond this limit and generating OAM spectra with multiple OAM modes can significantly enhance the scope of research. In this study, we explore vector fields with OAM dimensions exceeding ten, achieving polarization-controlled spectra in higher-dimensional OAM. Our findings not only offer a method for controlling high-dimensional OAM through polarization but also pave the way for potential applications in both classical and quantum realms utilizing high-dimensional vector states.

Research progress of integrated quantum light sources with orbital angular momentum

Quantum light sources are one of key devices for quantum information processing, and they are also the important foundation for applications such as in quantum computing, quantum communication, and quantum simulation. Improving the capacity of quantum information coding by using the quantum light source is a major challenge in the development of quantum information technology. Photons with a helical phase front can carry a discrete, unlimited but quantized amount of orbital angular momentum (OAM). The infinite number of states with different OAMs can greatly increase the capacity of optical communication and information processing in quantum regimes. To date photons carrying OAM have mainly been generated by using bulk crystals, which limits the efficiency and the scalability of the source. With the advancement of quantum photonic technology, many significant quantum photonic devices can now be realized on integrated chips. However, creating high-dimensional OAM quantum states at a micro-nano scale is still a challenge. And the research of harnessing high-dimensional OAM mode by using integrated quantum photonic technologies is still in its infancy. Here, the authors review the recent progress and discuss the integrated quantum light sources with OAM. The authors introduce the research progress of using OAM for both single photons and entangled photons and emphasize the exciting work on pushing boundaries in high-dimensional quantum states. This may pave the way for the research and practical applications of high-dimensional quantum light sources.

Remote transport of high-dimensional orbital angular momentum states and ghost images via spatial-mode-engineered frequency conversion

The efficient transport and engineering of photonic orbital angular momentum (OAM) lie at the heart of various related classical and quantum applications. Here, by leveraging the spatial-mode-engineered frequency conversion, we realize the remote transport of high-dimensional orbital angular momentum (OAM) states between two distant parties without direct transmission of information carriers. We exploit perfect vortices for preparing high-dimensional yet maximal O AM entanglement. Based on nonlinear sum-frequency generation working with a strong coherent wave packet and a single photon, we conduct the Bell-like state measurements for high-dimensional perfect vortices. We experimentally achieve an average transport fidelity 0.879 ± 0.048 and 0.796 ± 0.066 for a complete set of 3-dimensional and 5-dimensional OAM mutually unbiased bases, respectively. Furthermore, by exploring the full transverse entanglement, we construct another strategy of quantum imaging with interaction-free light. It is expected that, with the future advances in nonlinear frequency conversion, our scheme will pave the way for realizing truly secure high-dimensional quantum teleportation in the upcoming quantum network.

Twisting and entangling gravitons in high-dimensional orbital angular momentum states via photon-graviton conversion

Twisting and entangling gravitons in high-dimensional orbital angular momentum states via photon-graviton conversion

Orbital-angular-momentum-based optical clustering via nonlinear optics

Machine learning offers a convenient and intelligent tool for a variety of applications in the fields ranging from fundamental research to financial analysis. With the explosive growth of data streams, i.e., “big data,” optical machine learning with the inherent capacity for massive parallel processing is gradually attracting attention. Despite significant experimental and theoretical progress in this area, limited by the coherent manipulation of multibeams, high dimensional optical vector or matrix operation is still challenging. Here, by using the second harmonic generation of high dimensional orbital angular momentum superposition states, we present a compact and robust optical clustering machine, which is the crucial component in machine learning. In experiment, we conduct supervised clustering for classification of three- and eight-dimensional vectors and unsupervised clustering for text mining of 14-dimensional texts both with high accuracies. The presented optical clustering scheme could offer a pathway for constructing high speed and low energy consumption machine learning architectures.

High-Dimensional Entanglement-Enabled Holography.

As an important imaging technique, holography has been realized with different physical dimensions of light, including polarization, wavelength, and time. Recently, quantum holography has been demonstrated by utilizing polarization entangled state with the advantages of high robustness and enhanced spatial resolution, comparing with classical holography. However, the polarization is only a two-dimensional degree of freedom, which greatly limits the capacity of quantum holography. Here, we propose a method to realize high-dimensional quantum holography by using high-dimensional orbital angular momentum (OAM) entanglement. A high-capacity OAM-encoded quantum holographic system can be obtained by multiplexing a wide range of OAM-dependent holographic images. Proof-of-principle experiments with four- and six-dimensional OAM entangled states have been implemented and verify the feasibility of our idea. Our experimental results also demonstrate that the high-dimensional quantum holography shows a high robustness to classical noise. What is more, the level of security of the holographic imaging encryption system can be greatly improved in our high-dimensional quantum holography.

How gravitational fluctuations degrade the high-dimensional spatial entanglement

Twisted photons carrying orbital angular momentum (OAM) are competent candidates for future interstellar communications. However, the gravitational fluctuations are ubiquitous in spacetime. Thus a fundamental question arises naturally as to how the gravitational fluctuations affect the coherence and the degree of high-dimensional OAM entanglement when twisted photons travel across the textures of curved spacetime. Here, we consider the covariant scalar Helmholtz equations and the Minkowski metric with fluctuations of Gaussian distribution and formulate analytically the equations describing the motion for twisted light in the Laguerre-Gaussian mode space. It is seen that the OAM cannot remain conserved in the presence of gravitational fluctuations. Furthermore, two-photon density matrices are derived for interstellar OAM quantum entanglement distribution, and the degree of entanglement degradation is characterized by purity and negativity. It is revealed that the higher-dimensional OAM entanglement is more susceptible to spacetime fluctuations. We believe that our findings will be of fundamental importance for the future interstellar quantum communications with twisted photons.

High-dimensional orbital angular momentum entanglement from an ultrathin nonlinear film

Entanglement, as a crucial feature of quantum systems, is essential for various applications of quantum technologies. High-dimensional entanglement has the potential to encode arbitrary large amount of information and enhance robustness against eavesdropping and quantum cloning. The orbital angular momentum (OAM) entanglement can achieve the high-dimensional entanglement nearly for free stems due to its discrete and theoretically infinite-dimensional Hilbert space. A stringent limitation, however, is that the phase-matching condition limits the entanglement dimension because the coincidence rate decreases significantly for high-order modes. Here we demonstrate relatively flat high-dimensional OAM entanglement based on a spontaneous parametric down conversion (SPDC) from an ultrathin nonlinear lithium niobite crystal. The difference of coincidences between the different-order OAM modes significantly decreases. To further enhance the nonlinear process, this microscale SPDC source will provide a promising and integrated method to generate optimal high-dimensional OAM entanglement.

Control of harmonic orbital angular momentum in second-harmonic generation of perfect vortices

Nonlinear interaction between orbital angular momentum (OAM) modes has interesting effects and tremendous applications in both classical and quantum realms. Here we propose a strategy of using perfect vortices, which not only overcomes the spatial mode matching problem of nondegenerate OAM modes, but also reveals the OAM-only influence on the momentum matching by tuning the OAMs of the fundamental wave. We use perfect vortices of degenerate and nondegenerate OAM modes to clearly demonstrate the flexible control of OAM modes on nonlinear interaction by carefully exploring second-harmonic generation (SHG) in periodically poled crystal. We generate second-harmonic perfect vortices with the OAM order up to 40. Based on the observed phase-matching temperature shift caused by OAMs, we also use the SHG nonlinear process to distinctly confirm the OAM-only-induced subluminal effect. Our results pave the way toward unveiling the underlying physics behind nonlinear process of OAM modes and building high-capacity quantum links between systems operating at various wavelengths. The inverse process of SHG we developed, perfect-vortex-based spontaneous parametric down-conversion, may provide a promising solution for high-dimensional OAM entangled source.

Simple-Diffraction-Based Deep Learning to Reconstruct a High-Dimensional Orbital-Angular-Momentum Spectrum Via Single-Shot Measurement

Orbital-angular-momentum (OAM) complex-valued spectrum reconstruction routinely necessitates the measurements of a complete set of observables, which is rather time consuming and inefficient for high-dimensional OAM superposition state. Here we break this barrier to realize the full reconstruction of a high-dimensional OAM complex-valued spectrum via only a single-shot measurement, which benefits from the use of a residual convolutional neural network for learning the diffraction behaviors. In our experiment, the high-dimensional OAM states are diffracted by a simple aperture of pentagram that breaks the OAM conjugate symmetry. We achieve fidelity over 97.8% and 92.1% for high-dimensional pure and mixed OAM states (up to $d=15$), respectively. We also confirm the excellent robustness under strong noise environment. Our method will find potential applications in high-dimensional information encoding, such as large-alphabet communications, quantum imaging, and real-time quantum sensing.

High-Dimensional Entanglement of Photonic Angular Qudits

We propose a method for generation of entangled photonic states in high dimensions, the so-called qudits, by exploiting quantum correlations of Orbital Angular Momentum (OAM) entangled photons, produced via Spontaneous Parametric Down Conversion. Diffraction masks containing N angular slits placed in the path of twin photons define a qudit space of dimension N2, spanned by the alternative pathways of OAM-entangled photons. We quantify the high-dimensional entanglement of path-entangled photons by the Concurrence, using an analytic expression valid for pure states. We report numerical results for the Concurrence as a function of the angular aperture size for the case of high-dimensional OAM entanglement and for the case of high-dimensional path entanglement, produced by N × M angular slits. Our results provide additional means for preparation and characterization of entangled quantum states in high-dimensions, a fundamental resource for quantum simulation and quantum information protocols.

Propagation-invariant high-dimensional orbital angular momentum states

Photonic states encoded in spatial modes of paraxial light fields provide a promising platform for high-dimensional quantum information protocols and related studies, where several pioneering theoretical and experimental demonstrations have paved the path for future technologies. Crucially, critical issues encountered in free-space propagation still represent a major challenge. This is the case of asynchronous diffraction between spatial modes with different modal orders, which experience variations in their transverse structure upon free-space propagation. Here we address this issue by proposing an encoding method based on the use of Laguerre–Gaussian modes of the same modal order N to define a N + 1 dimensional space. Noteworthy, such modes endowed with orbital angular momentum (OAM) experience the same propagation aberrations featuring an identical Gouy phase and wavefront curvature. We demonstrate our proposal experimentally by using time-correlated-single-photon imaging combined with a digital propagation technique. Importantly, our technique allows to eliminate, without the use of imaging systems, all issues related to asynchronous diffraction, providing an accessible way to generate propagation-invariant OAM qudits for quantum optical protocols.

Diffraction-Induced Entanglement Loss of High-Dimensional Orbital Angular-Momentum States

Diffraction-Induced Entanglement Loss of High-Dimensional Orbital Angular-Momentum States

Manipulating the orbital-angular-momentum correlation of entangled two-photon states in three-dimensional nonlinear photonic crystals

Three-dimensional (3D) nonlinear photonic crystal (NPC) has recently been realized in experiment, which provides a powerful platform for quantum-state engineering. Here, we propose a fork-grating 3D NPC scheme to manipulate orbital-angular-momentum (OAM) correlations of entangled two-photon pairs. The spiral spectra, bandwidths, and generation rates of counterpropagating and copropagating photon pairs are theoretically analyzed. Our results show that 3D NPC is of practical significance to generate high-dimensional OAM entanglement for quantum precision measurement, quantum computing, and quantum communication.

High-dimensional orbital angular momentum multiplexing nonlinear holography

Nonlinear holography has been identified as a vital platform for optical multiplexing holography because of the appearance of new optical frequencies. However, due to nonlinear wave coupling in nonlinear optical processes, the nonlinear harmonic field is coupled with the input field, laying a fundamental barrier to independent control of the interacting fields for holography. We propose and experimentally demonstrate high-dimensional orbital angular momentum (OAM) multiplexing nonlinear holography to overcome this problem. By dividing the wavefront of the fundamental wave into different orthogonal OAM channels, multiple OAM and polarization-dependent holographic images in both the fundamental wave and second-harmonic wave have been reconstructed independently in the spatial frequency domain through a type-II second harmonic generation process. Moreover, this method can be easily extended to cascaded χ2 nonlinear optical processes for multiplexing in more wavelength channels, leading to potential applications in multicasting in optical communications, multiwavelength display, multidimensional optical storage, anticounterfeiting, and optical encryption.

Experimental certification of quantum dimensions and irreducible high-dimensional quantum systems with independent devices

Dimensionality plays an important role in various information-theoretic tasks and can be seen as a key resource for quantum information processing. In this work, for the first time to the best of our knowledge, we report an experimental test of classical and quantum dimensions in a prepare-and-measure scenario through a nonlinear dimension witness (NDW), where the preparer and the measurer have no shared randomness. We propose a theoretical method to certify whether the generated states can be decomposed as products of lower dimensional states with the NDW, certify the dimension of the high-dimensional system, and identify whether the quantum system is irreducible in a unified picture in our experiment. To demonstrate the practicability of this method, we experimentally witness the generation of classical and quantum systems encoded in the high-dimensional orbital angular momentum (OAM) state under the effects of atmospheric turbulence. Our results show that this nonlinear dimension witness is highly robust and can be used in the presence of noise and low detection efficiency; hence, we estimate the dimension in our experiment in a detection-loophole-free manner through the NDW. We believe our work opens new avenues for dimension witnesses, especially for device-independent estimation of quantum systems and quantum communications.

Increasing two-photon entangled dimensions by shaping input-beam profiles

Photon pair entangled in high dimensional orbital angular momentum (OAM) degree of freedom (DOF) has been widely regarded as a possible source in improving the capacity of quantum information processing. The need for the generation of a high dimensional maximally entangled state in the OAM DOF is therefore much desired. In this work, we demonstrate a simple method to generate a broader and flatter OAM spectrum, i.e. a larger spiral bandwidth (SB), of entangled photon pairs generated through spontaneous parametric down-conversion by modifying the pump beam profile. By investigating both experimentally and theoretically, we have found that an exponential pump profile that is roughly the inverse of the mode profiles of the single-mode fibers used for OAM detection will provide a much larger SB when compared to a Gaussian shaped pump.

Orbital-angular-momentum-based experimental test of Hardy's paradox for multisetting and multidimensional systems

Characterizing high-dimensional entangled states is of crucial importance in quantum information science and technology. Recent theoretical progress has been made to extend Hardy's paradox into a general scenario with multisetting and multidimensional systems, which enables the maximum probability of nonlocal events to surpass the bound that was limited in Hardy's original test. Hitherto, no experimental verification has been conducted to verify Hardy's paradox, as most of the previous experimental efforts were restricted to two-dimensional systems. Here, based on two-photon high-dimensional orbital angular momentum (OAM) entanglement, we report an experiment to demonstrate Hardy's paradox for multiple settings and multiple outcomes. We demonstrate the paradox for two-setting higher-dimensional OAM subspaces up to $d=7$, which reveals that the nonlocal events increase with dimension. Furthermore, we showcase the nonlocality with an experimentally recorded probability of 36.77% for a five-setting three-dimensional OAM subspace via entanglement concentration, thus showing a sharper contradiction between quantum mechanics and classical theory.

Intense circularly polarized attosecond pulse generation from solid targets irradiated with a two-color linearly polarized laser

Characterizing high-dimensional entangled states is of crucial importance in quantum information science and technology. Recent theoretical progress has been made to extend the Hardy's paradox into a general scenario with multisetting multidimensional systems, which can surpass the bound limited by the original version. Hitherto, no experimental verification has been conducted to verify such a Hardy's paradox, as most of previous experimental efforts were restricted to two-dimensional systems. Here, based on two-photon high-dimensional orbital angular momentum (OAM) entanglement, we report the first experiment to demonstrate the Hardy's paradox for multiple settings and multiple outcomes. We demonstrate the paradox for two-setting higher-dimensional OAM subspaces up to d = 7, which reveals that the nonlocal events increase with the dimension. Furthermore, we showcase the nonlocality with an experimentally recording probability of 36.77% for five-setting three-dimensional OAM subspace via entanglement concentration, and thus showing a sharper contradiction between quantum mechanics and classical theory.