High-purity Germanium Detector Research Articles

Measurement of γ-rays generated by neutron interaction with 16O at 30 MeV and 250 MeV

Abstract Deep understanding of γ-ray production from the fast neutron reaction in water is crucial for various physics studies at large-scale water Cherenkov detectors. We performed test experiments using quasi-mono energetic neutron beams (En = 30 and 250 MeV) at Osaka University’s Research Center for Nuclear Physics to measure γ-rays originating from the neutron-oxygen reaction with a high-purity germanium detector. Multiple γ-ray peaks which are expected to be from excited nuclei after the neutron-oxygen reaction were successfully observed. We measured the neutron beam flux using an organic liquid scintillator for the cross section measurement. With a spectral fitting analysis based on the tailored γ-ray signal and background templates, we measured cross sections for each observed γ-ray component. The results will be useful to validate neutron models employed in the on-going and future water Cherenkov experiments.

Estimation of the Effective Radiation Dose in Nuclear Medicine Workers from Dhaka by Measuring Radioactivity in Urine Sample Resulting from Internal Exposure

This study estimates the effective doses and activity concentration from 151 urine samples which are collected from 15 (Fifteen) occupational workers at National Institute of Nuclear Medicine and Allied Science (NINMAS) in Dhaka, Bangladesh. The radioactivity concentration in urine sample is due to intake of I-131, Tc-99m and F-18. The samples have been analyzed using High Purity Germanium (HPGe) detector. The radioactivity of I-131 and Tc-99m was found 0.91 ± 0.26 BqL-1 to 504.49 ± 6.03 BqL-1 and 0.15 ± 0.21 BqL-1 to 191.19 ± 6.98 BqL-1 respectively. Radioactivity of F-18 was found from 0.031 ± 0.022 BqL-1 to 0.282 ± 0.065 BqL-1. The effective doses of occupational workers have been also calculated using the radioactivity concentration and the dose coefficient according to ICRP publication 78. Jagannath University Journal of Science, Volume 11, Number 1, June 2024, pp. 64−80

ASSESSMENT OF THE LEVELS OF NATURAL RADIOACTIVITY AND THE POSSIBILITY OF RADIATION RISKS IN SOIL SAMPLES TAKEN FROM DIFFERENT LOCATIONS IN SOUTHERN ALMAZAR-ALKARAK, JORDAN

A wide study of environmental radioactivity levels in soil samples from Southern Almazar-Alkarak in Jordan was performed to develop a radiological map of the area. 15 soil samples were collected from different locations across the region and subjected to analysis using a high-purity germanium detector (HPGe). The study showed that the average levels of natural radionuclides 226Ra, 232Th, 238U and 40K were 34.5±0.98, 25.6±1.3, 32.2±3.7 and 278.5±15.7 Bq.kg−1, respectively. Also, to evaluate the radiological danger, the radium equivalent activity (Raeq) is calculated, absorbed gamma dose rate (D), annual effective dose equivalent (AEDE) and external hazard index (Hex), internal hazard index (Hin). The average values for these parameters were determined to be 92.5 Bq.kg−1, 43.0 nGy h−1, 52.7 µSv y−1 and 0.25Bq.kg−1, 0.34Bq.kg−1 respectively. The values of the gathered samples stay below the allowable limits. Consequently, the examined region does not present any radiation risk to the general population. Moreover, it has been discovered that there is no concentration of 137Cs radionuclide activity in the studied area.

Determination of natural radioactivity levels in soil samples from irrigated vegetable farming land in and around Addis Ababa, Ethiopia.

Soil samples were collected from vegetable agricultural areas in and around Addis Ababa, and their levels of radioactivity were measured. Gamma spectrometry with high-purity germanium detector was used to quantify radioactivity level. The average concentration of 226Ra, 232Th, and 40K were 32.8±2.1, 62.4±4.4, and 544.3±23.3Bqkg-1 respectively. The mean values of 232Th and 40K are higher, whereas the value of 226Ra is comparable with world average values. Radiological hazard indices, including radium equivalent activity (Raeq), absorbed dose rate (Dr), outdoor annual effective dose equivalent (Deff), external hazard index (Hex), internal hazard index (Hin), and gamma radiation representative level index (Iγ), were calculated based on the activity concentration of 226Ra, 232Th and 40K. The mean values were 163.9Bqkg-1, 78.7 nGy h-1, 0.10mSv y-1, 0.44, 0.53, and 0.60 respectively. All indices are lower than global recommended limit values. These results revealed that radiation hazard due to radionuclides in the soil of the study area is insignificant.

Estimation of radiological health risks due to 226Ra, 232Th, and 40K in foods consumed in Iraqi Kurdistan Region

ABSTRACT This study investigates the activity concentration of natural radionuclides in a diverse range of food samples in the Koya district markets food baskets, including both domestic and imported products. The samples cover annual crops (e.g. coffee, tea, kidney beans), tree nuts (e.g. almonds, pistachios), and other items (e.g. beef, fish, milk) by using a high-purity germanium (HPGe) detector. This research addresses a notable gap by providing baseline data on radionuclide concentrations and assessing potential health risks. Average activity concentrations for ²²⁶Ra, ²³²Th, and ⁴⁰K were 0.943, 0.367, and 191.8 Bq kg−1, respectively. Radium equivalent activity values ranged from 2.88–58.48 Bq kg−1, all below the safety limit. The average excess lifetime cancer risk (ELCR) was 0.154 mSv a−1, indicating safety for most samples, though coffee and tea showed higher levels. This study provides new data crucial for future research and regulatory monitoring, underscoring the need for further investigation into geological impacts on radionuclide levels.

Experimental evaluation of the impact of ZnO on the radiation shielding ability of B2O3–PbO–ZnO–CaO glass systems

In this study, we used the melt quenching process to develop inexpensive, new radiation shielding glasses. The prepared glasses have a general formula 40B2O3–20PbO-(y)ZnO-(40-y)CaO, (y = 20, 25, 30 and 35 mol%). These glasses' gamma-radiation shielding properties were experimentally measured using Am-241, Co-60, and Cs-137 sources and a High-Purity Germanium (HPGe) detector, revealing that incorporation of ZnO had a positive impact of the density of these glasses. Moreover, the incorporation of ZnO enhanced the prepared glasses' attenuation performance. With greater energy the half value layer increased, and by a factor of 45 with a 0.059–1.333 MeV energy increase. For the four studied glasses the radiation protection efficiency (RPE) values are 100 % efficient at low energies (0.059 MeV), with a drastic decrease in the values across all four samples as the energy increases from 0.06 to 0.662 MeV.

The 2024 LaBr[formula omitted](Ce) detector setup for the FAMU experiment

The FAMU experiment, led by INFN at the Rutherford Appleton Laboratory (UK), is designed to measure the Zemach radius of the proton in muonic hydrogen (μp) with uncertainty better than 1%. A set of LaBr3(Ce) scintillating crystals, complemented by a High-Purity Germanium (HPGe) detector, are used to detect the delayed muonic oxygen (μO) X-ray emission, which signals the muonic hydrogen spin flip excited with a tunable MIR laser. The detector setup is in continuous development. After two periods of measurement in 2023, the detector configuration is currently being upgraded for the 2024–2025 runs with new detectors read out by SiPMs to enhance signal-to-noise ratio and improve time performance. In particular, all ½” scintillators are being substituted with 1” ones, increasing the solid angle coverage and optimising energy resolution and timing performances.

Contributions of Cosmic-Ray Components to the HPGe Gamma Spectrometer Background Spectrum within the 0°-45° Zenith Angle Range

This study investigates the contributions of various cosmic-ray-induced components to the energy response of a High-Purity Germanium (HPGe) gamma spectrometer within the 0°-45° zenith angle range. The analysis focuses on muons, neutrons, protons, electrons, positrons, and photons. It also examines the impact of particle showers induced by muons interacting with the lead chamber and reaching the HPGe detector. Utilizing the GEANT4 simulation toolkit, we provide a detailed examination of these components' influence on the spectrum. The results confirm that within this zenith angle range, muons account for approximately 91% of the recorded cosmic-ray induced energy spectrum and contribute 54.6% to the overall cosmic-ray-induced background spectrum. The study also highlights the significant role of showers, especially those resulting from muon interactions with the lead shielding, in shaping the low-energy spectrum below 3 MeV.

Measurement of fast neutron induced (n,γ) reaction cross-section of 68Zn, 96Zr, 121Sb and 123Sb in the energy range of 1 to 2 MeV

The (n,γ) reaction cross-section for the elements 68Zn, 96Zr, 121Sb and 123Sb, present in the reactor structural/shielding materials, was measured by neutron activation technique in the neutron energy region of 1–2 MeV as very limited data is available in this energy range. Further, the neutron spectrum peaks in this energy region for the fast breeder reactors and proposed accelerator driven sub-critical systems. The natural strontium (natSr) element was used as a neutron flux monitor by considering effective combined reaction cross-section for 86Sr(n,γ)87Srm and 87Sr(n,n′)87Srm reactions. The pellets of mixture of sample and monitor were irradiated by a quasi-mono energetic fast neutron beam, generated by 7Li(p,n)7Be reaction at FOTIA, Bhabha Atomic Research Centre, Mumbai, India. The activity of activation products was measured by off-line gamma-ray spectrometry using High Purity Germanium Detector (HPGe). The present data with improved uncertainty and covariance analysis enhance the cross-section data base for better constraining the evaluated data and theoretical models. The theoretical (n,γ) reaction cross-sections were calculated using TALYS 1.96, which could reasonably explain the present data with the Fermi gas level density prescription.

Evaluating the radioactivity and health risks in oil and gas production areas: insights from Titas Gas Field, Bangladesh

ABSTRACT Conducting comprehensive studies of radioactivity and associated risk assessments in the oil and gas industry is crucial due to the potential accumulation of Naturally Occurring Radioactive Materials in production operations. This pioneering study investigates radioactivity levels in surface soil from the Titas Gas Field area in Bangladesh by a High Purity Germanium (HPGe) detector, a crucial resource of the nation’s energy infrastructure. In surface soil, the activity of 226Ra, 232Th, and 40K varied from 18–41 Bq/kg, 28–62 Bq/kg, and 280–600 Bq/kg, respectively. Particularly, the levels of 232Th exceeded the global average value for soil. These elevated 232Th levels are likely attributed to a combination of natural geological processes of enriching thorium bearing minerals, geochemical processes favouring thorium retention and human activities selectively impacting these radionuclides. The estimated of radiological risk reveals that some indices exceed recommended limits, hence pose a concern for public health. The study recommends periodic monitoring, public awareness campaigns, remediation efforts, and long-term management strategies to protect environmental and public health. The findings of this research underscore the critical need to recognise and address radiological hazards associated with gas extraction activities to safeguard the health and safety of workers and nearby communities in Bangladesh.

Pioneering study of radioactivity in soil near the Payra 1320 MW Thermal Power Plant, the largest coal-fired thermal power plant in Bangladesh

ABSTRACT Coal combustion increases atmospheric radioactivity, harming those live in the periphery of coal-fired thermal power plants (CFTPPs). A pioneering study has been performed using a high-purity germanium detector by analysing 30 soil samples collected from distances of 50, 600, 1200, and 3000 metres in the periphery of the largest 1320 MW CFTPP, Payra, Bangladesh. The activity concentrations of 226Ra, 232Th and 40K ranged from 19–32, 31–90, and 420–870 Bq/kg, respectively, with most of the samples show 232Th and 40K levels above global averages. Elevated levels of 232Th and 40K in soil around Payra thermal power plant stem from natural minerals, granitic rocks, ash disposal, coal combustion residues, and environmental factors. Radiological hazard indices, including dose rates and cancer risk, exceed global averages, indicating unsafe radiation exposure for coal miners and locals. These findings are crucial for planning coal-fired power plants and stress the need for municipal regulation of fly ash and health monitoring to mitigate risks for workers and residents.

Long-lived Gamma-Emitting Radionuclides in Commonly Consumed Imported Coffee Brands in Lagos and the Total Committed Effective Dose using a High Purity Germanium Detector

Long-lived Gamma-Emitting Radionuclides in Commonly Consumed Imported Coffee Brands in Lagos and the Total Committed Effective Dose using a High Purity Germanium Detector

Experimental and theoretical results of gamma shielding features for copper based shape memory alloys

In this study, the gamma ray attenuation characteristics for CuAlNi shape memory alloys with different proportions of Sn doping was investigated. We determined the mass attenuation coefficient (μ/ρ) of CuAlNiSn alloys both experimentally and theoretically within an energy range of 59.5–1332.5 keV. The experimental measurements were made using a high purity Germanium detector (HPGe) and theoretical calculations were made using WinXCOM program. To evaluate the gamma radiation shielding abilities of the alloy samples, the obtained (μ/ρ) values were used to determine the gamma protection parameters μ, HVL, TVL, MFP, and Zeff. In addition, the radiation protection efficiency (RPE) parameter was determined using gamma ray intensities in the absence and presence of the attenuator. Further analysis of the samples was conducted using a Rigaku Miniflex 600 model computer-controlled X-ray diffractometer (CuKα & λ = 1.5405 A0). The crystallographic structure of the alloys before and after irradiation was investigated. Other analysis which include EDX analysis (to investigate the chemical content) and SEM analysis (to investigate the microstructure) were conducted. According to result outcomes, gamma ray radiation did not affect the shape memory properties of structure. Another interesting observation is that, the radiation attenuation properties increase with increasing Sn concentration. Finally, we discovered that the CuAlNiSn4 alloy (which has the highest doping rate) provides good protection especially at low energy levels.

Calibration of a gamma ray Compton camera for radioactivity measurements

AbstractA dual-plane Compton imaging detector previously developed for prompt gamma imaging has been further tested and calibrated for quantitative radioactivity determination, specifically to assess radioactive debris from a reactor fuel element. The debris piece contains uranium isotopes and several long-lived fission products, including cesium-137 (Cs-137). The detector consists of two pixelated planes of cadmium-zinc-telluride (CZT) crystals which record gamma ray events interacting within these volumes. In addition to the energy spectrum obtained by pulse height analysis, the time-stamped events from each detector pixel are sorted by location into 3 categories for post-processing: intra-plane, inter-plane, and coincidence. An image reconstruction software enables spatial localization of the select gamma ray peak(s) from the spectrum, thereby separating the gamma ray by specific isotopes. We used the camera to image a small piece of debris for demonstration purposes. A measurement was performed alongside a high purity germanium (HPGe) detector, which could determine the isotopes' absolute activities and be used as a reference for the camera. In addition, a known isotopic point source was used to calibrate the camera’s energy detection efficiency in the same measurement geometry, correlating the image pixel intensity to the isotopic activity.

Determination of Excessive Lifetime Cancer Risk for Workers Exposed to Natural Radioactive Materials in Various Equipment in Oil and Gas Sector

In the oil and gas sector of Basrah, natural radioactive materials are accumulated in various equipment like wellheads, pumps, and separation vessels, often manifested as scales, sludge, and other forms of waste. Without proper preventive measures, these accumulations pose significant risks to workers, the public, and the environment. This study aims to assess the lifelong cancer risks associated with production processes and the handling of resultant waste, be it scale sediments, sludge, or soil. Sample collection across different regions was based on the evaluation of production and storage facilities. Using a high-purity germanium detector (HPGe), activity concentrations of 226Ra, 232Th, and 40K were measured. These concentrations were then used with standard equations to determine indoor effective dose rates. The regional-weighted (the lifetime risk of cancer is a measure of the cumulative risk of cancer over a specific age range and has a clear, intuitive appear) average of the lifetime excessive cancer risk was varied between (0.40 to 0.11 ×10-3) for ELCRoutdoor, (3.13 to 0.86 ×10-3) for ELCRindoor and (0.97 to 3 ×10-3) for ELCRtotal, significantly surpassing the global average value of (0.29x10-3). This disparity underscores the heightened risk posed by these activities, emphasizing the urgent need for enhanced safety measures and regulatory oversight to safeguard human health and the environment.

Total Radiological Dose and Safety Assessment of Workers in Radioactive Liquid Waste Storage Location in Al Tuwaitha Site

This study aims to determine the total effective dose (external and internal) in the radioactive liquid Waste Hall (WH) in the Radiochemistry Laboratories building (RCL) in Al- Tuwaitha site in order to estimate the radiation risk for workers in this place. The external effective dose was calculated by an indirect method using ThermoLuminescent Dosimeters (LiF: Mg, Ti (TLD-100)) by placing them in the waste hall for one month. The internal effective dose was estimated by collecting eight air samples (environmental samples) from different locations in WH using an air sampler pump (Sniffer) to collect air samples loaded with particles or dust which are deposited on cellulose filter papers (φ 125mm). This was done for two flow rates the lowest and the highest values of the air sampler pump of 5CFM and 20CFM, respectively.The filter papers were chemically treated using the digestion method. The radionuclides in these samples were measured using a gamma spectrometry system equipped with a high-purity germanium detector (HPGe), and the radioactivity concentration was measured using a gross alpha beta gamma system. The results showed 137Cs of low concentration was deposited on the filter paper. The total annual effective dose rate (external and internal) results showed that the highest in WH was (6358.97μSv/year) for the low probability scenario and (1589.74 μSv/year) for the realistic scenario.

Characteristic parameters and radon exhalation rates of aerated concrete blocks

ObjectiveTo understand the characteristic parameters and radon exhalation rates of aerated concrete blocks. MethodsA total of 39 nationally inspected samples were measured. Their dry density was determined based on their mass and volumes, their porosities were measured on the principle of volumetric expansion, and their radium content was determined using a high-purity germanium (HPGe) detector for gamma-ray spectroscopy. Furthermore, their diffusion lengths were quantified by establishing a combined cumulative and diffusion chamber, and their radon exhalation rates were measured through closed-box testing using a continuous radon monitor. ResultsThe aerated concrete blocks exhibited dry densities ranging from 464 to 840 ​kg/m3 [average: (654.0 ​± ​82.5) kg/m3], open porosities from 67.1 ​% to 81.1 % [average: (74.3 ​± ​3.3) %, radium (226Ra) content from 12.3 to 136 Bq/kg [average: (63.0 ​± ​30.4) Bq/kg], diffusion lengths from 0.49 to 1.01 ​m [average: (0.70 ​± ​0.15) m], and radon exhalation rates from 0.6 to 22.8 Bq·m−2·h−1 [average: (7.3 ​± ​5.3) Bq·m−2·h−1]. ConclusionAerated concrete blocks exhibit significantly higher porosities, diffusion lengths, and radon exhalation rates than traditional concrete and clay bricks. These blocks might contribute to the high indoor radon concentration observed in modern buildings in China.

A quantitative analysis on the effect of crystal parameters on full energy peak efficiency of a coaxial high purity Germanium detector for the energy range 50 keV-2.5 MeV

High Purity Germanium (HPGe) detectors are essential instruments in gamma-ray spectrometry, offering high sensitivity and exceptional energy resolution. The full-energy-peak (FEP) efficiency is a critical parameter that influences the accuracy of activity concentration measurements of radionuclides. This study examines the FEP efficiency of a coaxial HPGe detector, focusing on variations in crystal length, crystal radius, and crystal hole dimensions. For varying crystal lengths, the efficiency values show negligible differences at low energy (50 keV) but significant increases at higher energies, indicating that longer crystal lengths enhance efficiency. Similarly, the efficiency increases with larger crystal radii across all energy levels suggesting substantial efficiency gains even at low energies. However, variations in crystal hole radius and depth, exhibit minimal impact on FEP efficiency across all tested energy levels. These findings highlight that optimizing crystal length and radius is more crucial for changing detector efficiency compared to modifying hole dimensions, providing valuable insights for optimizing Monte Carlo models and detector design.

Spectral deconvolution approach for Beryllium-7 detection: Evaluating soil redistribution with NaI(Tl) detectors

Beryllium-7 is a cosmogenic radionuclide produced in the upper atmosphere through the spallation of cosmic rays and falls to Earth mainly by wet deposition. Given its short half-life (53 days) and strong adsorption to the clay present in the soil, 7Be inventory can be evaluated to obtain information about soil redistribution over periods of up to 6 months. By performing these measurements, one can infer the efficiency of soil management and conservation procedures. The isotope presence is measured using gamma-ray spectrometry to detect its decay emission, specifically a photon with an energy of 477.6 keV. Since other isotopes found in soil emit photons with similar energies, it is common to use High-Purity Germanium (HPGe) detectors due to their high energy resolution. However, these detectors are expensive and require cryogenic cooling during operation. An alternative is the Thallium-Activated Sodium Iodide (NaI(Tl)) detector, which is less costly and does not require cryogenic cooling, but has poorer resolution and cannot separate the emissions from 228Ac (463.0 keV), 7Be, and 208Tl (510.7 keV). This work aims to apply spectral deconvolution to quantify 7Be in soil samples collected from an agricultural mega-parcel situated on a hill slope and evaluate the soil redistribution experienced within. The activities of the interfering isotopes were quantified using other emissions, and the results were used to calculate the corresponding area in the desired region of the spectra. From this, 7Be activities were calculated and compared with the HPGe results to validate the deconvolution technique. The calculated activities for the three radioisotopes showed similar correspondence between the two detectors, indicating that the applied method is adequate for evaluating soil redistribution at lower costs. The calculated net soil deposition was 36.4 ± 6.4 kgm−2 for the NaI(Tl) detector and 26.4 ± 7.9 kgm−2 for the HPGe detector during the evaluated period. Furthermore, these results suggest that a similar approach can be applied to quantify other isotopes using NaI(Tl) detectors as an alternative to HPGe detectors.

Experimental study of gamma-ray attenuation capability of B2O3-ZnO-Na2O-Fe2O3 glass system

In the present work, a glass system with developed composition consisting of B2O3, ZnO, Na2O and Fe2O3 samples has been investigated. Glass samples were prepared using the melt quenching method and the density of the system was measured using Archimedes’ principle. Spectroscopic analysis using a gamma source and a high-purity germanium detector at four energies of 0.0595, 0.6617, 1.173, and 1.333 MeV emitted from Am-241, Cs-137, and Co-60 were used to determine the attenuation parameters of present glass composites. The sample containing 45 B2O3 + 10 Na2O + 40 ZnO + 5 Fe2O3 (coded BNZF-4) had the highest mass attenuation coefficient (MAC) value at all the energies discussed compared to the other composites. Whoever, the BNZF-1 sample had the lowest value at all ranges of energies. The transmission factors (TF, %) of the manufactured samples were calculated, at 0.0595 MeV (TF, %) values are 32.6429 and 6.4612 for samples BNZF-1 and BNZF-4, respectively. The statistical results demonstrated significantly better to increase the ZnO concentration in the sample, where the percentage of zinc oxide inside the prepared glass samples has the following direction BNZF -4 > BNZF -3 > BNZF -2 > BNZF -1. The significance of this study is that transparent, environmentally harmless glass composites with relatively high density have been prepared that can be used as shielding materials against gamma rays, especially at low energies.